Position-sensitive X-ray Detector Research Articles

Development of an X-ray imaging camera for targeted radionuclide therapy with astatine-211

The alpha-particle targeted radionuclide therapy (TRT) has been actively investigated for cancer treatment, and astatine-211 (211At) is one of the promising alpha-particle emitters. To evaluate the efficacy of radioactive pharmaceuticals, it is necessary to understand the 211At distribution in a body to accurately assess radiation dose in the targeted cells. In this study, an X-ray imaging camera was developed to investigate an in vivo211At imaging technique for the alpha-particle TRT, especially to apply for small animal investigations. The design of the X-ray imaging camera was optimized to measure Po K X-rays (77–92 keV) emitted during 211At decay. It comprised a monolithic NaI(Tl) scintillator, a position-sensitive photomultiplier, and a tungsten pinhole collimator. The intrinsic performance evaluation of the position-sensitive X-ray detector exhibited good energy resolution, spatial resolution, and response uniformity. Using point-like 211At sources, the 211At distribution was successfully obtained by the X-ray camera with a useful field-of-view of 20.4 × 20.4 mm2, a system spatial resolution of 1.6 mm, and a sensitivity of 2.4 × 10−4, equivalent to 101 cps/MBq, on the collimator axis at a 12.5 mm distance. This study demonstrated the imaging capability of 211At with high sensitivity and spatial resolution by the X-ray imaging camera with a pinhole collimator.

A wide-angle X-ray scattering laboratory setup for tracking phase changes of thin films in a chemical vapor deposition chamber.

The few-layer transition metal dichalcogenides (TMD) are an attractive class of materials due to their unique and tunable electronic, optical, and chemical properties, controlled by the layer number, crystal orientation, grain size, and morphology. One of the most commonly used methods for synthesizing the few-layer TMD materials is the chemical vapor deposition (CVD) technique. Therefore, it is crucial to develop in situ inspection techniques to observe the growth of the few-layer TMD materials directly in the CVD chamber environment. We demonstrate such an in situ observation on the growth of the vertically aligned few-layer MoS2 in a one-zone CVD chamber using a laboratory table-top grazing-incidence wide-angle X-ray scattering (GIWAXS) setup. The advantages of using a microfocus X-ray source with focusing Montel optics and a single-photon counting 2D X-ray detector are discussed. Due to the position-sensitive 2D X-ray detector, the orientation of MoS2 layers can be easily distinguished. The performance of the GIWAXS setup is further improved by suppressing the background scattering using a guarding slit, an appropriately placed beamstop, and He gas in the CVD reactor. The layer growth can be monitored by tracking the width of the MoS2 diffraction peak in real time. The temporal evolution of the crystallization kinetics can be satisfactorily described by the Avrami model, employing the normalized diffraction peak area. In this way, the activation energy of the particular chemical reaction occurring in the CVD chamber can be determined.

Observation of parametric X-ray radiation for the asymmetric Laue geometry

Angular distributions of parametric X-ray radiation from 255-MeV electrons in a thin Si crystal have been investigated for asymmetric Laue geometries using an imaging plate as a two-dimensional position-sensitive X-ray detector. The peak intensities of parametric X-ray radiation observed for (111) and (1¯1¯ 1) reflections, normalized by taking into account the effective target thickness and the transmission fraction of X-rays in the crystal, coincided within several percent. A large intensity difference depending on the asymmetry parameter, which is predicted by a dynamical theory dealing with the asymmetric Laue geometry, was not observed under the present experimental conditions. This indicates that the dependence of angular distributions of parametric X-ray radiation on the asymmetry parameter is negligibly weak, i.e., that it can be well explained by the well-established kinematical theory and dynamical theory as well as those for symmetric Laue and Bragg geometries.

Modelling of vignetting effects in full-field X-ray fluorescence imaging system based on pinhole optics

The full field X-ray fluorescence (FF-XRF) imaging is a technique capable of analysing the spatial distribution of elements in a sample. An alternative technique is the scanning macro-XRF method. Both techniques are powerful tools for non-destructive analysis of artworks mainly historical paintings. Technically, FF-XRF imaging is usually realised by coupling of a pinhole camera and a position sensitive and energy dispersive X-ray detector. The main advantages of the pinhole camera are its simplicity and infinite depth of field, however it introduces vignetting. For a visible light pinhole camera one distinguishes natural vignetting following the cos4 law and mechanical vignetting due to finite thickness of the camera. For an X-ray pinhole camera one has to take into account an additional component of vignetting due to absorption of X-rays in the air or other gas unless the setup is kept in vacuum. The goal of this study is to work out an analytical model of vignetting effects for a FF-XRF apparatus using an X-ray pinhole camera. Complete quantitative characterisation of the vignetting effects is a key step towards proper correction of the vignetting artefacts in recorded images. The elaborated analytical model has been applied to the images acquired with the FF-XRF apparatus being developed and an example of vignetting correction is presented.

