Ferromagnetic Resonance Technique Research Articles

Twofold and fourfold anisotropies in zinc ferrite thin films investigated by ferromagnetic resonance

By means of the ferromagnetic resonance (FMR) technique (at the $X$ band) we investigated the magnetic properties of ${\mathrm{ZnFe}}_{2}{\mathrm{O}}_{4}$ (ZFO) films grown on different substrates. Angular dependence of the FMR field showed the existence of twofold and fourfold anisotropies for the same material, grown on Si(111), MgO(100), and STO(100), respectively. By using a model that takes into consideration the relevant contributions to the energy, we were able to extract the following parameters: effective magnetization ${M}_{\mathrm{eff}}$, cubic magnetocrystalline anisotropy field, in-plane and out of plane uniaxial anisotropy fields, and the $g$ factor. The samples deposited on Si showed a twofold in-plane anisotropy while a fourfold magnetic anisotropy was observed for the ZFO/MgO and ZFO/${\mathrm{SrTiO}}_{3}$ samples. All samples showed a strong perpendicular uniaxial anisotropy above 1 kOe and low in-plane uniaxial and cubic anisotropy field, on the order of tens of oersteds. The FMR linewidth ($\mathrm{\ensuremath{\Delta}}H$) fitted from FMR data shows $\mathrm{\ensuremath{\Delta}}H$ values above 190 Oe for all samples, indicating high damping of this material to be $\ensuremath{\sim}{10}^{\ensuremath{-}2}$ for the ZFO/MgO. The present analysis compared the FMR data obtained for the in-plane and out of plane measurements. Likewise, the effective magnetization and perpendicular uniaxial anisotropy field by FMR were compared with the magnetic response obtained by a vibrating sample magnetometer.

Separation of Artifacts from Spin‐Torque Ferromagnetic Resonance Measurements of Spin‐Orbit Torque for the Low‐Symmetry Van der Waals Semi‐Metal ZrTe3

AbstractSpin‐orbit torques generated by exfoliated layers of the low‐symmetry semi‐metal ZrTe3 are measured using the spin‐torque ferromagnetic resonance (ST‐FMR) technique. When the ZrTe3 has a thickness greater than about 10 nm, artifacts due to spin pumping and/or resonant heating can cause the standard ST‐FMR analysis to overestimate the true magnitude of the torque efficiency by as much as a factor of 30, and to indicate incorrectly that the spin‐orbit torque depends strongly on the ZrTe3 layer thickness. Artifact‐free measurements can still be achieved over a substantial thickness range by the method developed recently to detect ST‐FMR signals in the Hall geometry as well as the longitudinal geometry. ZrTe3/Permalloy samples generate a conventional in‐plane anti‐damping spin torque efficiency = 0.014 ± 0.004, and an unconventional in‐plane field‐like torque efficiency = 0.003 ± 0.001. The out‐of‐plane anti‐damping torque is negligible. It is suggested that artifacts similarly interfere with the standard ST‐FMR analysis for other van der Waals samples thicker than about 10 nm.

Modulation of interfacial magnetic relaxation timeframes by partially uncoupled exchange bias

A set of partially uncoupled NiFe/Cu/IrMn exchange biased thin films with variable thickness of non-magnetic Cu spacer is characterized by ferromagnetic resonance (FMR) and Brillouin light scattering (BLS) techniques applied complementary to reveal time-scale dependent effects of uncoupling between ferromagnetic and antiferromagnetic layers on high-frequency magnetization dynamics. The results correlate with interfacial grain texture variations and static magnetization behavior. Two types of crystalline phases with correlated microwave response are revealed at the ferro–antiferromagnet interface in NiFe/Cu/IrMn thin films. The 1st phase forms well-textured NiFe/IrMn grains with NiFe (111)/IrMn (111) interface. The 2nd phase consists of amorphous NiFe/IrMn grains. Intercalation of NiFe/IrMn by Cu clusters results in relaxation of tensile strains at the NiFe/IrMn interface leading to larger size of grains in both the NiFe and IrMn layers. The contributions of well-textured and amorphous grains to the high-frequency magnetization reversal behavior are distinguished by FMR and BLS techniques. Generation of a spin-wave mode is revealed in the well-textured phase, whereas microwave response of the amorphous phase is found to originate from magnetization rotation dominated by a rotatable magnetic anisotropy term. Under fixed FMR frequency, the increase of Cu thickness results in higher magnetization rotation frequencies in the amorphous grains.

