Long-lived Isomeric States Research Articles

Long-sought isomer turns out to be the ground state of 76Cu

Isomers close to the doubly magic nucleus 78Ni (Z=28, N=50) provide essential information on the shell evolution and shape coexistence far from stability. The existence of a long-lived isomeric state in 76Cu has been debated for a long time. We have performed high-precision mass measurements of 76Cu with the JYFLTRAP double Penning trap mass spectrometer at the Ion Guide Isotope Separator On-Line facility and confirm the existence of such an isomeric state with an excitation energy Ex=64.8(25) keV. Based on the ratio of detected ground- and isomeric-state ions as a function of time, we show that the isomer is the shorter-living state previously considered as the ground state of 76Cu. The result can potentially change the conclusions made in previous works related to the spin-parity and charge radius of the 76Cu ground state. Additionally, the new 76Cu(n,γ) reaction Q-value has an impact on the astrophysical rapid neutron-capture process.

Nuclear Structure and Decay Data for A = 222 Isobars

Evaluated data are presented for 11 known A=222 nuclides (Bi, Po, At, Rn, Fr, Ra, Ac, Th, Pa, U, and Np), and relevant Jπ and T1/2 data for A=226 nuclei decaying by α-decay to A=222 nuclei. For 222Bi, only the isotopic identification is established with no measurement of its half-life. For 222Po, 222At, 222Fr, 222U, and 222Np, data are available only for the ground states, with static magnetic dipole and electric quadrupole moments, and charge radius measurements for the 222Fr ground state. For 222Ac and 222Pa, two low-lying levels are known from 226Pa α decay, and 226Np decay, respectively, but with no information about Jπ assignments and γ decays of these levels. For 222Pa, a long-lived isomeric state is known, decaying dominantly by α decay. 222Rn, 222Ra, and 222Th have been investigated in detail, the low-spin states by α decay and the high-spin studies of ground-state and octupole bands by in-beam γ-ray studies for all the three nuclei, as well as by Coulomb excitation for 222Rn and 222Ra. Low-spin levels in 222Ra have been investigated also through the β− decay of 222Fr. Half-lives of the excited states are known for 7 levels in 222Rn, 12 levels in 222Ra, and 3 levels in 222Th. Octupole deformations, with the presence of alternating-parity bands up to (16+) and (21−) in 222Rn, (20+) and (19−) in 222Ra, and (26+) and (25−) in 222Th, and with interband E1 transitions, have been established in these three nuclei. The present evaluation supersedes the previous A=222 ENSDF evaluations: (2011Si24), (1996El01), (1987El06) and (1977To14).

Studying Gamow-Teller transitions and the assignment of isomeric and ground states at N = 50

Direct mass measurements of neutron-deficient nuclides around the N=50 shell closure below 100Sn were performed at the FRS Ion Catcher (FRS-IC) at GSI, Germany. The nuclei were produced by projectile fragmentation of 124Xe, separated in the fragment separator FRS and delivered to the FRS-IC. The masses of 14 ground states and two isomers were measured with relative mass uncertainties down to 1×10−7 using the multiple-reflection time-of-flight mass spectrometer of the FRS-IC, including the first direct mass measurements of 98Cd and 97Rh. A new QEC=5437±67 keV was obtained for 98Cd, resulting in a summed Gamow-Teller (GT) strength for the five observed transitions (0+⟶1+) as B(GT)=2.94−0.28+0.32. Investigation of this result in state-of-the-art shell model approaches accounting for the first time experimentally observed spectrum of GT transitions points to a perfect agreement for N=50 isotones. The excitation energy of the long-lived isomeric state in 94Rh was determined for the first time to be 293±21 keV. This, together with the shell model calculations, allows the level ordering in 94Rh to be understood.

