Quantum Optics Research Articles

Optical manipulation in Rubidium-87 atomic medium using Kerr field: Dynamic insights into two-interfering electromagnetic waves

In this manuscript, we investigate the intricate dynamical properties arising from the interaction of two-interfering electromagnetic waves within a Rubidium-87 four-level N-type atomic medium. The study employs a probe field to interact with the atomic medium while incorporating two control fields one of which would be the Kerr field to modulate the system dynamics. The key parameters under scrutiny include the probe field detuning (ΔP/γ), control field parameters such as Rabi frequencies and detunings (Ω1,2/γ, Δ1,2/γ), and the angular orientation (θ) between the two-interfering waves. The research delves into the Energy density W, Momentum density P, Spin Angular momentum density S, Absorption rate Arate, Gradient force Fgrad, and Torque T associated with the two-interfering waves within the atomic medium. Through systematic variations in the aforementioned parameters, significant insights are gained into the nuanced behaviour of the system. The results showcase a rich tapestry of variations in the dynamical properties, shedding light on the underlying physics governing the interaction of electromagnetic waves in this unique atomic medium. This investigation not only contributes to the fundamental understanding of the dynamics within complex atomic systems but also holds potential applications in fields such as quantum information processing and quantum optics. The findings of this manuscript pave the way for further exploration and utilization of these intricate phenomena in the realm of advanced technologies and quantum communication.

On-chip quasi-light storage for long optical delays using Brillouin scattering

Efficient and extended light storage mechanisms are pivotal in photonics, particularly in optical communications, microwave photonics, and quantum networks, as they offer a direct route to circumvent electrical conversion losses and surmount bandwidth constraints. Stimulated Brillouin Scattering (SBS) is an established method to store optical information by transferring it to the acoustic domain, but current on-chip SBS efforts have limited bandwidth or storage time due to the phonon lifetime of several nanoseconds. An alternate approach known as quasi-light storage (QLS), which involves the creation of delayed replicas of optical data pulses via SBS in conjunction with a frequency comb, has been proposed to lift the storage time constraint; however, its realization has been confined to lengthy optical fibers, constraining integration with on-chip optical elements and form factors. Here, we present an experimental demonstration of QLS on a photonic chip leveraging the large SBS gain of chalcogenide glass, achieving delays of up to 500 ns for 1 ns long signal pulses, surpassing typical Brillouin storage processes' acoustic lifetime by more than an order of magnitude and waveguide transit time by two orders of magnitude. We experimentally and numerically investigate the dynamics of on-chip QLS and reveal that the interplay between the acoustic wave that stores the optical signal and subsequent optical pump pulses leads to a reshaping of the acoustic field. Our demonstrations illustrate the potential for achieving ultra-long storage times of individual pulses by several hundred pulse widths, marking a significant stride toward advancing the field of all-optical storage and delay mechanisms.

Study of Directional Couplers for Optical Qubit Quantum Operations

Study of Directional Couplers for Optical Qubit Quantum Operations

Limitations in design and applications of ultra-small mode volume photonic crystals

Ultra-small mode volume nanophotonic crystal cavities have been proposed as powerful tools for increasing coupling rates in cavity quantum electrodynamics systems. However, their adoption in quantum information applications remains elusive. In this work, we investigate possible reasons why, and analyze the impact of different low mode volume resonator design choices on their utility in quantum optics experiments. We analyze band structure features and loss rates of low mode volume bowtie cavities in diamond and demonstrate independent design control over cavity-emitter coupling strength and loss rates. Further, using silicon vacancy centers in diamond as exemplary emitters, we investigate the influence of placement imprecision. We find that the benefit on photon collection efficiency and indistinguishability is limited, while the fabrication complexity of ultra-small cavity designs increases substantially compared to conventional photonic crystals. We conclude that ultra-small mode volume designs are primarily of interest for dispersive spin-photon interactions, which are of great interest for future quantum networks.