Synthesis of magneto-dielectric coatings in electron-beam produced plasma in medium vacuum

Using sequential electron-beam evaporation of high-temperature dielectric (alumina ceramic) and magnetic (iron) targets in various gas atmospheres (helium, air, and oxygen) in medium vacuum (5–8 Pa), magneto-dielectric coatings with thickness of around 2 μm were deposited from a multicomponent beam plasma at a deposition rate of 0.2–0.3 μm/min. The coating magnetic properties were explored by the ferromagnetic resonance technique, revealing that their effective magnetization depends on the type of operating gas and varied from 4.2 to 6.8 kGs (for deposition in helium) to 0.3 kGs (in oxygen), which is characteristic of oxide ferromagnetic materials and is considerably lower than the corresponding value (∼22 kGs) for thin iron films formed by vacuum arc deposition in high vacuum. X-ray structural analysis of coatings deposited in medium vacuum in helium showed that the magnetic layer has a magnetite (Fe3O4) structure. The alumina ceramic layer provides the dielectric properties of the magneto-dielectric coating; a relative dielectric constant of 6.0 and a conductivity of 8.4 mS/m were achieved.

Facile Synthesis, Static, and Dynamic Magnetic Characteristics of Varying Size Double-Surfactant-Coated Mesoscopic Magnetic Nanoparticles Dispersed Stable Aqueous Magnetic Fluids.

The present work reports the synthesis of a stable aqueous magnetic fluid (AMF) by dispersing double-surfactant-coated Fe3O4 magnetic nanoparticles (MNPs) in water using a facile ambient scalable wet chemical route. MNPs do not disperse well in water, resulting in low stability. This was improved by dispersing double-surfactant (oleic acid and sodium oleate)-coated MNPs in water, where cross-linking between the surfactants improves the stability of the AMFs. The stability was probed by rheological measurements and all the AMF samples showed a good long-term stability and stability against a gradient magnetic field. Further, the microwave spin resonance behavior of AMFs was studied in detail by corroborating the experimental results obtained from the ferromagnetic resonance (FMR) technique to theoretical predictions by appropriate fittings. A broad spectrum was perceived for AMFs which indicates strong ferromagnetic characteristics. The resonance field shifted to higher magnetic field values with the decrease in particle size as larger-size MNPs magnetize and demagnetize more easily since their magnetic spins can align in the field direction more definitely. The FMR spectra was fitted to obtain various spin resonance parameters. The asymmetric shapes of the FMR spectra were observed with a decrease in particle sizes, which indicates an increase in relaxation time. The relaxation time increased with a decrease in particle sizes (sample A to D) from 37.2779 ps to 42.8301 ps. Further, a detailed investigation of the structural, morphological, and dc magnetic properties of the AMF samples was performed. Room temperature dc magnetic measurements confirmed the superparamagnetic (SPM) characteristics of the AMF and the M-H plot for each sample was fitted with a Langevin function to obtain the domain magnetization, permeability, and hydrodynamic diameter of the MNPs. The saturation magnetization and coercivity of the AMF samples increased with the increase in dispersed MNPs’ size of the samples. The improvement in the stability and magnetic characteristics makes AMFs suitable candidates for various biomedical applications such as drug delivery, magnetic fluid hyperthermia, and biomedicines.

Electric field control of magnetism in FePt/PMN-PT heterostructures

Laminar heterostructures composed by materials with different ferroic properties have been proposed for the control of magnetism with an applied voltage. We present here a study of the structural and magnetic properties of chemically disordered FePt ferromagnetic films of different thicknesses that have been sputter-deposited on ferroelectric PMN-PT (011) single crystals.By means of static and dynamic magnetic measurements we have found that it is possible to switch the magnetization easy axis by 90° if an electric field is applied in a direction perpendicular to the film plane. Using ferromagnetic resonance techniques we have estimated the strain induced magnetoelectric coupling of the FePt/PMN-PT heterostructure, obtaining ME=477(15) Oe m/MV for FePt thicknesses greater than 26 nm, which corresponds to an average magnetoelastic constant B=−13.2(1.1) MJ/m3. The associated saturation magnetostriction was estimated in λs∼90 ppm. Films thinner than 26 nm present corresponding values that are smaller by approximately 20%. A possible explanation for this difference is the well known transition from planar to stripe-like magnetic domains that occurs in FePt around this film thickness. However, this thickness dependence of ME is relatively smaller than that found in other ferromagnets such as Fe or FeGa, which makes FePt a potential candidate for thin film applications in magnetoelectronic devices.

