Gold Cone Research Articles

Optimizing design of irradiation uniformity of direct drive cone-in-shell target for fast ignition

The irradiation uniformity of a cone-in-shell target directly driven by laser beams has been considered. First, a model is established to include the influence of the cone on laser beam propagation. Then, the irradiation uniformity on the target surface outside the cone during the initial imprinting phase is analyzed, and highly uniform irradiation on the target surface outside the cone is achieved by optimizing the intensity distribution within laser beams, as well as the polar direct drive displacement. As an illustrative example, direct drive irradiation uniformity of a typical cone-in-shell target is improved for Shenguang III laser facility, the illumination non-uniformity is reduced from 5.8% to 1.1%. Irradiation on the cone surface outside the target is also analyzed, and it is found that for the laser-target configuration considered in this work, a gold cone thicker than 50μm is needed to avoid shock breakout. Moreover, sensitivity to beam uncertainties (power imbalance and pointing error) is analyzed, indicating that this scheme can tolerate a certain amount of beam errors.

Enhanced electron trapping and γ ray emission by ultra-intense laser irradiating a near-critical-density plasma filled gold cone

The radiation trapping effect (RTE) of electrons in the interaction of an ultra-intense laser and a near-critical-density plasma-filled gold cone is numerically investigated by using the particle-in-cell code EPOCH. It is found that, by using the cone, the threshold laser intensity for electron trapping can be significantly decreased. The trapped electrons located behind the laser front and confined near the laser axis oscillate significantly in the transverse direction and emit high-energy photons in the forward direction. With parameters optimized, a narrow photon angular distribution and a high-energy conversion efficiency from the laser to the photons can be obtained. The proposed scheme may offer possibilities to demonstrate the RTE of electrons in experiments at approachable laser intensities and serve as a novel table-top ray source.

Surface plasmon hurdles leading to a strongly localized giant field enhancement on two-dimensional (2D) metallic diffraction gratings.

An extensive numerical study of diffraction of a plane monochromatic wave by a single gold cone on a plane gold substrate and by a periodical array of such cones shows formation of curls in the map of the Poynting vector. They result from the interference between the incident wave, the wave reflected by the substrate, and the field scattered by the cone(s). In case of a single cone, when going away from its base along the surface, the main contribution in the scattered field is given by the plasmon surface wave (PSW) excited on the surface. As expected, it has a predominant direction of propagation, determined by the incident wave polarization. Two particular cones with height approximately 1/6 and 1/3 of the wavelength are studied in detail, as they present the strongest absorption and field enhancement when arranged in a periodic array. While the PSW excited by the smaller single cone shows an energy flux globally directed along the substrate surface, we show that curls of the Poynting vector generated with the larger cone touch the diopter surface. At this point, their direction is opposite to the energy flow of the PSW, which is then forced to jump over the vortex regions. Arranging the cones in a two-dimensional subwavelength periodic array (diffraction grating), supporting a specular reflected order only, resonantly strengthens the field intensity at the tip of cones and leads to a field intensity enhancement of the order of 10 000 with respect to the incident wave intensity. The enhanced field is strongly localized on the rounded top of the cones. It is accompanied by a total absorption of the incident light exhibiting large angular tolerances. This strongly localized giant field enhancement can be of much interest in many applications, including fluorescence spectroscopy, label-free biosensing, surface-enhanced Raman scattering (SERS), nonlinear optical effects and photovoltaics.

3D integration technology for sensor application using less than 5μm-pitch gold cone-bump connpdfection

Three-dimensional (3D) integrated circuit (IC) technology is an effective solution to reduce the manufacturing costs of advanced two-dimensional (2D) large-scale integration (LSI) while ensuring equivalent device performance and functionalities. This technology allows a new device architecture using stacked detector/sensor devices with a small dead sensor area and high-speed operation that facilitates hyper-parallel data processing. In pixel detectors or focal-plane sensor devices, each pixel area must accommodate many transistors without increasing the pixel size. Consequently, many methods to realize 3D-LSI devices have been developed to meet this requirement by focusing on the unit processes of 3D-IC technology, such as through-silicon via formation and electrical and mechanical bonding between tiers of the stack. The bonding process consists of several unit processes such as bump or metal contact formation, chip/wafer alignment, chip/wafer bonding, and underfill formation; many process combinations have been reported. Our research focuses on a versatile bonding technology for silicon LSI, compound semiconductor, and microelectromechanical system devices at temperatures of less than 200̂C for heterogeneous integration. A gold (Au) cone bump formed by nanoparticle deposition is one of the promising candidates for this purpose. This paper presents the experimental result of a fabricated prototype with 3-μm-diameter Au cone-bump connections with adhesive injection, and compares it with that of an indium microbump (μ-bump). The resistance of the 3-μm-diameter Au cone bump is approximately 6 Ω. We also investigated the influence of stress caused by the bump junction on the MOS characteristics.