Direct high-precision mass spectrometry of superheavy elements with SHIPTRAP

Direct mass measurements in the region of the heaviest elements were performed with the Penning-trap mass spectrometer SHIPTRAP at GSI Darmstadt. Utilizing the phase-imaging ion-cyclotron-resonance mass-spectrometry technique, the atomic masses of No251 (Z=102), Lr254 (Z=103), and Rf257 (Z=104) available at rates down to one detected ion per day were determined directly for the first time. The ground-state masses of No254 and Lr255,256 were improved by more than one order of magnitude. Relative statistical uncertainties as low as δm/m≈10−9 were achieved. Mass resolving powers of 11 000 000 allowed resolving long-lived low-lying isomeric states from their respective ground states in No251,254 and Lr254,255. This provided an unambiguous determination of the binding energies for odd-A and odd-odd nuclides previously determined only indirectly from decay spectroscopy.Received 24 June 2022Accepted 28 September 2022DOI:https://doi.org/10.1103/PhysRevC.106.054325Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI. Open access publication funded by the Max Planck Society.Published by the American Physical SocietyPhysics Subject Headings (PhySH)Research AreasBinding energy & massesNuclear structure & decaysPropertiesA ≥ 220TechniquesMass spectrometryPenning trapsRadioactive beamsNuclear Physics

Study of the 176Hf(n,2n)175Hf cross section at 18.9 MeV

Neutron nuclear reactions can provide significant information in the field of nuclear physics and applications. Hafnium (Hf) is one of the rare-earth isotopes with a relative large neutron total cross-section in the thermal neutron energy region and neutron induced reactions in reactor materials could lead to the production of long-lived isomeric states of Hf isotopes. Thus, the knowledge of neutron cross-sections on Hf isotopes is of great importance for basic research in Nuclear Physics as well as for applications concerning the interaction of neutrons with matter. In this study measurements of experimental cross section for the 176Hf(n,2n)175Hf and 180Hf(n,n΄γ)180mHf reactions were carried out, using the activation technique. The neutron beam energy at 18.9 MeV was produced via the 3H(d,n)4He reaction at the 5.5 MeV Tandem Van de Graaf accelerator laboratory of NCSR “Demokritos”. A thin metallic foil of natural Hf was used, while for the determination of the neutron flux at the target position a reference foil of Al was placed at the back of the Hf target. The irradiation was continuous for 28 hours leading to a total neutron fluence of 1010 n/cm2 and a BF3 detector was used for monitoring the neutron flux during the irradiation. After the end of irradiation, the activity of the Hf target and the Al foil were measured off-line by two HPGe detectors. Both detector efficiencies were obtained using a calibrated 152Eu source, placed in the same distance as the target and the reference foil. The 176Hf(n,2n)175Hf reaction has been corrected from the contribution of 177Hf(n,3n)175Hf and the 174Hf(n,γ)175Hf reactions and the 180Hf(n,n΄γ)180mHf reaction from the 179Hf(n,γ)180mHf. Theoretical calculations of the 174Hf(n,2n)175Hf, 176Hf(n,2n)175Hf and 180Hf(n,n΄γ)180mHf reaction cross-sections have also been performed using the nuclear statistical code “EMPIRE 3.2.3” and they have been compared with the data.

Search for fission from a long-lived isomer in No250 and evidence of a second isomer

