Top-gate thin-film transistors (TFTs) with amorphous aluminum-indium-zinc-oxide (a-AIZO) as channel layer and organic polymethylmethacrylate (PMMA) as dielectric layer were prepared via a solution process of dip coating method. The additive Al led to the band gap of AIZO films wider and effectively controlled the oxygen vacancies. This behaviour indicates that Al acted as an effective carrier suppressor in the IZO materials. Moreover, it was found that organic PMMA dielectric layer exhibited antireflection effect when it combined with a-AIZO film to form double-layer structure, showing the highly transparent of ∼94.7%. The a-AIZO-TFT with Al atomic content of 30% exhibited optimum device characteristics, with a high saturated mobility of 26.8 cm2 V−1 s−1, a small subthreshold swing of 0.24 V/decade, and slight hysteresis with Vth shift of ∼−1.26 V.
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