State-dependent Potentials Research Articles

Trapped Ion Quantum Computing Using Optical Tweezers and Electric Fields.

We propose a new scalable architecture for trapped ion quantum computing that combines optical tweezers delivering qubit state-dependent local potentials with oscillating electric fields. Since the electric field allows for long-range qubit-qubit interactions mediated by the center-of-mass motion of the ion crystal alone, it is inherently scalable to large ion crystals. Furthermore, our proposed scheme does not rely on either ground-state cooling or the Lamb-Dicke approximation. We study the effects of imperfect cooling of the ion crystal, as well as the role of unwanted qubit-motion entanglement, and discuss the prospects of implementing the state-dependent tweezers in the laboratory.

Prospects for single-photon sideband cooling of optically trapped neutral atoms

We propose a novel cooling scheme for realising single photon sideband cooling on particles trapped in a state-dependent optical potential. We develop a master rate equation from an ab-initio model and find that in experimentally feasible conditions it is possible to drastically reduce the average occupation number of the vibrational levels by applying a frequency sweep on the cooling laser that sequentially cools all the motional states. Notably, this cooling scheme works also when a particle experiences a deeper trap in its internal ground state than in its excited state, a condition for which conventional single photon sideband cooling does not work. In our analysis, we consider two cases: a two-level particle confined in an optical tweezer and Li atoms confined in an optical lattice, and find conditions for efficient cooling in both cases. The results from the model are confirmed by a full quantum Monte Carlo simulation of the system Hamiltonian. Our findings provide an alternative cooling scheme that can be applied in principle to any particle, e.g. atoms, molecules or ions, confined in a state-dependent optical potential.

Gravitational Redshift Tests with Atomic Clocks and Atom Interferometers

Atomic interference experiments can probe the gravitational redshift via the internal energy splitting of atoms and thus give direct access to test the universality of the coupling between matter-energy and gravity at different spacetime points. By including possible violations of the equivalence principle in a fully quantized treatment of all degrees of freedom, we characterize how the sensitivity to gravitational redshift violations arises in atomic clocks and atom interferometers, as well as their underlying limitations. Specifically, we show that: (i.) Contributions beyond linear order to trapping potentials lead to such a sensitivity of trapped atomic clocks. (ii.) While Bragg-type interferometers, even with a superposition of internal states, with state-independent, linear interaction potentials are at first insensitive to gravitational redshift tests, modified configurations, for example by relaunching the atoms, can mimic such tests tests under certain conditions. (iii.) Guided atom interferometers are comparable to atomic clocks. (iv.) Internal transitions lead to state-dependent interaction potentials through which light-pulse atom interferometers can become sensitive to gravitational redshift violations.

Non-adiabatic ring polymer molecular dynamics with spin mapping variables.

We present a new non-adiabatic ring polymer molecular dynamics (NRPMD) method based on the spin mapping formalism, which we refer to as the spin mapping NRPMD (SM-NRPMD) approach. We derive the path-integral partition function expression using the spin coherent state basis for the electronic states and the ring polymer formalism for the nuclear degrees of freedom. This partition function provides an efficient sampling of the quantum statistics. Using the basic properties of the Stratonovich-Weyl transformation, we further justify a Hamiltonian that we propose for the dynamical propagation of the coupled spin mapping variables and the nuclear ring polymer. The accuracy of the SM-NRPMD method is numerically demonstrated by computing the nuclear position and population auto-correlation functions of non-adiabatic model systems. The results obtained using the SM-NRPMD method agree very well with the numerically exact results. The main advantage of using the spin mapping variables over the harmonic oscillator mapping variables is numerically demonstrated, where the former provides nearly time-independent expectation values of physical observables for systems under thermal equilibrium. We also explicitly demonstrate that SM-NRPMD provides invariant dynamics upon various ways of partitioning the state-dependent and state-independent potentials.

General approach to state-dependent optical-tweezer traps for polar molecules

State-dependent optical tweezers can be used to trap a pair of molecules with a separation much smaller than the wavelength of the trapping light, greatly enhancing the dipole-dipole interaction between them. Here we describe a general approach to producing these state-dependent potentials using the tensor part of the ac Stark shift and show how it can be used to carry out two-qubit gates between pairs of molecules. The method is applicable to broad classes of molecules including bialkali molecules produced by atom association and those amenable to direct laser cooling.