In the present work, a $K$ isomeric state in $^{250}\mathrm{No}$, which is more stable against fission than the ground state, was experimentally studied. The aim was to measure the fission branch of this isomeric state. In total, 780 fission events attributed to the decay of $^{250}\mathrm{No}$ were detected. Among them 133 cases were attributed to the ground-state decay with a half-life of 4.0(4) $\ensuremath{\mu}\mathrm{s}$, which was populated by the deexcitation of the isomeric state via electromagnetic transitions with a half-life of 23(4) $\ensuremath{\mu}\mathrm{s}$. In addition, in two more cases, this long-lived isomeric state was populated in the deexcitation of a hitherto unknown, yet higher-lying and short-lived isomeric state with a half-life of $0.{7}_{\ensuremath{-}0.3}^{+1.4}\phantom{\rule{4pt}{0ex}}\ensuremath{\mu}\mathrm{s}$. No direct fission from the long-lived isomeric state, i.e., with a lifetime of longer than 40 $\ensuremath{\mu}\mathrm{s}$, was identified. This results in an upper limit of 0.035 for the branching ratio for fission. This is a significantly more strict limit than the previously known value of 0.5. Nonobservation of fission branching of the long-lived isomer is discussed relative to theoretical predictions and within various semiempirical ways, which resulted in an attribution of a lower limit of ${10}^{4}$ for the fission-hindrance factor, caused by the $K$ quantum number. The presences of multiple high-$K$ isomeric states seemingly is a widespread phenomenon in deformed heavy nuclei.

First coupling of the FRS particle identification and the FRS-Ion Catcher data acquisition systems: The case of 109In

For the first time, the FRagment Separator (FRS) and the Multiple-Reflection Time-Of-Flight Mass-Spectrometer (MR-TOF-MS) particle identification (PID) systems at GSI have been coupled. This new approach adds to the standard FRS PID an additional unambiguous identification of the fragments and the possibility to identify and count long-lived isomeric states (>ms). For this purpose, single-event timestamp information given by a common clock was used to correlate both systems. Two methods were implemented to improve the signal-to-background ratio by more than a factor 2 in the high resolution mass spectrum obtained with the MR-TOF-MS for the 109In isotope. Moreover, the coupling of the systems allows an improvement in the on-line monitoring of the FRS-Ion Catcher (IC) efficiency and extraction time. In addition, range calculations were implemented in the on-line monitoring; a powerful tool for real-time optimization of stopped beam experiments.

Mapping the N=40 island of inversion: Precision mass measurements of neutron-rich Fe isotopes

Nuclear properties across the chart of nuclides are key to improving and validating our understanding of the strong interaction in nuclear physics. We present high-precision mass measurements of neutron-rich Fe isotopes performed at the TITAN facility. The multiple-reflection time-of-flight mass spectrometer (MR-ToF-MS), achieving a resolving power greater than 600000 for the first time, enabled the measurement of Fe63–70, including first-time high-precision direct measurements (δm/m≈10−7) of Fe68–70, as well as the discovery of a long-lived isomeric state in Fe69. These measurements are accompanied by both mean-field and ab initio calculations using the most recent realizations which enable theoretical assignment of the spin-parities of the Fe69 ground and isomeric states. Together with mean-field calculations of quadrupole deformation parameters for the Fe isotope chain, these results benchmark a maximum of deformation in the N=40 island of inversion in Fe and shed light on trends in level densities indicated in the newly refined mass surface.Received 19 July 2021Revised 24 December 2021Accepted 16 March 2022DOI:https://doi.org/10.1103/PhysRevC.105.L041301©2022 American Physical SocietyPhysics Subject Headings (PhySH)Research AreasBinding energy & massesNuclear structure & decaysRare & new isotopesProperties59 ≤ A ≤ 89TechniquesAb initio calculationsMean field theoryTime-of-flight mass spectrometryNuclear Physics

High precision measurement of the half-life of the 391.6 keV metastable level in Pu239

Materials selection for rare event physics requires high performance detectors and customized analyses. In this context a novel $\beta$-$\gamma$ detection system, comprised of a liquid scintillator in coincidence with a HPGe, was developed with the main purpose of studying ultra trace contamination of uranium, thorium and potassium in liquid samples. In the search for $^{238}\textrm{U}$ contaminations through neutron activation analysis, since the activation product $^{239}\textrm{Np}$ decays to a relatively long-lived isomeric state of $^{239}\textrm{Pu}$, it is possible to perform a time selection of these events obtaining a strong background suppression. Investigating the time distribution of the coincidences between the $\beta^-$ decay of $^{239}\textrm{Np}$ and the delayed events following the de-excitation of the $^{239}\textrm{Pu}$ isomeric level at 391.6 keV, a precision measurement of the half-life of this level was conducted. The half-life of the 391.6 keV $^{239}\textrm{Pu}$ level resulted $190.2 \pm 0.2$ ns, thus increasing the precision by about a factor of 20 over previous measurements.

