Single Pulse Research Articles

Single-crystal silicon ablation with temporally delayed femtosecond laser double-pulse trains

Abstract A double-pulse femtosecond laser is used to process single-crystal silicon. Modulating the delay time was discovered to increase the ablation depth and improve the morphology of the ablated surface. The hole fabricated by a dual-pulse with a 200 ps interval is 24.4% deeper than that created by a single pulse of the same energy. Moreover, utilizing a dual pulse with an interval ranging from 100 to 1000 ps produces a considerably smoother ablation area as compared to the single pulse. The effect of the sub-pulse energy ratio of the double-pulse femtosecond laser on the size and morphology of the ablated area was also investigated. As the sub-pulse energy ratio decreases from 3:1 to 1:3, the size of the ablation area initially decreases and then increases, while the size of the ablation area is minimized when the sub-pulse ratio is 1:1, enabling precise control over the machining size. As the energy of the second sub-pulse increases, the ablation area becomes smoother due to the plasma heating of the double-pulse femtosecond laser.

Repetitive Transcranial Magnetic Stimulation Modulates Brain Connectivity in Children with Self-limited Epilepsy with Centrotemporal Spikes.

Interictal epileptiform discharges (IEDs) alter brain connectivity in children with epilepsy; this connectivity change may be a mechanism by which epilepsy induces cognitive deficits. Here, we test whether repetitive transcranial magnetic stimulation (rTMS), a non-invasive neuromodulation technique, modulates connectivity and reduces IEDs in children with epilepsy. Nineteen children with self-limited epilepsy with centrotemporal spikes (SeLECTS) participated in a cross-over study comparing the impact of active vs. sham rTMS on IEDs and brain connectivity. SeLECTS is an epilepsy syndrome affecting the motor cortex, and prior studies show that motor cortices become pathologically hyper-connected to frontal and temporal language cortices. Using a crossover design, we compared the effect of single doses of active versus sham motor cortex rTMS. Connectivity, which was quantified by the weighted phase lag index (wPLI), was measured before and after rTMS using single pulses of TMS combined with EEG (spTMS-EEG). Analyses focused on six regions: bilateral motor cortices and bilateral inferior frontal and superior temporal regions. IEDs were counted in the five minutes before and after rTMS. Active, but not sham, rTMS significantly and globally decreased wPLI connectivity between multiple regions, with the greatest reductions seen in the superior temporal region connections in the stimulated hemisphere. Additionally, there was a trend suggesting that rTMS decreases IED frequency. These findings underscore the potential of low-frequency rTMS to target pathologic hyperconnectivity and reduce IEDs in children with SeLECTS and potentially other pediatric epilepsy syndromes, offering a promising avenue for therapeutic intervention.

Design and optimization of a high thrust density air-breathing pulsed plasma thruster array

For satellites in Very Low Earth Orbit (VLEO) or the upper atmosphere, Air-Breathing Electric Propulsion (ABEP) can be used to counteract the drag effects of the atmosphere or provide attitude control without the need for onboard propellant storage. The Dense Plasma Focus (DPF) inspired the design of an ABEP Pulsed Plasma Thruster (TAMU PPT) which takes advantage of the simplicity, scalability, and high energy density of the DPF. This work details the design and testing of a PPT for use on satellites in the upper atmosphere. Testing was conducted at a variety of pressures and pulsing energies to determine which conditions provide maximum thrust and thrust to power ratios (TPR). It was found through single pulse experiments that a pressure of 6.3 hPa (corresponding to an altitude of about 35 km) and an energy per pulse of 9 J yield a TPR of 21 mN/kW. High frequency operation at 20 Hz in similar conditions showed a TPR of up to 28 mN/kW with a corresponding thrust of 4.8 mN. High speed imaging of the plasma plume found plasma velocities in excess of 2 km/s and identified metal ejecta with velocities up to 350 m/s. The pinching phenomenon associated with a DPF was also observed and a plasma jet velocity up to 50 km/s was recorded. The TPR of the TAMU PPT demonstrated in this work is comparable to that of other ABEP thrusters, however the TAMU PPT has an advantage when comparing thrust density. The TAMU PPT has a thrust density between 4.8 and 19 mN/cm2 while other ABEP thrusters have thrust densities between 0.019 and 0.36 mN/cm2.

