Synchrotron Radiation Research Articles

Runaway electron plateau current profile reconstruction from synchrotron imaging and Ar-II line polarization angle measurements in DIII-D

Current profile reconstructions are obtained for high current ( Ip≃550 kA) post-disruption runaway electron (RE) plateau plasmas in DIII-D. Two novel methods of measuring the RE current profile in high-current RE plateaus are introduced and compared: localization of the q = 2 rational surface using visible synchrotron emission (SE) imaging and the measurement of the polarization angle of line-integrated Ar-II line emission. The two methods are found to be consistent with each other within the data uncertainties. Different simulations of the RE current profile are compared with the measurements: the toroidal fluid RE model is found to best fit the data, within the measurement uncertainties. In addition to introducing two novel methods to measure the RE current profile and validating present simulation capabilities, this work demonstrates that instabilities can grow at q = 2 and q = 1 surfaces without necessarily causing a RE final loss instability. Numerical simulations are also presented to elucidate the role of these instabilities on synchrotron emission.

EMA beamline at Sirius: A versatile platform to probe glass and glass ceramics under extreme thermodynamic conditions

AbstractGlass and glass ceramics are very functional materials, albeit their structural complexity. Their relevance ranges from fundamental science problems in the fields of physics, chemistry, and geoscience, to applications in health areas, engineering, or technological matters that require high performance. Enhancing our understanding of these materials' performance and refining sample preparation methods remains paramount in this field. Synchrotron facilities offer a suite of powerful techniques for the detailed characterization of glasses and glass ceramics. These methods provide valuable insights into their atomic and molecular structure, phase transformations, mechanical behavior, and thermal properties, ultimately contributing to the development of improved materials for a wide range of applications. In‐depth investigations conducted under extreme conditions of pressure and temperature have yielded pivotal insights into densification mechanisms, phase transitions, crystallization kinetics, and their consequential macroscopic properties. The emergence of fourth‐generation synchrotrons brings in a wave of novel experimental possibilities that may exert a profound influence on this field in the coming decade. In this study, we unveil a selection of the remarkable capabilities now accessible to researchers at the Brazilian Synchrotron Light Source—Sirius, within the realm of extreme methods of analysis (EMA) beamline for investigating vitreous systems under extreme conditions.

The laser pump X-ray probe system at LISA P08 PETRA III.

Understanding and controlling the structure and function of liquid interfaces is a constant challenge in biology, nanoscience and nanotechnology, with applications ranging from molecular electronics to controlled drug release. X-ray reflectivity and grazing incidence diffraction provide invaluable probes for studying the atomic scale structure at liquid-air interfaces. The new time-resolved laser system at the LISA liquid diffractometer situated at beamline P08 at the PETRA III synchrotron radiation source in Hamburg provides a laser pump with X-ray probe. The femtosecond laser combined with the LISA diffractometer allows unique opportunities to investigate photo-induced structural changes at liquid interfaces on the pico- and nanosecond time scales with pump-probe techniques. A time resolution of 38 ps has been achieved and verified with Bi. First experiments include laser-induced effects on salt solutions and liquid mercury surfaces with static and varied time scales measurements showing the proof of concept for investigations at liquid surfaces.

Optical absorption spectra in the far-infrared range and phonons of CdSe1−xTex thin films

Optical reflection spectra of CdSe1-xTex thin films deposited on quartz substrates are measured using the synchrotron radiation in the spectral range of 20–500 cm−1. The absorption bands of CdSe, CdTe, CdSe0.75Te0.25, CdSe0.5Te0.5, and CdSe0.25Te0.75 films are localized in the range of 20–220 cm−1. The imaginary parts of the dielectric function ε2(λ−1) of CdTe1-xSex crystals calculated in the framework of the density functional theory are in good agreement with the experimental reflection spectra of CdTe1-xSex films. The eigenvectors of the dynamical matrix CdTe1-xSex crystals are analyzed for several phonon modes to understand the difference between the frequency dependences of the calculated vibration density of states and the imaginary part of dielectric function ε2(λ−1). Small features of the experimental reflective spectra of CdSe1-xTex films in the ranges 50–70 cm−1 and 80–120 cm−1 are explained using the analysis of results of the molecular dynamics. During comparative molecular dynamics calculations, it was found that the vibration density of states of a thin CdTe slab with a surface-to-volume number of atoms relation of NS/NV = 0.2, experienced a redshift of approximately 30 cm−1. This shift was observed in comparison with the CdTe single crystal.