Spin pumping contribution to the magnetization damping in Tm3Fe5O12/W bilayers

In this work, thulium iron garnet (Tm3Fe5O12 – TmIG (20 nm)/Tungsten(W)(t) bilayers, sputtered on top of gadolinium gallium garnet (111) substrate, were used to investigate spin pumping (SP) line broadening mechanism in Ferromagnetic Resonance (FMR). The TmIG, films prior and after tungsten cap layer deposition, were investigated employing FMR and X-ray diffraction techniques. The TmIG films showed (111) orientation and perpendicular magnetic anisotropy (PMA). Due to the interface TmIG/W, when the TmIG magnetization is in resonance a spin current is pumped out the TmIG into the W layer, increasing the damping of the magnetization. Measuring the out-of-plane angular dependence of the FMR resonance field and linewidth, we were able to obtain solely the SP contribution to the line broadening, filtering Gilbert, mosaicity, and two magnon scattering mechanisms.

Observation of the Out‐of‐Plane Polarized Spin Current from CVD Grown WTe2

AbstractWeyl semimetal Td‐phase WTe2 possesses the spin‐resolved band structure with strong spin–orbit coupling, holding promises as a useful spin source material. The noncentrosymmetric crystalline structure of Td‐WTe2 endows the generation of the out‐of‐plane polarized spin, which is of great interest in magnetic memory applications. Previously, WTe2 was explored in spin devices based on mechanically exfoliated single crystal flakes with a size of micrometers. For practical spintronics applications, it is highly desirable to implement wafer‐scale thin films. In this work, centimeter‐scale chemical vapor deposition (CVD) grown Td‐WTe2 thin films are used and the spin current generation is studied by the spin torque ferromagnetic resonance (ST‐FMR) technique. The in‐plane and out‐of‐plane spin conductivities of 7.36 × 103 () (Ωm)–1 and 1.76 × 103 () (Ωm)–1, respectively, are found in CVD‐growth 5 nm‐WTe2. The current‐induced magnetization switching in WTe2/NiFe is demonstrated at room temperature in the domain wall motion regime, which may invigorate potential spintronic device innovations based on Weyl semimetals.

Spin Injection Efficiency at Metallic Interfaces Probed by THz Emission Spectroscopy

AbstractTerahertz (THz) spin‐to‐charge conversion has become an increasingly important process for THz pulse generation and as a tool to probe ultrafast spin interactions at magnetic interfaces. However, its relation to traditional, steady state, ferromagnetic resonance techniques is poorly understood. Here, nanometric trilayers of Co/X/Pt (X = Ti, Au or an Au:W alloy) are investigated as a function of the “X” layer thickness, where THz emission generated by the inverse spin Hall effect is compared to the Gilbert damping of the ferromagnetic resonance. Through the insertion of the “X” layer it is shown that the ultrafast spin current injected in the non‐magnetic layer defines a direct‐spin‐conductance, whereas the Gilbert damping leads to an effective spin‐mixing‐conductance of the trilayer. Importantly, it is shown that these two parameters are connected to each other and that spin‐memory‐losses can be modeled via an effective Hamiltonian with Rashba fields. This work highlights that magneto‐circuit concepts can be successfully extended to ultrafast spintronic devices, as well as enhancing the understanding of spin‐to‐charge conversion processes through the complementarity between ultrafast THz spectroscopy and steady state techniques.

Recent progress on measurement of spin–charge interconversion in topological insulators using ferromagnetic resonance

Spin–orbit coupling (SOC) in materials plays a crucial role in interconversion between spin and charge currents. In reduced dimensions, SOC effects are enhanced and have been the focus of intensive experimental and theoretical research, both for their novel spin-dependent phenomena and for their potential exploitation in new spintronics devices. Thanks to the discovery of a family of two-dimensional materials, extensive research has been conducted to explore potential material systems to achieve high spin–charge interconversion rates as well as to allow detection and accurate measurement. This article reviews the prospect of topological insulators as a reliable material system for efficient spin–charge interconversion and recent experimental advances in detecting the charge-to-spin and spin-to-charge conversions on topological insulator surfaces via spin-torque ferromagnetic resonance and spin-pumping techniques, respectively.