PSR B0943+10: Mode Switch, Polar Cap Geometry, and Orthogonally Polarized Radiation

As one of the paradigm examples to probe into pulsar magnetospheric dynamics, PSR B0943+10 (J0946+0951) manifests representatively, showing a mode switch, orthogonal polarization, and subpulse drifting, frequently studied below 600 MHz. Here, both integrated and single pulses are studied at a high frequency (1.25 GHz) with FAST. The mode switch is studied using a profile decomposition method. A phase space evolution for the pulsar’s mode switch shows a strange-attractor-like pattern. The radiative geometry is proposed by fitting polarization position angles with the rotating vector model. The pulsar pulse profile is then mapped to the sparking locations on the pulsar surface, and the differences between the main pulse’s and the precursor component’s radiative processes may explain the X-ray’s synchronization with radio mode switch. Detailed single pulse studies on B0943+10's orthogonally polarized radiation are presented, which may support certain models of radiative transfer of polarized emission. In particular, the difference in orthogonal polarization modes’ circular polarization might reflect the cyclotron absorption in pulsar magnetospheres. B0943+10's B and Q modes evolve differently with frequency and have different proportions of orthogonal modes, which indicates possible magnetospheric changes during mode switch. For Q mode pulse profile, the precursor and the main pulse components are orthogonally polarized, and are probably originated from different depths in the magnetosphere. The findings could impact significantly on the pulsar electrodynamics and the radiative mechanism related.

Consecutive diagnosis of nanosecond pulsed discharge in a coaxial electrode configuration using a quadruple emICCD camera system

Abstract Understanding the rapid dynamics of the primary streamer is crucial for comprehending the nanosecond pulsed discharge process. To reveal the fast primary streamer process, this study introduces a newly developed quadruple emICCD camera system capable of capturing a sequence of four discharge images in single pulse, coupled with self-customized software for data analysis. A nanosecond pulse power with its FWHM of 10.5 ns was applied to a coaxial reactor, focusing on the dynamics of the primary streamer. Our research clarifies the spatiotemporal variations of the primary streamer’s properties and examines their relation with inner electrode diameter (i.d. 0.2–2.0 mm). Results showed that in a pulse-powered coaxial electrode, there are three stages in the primary streamer process and that i.d. serves as an important factor influencing the formation and propagation of streamers. Interestingly, we found that streamer head velocity, streamer width, and streamer area for individual streamers remain constant prior to streamer channels reaching the outer electrode. Furthermore, we also observed an initial increase followed by a decrease in both streamer head velocity and streamer width with increasing i.d values. This study sheds light on the fundamental properties of the primary streamer during nanosecond pulsed discharge, contributing valuable insights for future plasma applications.

Sudden Polarization Angle Jumps of the Repeating Fast Radio Burst FRB 20201124A

We report the first detection of polarization angle orthogonal jumps, a phenomenon previously only observed from radio pulsars, from a fast radio burst (FRB) source FRB 20201124A. We find three cases of orthogonal jumps in over 2000 bursts, all resembling those observed in pulsar single pulses. We propose that the jumps are due to the superposition of two orthogonal emission modes that could only be produced in a highly magnetized plasma, and they are caused by the line of sight sweeping across a rotating magnetosphere. The shortest jump timescale is of the order of 1 millisecond, which hints that the emission modes come from regions smaller than the light cylinder of most pulsars or magnetars. This discovery provides convincing evidence that FRB emission originates from the complex magnetosphere of a magnetar, suggesting an FRB emission mechanism that is analogous to radio pulsars despite a huge luminosity difference between two types of objects.

Fabrication of Photonic Crystal Structures on GaAs by Single Pulse Laser Interference Lithography

Fabrication of Photonic Crystal Structures on GaAs by Single Pulse Laser Interference Lithography

Investigation on Single Pulse Failure of Avalanche Transistors Triggered by Voltage Ramps in Marx Bank Circuits

Investigation on Single Pulse Failure of Avalanche Transistors Triggered by Voltage Ramps in Marx Bank Circuits

Effect of laser scanning frequency on the optical transmittance of the welded area in glass laser welding

Abstract When conventionally laser-welding transparent materials such as glass, researchers often primarily focus on the material’s joint strength, paying scant attention to variations in optical transmittance within the welding zone. However, in fields like biomedical applications, optical characteristics are also pivotal in characterizing the efficacy of welding. Therefore, this study investigated the relationship between scanning frequency and optical transmittance during laser welding. The findings indicate that a laser single pulse energy of 14.73 μJ, a repetition frequency of 500 kHz, a scanning speed of 600 mm/s, and an optimal scanning frequency of 45 times yielded the highest optical transmittance in the welding area. This resulted in a 13% increase in transmittance compared to stacking two glass pieces.

