Photonic Modes Research Articles

Probing PT-Symmetry Breaking of Non-Hermitian Topological Photonic States via Strong Photon-Magnon Coupling.

Light-matter interaction is crucial to both understanding fundamental phenomena and developing versatile applications. Strong coupling, robustness, and controllability are the three most important aspects in realizing light-matter interactions. Topological and non-Hermitian photonics have provided frameworks for robustness and control flexibility, respectively. How to engineer the properties of the edge state such as photonic density of state by using non-Hermiticity while ensuring topological protection has not been fully studied. Here we construct a parity-time-symmetric dimerized photonic lattice and probe the spontaneous PT-symmetry breaking of the edge states by utilizing the strong coupling between the photonic mode and a spin ensemble. Our Letter presents an accurate and almost noninvasive approach for investigating non-Hermitian topological states, while also offering methodologies for the implementation and manipulation of topological light-matter interactions.

Probing Purcell enhancement and photon collection efficiency of InAs quantum dots at nodes of the cavity electric field

The interaction of excitonic transitions with confined photonic modes enables tests of quantum physics and design of efficient optoelectronic devices. Here we study how key metrics such as Purcell factor, factor, and collection efficiency are determined by the non-cavity modes that exist in real devices, taking the well-studied micropillar cavity as an example. Samples with dots at different positions in the cavity field allow us to quantify the effect of the non-cavity modes and show that the zero-phonon line and the phonon-assisted emission into the cavity mode HE11 is suppressed by positioning dots at the field node. Published by the American Physical Society 2024

Photonic Molecule Approach to Multiorbital Topology.

The concepts of topology provide a powerful tool to tailor the propagation and localization of the waves. While electrons have only two available spin states, engineered degeneracies of photonic modes provide novel opportunities resembling spin degrees of freedom in condensed matter. Here, we tailor such degeneracies for the array of femtosecond laser written waveguides in the optical range exploiting the idea of photonic molecules: clusters of strongly coupled waveguides. In our experiments, we observe unconventional topological modes protected by the Z3 invariant arising due to the interplay of interorbital coupling and geometric dimerization mechanism. We track multiple topological transitions in the system with the change in the lattice spacings and excitation wavelength. This strategy opens an avenue for designing novel types of photonic topological phases and states.

Nonreciprocal Dissipation Engineering via Strong Coupling with a Continuum of Modes

Optical nonreciprocity plays a key role in almost every optical system, directing light flow and protecting optical components from backscattered light. Controllable forms of on-chip nonreciprocity are needed for the robust operation of increasingly sophisticated photonic integrated circuits (PICs) in the context of classical and quantum computation, networking, communications, and sensing. However, it has been challenging to achieve wideband, low-loss optical nonreciprocity on-chip. In this paper, we demonstrate strong coupling and Rabi-like energy exchange between photonic bands, possessing a continuum of modes, to unlock nonreciprocity and frequency translation over wide optical bandwidths in silicon. Using a traveling-wave phonon field to drive indirect interband photonic transitions, we demonstrate band hybridization that enables an intriguing form of nonreciprocal dissipation engineering. Using the converted mode to create a nonreciprocal dissipation channel, we demonstrate a frequency-neutral, low-loss (less than 1 dB) isolator with high nonreciprocal contrast (more than 14 dB) and broad operating bandwidth (more than 59 GHz). Additionally, through the implementation of complete interband conversion, we demonstrate a high extinction (more than 55 dB) optical frequency translation operation with near-unity efficiency. Published by the American Physical Society 2024

Strong light–matter interactions based on excitons and the abnormal all-dielectric anapole mode with both large field enhancement and low loss

The room temperature strong coupling between the photonic modes of micro/nanocavities and quantum emitters (QEs) can bring about promising advantages for fundamental and applied physics. Improving the electric fields (EFs) by using plasmonic modes and reducing their losses by applying dielectric nanocavities are widely employed approaches to achieve room temperature strong coupling. However, ideal photonic modes with both large EFs and low loss have been lacking. Herein, we propose the abnormal anapole mode (AAM), showing both a strong EF enhancement of ∼70-fold (comparable to plasmonic modes) and a low loss of 34 meV, which is much smaller than previous records of isolated all-dielectric nanocavities. Besides realizing strong coupling, we further show that by replacing the normal anapole mode with the AAM, the lasing threshold of the AAM-coupled QEs can be reduced by one order of magnitude, implying a vital step toward on-chip integration of nanophotonic devices.