Long-lived isomeric states and quasiparticle band structures in neutron-rich Gd162,164 nuclei from β decay

Long-lived isomeric states and quasiparticle band structures in neutron-rich <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mmultiscripts><mml:mi>Gd</mml:mi><mml:mprescripts /><mml:none /><mml:mrow><mml:mn>162</mml:mn><mml:mo>,</mml:mo><mml:mn>164</mml:mn></mml:mrow></mml:mmultiscripts></mml:math> nuclei from <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>β</mml:mi></mml:math> decay

Exotic Nuclear Structure of Neutron-rich Zn Isotopes

Nuclear structure of unstable nuclei, in particularly the nuclei near the magic number, has been one of the hot topics of nuclear physics study. Near the neutron magic number N=40, 50, rich nuclear structure phonomania appeared in the nickel region, in particularly for the neutron-rich isotopes, have stimulated intensive investigation from both theoretical and experimental aspects. In order to gain a better understanding of the nuclear structure in the nickel region, we choose to study the properties of neutron-rich Zn(Z=30) isotopes. In this paper, after a simple introduction of the laser spectroscopy experiment of Zn isotopes at CERN-ISOLDE, we reviewed the nuclear spins, magnetic moment, electric quadrupole moment and root mean square charge radius of the ground and long-lived isomeric states of 62–80Zn isotopes. Based on these properties, together with shell-model calculation from different interactions, we discussed systematically the nuclear structure phenomena, such as the shell structure evolution, magicity, deformation and shape coexistence, and the cross-shell excitation of correlated nucleons. At the end, on the basis of the current experimental data and nuclear structure information, as well as the theoretical prediction of energy level evolution of N=51 isotones in nickel region, we propose to measure the basic properties of 81,82Zn nuclei at the collinear resonance ionization spectroscopy setup at ISOLDE-CERN.

Isomer studies in the vicinity of the doubly-magic nucleus 100Sn: Observation of a new low-lying isomeric state in 97Ag

Long-lived isomeric states in 97Ag and 101−109In were investigated with the FRS Ion Catcher at GSI. In the isotope 97Ag, a long-lived (1/2−) isomeric state was discovered, and its excitation energy was determined to be 618(38) keV. This is simultaneously the first discovery of a nuclear isomeric state by multiple-reflection time-of-flight mass spectrometry. The measured excitation energies were compared to large-scale shell-model calculations, which indicated the importance of core excitation around 100Sn. Furthermore, advanced mean-field calculations for the 97Ag nucleus and relevant neighboring nuclei were performed, which have contributed to a better understanding of the repetitive appearance of certain isomeric structures in neighboring nuclei, and which have supported the discovery of the isomeric state in 97Ag in a global shell-evolution scheme.

Discovery of 68Br in secondary reactions of radioactive beams

The proton-rich isotope 68Br was discovered in secondary fragmentation reactions of fast radioactive beams. Proton-rich secondary beams of 70,71,72Kr and 70Br, produced at the RIKEN Nishina Center and identified by the BigRIPS fragment separator, impinged on a secondary 9Be target. Unambiguous particle identification behind the secondary target was achieved with the ZeroDegree spectrometer. Based on the expected direct production cross sections from neighboring isotopes, the lifetime of the ground or long-lived isomeric state of 68Br was estimated. The results suggest that secondary fragmentation reactions, where relatively few nucleons are removed from the projectile, offer an alternative way to search for new isotopes, as these reactions populate preferentially low-lying states.

