Massive arbitrary spin supermultiplets and massless (scalar and spin one-half) supermultiplets of the N = 2 Poincaré superalgebra in three-dimensional flat space are considered. Both the integer spin and half-integer spin supermultiplets are studied. For such massive and massless supermultiplets, a formulation in terms of light-cone gauge unconstrained superfields defined in a momentum superspace is developed. For the supermultiplets under consideration a superspace first derivative representation for all cubic interaction vertices is obtained. A superspace representation for dynamical generators of the N = 2 Poincaré superalgebra is also found.