Two-dimensional thin film lithium niobate photonic crystal waveguide for integrated photonic chips

The photonic crystal waveguide (PCW) possesses remarkable capabilities in manipulating light beams and light–matter interactions within the subwavelength range. This property renders it a highly promising structure for the miniaturization of optical devices. We delve into the mode characteristics in two-dimensional PCWs on thin film lithium niobate, establish the correlation between the single-mode region in the PCW and its photonic crystal duty cycle, and observe mode hybridization in the waveguide. A lithium niobate PCW with sidewall angles can realize single-mode transmission or mode conversion by adjusting the width of its defective waveguides, and it is theoretically and experimentally verified that a change in the width of the waveguide shifts the operating wavelength. The results of the mode analysis are useful in the design of waveguide structures for photonic crystal-based electro-optical modulators and optical sensors.

Non-Hermitian topology and criticality in photonic arrays with engineered losses

Integrated photonic systems provide a flexible platform where artificial lattices can be engineered in a reconfigurable fashion. Here, we show that one-dimensional photonic arrays with engineered losses allow the realization of topological excitations stemming from non-Hermiticity and bulk mode criticality. We show that a generalized modulation of the local photonic losses allows the creation of topological modes both in the presence of periodicity and even in the quasiperiodic regime. We demonstrate that a localization transition of all the bulk photonic modes can be engineered in the presence of a quasiperiodic loss modulation, and we further demonstrate that such a transition can be created in the presence of both resonance frequency modulation and loss modulation. We finally address the robustness of this phenomenology to the presence of next to the nearest neighbor couplings and disorder in the emergence of criticality and topological modes. Our results put forward a strategy to engineer topology and criticality solely from engineered losses in a photonic system, establishing a potential platform to study the impact of nonlinearities in topological and critical photonic matter. Published by the American Physical Society 2024

Broadband Beam-Scanning Phased Array Based on Microwave Photonics

A one-dimensional active broadband phased array based on microwave photonics that works in the Ku band is proposed to achieve a large instantaneous bandwidth. The phased array uses a feeding network based on microwave photonics to provide the true time delay and a wide operating bandwidth. The array is mainly composed of a broadband horn antenna, an RF transmitting/receiving module, an optical network module, and a temperature control module. The form of a horn was selected for the antenna unit, and it was fed through a waveguide to obtain a wide operating bandwidth. An optical fiber delay line that could realize the true time delay at different frequencies was adopted for the time-delay module of the optical network. To obtain a large time delay and small quantization error, a hybrid time-delay diagram utilizing electrical and optical time delays was used in the design. In addition, a temperature control module was added to the antenna system to enhance the stability of the photonic time-delay module. For verification, a prototype of the presented antenna system was designed, fabricated, and measured. The experimental results showed that the optical phased array antenna was able to scan ±20° from 12 GHz to 17 GHz, and the beam pointing did not appear to be offset over the wide operating bandwidth.

Rapid Switching of a C-Series Linear Accelerator Between Conventional and Ultrahigh-Dose-Rate Research Mode With Beamline Modifications and Output Stabilization

PurposeIn this study, a decommissioned C-series linear accelerator (linac) was configured to enable rapid and reliable conversion between the production of conventional electron beams and an Ultrahigh-dose-rate (UHDR) electron beamline to the treatment room isocenter for FLASH radiation therapy. Efforts to tune the beam resulted in a consistent, stable UHDR beamline. Methods and MaterialsThe linac was configured to allow for efficient switching between conventional and modified electron output modes within two minutes. Additions to the air system allow for retraction of the X-ray target from the beamline when the 10MV photon mode is selected. With the carousel set to an empty port, this grants access to the higher current pristine electron beam normally used to produce clinical photon fields. Monitoring signals related to the automatic frequency control (AFC) system allows for tuning of the waveguide while the machine is in a hold state so a stable beam is produced from the initial pulse. A pulse counting system implemented on a FPGA-based controller platform controls the delivery to a desired number of pulses. Beam profiles were measured with Gafchromic film. Pulse-by-pulse dosimetry was measured using a custom electrometer designed around the EdgeTM diode. ResultsThis method reliably produces a stable UHDR electron beam. Open field measurements of the 16cm (FWHM) gaussian beam saw average dose rates of 432Gy/s at treatment isocenter. Pulse overshoots were limited and ramp up was eliminated. Over the last year, there have been no recorded incidents that resulted in machine downtime due to the UHDR conversions. ConclusionStable 10MeV UHDR beams were generated to produce an average dose rate of 432Gy/s at the treatment room isocenter. With a reliable pulse-counting beam control system, consistent doses can be delivered for FLASH experiments with the ability to accommodate a wide range of field sizes, source-to-surface distances, and other experimental apparatus that may be relevant for future clinical translation.