Single-pulse ultrafast real-time simultaneous planar imaging of femtosecond laser-nanoparticle dynamics in flames

The creation of carbonaceous nanoparticles and their dynamics in hydrocarbon flames are still debated in environmental, combustion, and material sciences. In this study, we introduce single-pulse femtosecond laser sheet-compressed ultrafast photography (fsLS-CUP), an ultrafast imaging technique specifically designed to shed light on and capture ultrafast dynamics stemming from interactions between femtosecond lasers and nanoparticles in flames in a single-shot. fsLS-CUP enables the first-time real-time billion frames-per-second (Gfps) simultaneous two-dimensional (2D) imaging of laser-induced fluorescence (LIF) and laser-induced heating (LIH) that are originated from polycyclic aromatic hydrocarbons (PAHs) and soot particles, respectively. Furthermore, fsLS-CUP provides the real-time spatiotemporal map of femtosecond laser-soot interaction as elastic light scattering (ELS) at an astonishing 250 Gfps. In contrast to existing single-shot ultrafast imaging approaches, which are limited to millions of frames per second only and require multiple laser pulses, our method employs only a single pulse and captures the entire dynamics of laser-induced signals at hundreds of Gfps. Using a single pulse does not change the optical properties of nanoparticles for a following pulse, thus allowing reliable spatiotemporal mapping. Moreover, we found that particle inception and growth are derived from precursors. In essence, as an imaging modality, fsLS-CUP offers ultrafast 2D diagnostics, contributing to the fundamental understanding of nanoparticle’s inception and broader applications across different fields, such as material science and biomedical engineering.

Single-pulse three-dimensional parallel recording in glass using a feedback system.

High-quality three-dimensional computer-generated holograms (3D-CGHs) are crucial for programmable 3D femtosecond laser parallel recording (3D-FLPR). In this study, we introduced an innovative feedback approach for the rapid optimization of 3D-CGHs by incorporating the superposition of the calculated lens phases (CLPs) onto the 3D-CGHs within a feedback system. This feedback system, governed by coordinated control of a spatial light modulator (SLM) and a camera, served to avoid the poor quality of the ordinary CGH system. As a result, we successfully demonstrated coaxial 3D-FLPR in Ag-doped phosphate glass solely using a single fs laser pulse. Additionally, we regulated the energy distribution of the generated 3D multi-focus (3D-MF) to compensate the laser energy losses inside the glass. The presented single-pulse 3D parallel recording indicated the significant advancement facilitated by our method, particularly in enhancing the writing efficiency of optical storage.

Self-Heterodyne Diffractive Imaging of Ultrafast Electron Dynamics Monitored by Single-Electron Pulses.

The direct imaging of time-evolving molecular charge densities on atomistic scale and at femtosecond resolution has long been an elusive task. In this theoretical study, we propose a self-heterodyne electron diffraction technique based on single electron pulses. The electron is split into two beams, one passes through the sample and its interference with the second beam produces a heterodyne diffraction signal that images the charge density. Application to probing the ultrafast electronic dynamics in Mg-phthalocyanine demonstrates its potential for imaging chemical dynamics.

X-Band Single Chip Integrated Pulsed Electron Spin Resonance Microsystem.

We report on the design and characterization of a single chip integrated pulsed electron spin resonance detector operating at 9.1 GHz. The microsystem consists of an excitation microcoil, a detection microcoil, a low noise microwave preamplifier, a mixer, and an intermediate frequency (IF) amplifier. The chip area is about 0.7 mm2. To exemplify its possible applications, we report the results of single pulse, Rabi nutation, Hahn echo, two echoes, Carr-Purcell, and inversion recovery echo experiments performed on 0.02 and 0.05 nL samples of α, γ-bisdiphenylene-β-phenylallyl (BDPA) and 1% BDPA in polystyrene (BDPA:PS) at room temperature. The measured spin sensitivity is about 8 × 107 spins/Hz1/2 on a sensitive volume of about 0.1 nL. The microsystem power consumption is less than 100 mW, the radio frequency (RF) input bandwidth is 8.8 to 9.8 GHz, the IF output bandwidth is DC to 350 MHz, and the deadtime is less than 30 ns.

