Two-photon coherence in a DROP-FWM medium

Abstract

In this work, we report experimental studies on coherence in a medium exhibiting DROP (Double Resonance Optical Pumping)-FWM (Four Wave Mixing). Here 5S1/2(F) → 5P3/2(F/) → 5D (F//) two photon transition of hot 87Rb atoms is used. The 5S→5P connection is modified by introducing an additional beam phase coupled to the original beam linking F = 2 → F/ transition. The frequency of the additional beam is offset from that of the original beam by ≈ +10Γ (Γ is natural linewidth). Such a two-beam configuration in F→F/ manifold effectively satisfies conditions of Vee (V) linkage or degenerate two-level connection (DTLC), depending on the detuning of the 780nm laser. This transformation profoundly affects the behavior of the ensuing Ladder (Ξ) system. While the (I) Ξ +V condition is favorable for Electromagnetically Induced Transparency (EIT), the (ii) Ξ + DTLC brings in the effect of Electromagnetically Induced Absorption (EIA). The EIT-dominated situation is helpful for FWM to take place, and the EIA effect augments the stronger presence of DROP. This condition is verified by monitoring the blue fluorescence emanating from the 5D→6P3/2→5S1/2 decay route. The DROP effect follows the Amplified Spontaneous Emission (ASE) pattern in the media. The origin of blue photons is also due to FWM under EIT conditions. In the case of EIA, the dominant condition increment in blue fluorescence is due to increased stimulated emission. The blue photons mainly contributed by (i) FWM and (ii) increased participation of stimulated emission are directional in nature and phase coherent.