Band gap engineering and controlling transport properties of single photons in periodic and disordered Jaynes–Cummings arrays

We theoretically study the single-photon transport properties in periodic and position-disordered Jaynes–Cummings (or JC) arrays of waveguide-coupled microtoroidal ring resonators, each interacting with a single two-level quantum emitter. Employing the real-space formalism of quantum optics, we focus on various parameter regimes of cavity quantum electrodynamics (cQED) to gain better control of single-photon propagation in such a many-body quantum optical setting. As for some of the key findings, we observe that the periodic setting leads to the formation of the band structure in the photon transmission spectra, which is most evident in the strong coupling regime of cQED. However, under resonant conditions with no losses, the application of Bloch’s theorem indicates that the width of forbidden gaps can be altered by tuning the emitter-cavity coupling to small values. Moreover, in the disordered case, we find that the single-photon transmission curves show the disappearance of band formation. However, spectral features originating from cQED interactions observed for the single atom-cavity problem remain robust against weak-disordered conditions. The results of this work may find application in the study of quantum many-body effects in the optical domain as well as in different areas of quantum computation and quantum networking.

Spatial photoluminescence and lifetime mappings of quasi-2D perovskites coupled with a dielectric metasurface.

Light-matter interaction between quantum emitters and optical cavities plays a vital role in fundamental quantum photonics and the development of optoelectronics. Resonant metasurfaces are proven to be an efficient platform for tailoring the spontaneous emission (SE) of the emitters. In this work, we study the interplay between quasi-2D perovskites and dielectric TiO2 metasurfaces. The metasurface, functioning as an open cavity, enhances electric fields near its plane, thereby influencing the emissions of the perovskite. This is verified through angle-resolved photoluminescence (PL) studies. We also conducted reflectivity measurements and numerical simulations to validate the coupling between the quasi-2D perovskites and photonic modes. Notably, our work introduces a spatial mapping approach to study Purcell enhancement. Using fluorescence lifetime imaging microscopy (FLIM), we directly link the PL and lifetimes of the quasi-2D perovskites in spatial distribution when positioned on the metasurface. This correlation provides unprecedented insights into emitter distribution and emitter-resonator interactions. The methodology opens a new (to the best of our knowledge) approach for studies in quantum optics, optoelectronics, and medical imaging by enabling spatial mapping of both PL intensity and lifetime, differentiating between uncoupled quantum emitters and those coupled with different types of resonators.

Modulation of Second-Order Sideband Efficiency in an Atom-Assisted Optomechanical System

We propose an efficient scheme to enhance the generation of optical second-order sidebands (OSSs) in an atom-assisted optomechanical system. The cavity field is coupled with a strong driving field and a weak probe field, and a control field is applied to the atom. We use the steady-state method to analyze the nonlinear interaction in the system, which is different from the traditional linear analysis method. The existence of an auxiliary three-level atom driven by the control field significantly enhances the generation of an OSS. It is found that the efficiency of the OSS can be effectively modulated by adjusting the Rabi frequency of the control field, optomechanical cooperativity and atomic coupling strength. Our scheme provides a promising solution for controlling light propagation and has potential application in quantum optical devices and quantum information networks.

Superconducting nanowire single-photon detectors with saturated quantum efficiency at 1550 nm on single-crystal diamond substrates

Single-crystal diamond possesses exceptional physical and optical properties, rendering it an ideal platform for integrated quantum optics. The direct integration of broadband-sensitive and high-performance single-photon detectors on diamond holds significant implications for the realization of integrated diamond quantum optical circuits. In this study, we polished the diamond surface with RMS (root mean square) below 0.6 nm suitable for the deposition and patterning of NbN thin films through ion beam etching. Subsequently, we fabricated superconducting nanowire single-photon detectors directly on the polished diamond substrates and characterized for their electrical and optical properties. The NbN-SNSPD exhibited a high critical current density (2 MA cm−2), a saturated quantum efficiency (QE) below 2.5 K, and a maximum value of QE up to 88% at 4 K. These findings offer a promising solution for fully integrated quantum optical chips on single-crystal diamond substrates.