A variational asymmetric phase-field model of quasi-brittle fracture: Energetic solutions and their computation.

We derive the variational formulation of a gradient damage model by applying the energetic formulation of rate-independent processes and obtain a regularized formulation of fracture. The model exhibits different behaviour at traction and compression and has a state-dependent dissipation potential which induces a path-independent work. We will show how such formulation provides the natural framework for setting up a consistent numerical scheme with the underlying variational structure and for the derivation of additional necessary conditions of global optimality in the form of a two-sided energetic inequality. These conditions will form our criteria for making a better choice of the starting guess in the application of the alternating minimization scheme to describe crack propagation as quasistatic evolution of global minimizers of the underlying incremental functional. We will apply the procedure for two- and three-dimensional benchmark problems and we will compare the results with the solution of the weak form of the Euler-Lagrange equations. We will observe that by including the two-sided energetic inequality in our solution method, we describe, for some of the benchmark problems, an equilibrium path when damage starts to manifest, which is different from the one obtained by solving simply the stationariety conditions of the underlying functional.

Enhancing Dipolar Interactions between Molecules Using State-Dependent Optical Tweezer Traps.

We show how state-dependent optical potentials can be used to trap a pair of molecules in different internal states at a separation much smaller than the wavelength of the trapping light. This close spacing greatly enhances the dipole-dipole interaction and we show how it can be used to implement two-qubit gates between molecules that are 100 times faster than existing protocols and than rotational coherence times already demonstrated. We analyze complications due to hyperfine structure, tensor light shifts, photon scattering, and collisional loss, and conclude that none is a barrier to implementing the scheme.

On the variational modeling of non-associative plasticity

In this work, the energetic formulation for rate-independent dissipative materials is extended to consider non-associative plasticity models. In associative models, the fulfilment of the principle of maximum dissipation naturally leads to a variational formulation of the evolution problem. This is no longer true for non-associative models, which are generally presented in the literature in a non-variational form. However, recent studies have unveiled the possibility to recover a variational structure in non-associative plasticity by relying on a suitable state-dependent dissipation potential. Here, this idea is further elaborated in the framework of the energetic formulation, providing a systematic variational approach to non-associative plasticity. A clear link between the classical governing equations of non-associative plasticity and the energetic formulation is established, for which a state-dependent dissipation potential is derived from a generalization of the principle of maximum dissipation. The proposed methodology is then applied to recast specific non-associative plasticity models in variational form, highlighting the flexibility of the formulation. The examples include a Drucker-Prager model with combined isotropic-kinematic hardening and a ratcheting plasticity model. Several thermomechanical insights are provided for both examples. Moreover, exploiting the flexibility of the energetic formulation, extensions to gradient plasticity are devised, leading to representative finite element simulations.

Vortices in Fermi gases with spin-dependent rotation potentials

The rotation of two-component Fermi gases and the subsequent appearance of vortices have been the subject of numerous experimental and theoretical studies. Recent experimental advances in hyperfine state-dependent potentials and highly degenerate heteronuclear Fermi gases suggest that it would be feasible to create component-dependent rotation potentials in future experiments. In this study we use an effective field theory for Fermi gases to consider the effects of rotating only one component of the Fermi gas. We find that the superfluid band gap in bulk exists up to higher rotation frequencies because the superfluid at rest, far away from the vortex, has to resist only half of the rotational effects. The vortex remains the energetically favorable state above a critical frequency but exhibits a larger core size.

Effect of an echo sequence to a trapped single-atom interferometer with photon momentum kicks.

We investigate a single-atom interferometer (SAI) in an optical dipole trap (ODT) with photon momentum kicks. An echo sequence is used for the SAI. We find experimentally that interference visibilities of a counter-propagating Raman type SAI decay much faster than the co-propagating case. To understand the underlying mechanism, a wave-packet propagating simulation is developed for the ODT-guided SAI. We show that in state dependent dipole potentials, the coupling between external dynamics and internal states makes the atom evolve in different paths during the interfering process. The acquired momentum from counter-propagating Raman pulses forces the external motional wave packets of two paths be completely separated and the interferometer visibility decays quickly compared to that of the co-propagating Raman pulses process. Meanwhile, the echo interference visibility experiences revival or instantaneous collapse which depends on the π pulse adding time at approximate integer multiples or half integer multiples of the trap period.

