The aim of this paper is to present analytical and exact expressions for the frequency and buckling of large amplitude vibration of the symmetrical laminated composite beam (LCB) with simple and clamped end conditions. The equations of motion are derived by using Hamilton′s principle. The influences of axial force, Poisson effect, shear deformation, and rotary inertia are taken into account in the formulation. First, the geometric nonlinearity based on the von Karman′s assumptions is incorporated in the formulation while retaining the linear behavior for the material. Then, the displacement fields used for the analysis are coupled using the equilibrium equations of the composite beam. Substituting this coupled displacement fields in the potential and kinetic energies and using harmonic balance method, we obtain the ordinary differential equation in time domain. Finally, applying first order of homotopy analysis method (HAM), we get the closed form solutions for the natural frequency and deflection of the LCB. A detailed numerical study is carried out to highlight the influences of amplitude of vibration, shear deformation and rotary inertia, slenderness ratios, and layup in the case of laminates on the natural frequency and buckling load.