Controllable Preparation of Fused Silica Micro Lens Array through Femtosecond Laser Penetration-Induced Modification Assisted Wet Etching.

As an integrable micro-optical device, micro lens arrays (MLAs) have significant applications in modern optical imaging, new energy technology, and advanced displays. In order to reduce the impact of laser modification on wet etching, we propose a technique of femtosecond laser penetration-induced modification-assisted wet etching (FLIPM-WE), which avoids the influence of previous modification layers on subsequent laser pulses and effectively improves the controllability of lens array preparation. We conducted a detailed study on the effects of the laser single pulse energy, pulse number, and hydrofluoric acid etching duration on the morphology of micro lenses and obtained the optimal process parameters. Ultimately, two types of fused silica micro lens arrays with different focal lengths but the same numerical aperture (NA = 0.458) were fabricated using the FLPIM-WE technology. Both arrays exhibited excellent geometric consistency and surface quality (Ra~30 nm). Moreover, they achieved clear imaging at various magnifications with an adjustment range of 1.3×~3.0×. This provides potential technical support for special micro-optical systems.

Artificial synapse based on low-voltage Ni-doped CuI thin-film transistors for neuromorphic application

Inspired by the human brain's capacity as a powerful biological computer capable of simultaneously processing a vast array of cognitive tasks, many emerging artificial synapse devices have been developed in recent years. Electric-double-layer (EDL) transistors based on interfacial ion-modulation have attracted widespread attention for simulating synaptic plasticity and neural functions. Here, low-voltage EDL p-type thin-film transistors (TFTs) are fabricated on glass substrates, with Ni-doped cuprous iodide (Ni0.06Cu0.94I) as the channel and chitosan as the dielectric. The electrical performance of the Ni0.06Cu0.94I TFTs is investigated: current on/off ratio of 6.4 × 104, subthreshold swing of 33 mV/dec, threshold voltage of 1.38 V, operating voltage of 2 V, and saturation field-effect mobility of 15.75 cm2 V−1 s−1. A dual in-plane gate OR logic operation is demonstrated. Importantly, by applying single voltage pulses, dual voltage pulses, and multiple voltage pulses to the gate, the Ni0.06Cu0.94I transistors exhibited typical synaptic characteristics, including short-term potentiation, short-term depression, long-term potentiation, long-term depression, paired-pulse facilitation, and spiking-rate-dependent plasticity. Furthermore, the synaptic transistor can also simulate the learning–forgetting–relearning process of the human brain. These remarkable behaviors of voltage-stimulated synaptic transistors have potential for neuromorphic applications in future artificial systems.

Characterization of Micro-Holes Drilled Using a UV Femtosecond Laser in Modified Polyimide Flexible Circuit Boards.

Modified polyimide (MPI) flexible printed circuits (FPCs) are used as chip carrier boards. The quality of the FPC directly affects the reliability of the integrated circuit. Furthermore, micro-holes are critical components of FPCs. In this study, an ultraviolet (UV) femtosecond laser is used to drill micro-holes in double-layer flexible circuit boards with MPI as the substrate. The morphology of the micro-hole wall in the copper foil and MPI layer is observed, and the effects of the laser processing parameters on the diameter and depth of the micro-holes are analyzed. The drilling process and mechanism of micro-holes obtained using a UV femtosecond laser in MPI FPCs are discussed. The results show that the morphology of femtosecond laser-machined copper is closely related to the laser energy, and a periodic structure is observed during the machining process. Copper, MPI, and copper oxides are the most common molten deposits in micro-holes during drilling. The depth of the micro-holes increases with an increase in the energy of a single pulse, scanning time, and scanning overlap rate of the laser beam. However, the diameter exhibits no discernible alteration. The material removal rate increased significantly when laser processing was applied to the MPI resin layer.