Dissociative adsorption of supersonic CH3Cl on Cu oxide Surfaces: Cu2O(111) and bulk Cu2O precursor “29”-Structure on Cu(111)

To examine the elementary steps of the Rochow-Müller process we placed copper oxides, viz., Cu2O(111) and the bulk Cu2O precursor “29”-structure on Cu(111), under supersonic molecular beams (SSMB) of CH3Cl. The SSMB energies range from 0.5-1.9 eV. We employed X-ray photoemission spectroscopy (XPS) in conjunction with synchrotron radiation (SR) to determine the resulting adsorbed species present. We identified two reaction paths, viz., Reaction I and Reaction II. Reaction I involves dissociative adsorption of CH3Cl. In Reaction II, CH3Cl also dissociates, but with Cl as the dominant adsorbed species (higher than that of adsorbed carbonaceous species, as observed for Reaction I). For the incident energies and exposure conditions considered, we found Reaction II as the dominant reaction path for CH3Cl reaction on both Cu2O(111) and the “29”-structure on Cu(111).

Structural phase transitions in multicomponent La0.2Nd0.2Sm0.2Gd0.2RE50.2NbO4 (RE5 = Ho, Y, Tb, Eu, Pr) oxides

AbstractIn this work, the influence of compositional complexity on the structural and thermal properties of multicomponent rare‐earth ortho‐niobates from the La0.2Nd0.2Sm0.2Gd0.2RE50.2NbO4 (RE5 = Ho, Y, Tb, Eu, Pr) series was investigated. Based on X‐ray powder diffraction studies using synchrotron radiation, it was found that all tested materials were pure single‐phase compositions and showed stability in the monoclinic I2/c crystal structure at room temperature. High‐temperature X‐ray powder diffraction studies and dilatometry studies confirmed the presence of a structural phase transition between low‐temperature (I2/c) and high‐temperature (I41/a) polymorphs. The structural phase transition temperatures are between 676°C and 701°C. Interestingly, despite their compositional complexity, the structural phase transition temperature behaves similarly to conventional ortho‐niobates, that is, it depends on the radius of the A‐cation; that is, as the ionic radius increases, the phase transition temperature decreases. The transition has been categorized as a second‐order phase transition based on the observed relationship between the Landau order parameter and spontaneous strain. The coexistence of the tetragonal and monoclinic phases has been seen in all compositions around the temperature of the structural phase transition. The presence of two orientation states in the monoclinic structure leads to the so‐called spontaneous strain, which consists of longitudinal (u) and shear (v) strain components. The values of these strains at 300°C range between 2.42 and 2.58 × 10−2 for longitudinal, 2.98 and 3.04 × 10−2 for shear, and 5.46 and 5.57 × 10−2 for scalar spontaneous strain. It was found that the spontaneous strain in each of the materials under test was very little impacted by the variation in the complexity of the A sublattice's composition. In addition, thermal expansion coefficients of both polymorphs were determined, which range from 12.7 × 10−6 K−1 to 13.2 × 10−6 K−1 for the monoclinic structure and 9.7 × 10−6 K−1 to 9.9 × 10−6 K−1 for the tetragonal one.

Decoding the Nature of Coherent Radio Emission in Pulsars I: Observational Constraints