Designing Variational Ansatz for Quantum‐Enabled Simulation of Non‐Unitary Dynamical Evolution ‐ An Excursion into Dicke Supperradiance

AbstractAdaptive Variational Quantum Dynamics (AVQD) algorithms offer a promising approach to providing quantum‐enabled solutions for systems treated within the purview of open quantum dynamical evolution. In this study, the unrestricted‐vectorization variant of AVQD is employed to simulate and benchmark various non‐unitarily evolving systems. Exemplification of how construction of an expressible ansatz unitary and the associated operator pool can be implemented to analyze examples such as the Fenna–Matthews–Olson complex (FMO) and even the permutational invariant Dicke model of quantum optics. Furthermore, an efficient decomposition scheme is shown for the ansatz used, which can extend its applications to a wide range of other open quantum system scenarios in near future. In all cases the results obtained are in excellent agreement with exact numerical computations that bolsters the effectiveness of this technique. The successful demonstrations pave the way for utilizing this adaptive variational technique to study complex systems in chemistry and physics, like light‐harvesting devices, thermal, and opto‐mechanical switches, to name a few.

Vortex beam induced spatial modulation of quantum-optical effects in a coherent atomic medium

We have studied two-dimensional absorption, gain, and corresponding refractive index profiles in a ladder-type three-level atomic system interacting with three coherent fields. One is a weak probe field considered as a plane wave, while the other two are the control fields taken as two Laguerre–Gaussian doughnut beams. Position dependence of two vortex beams induces the spatially modulated coherence at the condition of resonance, which enables us to obtain space-dependent absorption, transparency, gain without inversion (GWI), and refractive index enhancement in the present scheme. The azimuthal modulation of coherence effects is attributed to the presence of optical angular momentum of the vortex beams. Under the influence of an additional travelling wave field with the presence of two vortex beams, the present model leads us to obtain an ultra-large enhancement of refractive index at the resonant detuning of the fields. This phenomenon makes the atom-field system to play the equivalent role of a high-refractive-index prism. The role of near dipole–dipole (NDD) interaction on the modulation of position-dependent coherence effects has also been investigated. It has been shown that, without any inclusion of the travelling wave field in the system, the phenomenon of resonant enhancement of refractive index may also occur in the presence of NDD effect. The new way of generating spatially controlled GWI and nonlinear refractive index enhancement is specific to the present model. This work seems to be useful for finding its applications in spatially modulated coherence controlled electromagnetically induced transparency-based quantum devices like quantum optical memory, switches, and quantum logic gates, where the refractive index switching phenomenon is a prerequisite.

A new teaching-learning sequence to promote secondary school students’ learning of quantum physics using Dirac notation

This paper describes the design of a new teaching-learning sequence on quantum physics aimed at upper secondary school students. In this teaching-learning sequence, GeoGebra simulations and interactive screen experiments are used to investigate the behaviour of a single photon at beam splitter and single photon interference in a Michelson interferometer. We propose a minimal formalism using Dirac notation, which avoids complex numbers and elaborate vector calculus, to make a quantitative description of the quantum optics experiments accessible to secondary school students. With this new educational pathway, we take into account findings from physics education research, which suggest that the introduction of a mathematical formalism tailored to students’ abilities might help them to overcome naive-realist views of quanta or space-time descriptions of quantum phenomena, while at the same time facilitating a transition to a functional understanding of quantum models.