High-energy-density electron jet generation from an opening gold cone filled with near-critical-density plasma

By using two-dimensional particle-in-cell simulations, we propose a scheme for strong coupling of a petawatt laser with an opening gold cone filled with near-critical-density plasmas. When relevant parameters are properly chosen, most laser energy can be fully deposited inside the cone with only 10% leaving the tip opening. Due to the asymmetric ponderomotive acceleration by the strongly decayed laser pulse, high-energy-density electrons with net laser energy gain are accumulated inside the cone, which then stream out of the tip opening continuously, like a jet. The jet electrons are fully relativistic, with speeds around 0.98−0.998 c and densities at 1020/cm3 level. The jet can keep for a long time over 200 fs, which may have diverse applications in practice.

Coupling single quantum dots to plasmonic nanocones: optical properties.

Coupling a single quantum emitter, such as a fluorescent molecule or a quantum dot (QD), to a plasmonic nanostructure is an important issue in nano-optics and nano-spectroscopy, relevant for a wide range of applications, including tip-enhanced near-field optical microscopy, plasmon enhanced molecular sensing and spectroscopy, and nanophotonic amplifiers or nanolasers, to mention only a few. While the field enhancement of a sharp nanoantenna increasing the excitation rate of a very closely positioned single molecule or QD has been well investigated, the detailed physical mechanisms involved in the emission of a photon from such a system are, by far, less investigated. In one of our ongoing research projects, we try to address these issues by constructing and spectroscopically analysing geometrically simple hybrid heterostructures consisting of sharp gold cones with single quantum dots attached to the very tip apex. An important goal of this work is to tune the longitudinal plasmon resonance by adjusting the cones' geometry to the emission maximum of the core-shell CdSe/ZnS QDs at nominally 650 nm. Luminescence spectra of the bare cones, pure QDs and hybrid systems were distinguished successfully. In the next steps we will further investigate, experimentally and theoretically, the optical properties of the coupled systems in more detail, such as the fluorescence spectra, blinking statistics, and the current results on the fluorescence lifetimes, and compare them with uncoupled QDs to obtain a clearer picture of the radiative and non-radiative processes.

Effect of defocusing on picosecond laser-coupling into gold cones

Here, we show that defocusing of the laser in the interaction of a picosecond duration, 1.053 μm wavelength, high energy pulse with a cone-wire target does not significantly affect the laser energy coupling efficiency, but does result in a drop in the fast electron effective temperature. This may be beneficial for fast ignition, since not only were more electrons with lower energies seen in the experiment but also the lower prepulse intensity will reduce the amount of preplasma present on arrival of the main pulse, reducing the distance the hot electrons have to travel. We used the Vulcan Petawatt Laser at the Rutherford Appleton Laboratory and gold cone targets with approximately 1 mm long, 40 μm diameter copper wires attached to their tip. Diagnostics included a quartz crystal imager, a pair of highly oriented pyrolytic graphite crystal spectrometers and a calibrated CCD operating in the single photon counting regime, all of which looked at the copper Kα emission from the wire. A short pulse optical probe, delayed 400 ps relative to the main pulse was employed to diagnose the extent of plasma expansion around the wire. A ray-tracing code modeled the change in intensity on the interior surface of the cone with laser defocusing. Using a model for the wire copper Kα emission coupled to a hybrid Vlasov-Fokker-Planck code, we ran a series of simulations, holding the total energy in electrons constant whilst varying the electron temperature, which support the experimental conclusions.