Radio observations from normal pulsars indicate that the coherent radio emission is excited by curvature radiation from charge bunches. In this review, we provide a systematic description of the various observational constraints on the radio emission mechanism. We have discussed the presence of highly polarized time samples where the polarization position angle follow two orthogonal well-defined tracks across the profile that closely match the rotating vector model in an identical manner. The observations also show the presence of circular polarization, with both the right and left handed circular polarization seen across the profile. Other constraints on the emission mechanism are provided by the detailed measurements of the spectral index variation across the profile window, where the central part of the profile, corresponding to the core component, has a steeper spectrum than the surrounding cones. Finally, the detailed measurements of the subpulse drifting behaviour can be explained by considering the presence of non-dipolar field on the stellar surface and the formation of the partially screened gap (PSG) above the polar cap region. The PSG gives rise to a non-stationary plasma flow that has a multi-component nature, consisting of highly energetic primary particles, secondary pair plasma, and iron ions discharged from the surface, with large fragmentation resulting in dense plasma clouds and lower-density inter-cloud regions. The physical properties of the outflowing plasma and the observational constraints lead us to consider coherent curvature radiation as the most viable explanation for the emission mechanism in normal pulsars, where propagation effects due to adiabatic walking and refraction are largely inconsequential.

High Harmonic Generation Seeding Echo-Enabled Harmonic Generation toward a Storage Ring-Based Tender and Hard X-ray-Free Electron Laser

To align with the global trend of integrating synchrotron light source (SLS) and free electron laser (FEL) facilities on one site, in line with examples such as SPring-8 and SACLA in Japan and ELETTRA and FERMI in Italy, we actively explore FEL options leveraging the ultralow-emittance electron beam of the NSLS-II upgrade. These options show promising potential for synergy with storage ring (SR) operations, thereby significantly enhancing our facility’s capabilities. Echo-enabled harmonic generation (EEHG) is well-suited to SR-based FELs, and has already been demonstrated with the capability of generating extremely narrow bandwidth as well as high brightness, realized using diffraction-limited short pulses in transverse planes and Fourier transform-limited bandwidth in the soft X-ray spectrum. However, regarding a conventional EEHG scheme, the combination of the shortest seed laser wavelength (256 nm) and highest harmonic (200) sets the short wavelength limit to λ = 1.28 nm. To further extend the short wavelength limit down to the tender and hard X-ray region, a vital option is to shorten the seed laser wavelength. Thanks to recent advances in high harmonic generation (HHG), packing 109 photons at one harmonic within a few-femtosecond pulse could turn such a novel HHG source into an ideal seeding for EEHG. Thus, compared to the cascaded EEHG, the HHG seeding option could not only lower the cost, but also free the SR space for accommodating more user beamlines. Moreover, to mitigate the SASE background noise on the sample and detector, we combine the HHG seeding EEHG with the crab cavity short pulse scheme for maximum benefit.

Glucocorticoids disrupt longitudinal advance of cortical bone basic multicellular units in the rabbit distal tibia

Glucocorticoids (GCs) are the leading cause of secondary osteoporosis. The emerging perspective, derived primarily from 2D histological study of trabecular bone, is that GC-induced bone loss arises through the uncoupling of bone formation and resorption at the level of the basic multicellular unit (BMU), which carries out bone remodeling. Here we explore the impact of GCs on cortical bone remodeling in the rabbit model. Based upon the rapid reduction of bone formation and initial elevation of resorption caused by GCs, we hypothesized that the rate of advance (longitudinal erosion rate; LER) of cortical BMUs would be increased. To test this hypothesis we divided 20 female New Zealand White rabbits into four experimental groups: ovariohysterectomy (OVH), glucocorticoid (GC), OVH + GC and SHAM controls (n = 5 animals each). Ten weeks post-surgery (OVH or sham), and two weeks after the initiation of dosing (daily subcutaneous injections of 1.5 mg/kg of methylprednisolone sodium succinate in the GC-treated groups and 1 ml of saline for the others), the right tibiae were scanned in vivo using Synchrotron Radiation (SR) in-line phase contrast micro-CT at the Canadian Light Source. After an additional 2 weeks of dosing, the rabbits were euthanized and ex vivo images were collected using desktop micro-CT. The datasets were co-registered in 3D and LER was calculated as the distance traversed by BMU cutting-cones in the 14-day interval between scans. Counter to our hypothesis, LER was greatly reduced in GC-treated rabbits. Mean LER was lower in GC (4.27 μm/d; p < 0.001) and OVH + GC (4.19 μm/d; p < 0.001), while similar in OVH (40.13 μm/d; p = 0.990), compared to SHAM (40.44 μm/d). This approximately 90 % reduction in LER with GCs was also associated with an overall disruption of BMU progression, with radial expansion of the remodeling space occurring in all directions. This unexpected outcome suggests that GCs do not simply uncouple formation and resorption within cortical BMUs and highlights the value of the time-lapsed 4D approach employed.

