Superconductor Thin Films Research Articles

Correction: Fabrication and Characterization of Boron-Implanted Silicon Superconducting Thin Films on SOI Substrates for Low-Temperature Detectors

Correction: Fabrication and Characterization of Boron-Implanted Silicon Superconducting Thin Films on SOI Substrates for Low-Temperature Detectors

Superconducting resonator parametric amplifiers with intrinsic separation of pump and signal tones

Abstract Superconducting resonator parametric amplifiers achieve ultra-low-noise amplification through the nonlinear kinetic inductance of thin-film superconductors. One of the main challenges to the operation of these devices is the separation of the strong pump tone from the signal tone after amplification has been achieved. In this paper, we propose and experimentally demonstrate a pump separation method based on operating a half-wave superconducting resonator amplifier behind a cryogenic circulator. Our pump separation scheme does not involve post-amplification interference, and thereby avoids the delicate phase matching of two different pump paths. We demonstrate the scheme using two-port half-wave resonator amplifiers based on superconducting NbN thin-films. We present measurements of gain profiles and degrees of pump separation for amplifiers having different coupling quality factors. On an amplifier having a coupling quality factor of ~2000, we measured a peak signal gain of 15 dB whilst achieving pump separation of 12 dB. The amplifier was stable for continuous measurements, and the gain drift was measured to be 0.15 dB over an hour. The same amplifier was operated at 3.2 K and achieved a peak signal gain of 11 dB whilst having a pump separation factor of 10.5 dB. The pump separation scheme, and these promising results, will advance the development of superconducting resonator amplifiers as an important technology in quantum sensing.

Effect of Proton Irradiation on Thin-Film YBa2Cu3O7-δ Superconductor.

We investigated the effect of 0.6 MeV proton irradiation on the superconducting and normal-state properties of thin-film YBa2Cu3O7-δ superconductors. A thin-film YBCO superconductor (≈567 nm thick) was subject to a series of proton irradiations with a total fluence of 7.6×1016 p/cm2. Upon irradiation, Tc was drastically decreased from 89.3 K towards zero with a corresponding increase in the normal-state resistivity above Tc. This increase in resistivity, which indicates an increase in defects inside the thin-film sample, can be converted to the dimensionless scattering rate. We found that the relation between Tc and the dimensionless scattering rate obtained during proton irradiation approximates the generalized d-wave Abrikosov-Gor'kov theory better than the previous results obtained from electron irradiations. This is an unexpected result, since the electron irradiation is known to be most effective to suppress superconductivity over other heavier ion irradiations such as proton irradiation. In comparison with the previous irradiation studies, we found that the result can be explained by two facts. First, the dominant defects created by 0.6 MeV protons can be point-like when the implantation depth is much longer than the sample thickness. Second, the presence of defects on all element sites is important to effectively suppress Tc.

Current induced hidden states in Josephson junctions

Josephson junctions enable dissipation-less electrical current through metals and insulators below a critical current. Despite being central to quantum technology based on superconducting quantum bits and fundamental research into self-conjugate quasiparticles, the spatial distribution of super current flow at the junction and its predicted evolution with current bias and external magnetic field remain experimentally elusive. Revealing the hidden current flow, featureless in electrical resistance, helps understanding unconventional phenomena such as the nonreciprocal critical current, i.e., Josephson diode effect. Here we introduce a platform to visualize super current flow at the nanoscale. Utilizing a scanning magnetometer based on nitrogen vacancy centers in diamond, we uncover competing ground states electrically switchable within the zero-resistance regime. The competition results from the superconducting phase re-configuration induced by the Josephson current and kinetic inductance of thin-film superconductors. We further identify a new mechanism for the Josephson diode effect involving the Josephson current-induced phase. The nanoscale super current flow emerges as a new experimental observable for elucidating unconventional superconductivity, and optimizing quantum computation and energy-efficient devices.