Effect of processing parameters on the defects state in Ni0.65Zn0.35Al0.8Fe1.2O4 thin films

Ferromagnetic resonance (FMR) technique is used to investigate the effect of oxygen partial pressure (PO2) and substrate temperature (TS) on the defect properties of Ni0.65Zn0.35Al0.8Fe1.2O4 (NZAFO) thin films. NZAFO thin films are deposited on MgAl2O4 (MAO) (100) substrates using pulsed laser deposition technique under various PO2 and TS. The FMR study reveals that the FMR parameters such as linewidth, line intensity and g-factor of the NZAFO thin films are sensitive to the variations in PO2 and TS. The observed changes in the FMR parameters are attributed to the variation of density and uniformity of defects in NZAFO thin films. Thus the significance of the present work suggests that the FMR may serve as an effective tool to monitor the growth condition of complex oxide films.

Crystallographic direction related spin current transmission in MgO(001)/Fe0.79Si0.21(001)/Pt(111) epitaxial bilayers

Spin-pumping and spin-orbit torque efficiencies in ferromagnetic/heavy metal bilayers, which usually consist of the polycrystalline grains, are related to the spin current transmission from ferromagnets to heavy metals and vice versa, respectively. In this work, epitaxial ${\mathrm{Fe}}_{0.79}{\mathrm{Si}}_{0.21}(001)/\mathrm{Pt}(111)$ films were fabricated to investigate the spin-pumping efficiency and spin-orbit torque efficiency by ferromagnetic resonance and harmonic Hall resistance measurement techniques, respectively. Ferromagnetic resonance results show that the incremental magnetic damping constants in epitaxial ${\mathrm{Fe}}_{0.79}{\mathrm{Si}}_{0.21}(001)/\mathrm{Pt}(111)$, compared with those of the epitaxial ${\mathrm{Fe}}_{0.79}{\mathrm{Si}}_{0.21}(001)/\mathrm{Al}{\mathrm{O}}_{x}$ reference sample, depend on whether the external magnetic field is applied along the in-plane easy or hard axes of ${\mathrm{Fe}}_{0.79}{\mathrm{Si}}_{0.21}$. The Pt thickness-dependent anisotropic damping constant was ascribed to the anisotropic spin current absorption in epitaxial Pt(111) layer. When electric currents were applied along the easy and hard axes of ${\mathrm{Fe}}_{0.79}{\mathrm{Si}}_{0.21}$ in epitaxial ${\mathrm{Fe}}_{0.79}{\mathrm{Si}}_{0.21}(001)/\mathrm{Pt}(111)$ bilayers, a large difference between spin-orbit torques generated from Pt(111) was observed by a harmonic Hall resistance measurement method. Both of the results suggest that spin current transmission efficiency is related to the anisotropic spin Hall effect of epitaxial Pt(111) layer due to the different spin-orbit interaction energies along the different crystallographic directions of Pt.

Drag effect induced large anisotropic damping behavior in magnetic thin films with strong magnetic anisotropy

The determination of intrinsic Gilbert damping is one of the central interests in the field of spintronics. However, some external factors in magnetic films tend to play a remarkable role in the magnetization dynamics. Here, we present a comprehensive study of the magnetic relaxation in ferromagnetic films with various in-plane magnetic anisotropy via ferromagnetic resonance technique. We find that the magnetic drag effect can result in the resonant linewidth broadening and the nonlinear dependence of linewidth on frequency stemming from field-magnetization misalignment. As a result, this could lead to the imprecise extraction of the key dynamic parameter-Gilbert damping and cause the confusing behaviors of ultra-low and anisotropic damping in thin films and multi-layers with high magnetic anisotropy. Our results provide a crucial way for the accurately quantitative estimation of the Gilbert damping in spintronics measurements.

Spin-orbit torque induced magnetization dynamics and switching in a CoFeB/Ta/CoFeB system with mixed magnetic anisotropy

Spin-orbit torque (SOT) induced magnetisation switching in CoFeB/Ta/CoFeB trilayer with two CoFeB layers exhibiting in-plane magnetic anisotropy (IPMA) and perpendicular magnetic anisotropy (PMA) is investigated. Interlayer exchange coupling (IEC), measured using ferromagnetic resonance technique is modified by varying thickness of Ta spacer. The evolution of the IEC leads to different orientation of the magnetic anisotropy axes of two CoFeB layers: for thicker Ta layer where magnetisation prefers antiferromagnetic ordering and for thinner Ta layer where ferromagnetic coupling exists. Magnetisation state of the CoFeB layer exhibiting PMA is controlled by the spin-polarized current originating from SOT in $\mu m$ sized Hall bars. The evolution of the critical SOT current density with Ta thickness is presented, showing an increase with decreasing $t_\mathrm{Ta}$, which coincides with the coercive field dependence. In a narrow range of $t_\mathrm{Ta}$ corresponding to the ferromagnetic IEC, the field-free SOT-induced switching is achieved.