A novel generation design dipole magnet power supply of booster to storage ring transport line in NSRRC

The Taiwan Light Source (TLS) is a synchrotron radiation facility located in Taiwan. The booster ring at TLS injects electrons into the storage ring, which then circulates the electrons to produce synchrotron radiation for various experiments. The Taiwan Light Source (TLS) has been in service for more than 20 years, and some of the power supplies used in the facility are old and hard to maintain repair and the component are phase-out. The upgrade is specifically aimed at replacing the power supply for the BTS (Booster to Storage ring) transmission line with a new machine. During the regular shunt down time, dipole magnet power supply replacements were completed. The main reason for using the Chroma 62075H-30E power supply is commonality, for this machine is widely used in Taiwan Photon Source (TPS), and the output current of the power supply is paralleled to a dipole magnet. Therefore, a total of 17 power supplies are used in this upgrade planned to be executed. This novel generation upgrade design is important because the power supply for the BTS transmission line is critical for the operation of the facility, as it is responsible for maintaining the electron beam at a stable energy level as it is injected from the booster ring into the storage ring. A more reliable and efficient power supply can help improve the stability and quality of the electron beam, leading to better experimental results and more efficient use of the facility. Overall, this novel generation upgrade design is part of the ongoing effort to modernize and improve the infrastructure of the TLS, ensuring that it remains a state-of-the-art research facility for years to come.

Comparison of two vacuum system technologies for the synchrotron storage ring: case study of Iranian Light Source Facility

The current study compares two vacuum system designs for the Iranian Light Source Facility (ILSF) storage ring: conventional vacuum system design with stainless-steel vacuum chambers that are pumped by Non-Evaporable Getter (NEG) cartridges and ion pumps. In this design, all synchrotron radiation is absorbed by the local photon absorbers. In the second design, the water-cooled copper tubes that are coated with NEG materials are used as the vacuum chambers. This study will illustrate the advantages of using the NEG-coated vacuum chambers over the conventional design with the stainless-steel chambers. Since the two designs for ILSF are now completed, some of the details of this comparison might be interesting to other light sources, especially those that have plans to upgrade to a 4th generation.

Real-time structural characterization of protein response to a caged compound by fast detector readout and high-brilliance synchrotron radiation

Protein dynamics are essential to biological function, and methods to determine such structural rearrangements constitute a frontier in structural biology. Synchrotron radiation can track real-time protein dynamics, but accessibility to dedicated high-flux single X-ray pulse time-resolved beamlines is scarce and protein targets amendable to such characterization are limited. These limitations can be alleviated by triggering the reaction by laser-induced activation of a caged compound and probing the structural dynamics by fast-readout detectors. In this work, we established time-resolved X-ray solution scattering (TR-XSS) at the CoSAXS beamline at the MAX IV Laboratory synchrotron. Laser-induced activation of caged ATP initiated phosphoryl transfer in the adenylate kinase (AdK) enzyme, and the reaction was monitored up to 50ms with a 2-ms temporal resolution achieved by the detector readout. The time-resolved structural signal of the protein showed minimal radiation damage effects and excellent agreement to data collected by a single X-ray pulse approach.

Effect of post-weld heat treatment on the microstructure, phase composition and mechanical properties of dissimilar Al-Mg-Li/Al-Cu-Li laser welded joints