Superconductivity in thin films of RuN

Superconductivity in thin films of RuN

Pressure tuning of superconductivity in TiN thin films

Titanium nitride (TiN) thin films are used for the fabrication of superconducting devices due to their chemical stability against oxidization and high quality at interfaces. The high-pressure technique serves as a useful tool to understand the mechanical and electrical properties of materials, which is crucial for practical applications. However, high-pressure transport measurements of thin films are extremely difficult due to the limited sample space of high-pressure cells and the fragility of thin films. Here, we successfully carried out high-pressure electrical transport and Raman measurements on TiN films up to ∼50 GPa. The superconducting transition temperature gradually decreases with increasing pressure, which can be attributed to the decrease of electron -phonon coupling and is consistent with our first-principles calculations. In addition, the coexistence of a symmetry-enforced Dirac nodal chain and a nodal box is revealed by our calculations in TiN. Our work provides a promising way to study the physical properties of thin films at high pressure, which would broaden the high-pressure research field.

Correlating critical current density, quench protection, relaxation time and entropy in superconductors after disturbances—Intermediate summary

<p>This paper summarizes results recently obtained from simulation of transient temperature excursions in filamentary and thin film superconductors. Under multi-component heat transfer in the complicated conductor cross sections and materials composition of present High Temperature Superconductors, numerical, Finite Element and Monte Carlo simulations are applied to solve Fourier’s differential equation with high spatial and temporal resolution. The overall aim was to encircle the quench problem in superconductors and to provide new stability criteria from correlations between superconductor critical current density, density of electron pairs, and relaxation time and entropy. Relaxation, correlation and entropy analysis presented in this paper extends the spectrum of standard methods to avoid quench to a new tool. As results, quench starts always locally, and as a highlight of this investigation, a second “critical” temperature, <em>T<sub>Quench</sub></em>, has been identified that with high probability exists below standard critical temperature. Entropy is the driving force for relaxation of the superconductor to new equilibrium after a disturbance.<strong></strong></p>

Structure and Superconductivity of Epitaxial and Polycrystalline VN Thin Films

Structure and Superconductivity of Epitaxial and Polycrystalline VN Thin Films

Inverse Spin-Hall Effect and Spin Swapping in Spin-Split Superconductors.

When a spin-splitting field is introduced to a thin film superconductor, the spin currents polarized along the field couples to energy currents that can only decay via inelastic scattering. We study spin and energy injection into such a superconductor where spin-orbit impurity scattering yields inverse spin-Hall and spin-swapping currents. We show that the combined presence of a spin-splitting field, superconductivity, and inelastic scattering gives rise to a strong enhancement of the ordinary inverse spin-Hall effect, as well as unique inverse spin-Hall and spin-swapping signals orders of magnitude stronger than the ordinary inverse spin-Hall signal. These can be completely controlled by the orientation of the spin-splitting field, resulting in a long-range charge and spin accumulations detectable much further from the injector than in the normal state. While the enhanced inverse spin-Hall signals offer a major improvement in spin detection sensitivity, the unique spin-swap signals can be utilized for designing devices where both the spin and current directions are controlled and altered throughout the geometry.

Fabrication and Characterization of Boron-Implanted Silicon Superconducting Thin Films on SOI Substrates for Low-Temperature Detectors

Fabrication and Characterization of Boron-Implanted Silicon Superconducting Thin Films on SOI Substrates for Low-Temperature Detectors

Theory of superconductivity in thin films under an external electric field

Theory of superconductivity in thin films under an external electric field

A Simple Model for the Induction Current Distribution in a Thin Superconducting Film

A Simple Model for the Induction Current Distribution in a Thin Superconducting Film

Steering of Vortices by Magnetic Field Tilting in Open Superconductor Nanotubes.

