Vibration neutralizers are single-degree-of-freedom devices affixed to vibrating structures in order to reduce the response at a specific troublesome harmonic excitation frequency. As this frequency may vary over time, it becomes imperative to track and adjust the neutralizer to maintain the optimal performance. Recent years have witnessed the emergence of adaptive tunable vibration neutralizers, offering real-time adjustment capabilities through external actions. Thanks to real-time control algorithms, these devices enable the automatic mitigation of vibration levels in mechanical structures. A particularly successful algorithm for the automatic tuning of these devices leverages the phase angle between the base acceleration and the neutralizer’s mass. This study critically examines the justification for employing such an algorithm and scrutinizes its optimal applicability limits, particularly in the context of viscous and structurally damped systems. The findings reveal that this algorithm accurately approximates optimum tuning for systems with low damping. Moreover, from an engineering perspective, the algorithm remains acceptable even for heavily damped structures. Through a focused and comprehensive analysis, this paper provides valuable insights into the efficacy and limitations of the phase-angle-based tuning algorithm, contributing to the advancement of adaptive vibration control strategies in smart structures.