Position-Sensitive Magnetic Calorimeters for Lynx

We describe the performance of position-sensitive metallic magnetic calorimeter X-ray detectors for potential future astrophysics missions, such as Lynx. The motivation behind this is to achieve a large focal plane area by increasing the number of pixels compared to the number of readout channels (called hydra). The detector consists of a $$5 \times 5$$ array of gold absorbers thermally coupled to a paramagnetic sensor. Since each absorber has a different thermal link to the sensor, it generates a different pulse shape and enables discrimination of pixel position. Recently, we have been successfully able to discriminate 25 averaged pulse shapes by means of rise-time and pulse height. The measured pulse shapes and distribution agree well with the modeling results. The estimated energy resolutions based on the pulse height and noise data we measured are 2.8–3.7 eV for $$\hbox {MnK}\alpha $$ X-ray photons at 50 mK.

X-ray diffraction methods for structural diagnostics of materials: progress and achievements

The development of X-ray diffractometry at the turn of the 21st century is presented. The review covers instrumentation development for structural studies based on the use of both standard continuously radiating X-ray generators and state-of-the-art sources of ultrashort and ultra-bright X-ray pulses. The latter technique enables investigation of the structural dynamics of condensed matter in a 4D space–time continuum with a resolution reaching a tenth of a femtosecond. New engineering approaches to enhancing the sensitivity, accuracy, and efficiency of X-ray diffraction experiments are discussed, including new and promising X-rays sources, reflective collimating and focusing X-ray optical devices, and fast low-noise and radiation-resistant position-sensitive X-ray detectors, as well as a new generation of X-ray diffractometers developed based on these elements. The presentation is focused on modern engineering solutions that enable academic and applied-research laboratories to perform X-ray diffraction studies on-site, which earlier were only feasible using synchrotron radiation sources at international resource sharing centers.

Time and position sensitive photon detector for coincidence measurements in the keV energy range.

The detection efficiency η of any particle detector is important, concerning acquisition time, but becomes even more critical when two particles are detected in coincidence, with a total efficiency η1η2, in order to allow a deeper understanding of complex processes induced by light or particle interaction with matter. Efficiency and resolution of a time and position sensitive x-ray detector are reported here. This system consists of a multilayer transmission photocathode and two micro-channel plates (MCPs) equipped with a delay line anode (DLA). The efficiency is found to be about 20% for Al Kα photons, while the spatial resolution is comparable to that of a standard DLA detector (about 100 μm). The fast response time of the detector combined with its efficiency should allow coincidence experiments between x-ray photons and other particles (electron, ions, etc.).

Investigations of fast processes by X-ray diffraction methods at the Siberian Synchrotron and Terahertz Radiation Center

A unique instrumentation complex that includes wigglers, X-ray position sensitive detectors, diffractometers, and explosion chambers and enables a 73 ps X-ray diffraction time resolution (exposure time) has been developed at the Siberian Synchrotron and Terahertz Radiation Center, a research collaboration operating at the Budker Institute of Nuclear Physics, Siberian Branch of the Russian Academy of Sciences. A number of techniques have been developed and implemented with which nanosecond-resolution investigations of the nucleation and growth dynamics became possible for the first time for diamond and metal nanoparticles under explosion and shock wave conditions. Studies with millisecond resolution of the structural transformation dynamics of chemical reactions, investigations of the kinetics of self-propagating high-temperature synthesis, and obtaining information on the state of catalysts are also among the new possibilities developed.

Single crystal CVD diamond membranes as Position Sensitive X-ray Detector

Transparent X-ray Beam Position Monitor (XBPM) has been specifically developed for low energy X-ray beamlines (1.4 keV < E < 5 keV) allowing to transmit more than 80% of 2 keV energy beam. The detector is based on a free-standing single crystal CVD diamond membrane of 4 μm thickness with position-sensitive DLC (Diamond-Like Carbon) resistive electrodes in duo-lateral configuration. The measured X-ray beam induced current (XBIC) due to the interaction of X-rays with diamond membrane allows precise monitoring of the absolute beam flux and the beam position (by the reconstruction of its center-of-gravity) at beam transmissions reaching 95%. This detector has been installed at SOLEIL synchrotron on the SIRIUS beamline monochromator output and it has shown charge collection efficiency (CCE) reaching 100% with no lag-effects and excellent beam intensity sensitivity monitoring. X-ray beam mapping of the detector showed an XBIC response inhomogeneity of less than 10% across the membrane, corresponding mainly to the measured variation of the diamond plate thickness. The measured beam position resolution is at sub-micron level depending on the beam flux and the readout electronics bandwidth.