In planar superconductor thin films, the places of nucleation and arrangements of moving vortices are determined by structural defects. However, various applications of superconductors require reconfigurable steering of fluxons, which is hard to realize with geometrically predefined vortex pinning landscapes. Here, on the basis of the time-dependent Ginzburg-Landau equation, we present an approach for the steering of vortex chains and vortex jets in superconductor nanotubes containing a slit. The idea is based on the tilting of the magnetic field B at an angle α in the plane perpendicular to the axis of a nanotube carrying an azimuthal transport current. Namely, while at α=0∘, vortices move paraxially in opposite directions within each half-tube; an increase in α displaces the areas with the close-to-maximum normal component |Bn| to the close(opposite)-to-slit regions, giving rise to descending (ascending) branches in the induced-voltage frequency spectrum fU(α). At lower B values, upon reaching the critical angle αc, the close-to-slit vortex chains disappear, yielding fU of the nf1 type (n≥1: an integer; f1: the vortex nucleation frequency). At higher B values, fU is largely blurry because of multifurcations of vortex trajectories, leading to the coexistence of a vortex jet with two vortex chains at α=90∘. In addition to prospects for the tuning of GHz-frequency spectra and the steering of vortices as information bits, our findings lay the foundation for on-demand tuning of vortex arrangements in 3D superconductor membranes in tilted magnetic fields.

Superconducting nitridized-aluminum thin films

We report the direct observation of superconductivity in nitridized-aluminum thin films. The films are produced by sputtering deposition of aluminum in a controlled mixture of nitrogen diluted in argon. The concentration of applied nitrogen directly determines the properties of the superconducting thin films. We observe samples displaying critical temperatures up to 3.38 ± 0.01 K and resilience to in-plane magnetic fields well above 1 T, with good reproducibility of the results. This work represents an unambiguous demonstration of tunable superconductivity in aluminum-based nitridized thin films. Our results put forward nitridized aluminum as a promising material to be employed in superconducting quantum circuits for quantum technology applications.

Levitation force measurement and characteristics analysis of double sided high temperature superconducting thin film device

In this paper, the levitation characteristics of double sided high temperature superconducting (HTS) thin film device is proposed and measured. Based on the unique advantages such as, passive self-stable levitation, higher payload, lower energy consumption, less maintenance cost, etc., HTS-magnetic levitation (maglev) technology has been applied in the traditional fields (rail transit and energy storage fields) and novel fields (astrophysics, space station microgravity, vibration isolation fields). As the key core components, HTS device should meet the requirements of volume, weight and cost, to improve the system operation efficiency. Thus, considering the low profile, miniaturization and lightweight characteristics of the double sided YBa2Cu3O7-x (YBCO) thin film, we measured its levitation and relaxation characteristics. Meanwhile, we also designed the YBCO thin film with meander-lines, to explore the levitation characteristic evolution mechanism. It can be found from the experimental results that, the single piece of YBCO thin film with/without meander-lines can offer the levitation force more than 400 mN and 800 mN, respectively. The signature of this work is that the double sided YBCO thin film has the potential to be employed as the core device in the special application fields (such as astrophysics and space station), to supply the sufficient micro levitation force in limited volume and weight.

Gauge Theories of Josephson Junction Arrays: Why Disorder Is Irrelevant for the Electric Response of Disordered Superconducting Films

We review the topological gauge theory of Josephson junction arrays and thin film superconductors, stressing the role of the usually forgotten quantum phase slips, and we derive their quantum phase structure. A quantum phase transition from a superconducting to the dual, superinsulating phase with infinite resistance (even at finite temperatures) is either direct or goes through an intermediate bosonic topological insulator phase, which is typically also called Bose metal. We show how, contrary to a widely held opinion, disorder is not relevant for the electric response in these quantum phases because excitations in the spectrum are either symmetry-protected or neutral due to confinement. The quantum phase transitions are driven only by the electric interaction growing ever stronger. First, this prevents Bose condensation, upon which out-of-condensate charges and vortices form a topological quantum state owing to mutual statistics interactions. Then, at even stronger couplings, an electric flux tube dual to Abrikosov vortices induces a linearly confining potential between charges, giving rise to superinsulation.