Butt joints of the V-1461 and 1424 heat treated aluminum–lithium alloys of the third generation were welded with a CO2 laser and studied in detail for the first time. In particular, spatial distributions of the formed phases and their evolution upon post-weld heat treatment (PWHT), determining the mechanical properties of the joints, were investigated. The PWHT included quenching and subsequent artificial aging. The key factors, affecting the metallurgical processes in a weld pool, were the following: 1) the alloying elements and the thermal properties of the alloys, 2) the dynamics of the local non-equilibrium melting, the convective transfer of the molten metal in the weld pool and its subsequent solidification, 3) the cooling rate, and 4) the PWHT procedure. By using synchrotron radiation and scanning electron microscopy, new θ(Al2Cu), T1(Al2CuLi) and S1(Al2MgLi) phases were found in the weld metal that were absent in both base metals. This phenomenon reduced the mechanical properties of the joints to the levels, corresponding to about 50 % of the 1424 alloy as the weakest one. Quenching contributed to the formation of the δ′(Al3Li) strengthening phase in the weld metal. As a result, the ultimate tensile strength increased up to 70 % and elongation up to 95 % of the corresponding levels of the 1424 alloy. Artificial aging made it possible to form the T1(Al2CuLi) strengthening phase, to increase the content of the δ′(Al3Li) one, as well as to improve the mechanical properties of the joint. In this case, the ultimate tensile strength was 411 MPa, the yield point was 327 MPa and elongation was 1.7 %. These values were close to those for the 1424 alloy (about 80 %, 89 % and 23 %, respectively).

Stochastic Averaging of Radiative Transfer Coefficients for Relativistic Electrons

Synchrotron emissivities, absorptivities, and Faraday rotation and conversion coefficients are needed in modeling a variety of astrophysical sources, including Event Horizon Telescope (EHT) sources. We develop a method for estimating transfer coefficients that exploits their linear dependence on the electron distribution function, decomposing the distribution function into a sum of parts each of whose emissivity can be calculated easily. We refer to this procedure as stochastic averaging and apply it in two contexts. First, we use it to estimate the emissivity of an isotropic κ distribution function with a high-energy cutoff. The resulting coefficients can be evaluated efficiently enough to be used directly in ray-tracing calculations, and we provide an example calculation. Second, we use stochastic averaging to assess the effect of subgrid turbulence on the volume-averaged emissivity and along the way provide a prescription for a turbulent emissivity. We find that for parameters appropriate to EHT sources turbulence reduces the emissivity slightly. In the infrared, turbulence can dramatically increase the emissivity.

A computing module for speeding up the bunch-by-bunch measurement of transverse positions and transverse profiles within injection period

The Multi-Bend-Achromat (MBA) structure of the Diffraction-limited Synchrotron Light Source (DLSR) makes the dynamic range of its injection significantly smaller, thus posing a more demanding challenge for the stable injection of beams. To investigate the possible instabilities during the injection process, multi-anode photomultiplier tubes (MAPMT) are used in bunch-by-bunch measurements to obtain the transverse positions and transverse profiles of the bunched beams as they are injected. However, the data processing time witnessed in prior measurements posed a significant challenge in obtaining this information in time, thus failing to meet the stringent demands of online measurements. Consequently, this paper proposes one computing module, engineered to enhance the speed of bunch-by-bunch measurements of transverse positions and profiles. This solution is capable of delivering measurement results for each bunch in the filling pattern, all within the specified injection period.

A study of the latest updates of the readout system for the hybird-pixel detector at HEPS

The High Energy Photon Source (HEPS) represents a fourth-generation light source. This facility has made unprecedented advancements in accelerator technology, necessitating the development of new detectors to satisfy physical requirements such as single-photon resolution, large dynamic range, and high frame rates. Since 2016, the Institute of High Energy Physics has introduced the first user-experimental hybrid pixel detector, progressing to the fourth-generation million-pixel detector designed for challenging conditions, with the dual-threshold single-photon detector HEPS-Beijing PIXel (HEPS-BPIX) set as the next-generation target. HEPS-BPIX will employ the entirely new Application-Specific Integrated Circuit (ASIC) BP40 for pixel information readout. Data flow will be managed and controlled through readout electronics based on a two-tier Field-Programmable Gate Array (FPGA) system: the Front-End Electronics (FEE) and the Input-Output Board (IOB) handle the fan-out for 12 ASICs, and the μ4FCP is tasked with processing serial data on high-speed links, transferring pixel-level data to the back-end RTM and μTCA chassis, or independently outputting through a network port, enabling remote control of the entire detector. The new HEPS-BPIX firmware has undergone a comprehensive redesign and update to meet the electronic characteristics of the new chip and to improve the overall performance of the detector. We provide an overview of the core subunits of HEPS-BPIX, emphasizing the readout system, evaluating the new hardware and firmware, and highlighting some of its innovative features and characteristics.