Cadmium-Zinc-Telluride Imager On-Board Astrosat:A Multi-Faceted Hard X-Ray Instrument

The AstroSat satellite is designed to make multi-waveband observations of astronomical sources and the Cadmium Zinc Telluride Imager (CZTI) instrument of AstroSat covers the hard X-ray band. CZTI has a large area position sensitive hard X-ray detector equipped with a Coded Aperture Mask, thus enabling simultaneous background measurement. Ability to record simultaneous detection of ionizing interactions in multiple detector elements is a special feature of the instrument and this is exploited to provide polarization information in the 100 - 380 keV region. CZTI provides sensitive spectroscopic measurements in the 20 - 100 keV region, and acts as an all sky hard X-ray monitor and polarimeter above 100 keV. During the first year of operation, CZTI has recorded several gamma-ray bursts, measured the phase resolved hard X-ray polarization of the Crab pulsar, and the hard X-ray spectra of many bright Galactic X-ray binaries. The excellent timing capability of the instrument has been demonstrated with simultaneous observation of the Crab pulsar with radio telescopes like GMRT and Ooty radio telescope.

Chemical speciation using high energy resolution PIXE spectroscopy in the tender X-ray range

High energy resolution X-ray emission spectroscopy employing wavelength dispersive (WDS) crystal spectrometers can provide energy resolution on the level of core-hole lifetime broadening of the characteristic emission lines. While crystal spectrometers have been traditionally used in combination with electron excitation for major and minor element analysis, they have been rarely considered in proton induced X-ray emission (PIXE) trace element analysis mainly due to low detection efficiency. Compared to the simplest flat crystal WDS spectrometer the efficiency can be improved by employing cylindrically or even spherically curved crystals in combination with position sensitive X-ray detectors. When such spectrometer is coupled to MeV proton excitation, chemical bonding effects are revealed in the high energy resolution spectra yielding opportunity to extend the analytical capabilities of PIXE technique also towards chemical state analysis. In this contribution we will focus on the high energy resolution PIXE (HR-PIXE) spectroscopy in the tender X-ray range performed in our laboratory with our home-built tender X-ray emission spectrometer. Some general properties of high energy resolution PIXE spectroscopy in the tender X-ray range are presented followed by an example of sulfur speciation in biological tissue illustrating the capabilities as well as limitations of HR-PIXE method used for chemical speciation in the tender X-ray range.

Angular distributions of parametric X-ray radiation from a diamond crystal

Angular distributions of parametric X-ray radiation (PXR) from 255MeV electrons incident on a 50μm thick diamond crystal are presented. Almost all experiments on the angular distributions of PXR have been performed using Si crystals. The purpose of the present work is to extend this research to diamond crystals. An imaging plate was adopted as a two-dimensional position-sensitive X-ray detector, and high-quality PXR angular distribution data were successfully obtained. The measured PXR angular distributions were compared with those predicted theoretically and good agreement was obtained. The cause of the slight difference observed around the center position (Bragg direction) is also discussed.

Basic design of a multi wire proportional counter using Garfield++ for ILSF

The Iranian Light Source Facility (ILSF) is a new 3 GeV third generation synchrotron radiation facility in Middle East, which at the time being is in its design stage. An important aspect for the scientific success of this new source will be the availability of well adapted detectors. Position-sensitive X-ray detectors have played an important role in synchrotron radiation X-ray experiments for many years and are still in use. An operational one-dimensional multiwire position sensitive detector with delay line readout produced by ILSF showed a position resolution of 230 μm. In this paper, we introduce a 2-D position sensitive gas detector based on a multiwire proportional chamber which will be used in small/wide angle scattering and diffraction experiments with synchrotron radiation at the ILSF. The parameters of its components, including the gas filling, gas pressure, temperature, the geometry of anode and cathodes planes as well as the expected performance of the designed system will be described in the following. For the design and the simulation of MWPC the Elmer and Garfield++ codes have been employed. We have built and tested a MWPC as a prototype at ILSF. The results obtained so far show a good position sensing. After primary test the detector has been optimized and is now ready for test at Elettra.