New and comprehensive β - and βp -decay spectroscopy results in the vicinity of Sn100

A decay spectroscopy experiment on proton-rich nuclei in the vicinity of the doubly magic Sn100 was carried out at RIKEN Nishina Center. More than 20 nuclei with 43≤Z≤50 and N≤51, produced by fragmentation reactions were investigated via analyses of β-decay, βp-decay, and subsequent γ-ray data. Owing to higher statistics, the precision on the half-lives of many of the ground states and isomers was improved. β-decay endpoint energies of 11 states in 8 nuclei were measured for the first time, and the corresponding QEC and excitation energies were generally consistent with various mass models. Many β-delayed proton emission branching ratios were measured either for the first time or with higher precision compared to literature values, and some of them differed by more than 2σ. Many of the large discrepancies were associated with nuclei with long-lived isomeric states, highlighting large systematic uncertainties involved in these measurements. Twenty-five new γ rays were observed, and ten new states are proposed with unambiguous excitation energies, spins, and parities. Most of the energies of the excited states were consistent within 300 keV or 20%, whichever was greater, compared to shell model predictions in the proton/neutron (p1/2,g9/2) model space assuming a Sr76 core. A signature of a new (1/2-) isomer in Cd97 with T1/2=0.73(7) s was found, in good agreement with shell model predictions.

Measurements and analysis of [formula omitted]Hf production cross sections under [formula omitted]Ta and [formula omitted]W irradiation by protons with 0.04–2.6 GeV energies

This paper presents the results of experimental determination and computational simulation of the independent cross sections of 178m2Hf production in natTa and natW thin targets irradiated by mono-energetic proton beams in the energy range from ∼0.04 up to 2.6 GeV. The cross sections were determined using the γ-spectrometry technique without chemical separation of irradiated samples. The obtained experimental results were compared with the results of simulations based on the modified CEM03.03-ext intranuclear cascade model, which allows to analyze both the cross sections of residual nuclei production and the probabilities of long-lived isomeric states formation. Verification of the isomeric yield calculation model was demonstrated based on experimental data on high-spin isomer production cross sections in 208Pb target irradiated by protons.

Detailed spectroscopy of Bi195

An experiment focused on the study of shape coexistence and new high-spin structures in $^{195}\mathrm{Bi}$ has been performed. The nucleus is in a transitional region of the bismuth isotope chain. A large number of new states have been found, resulting in a significant extension of the previously known level scheme. Several new collective structures have been identified. A strongly coupled rotational band built upon the $13/{2}^{+}$ isomeric state was extended up to ${I}^{\ensuremath{\pi}}=(49/{2}^{+})$ and an energy of 5706 keV. The ${I}^{\ensuremath{\pi}}=31/{2}^{+}$ member of the $\ensuremath{\pi}{i}_{13/2}$ band was also found to feed a new long-lived isomeric state with an excitation energy of 2616 keV and a spin and parity of ${I}^{\ensuremath{\pi}}=29/{2}^{+}$. The half-life of the $29/{2}^{+}$ isomeric state was determined to be $1.49(1)\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}\mathrm{s}$. It decays via the emission of 457-keV $E2$ and 236-keV $E1$ transitions, respectively. A low-energy 46-keV $E2$ transition has been identified to depopulate the ($29/{2}^{\ensuremath{-}}$) isomeric state, with a measured half-life of ${T}_{1/2}=614(5)\phantom{\rule{0.28em}{0ex}}\mathrm{ns}$. This transition allows the excitation energy of the isomeric state to be determined as 2381 keV. The feeding patterns of both $29/{2}^{+}$ and ($29/{2}^{\ensuremath{-}}$) isomeric states have also been described. This is the first time collective structures have also been observed up to high spins and excitation energies in the neutron-deficient $^{195}\mathrm{Bi}$ nucleus. Evidence for the manifestation of shape coexistence in $^{195}\mathrm{Bi}$ is also discussed.