Controlling Molecular Photoisomerization in Photonic Cavities through Polariton Funneling.

Strong coupling between photonic modes and molecular electronic excitations, creating hybrid light-matter states called polaritons, is an attractive avenue for controlling chemical reactions. Nevertheless, experimental demonstrations of polariton-modified chemical reactions remain sparse. Here, we demonstrate modified photoisomerization kinetics of merocyanine and diarylethene by coupling the reactant's optical transition with photonic microcavity modes. We leverage broadband Fourier-plane optical microscopy to noninvasively and rapidly monitor photoisomerization within microcavities, enabling systematic investigation of chemical kinetics for different cavity-exciton detunings and photoexcitation conditions. We demonstrate three distinct effects of cavity coupling: first, a renormalization of the photonic density of states, akin to a Purcell effect, leads to enhanced absorption and isomerization rates at certain wavelengths, notably red-shifting the onset of photoisomerization. This effect is present under both strong and weak light-matter couplings. Second, kinetic competition between polariton localization into reactive molecular states and cavity losses leads to a suppression of the photoisomerization yield. Finally, our key result is that in reaction mixtures with multiple reactant isomers, exhibiting partially overlapping optical transitions and distinct isomerization pathways, the cavity resonance can be tuned to funnel photoexcitations into specific reactant isomers. Thus, upon decoherence, polaritons localize into a chosen isomer, selectively triggering the latter's photoisomerization despite initially being delocalized across all isomers. This result suggests that careful tuning of the cavity resonance is a promising avenue to steer chemical reactions and enhance product selectivity in reaction mixtures.

Kinetic theory formulation of the P - and CP -odd terms in the photon self-energy in a medium

In an optically active medium, such as a plasma that contains a neutrino background, the left-handed and right-handed polarization photon modes acquire different dispersion relations. We study the propagation of photons in such a medium, which is otherwise isotropic, within the framework of the covariant collissionless Boltzmann equation incorporating a term that parametrizes the optical activity. Using the linear response approximation, we obtain the formulas for the components of the photon polarization tensor, expressed in terms of integrals over the momentum distribution function of the background particles. The main result here is the formula for the P- and CP-breaking component of the photon polarization tensor in terms of the parameter involved in the new term we consider in the Boltzmann equation to describe the effects of optical activity. We discuss the results for some particular cases, such as long-wavelength and nonrelativistic limits, for illustrative purposes. We also discuss the generalizations of the P- and CP-breaking term we included in the Boltzmann equation. In particular we consider the application to a plasma with a neutrino background and establish contact with calculations of the photon self-energy in those systems in the framework of thermal field theory. Published by the American Physical Society 2024

Microscopic nonlinear optical activities and ultrafast carrier dynamics in layered AgInP2S6

Since the emergence of graphene, transition metal dichalcogenides, and black phosphorus, two-dimensional materials have attracted significant attention and have driven the development of fundamental physics and optoelectronic devices. Metal phosphorus trichalcogenides (MPX3), due to their large bandgap of 1.3–3.5 eV, enable the extension of optoelectronic applications to visible and ultraviolet (UV) wavelengths. Micro-Z/I-scan (μ-Z/I-scan) and micro-pump-probe (μ-pump-probe) setups were used to systematically investigate the third-order nonlinear optical properties and ultrafast carrier dynamics of the representative material AgInP2S6. UV-visible absorption spectra and density functional theory (DFT) calculations revealed a quantum confinement effect, in which the bandgap decreased with increasing thickness. The two-photon absorption (TPA) effect is exhibited under the excitation of both 520 and 1040 nm femtosecond pulses, where the TPA coefficient decreases as the AgInP2S6 thickness increases. In contrast, the TPA saturation intensity exhibits the opposite behavior that the TPA saturation is more likely to occur under visible excitation. After the valence band electrons undergo photon transitions to the conduction band, the non-equilibrium carriers relax through non-radiative and defect-assisted recombination. These findings provide a comprehensive understanding of the optical response process of AgInP2S6 and are a valuable reference for the development of optoelectronic devices.