Magnetoelastic interactions and magnetic damping in Co2Fe0.4Mn0.6Si and Co2FeGa0.5Ge0.5 Heusler alloys thin films for spintronic applications

Co2Fe0.4Mn0.6Si (CFMS) and Co2FeGa0.5Ge0.5 (CFGG) Heusler alloys are among the most promising thin film materials for spintronic devices due to a high spin polarization, low magnetic damping and giant/tunneling magnetoresistance ratios. Despite numerous investigations of Heusler alloys magnetic properties performed up to now, magnetoelastic effects in these materials remain not fully understood; due to quite rare studies of correlations between magnetoelastic and other magnetic properties, such as magnetic dissipation or magnetic anisotropy. In this research we have investigated epitaxial CFMS and CFGG Heusler alloys thin films of thickness in the range of 15–50 nm. We have determined the magnetoelastic tensor components and magnetic damping parameters as a function of the magnetic layer thickness. Magnetic damping measurements revealed the existence of non-Gilbert dissipation related contributions, including two-magnon scattering and spin pumping phenomena. Magnetoelastic constant B11 values and the effective magnetic damping parameter αeff values were found to be in the range of − 6 to 30 × 106 erg/cm3 and between 1 and 12 × 10–3, respectively. The values of saturation magnetostriction λS for CFMS Heusler alloy thin films were also obtained using the strain modulated ferromagnetic resonance technique. The correlation between αeff and B11, depending on magnetic layer thickness was determined based on the performed investigations of the above mentioned magnetic properties.

Spin-Wave Dynamics in an Artificial Kagome Spin IceSupported by the State Grid Corporation of China via the Science and Technology Project: Research on Electromagnetic Measurement Technology Based on EIT and TMR (Grant No. JL71-18-007).

Artificial spin ice (ASI) structures have significant technological potential as reconfigurable metamaterials and magnetic storage media. We investigate the field/frequency-dependent magnetic dynamics of a kagome ASI made of 25-nm-thick permalloy nanomagnet elements, combining magnetoresistance (MR) and microscale ferromagnetic resonance (FMR) techniques. Our FMR spectra show a broadband absorption spectrum from 0.2 GHz to 3 GHz at H below 0.3 kOe, where the magnetic configuration of the kagome ASI is in the multidomain state, because the external magnetic field is below the obtained coercive field H c ∼ 0.3 kOe, based on both the low-field range MR loops and simulations, suggesting that the low-field magnetization dynamics of kagome ASI is dominated by a multimode resonance regime. However, the FMR spectra exhibit five distinctive resonance modes at the high-field quasi-uniform magnetization state. Furthermore, our micromagnetic simulations provide additional spatial resolution of these resonance modes, identifying the presence of two high-frequency primary modes, localized in the horizontal and vertical bars of the ASI, respectively; three other low-frequency modes are mutually exclusive and separately pinned at the corners of the kagome ASI by an edge-induced dipolar field. Our results suggest that an ASI structural design can be adopted as an efficient approach for the development of low-power filters and magnonic devices.

Microresonators and Microantennas—Tools to Explore Magnetization Dynamics in Single Nanostructures

The phenomenon of magnetic resonance and its detection via microwave spectroscopy provide insight into the magnetization dynamics of bulk or thin film materials. This allows for direct access to fundamental properties, such as the effective magnetization, g-factor, magnetic anisotropy, and the various damping (relaxation) channels that govern the decay of magnetic excitations. Cavity-based and broadband ferromagnetic resonance techniques that detect the microwave absorption of spin systems require a minimum magnetic volume to obtain a sufficient signal-to-noise ratio (S/N). Therefore, conventional techniques typically do not offer the sensitivity to detect individual micro- or nanostructures. A solution to this sensitivity problem is the so-called planar microresonator, which is able to detect even the small absorption signals of magnetic nanostructures, including spin-wave or edge resonance modes. As an example, we describe the microresonator-based detection of spin-wave modes within microscopic strips of ferromagnetic A2 Fe60Al40 that are imprinted into a paramagnetic B2 Fe60Al40-matrix via focused ion-beam irradiation. While microresonators operate at a fixed microwave frequency, a reliable quantification of the key magnetic parameters like the g-factor or spin relaxation times requires investigations within a broad range of frequencies. Furthermore, we introduce and describe the step from microresonators towards a broadband microantenna approach. Broadband magnetic resonance experiments on single nanostructured magnetic objects in a frequency range of 2–18 GHz are demonstrated. The broadband approach has been employed to explore the influence of lateral structuring on the magnetization dynamics of a Permalloy (Ni80Fe20) microstrip.

