High precision measurement of the half-life of the 391.6 keV metastable level in Pu239

Abstract

Materials selection for rare event physics requires high performance detectors and customized analyses. In this context a novel $\beta$-$\gamma$ detection system, comprised of a liquid scintillator in coincidence with a HPGe, was developed with the main purpose of studying ultra trace contamination of uranium, thorium and potassium in liquid samples. In the search for $^{238}\textrm{U}$ contaminations through neutron activation analysis, since the activation product $^{239}\textrm{Np}$ decays to a relatively long-lived isomeric state of $^{239}\textrm{Pu}$, it is possible to perform a time selection of these events obtaining a strong background suppression. Investigating the time distribution of the coincidences between the $\beta^-$ decay of $^{239}\textrm{Np}$ and the delayed events following the de-excitation of the $^{239}\textrm{Pu}$ isomeric level at 391.6 keV, a precision measurement of the half-life of this level was conducted. The half-life of the 391.6 keV $^{239}\textrm{Pu}$ level resulted $190.2 \pm 0.2$ ns, thus increasing the precision by about a factor of 20 over previous measurements.