Evolution of nuclear structure in neutron-rich odd-Zn isotopes and isomers

Collinear laser spectroscopy was performed on Zn (Z=30) isotopes at ISOLDE, CERN. The study of hyperfine spectra of nuclei across the Zn isotopic chain, N=33–49, allowed the measurement of nuclear spins for the ground and isomeric states in odd-A neutron-rich nuclei up to N=50. Exactly one long-lived (>10 ms) isomeric state has been established in each 69–79Zn isotope. The nuclear magnetic dipole moments and spectroscopic quadrupole moments are well reproduced by large-scale shell–model calculations in the f5pg9 and fpg9d5 model spaces, thus establishing the dominant term in their wave function. The magnetic moment of the intruder Iπ=1/2+ isomer in 79Zn is reproduced only if the νs1/2 orbital is added to the valence space, as realized in the recently developed PFSDG-U interaction. The spin and moments of the low-lying isomeric state in 73Zn suggest a strong onset of deformation at N=43, while the progression towards 79Zn points to the stability of the Z=28 and N=50 shell gaps, supporting the magicity of 78Ni.

Application of isochronous mass spectrometry for the study of angular momentum population in projectile fragmentation reactions

Isochronous mass spectrometry was applied to measure isomeric yield ratios of fragmentation reaction products. This approach is complementary to conventional gamma-ray spectroscopy in particular for measuring yield ratios for long-lived isomeric states. Isomeric yield ratios for the high-spin I = 19/2 states in the mirror nuclei 53Fe and 53Co are measured to study angular momentum population following the projectile fragmentation of 78Kr at energies of 480A MeV on a beryllium target. The 19/2 state isomeric ratios of 53Fe produced from different projectiles in the literature have also been extracted as a function of mass number difference between projectile and fragment (mass loss). The results are compared to ABRABLA07 model calculations. The isomeric ratios of 53Fe produced using different projectiles suggest that the theory underestimates not only the previously reported dependence on the spin but also the dependence on the mass loss.

Long-lived K isomer and enhanced γ vibration in the neutron-rich nucleus 172Dy: Collectivity beyond double midshell

The level structure of 172Dy has been investigated for the first time by means of decay spectroscopy following in-flight fission of a 238U beam. A long-lived isomeric state with T1/2 = 0.71(5) s and K π = 8 − has been identified at 1278 keV, which decays to the ground-state and γ-vibrational bands through hindered electromagnetic transitions, as well as to the daughter nucleus 172Ho via allowed β decays. The robust nature of the K π = 8 − isomer and the ground-state rotational band reveals an axially-symmetric structure for this nucleus. Meanwhile, the γ-vibrational levels have been identified at unusually low excitation energy compared to the neighboring well-deformed nuclei, indicating the significance of the microscopic effect on the non-axial collectivity in this doubly mid-shell region. The underlying mechanism of enhanced γ vibration is discussed in comparison with the deformed Quasiparticle Random-Phase Approximation based on a Skyrme energy-density functional.

The Collinear Fast Beam laser Spectroscopy (Cfbs) experiment at Triumf

Laser spectroscopy experiments at radioactive ion beam facilities around the world investigate properties of exotic nuclei for scientific endeavours such as, but not limited to, the investigation of nuclear structure. Advancements in experimental sensitivity and performance are continuously needed in order to extend the reach of nuclei that can be measured. The collinear fast beam laser spectroscopy (Cfbs) setup at Triumf, coupled to an out-of-plane radio-frequency quadrupole Paul trap, enables measurements of some of the most fundamental nuclear properties for long-lived ground and isomeric states. The first comprehensive overview of the Cfbs experiment is provided along with descriptions of key developments that extend the reach of laser spectroscopy experiments. A novel data acquisition technique structured around three-dimensional spectra is presented, where the integration of a custom multi-channel-scalar provides photon counts correlated with arrival time and acceleration voltage for post-experiment analysis. In addition, new rapid light manipulation techniques are discussed that suppress undesirable hyperfine pumping effects and regain losses in experimental efficiency.