Localized enhancement of electric field in tip-enhanced Raman spectroscopy using radially and linearly polarized light

Finite-Difference Time-Domain (FDTD) calculations are used to characterize the electric field in the vicinity of a sharp silver or gold cone with an apex diameter of 10 nm. The simulations are utilized to predict the intensity and the distribution of the locally enhanced electric field in tip-enhanced Raman spectroscopy (TERS). A side-by-side comparison of the enhanced electric field induced by a radially and a linearly polarized light in both gap-mode and conventional TERS setup is performed. For this purpose, a radially polarized source is introduced and integrated into the FDTD modeling. Additionally, the optical effect of a thin protective layer of alumina on the enhancement of the electric field is investigated.

FIREX foam cryogenic target development: residual void reduction and estimation with solid hydrogen refractive index measurements

Voidless fuel solidification within a foam material is attempted for the development of a Fast Ignition Realization EXperiment (FIREX) target. A typical target consists of a foam shell with a thin solid fuel layer, a gold cone guide and a glass fill tube. The foam layer is formed with aggregations of tiny cells. The porous foam material has the advantage of forming a uniform layer in a liquid state by the effect of capillarity. Random liquid–solid transitions of fuel, however, would cause void spaces in each cell because of their different densities. To form a voidless solid fuel layer in the FIREX target, we propose a layering method, which includes the process of controlled solidification and simultaneous liquid fuel supply to the liquid/solid interface. Normal H2 is used as a surrogate fuel for our experiments. By applying a resorcinol/formalin aerogel, which has been developed in the Institute of Laser Engineering, Osaka University, instead of a foam material, formation of a solid H2 layer with reduced void spaces is preliminarily demonstrated. Related solid H2 refractive indices are measured to estimate the void fraction. Eventually, its filling factor reaches ∼99%. Furthermore, the application of the proved method is numerically simulated on the FIREX target. The method is confirmed to be applicable in it with a cone guide heating technique.

Ultra-Precision Turning Technology of Gold Cone in Fast Ignition

Fast Ignition (FI) attracts much attention owing to its advantages. The fabrication of fast ignition targets is one of the key technologies in FI study. Based on the single point diamond turning (SPDT) technology, Diamond post-turning method is adopted in this paper for the fabrication of gold cone. It not only helps to reduce the end-effect of cone mandrel and consequently improve the coaxiality of internal and external cone surface, but also helps to improve the quality of cone surface and the wall thickness consistency. Besides, the processing parameter of diamond post-turning is experimentally studied in this paper for its effect on the cone surface roughness. According to results, the cone surface roughness is Ra 9.21nm, the wall thickness consistency is 3μm and the cone end surface roughness is Ra5.72nm。

Ion beam focusing with cone optics for WDM experiments

Beam focusing properties of cone optics were systematically investigated by Monte Carlo simulations under various combinations of beam and cone parameters. To optimize the cone optic design for accelerator-driven WDM experiments, the beam intensity gains after cone focusing were evaluated from the simulation results as functions of cone wall material and shape parameters such as taper angle and wall curvature. The uniformity of the cone-focused beam was also examined by considering not only various cone parameters but also the cases involving the misalignment of the cone optic. From the results, a parabolic gold cone was found to be the best choice at least for relatively light ions such as lithium having MeV energies. It is also found that although smaller taper angle improves the total beam transport efficiency in the optic, it brings more difficulties in the alignment of the optic because the alignment accuracy should be less than a half of the taper angle to obtain acceptable uniformity in the beam energy deposition on the target.

Hot-electron generation from laser–pre-plasma interactions in cone-guided fast ignition

Two-dimensional particle-in-cell (PIC) simulations were performed for the cone-in-shell integrated fast-ignition experiments at the Omega Laser Facility [W. Theobald et al., Phys. Plasmas 18, 056305 (2011)]. The initial plasma density profile in the PIC simulations was taken from hydrodynamic simulations of the prepulse interaction with the gold cone. Hot-electron generation from laser–pre-plasma interactions and transport up to 100× the critical density (nc) was studied. The simulation showed a mean divergence half-angle of 68° and 50% absorption for the hot electrons. The simulation results show that the generated hot electrons were dominated in number by low-energy electrons but in energy by multi-MeV electrons. Electron transport between 5 and 100 nc was ballistic. In the late stage of the simulation, all the results were largely independent of polarization, indicating a stochastic hot-electron–generation mechanism.