L-series X-ray fluorescence cross section measurements for 72Hf employing synchrotron radiation

In the present work, the Hf target was irradiated by tuning the energy (Ep) of synchrotron radiation across the Li (i = 1–3) edge-energies ranging from 9.6 keV to 14.0 keV in order to measure the cross sections for production of the fluorescent Lk X-rays (k = l, α, η, β1,6, β3, β4, β2,15, β5,7, β9,10, γ1,5, γ2,3,6,8, γ4). These measurements were performed with the aim to check the validity of independent particle approximation (IPA) models at incident photon energies in proximity to the Li absorption edges of a heavy transition element. The measured cross sections were compared with three sets of values calculated using the X-ray emission rates based on the Dirac-Fock model, the Li (i = 1–3) sub-shell photoionization cross-sections based on the non-relativistic Hartree-Fock-Slater model and three sets of the fluorescence (ωi) and Coster-Kronig (fji) yields.

On the Theory of Diffraction of Limited Synchrotron Radiation Beams in Single Crystal in the Laue Case

On the Theory of Diffraction of Limited Synchrotron Radiation Beams in Single Crystal in the Laue Case

Optical Spectropolarimetric Variability Properties in Blazars PKS 0637–75 and PKS 1510–089

Spectropolarimetry is a powerful tool to investigate the central regions of active galactic nuclei (AGNs) as polarization signatures are key to probing magnetic field structure, evolution, and the physics of particle acceleration in jets. Optical linear polarization of blazars is typically greater than a few percent, indicating the emission is dominated by nonthermal synchrotron radiation, while polarization less than a few percent is common for other type 1 AGNs. We present a spectropolarimetric study of PKS 0637–75 and PKS 1510–089 to determine how the head-on orientation of a jet and dominant emission processes influence polarimetric variations in the broad lines and continuum. Observations were obtained biweekly from the Robert Stobie Spectrograph on the Southern African Large Telescope. Variability in the continuum polarization is detected for both PKS 0637–75 and PKS 1510–089, with a total average level of 2.5% ± 0.1% and 7.5% ± 0.1%, respectively. There is no clear polarization in the broad Balmer emission lines and weak polarization in Mg ii as the average level across all observations is 0.2% ± 0.1% for Hβ, 0.2% ± 0.3% for Hγ, and 0.6% ± 0.2% for Mg ii. We find that polarization measurements confirm the conclusions drawn from spectral energy distribution modeling of the disk–jet contributions to the emission as optical polarization and time variability for PKS 0637–75 are shown to be dominated by accretion disk emission while those of PKS 1510–089 are due to both disk and jet emission, with greater jet contribution during flaring states.

In-situ Synchrotron Radiation XRD Crystal Structure and Microstructure Analysis of CaO-ZrO2 solid-solution at 1100°C with Prolonged Heating

Abstract The structural analysis of the CaO-ZrO2 solid-solutions was carried out using in-situ synchrotron radiation X-ray diffraction (SR-XRD). CaO-ZrO2 solid-solutions with 0, 2.5, and 5 at.% CaO contents were synthesized via a solid-solid ball milling technique. The amorphous ZrO2 powder was synthesized via co-precipitation using ZrCl4 and NH4OH as precursors, while the CaO powder was purified from a local limestone. In-situ SR-XRD measurements were conducted on the CaO-ZrO2 mixtures by independently heating them to 1100°C for different holding times of 0, 12, 24, and 36 minutes using a DHS furnace. Qualitative analysis of all SR-XRD patterns showed that only tetragonal zirconia (t-ZrO2) was present. The crystallite size of tetragonal zirconia ranged from 17 to 22 nm, depending on calcination holding time and CaO addition. Further analysis showed that the tetragonality (c/a) parameter remained relatively constant over the 36-minute holding time. However, the introduction of CaO led to an insignificant reduction in tetragonality, averaging 0.292%.