Transmission-mode diamond X-ray position sensitive detector and its applications in synchrotron radiation beamlines

Transmission-mode diamond X-ray position sensitive detector and its applications in synchrotron radiation beamlines

Element Mapping in Organic Samples Utilizing a Benchtop X-Ray Fluorescence Emission Tomography (XFET) System.

X-ray fluorescence computed tomography (XFCT) is an emerging imaging modality that maps the three-dimensional distribution of elements, generally metals, in ex vivo specimens and potentially in living animals and humans. Building on our previous synchrotron-based work, we experimentally explored the use of a benchtop X-ray fluorescence computed tomography system for mapping trace-metal ions in biological samples. This system utilizes a scanning pencil-beam to stimulate the object and then relies on a detection system, with single or multiple slit apertures placed in front of position-sensitive X-ray detectors, to collect the fluorescence X-rays and to form 3-D elemental map without the need for tomographic imaging reconstruction. The technique was used to generate images of the elemental distributions of a triple-tube phantom and an osmium-stained zebrafish.

Combined linear polarization and angular distribution measurements of x-rays for precise determination of multipole-mixing in characteristic transitions of high-Z systems

By applying novel-type position sensitive x-ray detectors as Compton polarimeters we recently performed a study of the linear polarization of Lyman- radiation following radiative electron capture into initially bare uranium ions. It was found that a model-independent determination of the ratio of the E1 and M2 transition amplitudes, and consequently of the corresponding transition rates, is feasible by combining the linear polarization data with a measurement of the angular distribution of the emitted radiation. In this work a detailed description of the underlying experimental technique for combined measurements of the linear polarization and the angular distribution of characteristic transitions in high-Z ions is presented. Special emphasis is given to the application of two, two-dimensional position-sensitive x-ray detectors for Compton polarimetry of hard x-rays. Moreover, we demonstrate the polarimeter efficiency of such detector systems can be significantly improved if events, where the charge is spread over neighboring segments, are reconstructed to be used in the polarization analysis.

Position sensitive and energy dispersive x-ray detector based on silicon strip detector technology

A new position sensitive detector with a global energy resolution for the entire detector of about 380 eV FWHM for 8.04 keV line at ambient temperature is presented. The measured global energy resolution is defined by the energy spectra summed over all strips of the detector, and thus it includes electronic noise of the front-end electronics, charge sharing effects, matching of parameters across the channels and other system noise sources. The target energy resolution has been achieved by segmentation of the strips to reduce their capacitance and by careful optimization of the front-end electronics. The key design aspects and parameters of the detector are discussed briefly in the paper. Excellent noise and matching performance of the readout ASIC and negligible system noise allow us to operate the detector with a discrimination threshold as low as 1 keV and to measure fluorescence radiation lines of light elements, down to Al Kα of 1.49 keV, simultaneously with measurements of the diffraction patterns. The measurement results that demonstrate the spectrometric and count rate performance of the developed detector are presented and discussed in the paper.

Compton polarimetry using double-sided segmented x-ray detectors

Hard x-ray polarimetry of radiation emitted in collisions of heavy ions, electrons or photons with matter provides detailed information on the collision dynamics as well as of the atomic structure in the presence of extreme field strengths. Moreover, it also opens a route for polarization diagnosis of spin-polarized ion and electron beams which, for example, might be useful in future parity non-conservation studies. Owing to recent progress in the development of highly segmented solid-state detectors, a novel type of polarimeter for the hard x-ray regime has become available. Applied as Compton polarimeters, two-dimensional position-sensitive x-ray detectors now allow for precise and efficient measurements of x-ray linear polarization properties. In this report recent polarimetry studies using such detector systems are reviewed.

Position-sensitive soft X-ray detectors and their application

The designs and characteristics of linear and curved position-sensitive gas-filled detectors of soft X rays are described. The best result obtained with a gas mixture based on xenon is near 40 μm (CuKα). The information of their use in X-ray scientific equipment is presented.

Development and optimization of the production technology of large-size position-sensitive detectors

Results of development and optimization of the production technology of large-size semiconductor position-sensitive X-ray detectors, based on Si(Li)-p-i-n structures and intended for tomographic and environmental problems, are described. The detectors with a 50 × 50 × 2-mm-size sensitive area with 8, 16, and 32 strips were produced. With a voltage of 100–500 V, the energy resolution is 50 and 75–80 keV for electrons with an energy of 1 MeV and for α particles with an energy of 7.65 MeV, respectively, when the dark current is 0.5–1 μA, the capacitance value is 300 pF, and noise is 40 keV.