High-Field Optical Cesium Magnetometer for Magnetic Resonance Imaging

We present a novel high-field optical quantum magnetometer based on saturated absorption spectroscopy on the extreme angular-momentum states of the cesium D2 line. With key features including continuous readout, high sampling rate, and sensitivity and accuracy in the ppm range, it represents a competitive alternative to conventional techniques for measuring magnetic fields of several teslas. The prototype has four small separate field probes, and all support electronics and optics are fitted into a single 19-inch rack to make it compact, mobile, and robust. The field probes are fiber coupled and made from nonmetallic components, allowing them to be easily and safely positioned inside a 7 T MRI scanner. We demonstrate the capabilities of this magnetometer by measuring two different MRI sequences, and we show how it can be used to reveal imperfections in the gradient coil system, to highlight the potential applications in medical MRI. We propose the term EXAAQ (EXtreme Angular-momentum Absorption-spectroscopy Quantum) magnetometry, for this novel method. Published by the American Physical Society 2024

On the properties of the anisotropic multivariate Hermite-Gauss functions

The Hermite-Gauss basis functions have been extensively employed in classical and quantum optics due to their convenient analytic properties. A class of multivariate Hermite-Gauss functions, the anisotropic Hermite-Gauss functions, arise by endowing the standard univariate Hermite-Gauss functions with a positive definite quadratic form. These multivariate functions admit useful applications in optics, signal analysis and probability theory, however they have received little attention in literature. In this paper, we examine the properties of these functions, with an emphasis on applications in computational optics.

Transient temperature dynamics of reservoirs connected through an open quantum system.

The dynamics of open quantum systems connected with several reservoirs attract great attention due to their importance in quantum optics, biology, quantum thermodynamics, transport phenomena, etc. In many problems, the Born approximation is applicable, which implies that the influence of the open quantum system on the reservoirs can be neglected. However, in the case of long-time dynamics or mesoscopic reservoirs, the reverse influence can be crucial. In this paper, we investigate the transient dynamics of several bosonic reservoirs connected through an open quantum system. We use an adiabatic approach to study the temporal dynamics of temperatures of the reservoirs during relaxation to thermodynamic equilibrium. We show that there are various types of temperature dynamics that strongly depend on the values of dissipative rates and initial temperatures. We demonstrate that temperatures of the reservoirs, including the hottest and coldest ones, can exhibit nonmonotonic behavior. Moreover, there are moments of time during which the reservoir with an initially intermediate temperature becomes the hottest or coldest reservoir. The obtained results pave the way for managing energy flows in mesoscale and nanoscale systems.

Spectral quasi-clustering estimates for certain semiregular systems

We show a quasi-clustering result for a subclass of the class of Semiregular Metric Globally Elliptic Systems (SMGES) including certain quantum optics models (such as Jaynes-Cummings and its generalizations) which describe light-matter interaction. More precisely, we show that for the class of systems with polynomial coefficients we consider, the spectrum concentrates within the union of intervals (not necessarily disjoint, but at most intersecting in an a priori finite number) centered at a sequence determined in terms of invariants of the (total) symbol and width decreasing as the centers go to infinity.

Ultrafast photoluminescence and multiscale light amplification in nanoplasmonic cavity glass.

Interactions between plasmons and exciton nanoemitters in plexcitonic systems lead to fast and intense luminescence, desirable in optoelectonic devices, ultrafast optical switches and quantum information science. While luminescence enhancement through exciton-plasmon coupling has thus far been mostly demonstrated in micro- and nanoscale structures, analogous demonstrations in bulk materials have been largely neglected. Here we present a bulk nanocomposite glass doped with cadmium telluride quantum dots (CdTe QDs) and silver nanoparticles, nAg, which act as exciton and plasmon sources, respectively. This glass exhibits ultranarrow, FWHM = 13 nm, and ultrafast, 90 ps, amplified photoluminescence (PL), λem≅503 nm, at room temperature under continuous-wave excitation, λexc = 405 nm. Numerical simulations confirm that the observed improvement in emission is a result of a multiscale light enhancement owing to the ensemble of QD-populated plasmonic nanocavities in the material. Power-dependent measurements indicate that >100 mW coherent light amplification occurs. These types of bulk plasmon-exciton composites could be designed comprising a plethora of components/functionalities, including emitters (QDs, rare earth and transition metal ions) and nanoplasmonic elements (Ag/Au/TCO, spherical/anisotropic/miscellaneous), to achieve targeted applications.

