During the high-speed winding of polyester filament, a contact roller must be applied to press on the filament package’s surface to ensure the filament is placed stably and precisely on the package surface. Thus, a twin-rotor system with contact coupling characteristics between the contact roller and the filament package is formed. Identifying the contact parameters between the contact roller and the package are prerequisite to precisely analyze the dynamic behavior of the winding system, as well as to determine the technical parameters. In this paper, an approach was proposed to identify the equivalent contact stiffness and contact damping coefficients by means of coordination through experiment and simulation. First, based on the forced non-resonance method of a single-degree-of-freedom system, the testing scheme was drawn up in consideration of the winding process parameters. Then, an experimental device for the twin-rotor system was developed, and the dynamic contact parameters just in the working frequency band corresponding to low linear speed of winding were obtained by the experiment, due to the requirement of the forced non-resonance theory and economic limitations of the experimental device. Third, the basic parameters including equivalent radial Young’s modulus and damping ratio of the package were obtained through experimental test. Furthermore, the contact parameters in the working frequency band corresponding to high linear speed of winding were obtained through simulation. Finally, the curve fitting of contact parameters was finished; in addition, the comparative results between the simulation and the experiment are in good agreement. The dynamic contact parameters present nonlinear frequency variation characteristics.