Resonant Antenna Probes for Tip-Enhanced Infrared Near-Field Microscopy

We report the development of infrared-resonant antenna probes for tip-enhanced optical microscopy. We employ focused-ion-beam machining to fabricate high-aspect ratio gold cones, which replace the standard tip of a commercial Si-based atomic force microscopy cantilever. Calculations show large field enhancements at the tip apex due to geometrical antenna resonances in the cones, which can be precisely tuned throughout a broad spectral range from visible to terahertz frequencies by adjusting the cone length. Spectroscopic analysis of these probes by electron energy loss spectroscopy, Fourier transform infrared spectroscopy, and Fourier transform infrared near-field spectroscopy corroborates their functionality as resonant antennas and verifies the broad tunability. By employing the novel probes in a scattering-type near-field microscope and imaging a single tobacco mosaic virus (TMV), we experimentally demonstrate high-performance mid-infrared nanoimaging of molecular absorption. Our probes offer excellent perspectives for optical nanoimaging and nanospectroscopy, pushing the detection and resolution limits in many applications, including nanoscale infrared mapping of organic, molecular, and biological materials, nanocomposites, or nanodevices.

Impact of extended preplasma on energy coupling in kilojoule energy relativistic laser interaction with cone wire targets relevant to fast ignition

Cone-guided fast ignition laser fusion depends critically on details of the interaction of an intense laser pulse with the inside tip of a cone. Generation of relativistic electrons in the laser plasma interaction (LPI) with a gold cone and their subsequent transport into a copper wire have been studied using a kJ-class intense laser pulse, OMEGA EP (850 J, 10 ps). We observed that the laser-pulse-energy-normalized copper Kα signal from the Cu wire attached to the Au cone is significantly reduced (by a factor of 5) as compared to that from identical targets using the Titan laser (150 J, 0.7 ps) with 60 × less energy in the prepulse. We conclude that the decreased coupling is due to increased prepulse energy rather than 10 ps pulse duration, for which this effect has not been previously explored. The collisional particle-in-cell code PICLS demonstrates that the preformed plasma has a significant impact on generation of electrons and their transport. In particular, a longer scale length preplasma significantly reduces the energy coupling from the intense laser to the wire due to the larger offset distance between the relativistic critical density surface and the cone tip as well as a wider divergence of source electrons. We also observed that laser-driven plasma ionization increase in the LPI region can potentially alter the electron density profile during the laser interaction, forcing the electron source to be moved farther away from the cone tip which contributes to the reduction of energy coupling.

Implosion and heating experiments of fast ignition targets by Gekko-XII and LFEX lasers

The FIREX-1 project, the goal of which is to demonstrate fuel heating up to 5 keV by fast ignition scheme, has been carried out since 2003 including construction and tuning of LFEX laser and integrated experiments. Implosion and heating experiment of Fast Ignition targets have been performed since 2009 with Gekko-XII and LFEX lasers. A deuterated polystyrene shell target was imploded with the 0.53- μm Gekko-XII, and the 1.053- μm beam of the LFEX laser was injected through a gold cone attached to the shell to generate hot electrons to heat the imploded fuel plasma. Pulse contrast ratio of the LFEX beam was significantly improved. Also a variety of plasma diagnostic instruments were developed to be compatible with harsh environment of intense hard x-rays (γ rays) and electromagnetic pulses due to the intense LFEX beam on the target. Large background signals around the DD neutron signal in time-of-flight record of neutron detector were found to consist of neutrons via (γ,n) reactions and scattered gamma rays. Enhanced neutron yield was confirmed by carefully eliminating such backgrounds. Neutron enhancement up to 3.5 × 107 was observed. Heating efficiency was estimated to be 10–20% assuming a uniform temperature rise model.

Characterization of relativistic electrons generated by a cone guiding laser pulse

We demonstrated the interaction of a gold cone target with a femto second (fs) laser pulse above the relativistic intensity of 1.37 × 1018 μm 2W/cm2. Relativistic electrons with energy above 2 MeV were observed. A 25%-40% increase of the electron temperature is achieved compared to the case when a plane gold target is used. The electron temperature increase results from the guiding of the laser beam at the tip and the intense quasistatic magnetic field in the cone geometry. The behavior of the relativistic electrons is verified in our 2D-PIC simulations.