Enhanced optical nonlinearity of epsilon-near-zero metasurface by quasi-bound state in the continuum

Bound states in the continuum (BICs) provide a powerful way to enhance the nonlinear properties of materials, epsilon-near-zero (ENZ) materials are considered as promising candidates with strong nonlinearities. However, the realization of BIC based on ENZ materials in the near-infrared (NIR) is very challenging due to the large loss in the NIR. Here, a high-quality quasi-BIC based on the ENZ metasurface is proposed for the first time, which is composed of patterned ENZ films embedded in a dielectric-metal hybrid structure, and realizes destructive interference between the Berreman mode and photonic mode to form the Friedrich-Wintergen BIC (FW-BIC). The electric field is strongly confined in the ENZ film, resulting in considerable field enhancement, and the nonlinear refractive index coefficient is 1.63 × 10−12 m2/W, which is three orders of magnitude larger than that of the ITO film. The instantaneous response time is 600 fs and extremely high modulation speed up to the THz level. Benefiting from the perfect absorption and narrow linewidth of quasi-BIC and the change in refractive index of the metasurface induced by Kerr nonlinearity, the absolute modulation is from near-zero to 92% with an extinction ratio of 23.2 dB. It provides a promising platform for the development of integrated ultrafast high-speed photonics.

Two-photon coherence in a DROP-FWM medium

In this work, we report experimental studies on coherence in a medium exhibiting DROP (Double Resonance Optical Pumping)-FWM (Four Wave Mixing). Here 5S1/2(F) → 5P3/2(F/) → 5D (F//) two photon transition of hot 87Rb atoms is used. The 5S→5P connection is modified by introducing an additional beam phase coupled to the original beam linking F = 2 → F/ transition. The frequency of the additional beam is offset from that of the original beam by ≈ +10Γ (Γ is natural linewidth). Such a two-beam configuration in F→F/ manifold effectively satisfies conditions of Vee (V) linkage or degenerate two-level connection (DTLC), depending on the detuning of the 780nm laser. This transformation profoundly affects the behavior of the ensuing Ladder (Ξ) system. While the (I) Ξ +V condition is favorable for Electromagnetically Induced Transparency (EIT), the (ii) Ξ + DTLC brings in the effect of Electromagnetically Induced Absorption (EIA). The EIT-dominated situation is helpful for FWM to take place, and the EIA effect augments the stronger presence of DROP. This condition is verified by monitoring the blue fluorescence emanating from the 5D→6P3/2→5S1/2 decay route. The DROP effect follows the Amplified Spontaneous Emission (ASE) pattern in the media. The origin of blue photons is also due to FWM under EIT conditions. In the case of EIA, the dominant condition increment in blue fluorescence is due to increased stimulated emission. The blue photons mainly contributed by (i) FWM and (ii) increased participation of stimulated emission are directional in nature and phase coherent.

Hermitian and non-Hermitian topology from photon-mediated interactions

As light can mediate interactions between atoms in a photonic environment, engineering it for endowing the photon-mediated Hamiltonian with desired features, like robustness against disorder, is crucial in quantum research. We provide general theorems on the topology of photon-mediated interactions in terms of both Hermitian and non-Hermitian topological invariants, unveiling the phenomena of topological preservation and reversal, and revealing a system-bath topological correspondence. Depending on the Hermiticity of the environment and the parity of the spatial dimension, the atomic and photonic topological invariants turn out to be equal or opposite. Consequently, the emergence of atomic and photonic topological boundary modes with opposite group velocities in two-dimensional Hermitian topological systems is established. Owing to its general applicability, our results can guide the design of topological systems.

The use of NADH anisotropy to investigate mitochondrial cristae alignment

Life may be expressed as the flow of electrons, protons, and other ions, resulting in large potential difference. It is also highly photo-sensitive, as a large proportion of the redox capable molecules it relies on are chromophoric. It is thus suggestive that a key organelle in eukaryotes, the mitochondrion, constantly adapt their morphology as part of the homeostatic process. Studying unstained in vivo nano-scale structure in live cells is technically very challenging. One option is to study a central electron carrier in metabolism, reduced nicotinamide adenine dinucleotide (NADH), which is fluorescent and mostly located within mitochondria. Using one and two-photon absorption (340–360 nm and 730 nm, respectively), fluorescence lifetime imaging and anisotropy spectroscopy of NADH in solution and in live cells, we show that mitochondria do indeed appear to be aligned and exhibit high anisotropy (asymmetric directionality). Aqueous solution of NADH showed an anisotropy of ~ 0.20 compared to fluorescein or coumarin of < 0.1 and 0.04 in water respectively and as expected for small organic molecules. The anisotropy of NADH also increased further to 0.30 in the presence of proteins and 0.42 in glycerol (restricted environment) following two-photon excitation, suggesting more ordered structures. Two-photon NADH fluorescence imaging of Michigan Cancer Foundation-7 (MCF7) also showed strong anisotropy of 0.25 to 0.45. NADH has a quantum yield of fluorescence of 2% compared to more than 40% for photoionisation (electron generation), when exposed to light at 360 nm and below. The consequence of such highly ordered and directional NADH patterns with respect to electron ejection upon ultra-violet (UV) excitation could be very informative—especially in relation to ascertaining the extent of quantum effects in biology, including electron and photonic cascade, communication and modulation of effects such as spin and tunnelling.