Sideband cooling of molecules in optical traps

Sideband cooling is a popular method for cooling atoms to the ground state of an optical trap. Applying the same method to molecules requires a number of challenges to be overcome. Strong tensor Stark shifts in molecules cause the optical trapping potential, and corresponding trap frequency, to depend strongly on rotational, hyperfine and Zeeman state. Consequently, transition frequencies depend on the motional quantum number and there are additional heating mechanisms, either of which can be fatal for an effective sideband cooling scheme. We develop the theory of sideband cooling in state-dependent potentials, and derive an expression for the heating due to photon scattering. We calculate the ac Stark shifts of molecular states in the presence of a magnetic field, and for any polarization. We show that the complexity of sideband cooling can be greatly reduced by applying a large magnetic field to eliminate electron- and nuclear-spin degrees of freedom from the problem. We consider how large the magnetic field needs to be, show that heating can be managed sufficiently well, and present a simple recipe for cooling to the ground state of motion.

Controlling the dynamical scale factor in a trapped atom Sagnac interferometer

Sagnac interferometers with massive particles promise unique advantages in achieving high precision measurements of rotation rates over their optical counterparts. Recent proposals and experiments are exploring non-ballistic Sagnac interferometers where trapped atoms are transported along a closed path. This is achieved by using superpositions of internal quantum states and their control with state-dependent potentials. We address emergent questions regarding the dynamical behavior of Bose-Einstein condensates in such an interferometer and its impact on rotation sensitivity. We investigate complex dependencies on atomic interactions as well as trap geometries, rotation rates, and speed of operation. We find that temporal transport profiles obtained from a simple optimization strategy for non-interacting particles remain surprisingly robust also in the presence of interactions over a large range of realistic parameters. High sensitivities can be achieved for short interrogation times far from the adiabatic regime. This highlights a route to building fast and robust guided ring Sagnac interferometers with fully trapped atoms.

Pulsed Quantum-State Reconstruction of Dark Systems.

We propose a novel strategy to reconstruct the quantum state of dark systems, i.e., degrees of freedom that are not directly accessible for measurement or control. Our scheme relies on the quantum control of a two-level probe that exerts a state-dependent potential on the dark system. Using a sequence of control pulses applied to the probe makes it possible to tailor the information one can obtain and, for example, allows us to reconstruct the density operator of a dark spin as well as the Wigner characteristic function of a harmonic oscillator. Because of the symmetry of the applied pulse sequence, this scheme is robust against slow noise on the probe. The proof-of-principle experiments are readily feasible in solid-state spins and trapped ions.

Self-oscillation excitation under condition of positive dissipation in a state-dependent potential well

The self-oscillatory dynamics is considered as motion of a particle in a potential field in the presence of dissipation. Described mechanism of self-oscillation excitation is not associated with peculiarities of a dissipation function, but results from properties of a potential, whose shape depends on a system state. Moreover, features of a potential function allow to realize the self-oscillation excitation in a case of the dissipation function being positive at each point of the phase space. The phenomenon is explored both numerically and experimentally on the example of a double-well oscillator with a state-dependent potential and dissipation. After that a simplified single-well model is studied.

Spontaneous spin squeezing in a rubidium BEC

We describe an experiment where spin squeezing occurs spontaneously within a standard Ramsey sequence driving a two-component Bose–Einstein condensate (BEC) of 87Rb atoms trapped in an elongated magnetic trap. The squeezing is generated by state-dependent collisional interactions, despite the near-identical scattering lengths of the spin states in 87Rb. In our proof-of-principle experiment, we observe a metrological spin squeezing that reaches 1.3 ± 0.4 dB for 5000 atoms, with a contrast of 90 ± 1%. The method may be applied to realize spin-squeezed BEC sources for atom interferometry without the need for cavities, state-dependent potentials or Feshbach resonances.

