AbstractIn order to expand the application of magnetorheological elastomers (MREs) in the field of sensor technology and improve their dielectric properties, a type of MRE with modified graphene, graphene/silicone rubber‐based magnetorheological elastomer (GR/RTV‐MRE), is proposed and its dielectric sensing properties were investigated. A model for calculating the relative permittivity of MRE was developed and combined with VASP software simulation to obtain the relative permittivity of GR/RTV‐MRE with different graphene contents. Combining the silicone rubber matrix with 30 vol% micro‐sized (ca 3.5 μm) spherical carbonyl iron particles, GR/RTV‐MRE samples with different graphene contents were prepared and tested for their relative permittivity. There is an error of approximate 7% between the test results and the simulation results, and the relative permittivity of GR/RTV‐MRE with a graphene content of 3 vol% reaches a maximum value of 35.400. An experimental platform for compressive properties was constructed and the compressive modulus of GR/RTV‐MRE with a graphene content of 3 vol% was tested under a magnetic field of 0–1 T. The results show that the modulus of compressibility is positively correlated with the magnetic field intensity in the range 0–0.9 T, up to 3.98 MPa, and is almost constant in the range 0.9–1 T. GR/RTV‐MRE with a graphene content of 3 vol% was used as the dielectric of a capacitive type transducer. The sensitivity of the capacitive sensor was measured to be 0.07 kPa−1 with a linear fitting of 99.6%. It is shown that GR/RTV‐MRE with 3 vol% graphene has good dielectric sensing capability. © 2022 Society of Industrial Chemistry.
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