Integrated experiments of fast ignition targets by Gekko-XII and LFEX lasers

Implosion and heating experiments at the Institute of Laser Engineering, Osaka University on Fast Ignition (FI) targets for the FIREX-1 project have been performed with Gekko-XII laser for implosions and LFEX laser for heating. We tried to reduce the prepulse level in the LFEX laser system and have improved the plasma diagnostics to observe the plasma in the harsh hard X-ray environment. A plastic (CD) shell target, 7-μm thick and 500 μm in diameter with a hollow gold cone was used in this experiment to guide the short-pulse laser at the time of the maximum compression. The shell target was imploded with 9 or 12 beams of Gekko-XII laser (527 nm) with energy of 300 J/beam in a 1.5 ns pulse. Two of the four LFEX laser (1053 nm) beams were injected into the inside bottom of the cone with an energy up to 0.7 kJ/beam in a 1.5 ps pulse at the time around the maximum implosion. We have observed neutron enhancement up to 3.5 × 107 with total heating energy of 300 J, which is higher than the yield obtained in the previous experiment in 2002 [R. Kodama et al. Nature 418, 933 (2002)]. We found the estimated heating efficiency is at a level of 10–20%. Fuel heating to 5 keV is expected when the full output of LFEX is used.

Cone-guided fast ignition with ponderomotively accelerated carbon ions

Carbon ions are used to heat the precompressed deuterium–tritium (DT) fuel in a cone-guided fast ignitor scheme with an areal mass density of about 2.6 g cm−2. An ultra-intense laser pulse with a focal intensity of 1.45 × 1022 W cm−2 accelerates the carbon ions to an energy of 450 MeV from a homogeneous layer of 0.2 g/cm3 density, which fills the head of the gold cone. Pellet ignition was observed in hybrid numerical simulations for a laser energy of about 65 kJ in a rectangular pulse of 4 ps duration. This corresponds to estimated overall efficiencies of more than 24% for ion acceleration and 17% for core heating. Reducing the laser intensity to the value 5 × 1021 W cm−2, carbon ions with the energy of 175 MeV will be accelerated, and ignition occurred in hydrodynamic simulations for a laser energy of 115 kJ at a reduced heating efficiency of 6%. The comparison with ignition of a large-scale DT pellet, showing similar hydrodynamic characteristics and heated by in situ accelerated DT ions with 10 MeV mean energy, demonstrates the advantage of the carbon ion ignitor beam due to the more effective acceleration and expected higher directionality.

Gold Nanocone Near-Field Scanning Optical Microscopy Probes

Near-field scanning optical microscopy enables the simultaneous topographical and subdiffraction limited optical imaging of surfaces. A process is presented for the implementation of single individually engineered gold cones at the tips of atomic force microscopy cantilevers. These cantilevers act as novel high-performance optical near-field probes. In the fabrication, thin-film metallization, electron beam induced deposition of etch masks, and Ar ion milling are combined. The cone constitutes a well-defined highly efficient optical antenna with a tip radius on the order of 10 nm and an adjustable plasmon resonance frequency. The sharp tip enables high resolution topographical imaging. By controllably varying the cone size, the resonance frequency can be adapted to the application of choice. Structural properties of these sharp-tipped probes are presented together with topographical images recorded with a cone probe. The antenna functionality is demonstrated by gathering the near-field enhanced Raman signature of individual carbon nanotubes with a gold cone scanning probe.

Present states and future prospect of fast ignition realization experiment (FIREX) with Gekko and LFEX Lasers at ILE

Abstract The fast ignition realization experiment (FIREX) project is progressing. The new short pulse laser system, LFEX laser, has been completely assembled and one of the four beamlets is now in operation. A fast-ignition experiment was performed using this single short pulse combined with the Gekko XII implosion laser. The energy of the GXII implosion laser was about 2 kJ and the pulse width was 1.5 ns. The energy of the LFEX laser was increased upto 800 J and two pulse durations 5 and 1.6 ps were compared. Targets were deuterated plastic shells with gold cones. It was found that the neutron yield was increased by a factor of 30 as a result of the fast electron-induced heating in LFEX 1.6 ps shot. The estimated coupling efficiency between the LFEX laser pulse and the compressed fuel was low (less than 5%). This may be due to pre-plasma formed by light arriving at the target before the main laser pulse. Further investigations and attempts to overcome these problems are now in progress.