Dressed state dynamics of two-component Bose-Einstein Condensates in state-dependent potentials

Dressed potentials realized by coupling state-dependent bare potentials with external fields have important applications in trapping and manipulating atoms. Here, we study the dynamics of dressed states for coupled two-component Bose-Einstein condensates (BECs) in state-dependent potentials. Through both analytical and numerical methods, we find that the dressed state dynamics sensitively depend on both the inter-component coupling strength and the initial state. If the inter-component coupling is strong enough and the initial wave packet is located at the potential minimum, the dressed states can be decoupled and the Josephson oscillations and macroscopic quantum self-trapping appear. However, if the initial wave packet is located far away from the potential minimum, the wave packet will acquire a large kinetic energy and Landau-Zener transitiozs between the dressed states occur at the avoided-crossing point. Further, we give the validity ranges and conditions for the formation of adiabatic potentials, where the influences of Landau-Zener transitions can be ignored. Our results give an insight on how the inter-component coupling affects the dressed state dynamics and how to realize adiabatic potentials with BECs in state-dependent potentials.

Improving the lifetime in optical microtraps by using elliptically polarized dipole light

Tightly focused optical dipole traps induce vector light shifts ("fictitious magnetic fields") which complicate their use for single-atom trapping and manipulation. The problem can be mitigated by adding a larger, real magnetic field, but this solution is not always applicable; in particular, it precludes fast switching to a field-free configuration. Here we show that this issue can be addressed elegantly by deliberately adding a small elliptical polarization component to the dipole beam. In our experiments with single $^{87}$Rb atoms in a chopped trap, we observe improvements up to a factor 11 of the trap lifetime compared to the standard, seemingly ideal linear polarization. This effect results from a modification of heating processes via spin-state diffusion in state-dependent trapping potentials. We develop Monte-Carlo simulations of the evolution of the atom's internal and motional states and find that they agree quantitatively with the experimental data. The method is general and can be applied in all experiments where the longitudinal polarization component is non-negligible.

Coherent state mapping ring polymer molecular dynamics for non-adiabatic quantum propagations.

We introduce the coherent-state mapping ring polymer molecular dynamics (CS-RPMD), a new method that accurately describes electronic non-adiabatic dynamics with explicit nuclear quantization. This new approach is derived by using coherent-state mapping representation for the electronic degrees of freedom (DOF) and the ring-polymer path-integral representation for the nuclear DOF. The CS-RPMD Hamiltonian does not contain any inter-bead coupling term in the state-dependent potential and correctly describes electronic Rabi oscillations. A classical equation of motion is used to sample initial configurations and propagate the trajectories from the CS-RPMD Hamiltonian. At the time equivalent to zero, the quantum Boltzmann distribution (QBD) is recovered by reweighting the sampled distribution with an additional phase factor. In a special limit that there is one bead for mapping variables and multiple beads for nuclei, CS-RPMD satisfies detailed balance and preserves an approximate QBD. Numerical tests of this method with a two-state model system show very good agreement with exact quantum results over a broad range of electronic couplings.

Einstein-Podolsky-Rosen-entangled Bose-Einstein condensates in state-dependent potentials: A dynamical study

We study generation of non-local correlations by atomic interactions in a pair of bi-modal Bose-Einstein Condensates in state-dependent potentials including spatial dynamics. The wave-functions of the four components are described by combining a Fock state expansion with a time-dependent Hartree-Fock Ansatz, so that both the spatial dynamics and the local and non-local quantum correlations are accounted for. We find that despite the spatial dynamics, our protocole generates enough non-local entanglement to perform an EPR steering experiment with two spatially separated con-densates of a few thousands of atoms.

Microwave coherent manipulation of cold atoms in optically induced fictitious magnetic traps on an atom chip**Project supported by the National Key Research and Development Program of China (Grant No. 2016YFA0302800) and the National Natural Science Foundation of China (Grant No. 11674361).

We propose a novel on-chip platform for controlling and manipulating cold atoms precisely and coherently. The scheme is achieved by producing optically induced fictitious magnetic traps (OFMTs) with 790 nm (for 87Rb) circularly polarized laser beams and state-dependent potentials simultaneously for two internal atomic states with microwave coplanar waveguides. We carry out numerical calculations and simulations for controlled collisional interactions between OFMTs and addressable single atoms’ manipulation on our designed hybrid atom chips. The results show that our proposed platform is feasible and flexible, which has wide applications including collisional dynamics investigation, entanglement generation, and scalable quantum gates implementation.