Lindblad Master Equation Capable of Describing Hybrid Quantum Systems in the Ultrastrong Coupling Regime.

Despite significant theoretical efforts devoted to studying the interaction between quantized light modes and matter, the so-called ultrastrong coupling regime still presents significant challenges for theoretical treatments and prevents the use of many common approximations. Here we demonstrate an approach that can describe the dynamics of hybrid quantum systems in any regime of interaction for an arbitrary electromagnetic (EM) environment. We extend a previous method developed for few-mode quantization of arbitrary systems to the case of ultrastrong light-matter coupling, and show that even such systems can be treated using a Lindblad master equation where decay operators act only on the photonic modes by ensuring that the effective spectral density of the EM environment is sufficiently suppressed at negative frequencies. We demonstrate the validity of our framework and show that it outperforms current state-of-the-art master equations for a simple model system, and then study a realistic nanoplasmonic setup where existing approaches cannot be applied.

Cavity-modified molecular dipole switching dynamics.

Polaritonic states, which are formed by resonances between a molecular excitation and the photonic mode of a cavity, have a number of useful properties that offer new routes to control molecular photochemistry using electric fields. To provide a theoretical description of how polaritonic states affect the real-time electron dynamics in molecules, a new method is described where the effects of strong light-molecule coupling are implemented using real-time electronic structure theory. The coupling between the molecular electronic states and the cavity is described by the Pauli-Fierz Hamiltonian, and transitions between polaritonic states are induced via an external time-dependent electric field using time-dependent configuration interaction (TDCI) theory, producing quantum electrodynamics TDCI (QED-TDCI). This method is used to study laser-induced ultrafast charge transfer and dipole-switching dynamics of the LiCN molecule inside a cavity. The increase in cavity coupling strength is found to have a significant impact on the energies and transition dipole moments of the molecule-cavity system. The convergence of the polaritonic state energies as a function of the number of included electronic and photonic basis states is discussed.

Design of ultra-low noise amplifier for quantum applications (QLNA)

The present article primarily focuses on the design of an ultra-low-noise amplifier specifically tailored for quantum applications. The circuit design places a significant emphasis on improving the noise figure, as quantum-associated applications require the circuit's noise temperature to be around 0.4 K. This requirement aims to achieve performance comparable to the Josephson Junction amplifier. Although this task presents considerable challenges, the work concentrates on engineering the circuit to minimize mismatch and reflection coefficients, while simultaneously enhancing circuit transconductance. These efforts aim to improve the noise figure as efficiently as possible. The results of this study indicate the possibility of achieving a noise figure of approximately 0.009 dB for a unique circuit design operating at 10 K. In a departure from traditional approaches, this study employs quantum mechanical theory to analyze the circuit comprehensively. By employing quantum theory, the researchers derive relationships that highlight the crucial quantities upon which the circuit design should focus to optimize the noise figure. For example, the circuit's gain power, which depends on the circuit's photonic modes, is theoretically derived and found to affect the noise figure directly. Ultimately, by merging quantum theory with engineering approaches, this study successfully designs a highly efficient circuit that significantly minimizes the noise figure in a quantum application setting.

Continuous wave terahertz detection using 1550nm pumped nonlinear photoconductive GaAs metasurfaces.

Terahertz (THz) continuous wave (CW) spectroscopy systems can offer extremely high spectral resolution over the THz band by photo-mixing high-performance telecommunications-band (1530-1565 nm) lasers. However, typical THz CW detectors in these systems use narrow band-gap photoconductors, which require elaborate material growth and generate relatively large detector noise. Here we demonstrate that two-step photon absorption in a nano-structured low-temperature grown GaAs (LT-GaAs) metasurface which enables switching of photoconductivity within approximately one picosecond. We show that LT-GaAs can be used as an ultrafast photoconductor in CW THz detectors despite having a bandgap twice as large as the telecommunications laser photon energy. The metasurface design harnesses Mie modes in LT GaAs resonators, whereas metallic electrodes of THz detectors can be designed to support an additional photonic mode, which further increases photoconductivity at a desired wavelength.