High-dimensional Poincaré beams generated through cascaded metasurfaces for high-security optical encryption

Optical encryption plays an increasingly important role in the field of information security owing to its parallel processing capability and low power consumption. Employing the ultrathin metasurfaces in optical encryption has promoted the miniaturization and multifunctionality of encryption systems. Nevertheless, with the few number of degrees of freedom (DoFs) multiplexed by single metasurface, both key space and encoding space are limited. To address this issue, we propose a high-security and large-capacity optical encryption scheme based on perfect high-dimensional Poincaré beams with expanded DoFs. By cascading two arrayed metasurfaces, more beam properties can be independently engineered, which gives rise to the extensively expanded key and encoding spaces. Our work provides a promising strategy for optical encryption with high security level and large information capacity and might facilitate the applications of Poincaré beams in optical communications and quantum information.

Topological protection of dual-polarization biphoton states in photonic crystals

Polarization control is a major issue in topological quantum optics that limits reliable generation and transmission of quantum states. This study presents what we believe to be a novel topological photonic crystal design that provides topological protection for biphoton pairs for both TE and TM polarization. By well-designed cell configurations within the lattice, two topological boundaries emerge that can accommodate TM and TE modes at the same time. By adjusting the dispersion curves, we can further design nonlinear four-wave mixing processes within the topological photonic crystals and provide theoretical explanations for the entanglement of the dual-polarization biphoton states. Numerical results confirm the robust transport of entangled photon pairs, even when subjected to sharp bending. Moreover, combining the dual-polarization topological photonic crystal with a polarization beam splitter enables the preparation of polarization-encoded maximally entangled states. Our work exhibits significant potential for applications in robust optical quantum information processing and quantum secure communication.

Role of Pyramidal Low-Dimensional Semiconductors in Advancing the Field of Optoelectronics

Numerous optoelectronic devices based on low-dimensional nanostructures have been developed in recent years. Among these, pyramidal low-dimensional semiconductors (zero- and one-dimensional nanomaterials) have been favored in the field of optoelectronics. In this review, we discuss in detail the structures, preparation methods, band structures, electronic properties, and optoelectronic applications (photocatalysis, photoelectric detection, solar cells, light-emitting diodes, lasers, and optical quantum information processing) of pyramidal low-dimensional semiconductors and demonstrate their excellent photoelectric performances. More specifically, pyramidal semiconductor quantum dots (PSQDs) possess higher mobilities and longer lifetimes, which would be more suitable for photovoltaic devices requiring fast carrier transport. In addition, the linear polarization direction of exciton emission is easily controlled via the direction of magnetic field in PSQDs with C3v symmetry, so that all-optical multi-qubit gates based on electron spin as a quantum bit could be realized. Therefore, the use of PSQDs (e.g., InAs, GaN, InGaAs, and InGaN) as effective candidates for constructing optical quantum devices is examined due to the growing interest in optical quantum information processing. Pyramidal semiconductor nanorods (PSNRs) and pyramidal semiconductor nanowires (PSNWRs) also exhibit the more efficient separation of electron-hole pairs and strong light absorption effects, which are expected to be widely utilized in light-receiving devices. Finally, this review concludes with a summary of the current problems and suggestions for potential future research directions in the context of pyramidal low-dimensional semiconductors.

Observation of amplitude squeezing in a constant-current-driven distributed feedback quantum dot laser with optical feedback

We illustrate the generation of single-mode amplitude squeezing in a distributed feedback quantum dot laser driven by a constant-current pump. Achieving broadband amplitude squeezing of 1.7 dB over a 10 GHz range at room temperature is realized by suppressing carrier noise and implementing optical feedback. The noise-corrected squeezing level reached 5.1 dB. Furthermore, the examination of the zero-delay second-order correlation function demonstrates the robust feedback stability of the amplitude-squeezed state in the quantum dot laser compared to a reference quantum well laser. This investigation lays the groundwork for future advancements in integrated optical quantum chips.