Tuning Critical Field, Critical Current, and Diode Effect of Narrow Thin-Film Superconductors Through Engineering Inhomogeneous Pearl Length

Tuning Critical Field, Critical Current, and Diode Effect of Narrow Thin-Film Superconductors Through Engineering Inhomogeneous Pearl Length

Roles of Fe-ion irradiation on MgB2 thin films: Structural, superconducting, and optical properties

The effects of Fe-ion irradiation on the crystal structure and superconducting properties of MgB2 thin films were investigated. Pristine samples were prepared using hybrid physical-chemical vapor deposition (HPCVD), and ion irradiation was performed at three different doses of 5 × 1013, 1 × 1014, and 2 × 1014 ions/cm2. The measured temperature-dependent resistivity showed that as the irradiation dose increased from pristine to most irradiated, the superconducting critical temperature, Tc, significantly decreased from 38.33 to 3.02 K. The crystal structures of the films were investigated by X-ray diffraction (XRD) and X-ray absorption spectroscopy (XAS) measurements. The results showed that the higher the dose, the greater the change in crystal structure, such as the lattice constant and bond length. This suggests that the destruction of the crystal structure at higher doses leads to the degradation of superconductivity in the irradiated MgB2 thin films. Raman spectroscopy showed that the electron-phonon coupling constant decreased with increasing irradiation dose, which was directly related to the reduction of Tc in the samples. The optical conductivity indicates that the charge-carrier density of the σ-band plays an important role in the superconductivity of ion-irradiated MgB2.

Smooth, homogeneous, high-purity Nb3Sn superconducting RF resonant cavity by seed-free electrochemical synthesis

Workbench-size particle accelerators, enabled by Nb3Sn-based superconducting radio-frequency (SRF) cavities, hold the potential of driving scientific discovery by offering a widely accessible and affordable source of high-energy electrons and x-rays. Thin-film Nb3Sn RF superconductors with high quality factors, high operation temperatures, and high-field potentials are critical for these devices. However, surface roughness, non-stoichiometry, and impurities in Nb3Sn deposited by conventional Sn-vapor diffusion prevent them from reaching their theoretical capabilities. Here we demonstrate a seed-free electrochemical synthesis that pushes the limit of chemical and physical properties in Nb3Sn. Utilization of electrochemical Sn pre-deposits reduces the roughness of converted Nb3Sn by five times compared to typical vapor-diffused Nb3Sn. Quantitative mappings using chemical and atomic probes confirm improved stoichiometry and minimized impurity concentrations in electrochemically synthesized Nb3Sn. We have successfully applied this Nb3Sn to the large-scale 1.3 GHz SRF cavity and demonstrated ultra-low BCS surface resistances at multiple operation temperatures, notably lower than vapor-diffused cavities. Our smooth, homogeneous, high-purity Nb3Sn provides the route toward high efficiency and high fields for SRF applications under helium-free cryogenic operations.

Fabrication Development for SPT-SLIM, a Superconducting Spectrometer for Line Intensity Mapping

Line Intensity Mapping (LIM) is a new observational technique that uses low-resolution observations of line emission to efficiently trace the large-scale structure of the Universe out to high redshift. Common mm/sub-mm emission lines are accessible from ground-based observatories, and the requirements on the detectors for LIM at mm-wavelengths are well matched to the capabilities of large-format arrays of superconducting sensors. We describe the development of an <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"><tex-math notation="LaTeX">$R$</tex-math></inline-formula> = <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"><tex-math notation="LaTeX">$\lambda / \Delta \lambda = 300$</tex-math></inline-formula> on-chip superconducting filter-bank spectrometer covering the 120–180 GHz band for future mm-LIM experiments, focusing on SPT-SLIM, a pathfinder LIM instrument for the South Pole Telescope. Radiation is coupled from the telescope optical system to the spectrometer chip via an array of feedhorn-coupled orthomode transducers. Superconducting microstrip transmission lines then carry the signal to an array of channelizing half-wavelength resonators, and the output of each spectral channel is sensed by a lumped element kinetic inductance detector (leKID). Key areas of development include incorporating new low-loss dielectrics to improve both the achievable spectral resolution and optical efficiency and development of a robust fabrication process to create a galvanic connection between ultra-pure superconducting thin-films to realize multi-material (hybrid) leKIDs. We provide an overview of the spectrometer design, fabrication process, and prototype devices.