Enhanced spin-orbit torque efficiency in Pt100–x Ni x alloy based magnetic bilayer* *Project supported by the National Natural Science Foundation of China (Grant Nos. 51901025 and 51625101), the Fundamental Research Funds for the Central Universities, China (Grant No. 310421101), and the Beijing Natural Science Foundation, China (Grant No. Z190007).

The binary alloy/ferromagnetic metal heterostructure has drawn extensive attention in the research field of spin–orbit torque (SOT) due to the potential enhancement of SOT efficiency via composition engineering. In this work, the magnetic properties and SOT efficiency in the Pt100 – x Ni x /Ni78Fe22 bilayers were investigated via the spin-torque ferromagnetic resonance (ST-FMR) technique. The effective magnetic anisotropy field and effective damping constant extracted by analyzing the ST-FMR spectra show a weak dependence on the Ni concentration. The effective spin-mixing conductance of 8.40 × 1014 Ω−1 ⋅ m−2 and the interfacial spin transparency T in of 0.59 were obtained for the sample of Pt70Ni30/NiFe bilayer. More interestingly, the SOT efficiency that is carefully extracted from the angular dependence of ST-FMR spectra shows a nonmonotonic dependence on the Ni concentration, which reaches the maximum at x = 18. The enhancement of the SOT efficiency by alloying the Ni with Pt shows potential in lowering the critical switching current. Moreover, alloying relatively cheaper Ni with Pt may promote to reduce the cost of SOT devices.

Giant spin torque efficiency in single-crystalline antiferromagnet Mn2Au films

Antiferromagnetic (AFM) materials have attracted wide attention in spin-orbit torque (SOT)-based spintronic due to its abundant spin-dependent properties and unique advantage of immunity against external field perturbations. To act as the charge-to-spin conversion source in energy-saving spintronic devices, it is of great importance for the AFM material to possess a large spin torque efficiency (ξDL). In this work, using the spin torque ferromagnetic resonance (ST-FMR) technique and a Mn2Au/NiFe(Py) bilayer system, we systemically study the ξDL of AFM Mn2Au films with different crystal structures. Compared with polycrystalline Mn2Au with effective ξDL < 0.051, we show a much larger ξDL of ~0.333 in single-crystal Mn2Au, which arises from the large spin Hall conductivity instead of electrical resistivity. Moreover, with a further contribution of interfacial effects, the effective ξDL of single-crystalline Mn2Au/Py system increases to 0.731, which is more than two times larger than the value of ∼0.22 reported for the Mn2Au/CoFeB system. By utilizing the large ξDL of Mn2Au in a perpendicularly magnetized MnGa/Mn2Au system, energy-efficient deterministic magnetization switching with a current density at ~106 A cm−2 is achieved. Our results reveal a significant potential of Mn2Au as an efficient SOT source and shed light on its application in future AFM material-based SOT integration technology.

Magnetization dynamics in ordered spin structures revealed by diffractive and reflectometry ferromagnetic resonance

Synchrotron radiation based techniques provide unique insight into both the element and time resolved magnetization behavior in magnetic spin systems. Here, we highlight the power of two recent developments, utilizing x-ray scattering techniques to reveal the precessional magnetization dynamics of ordered spin structures in the GHz regime, both in diffraction and reflection configurations. Our recently developed diffraction and reflectometry ferromagnetic resonance (DFMR and RFMR) techniques provide novel ways to explore the dynamics of modern magnetic materials, thereby opening up new pathways for the development of spintronic devices. In this paper we provide an overview of these techniques, and discuss the new understanding they provide into the magnetization dynamics in the chiral magnetic structure in Y-type hexaferrite and the depth dependence to the magnetization dynamics in a [CoFeB/MgO/Ta]4 multilayer.