RRAT J1913+1330: An Extremely Variable and Puzzling Pulsar

Rotating radio transients (RRATs) are neutron stars that emit sporadic radio bursts. We detected 1955 single pulses from RRAT J1913+1330 using the 19 beam receiver of the Five-hundred-meter Aperture Spherical radio Telescope. These pulses were detected in 19 distinct clusters, with 49.4% of them occurring with a waiting time of one rotation period. The energy distribution of these individual pulses exhibited a wide range, spanning 3 orders of magnitude, reminiscent of repeating fast radio bursts (FRBs). Furthermore, we observed abrupt variations in pulse profile, width, peak flux, and fluence between adjacent sequential pulses. These findings suggest that this RRAT could be interpreted as a pulsar with extreme pulse-to-pulse modulation. The presence of sequential pulse trains during active phases, along with significant pulse variations in profile, fluence, flux, and width, should be intrinsic to a subset of RRATs. Our results indicate that J1913+1330 represents a peculiar source that shares certain properties with populations of nulling pulsars, giant pulses, and FRBs from different perspectives. The dramatic pulse-to-pulse variation observed in J1913+1330 could be attributed to unstable pair creation above the polar cap region and the variation of the site where streaming pairs emit coherently. Exploring a larger sample of RRATs exhibiting similar properties to J1913+1330 has the potential to significantly advance our understanding of pulsars, RRATs, and FRBs.

Infrared microlens formation on chalcogenide polymer surface via femtosecond laser pulse ablation

In this study, we introduced micro-optical surface formation via femtosecond (fs) laser pulse scanning to chalcogenide polymer (ChP), a promising material for cost-effective infrared applications. Employing this method, we successfully fabricated a large-area poly(sulfur-random-(1,3-diisopropenylbenzene)) (S-r-DIB) microlens array (MLA) component. Each micro-concave spherical surface was crafted with a single fs laser pulse, serving as a micro-concave lens surface. We achieved a quasi-periodic MLA sample with over 2 × 105 micro-lenslets within a 10 mm × 10 mm footprint. Additionally, precise locating of laser pulse irradiation enabled us to create a hexagonal MLA with a filling factor over 37 %. Morphological investigations and imaging tests confirmed the adequate surface quality of the fabricated components, with its uniformity revealed by the virtual foci grid in near infrared region. To elucidate the forming conditions and mechanisms, we studied the evolution of surface morphology under various laser irradiation conditions. Laser induced damage thresholds of S70-r-DIB30 were experimentally determined for both 800 nm and 400 nm wavelengths under single- and multi-pulse irradiation scenarios. We identified the optimal fabrication fluence window as 115–205 mJ/cm2 with 800 nm single-pulse irradiation. The bandgap of the S70-r-DIB30 was estimated as 2.06 eV, and energy band analysis confirmed distinctions in ablation morphology. Furthermore, we investigated sub-surface morphology evolution using orthogonal ultrafast pump–probe imaging, revealing diversity compared to traditional inorganic and polymeric optical materials due to differing absorption and etching mechanisms. The elastic wave velocity of 3.2 km/s in this ChP and etching velocity of 0.7 μm/pulse were experimentally determined. These findings deepen our understanding of ChP material interaction with fs lasers, offering insights for potential applications such as surface engineering, substrate cutting, and micro-structure formation.

Unveiling Ultrafast-Weak-Field Coherent Control of Indirect Dissociation Reactions.

Coherent control of molecular photodissociation through one-photon transitions has become a topic of interest in physical chemistry. Previous studies have shown that modulating the spectral phase of a single ultrafast laser pulse while keeping its spectral amplitude constant does not affect the dissociation yield of reactions originating from a pure eigenstate of the ground electronic state. Here, we explore the indirect photodissociation reaction of NaI molecules using theoretical and numerical methods. Our findings show that, in contrast to the outcomes achieved with negatively chirped pulses, time-dependent population of the eigenstates of the excited adiabatic potential induced by positively chirped laser pulses, acting as intermediates in the reaction, cannot be periodically restored to that caused by the unchirped pulse. This gives rise to an intriguing phenomenon: the sign of the pulse's chirp rate influences the distribution of dissociation fragments in coordinate and momentum space over extended periods. This work highlights the potential of using spectral-phase modulated pulses to manipulate indirect photodissociation reactions, offering a way to modify the transient photofragment distributions by controlling reaction intermediates.

Dynamic response of dry sands subjected to dual patch impact loads of a wheeled helicopter

Dual patch impact loads are applied through two tires attached to a single landing gear during the landing of wheeled helicopters. To investigate the dynamic response of dry sands under dual patch impact loads from wheeled helicopters, model tests and validated numerical simulations were performed. The findings reveal that the settlement pattern in the shallow sand layer exhibits a characteristic W-shape, with the maximum settlement occurring directly beneath the center of each tamper. The time-history curve of the vertical dynamic pressure along the centerline of each tamper shows a single peak pulse with a duration of approximately 0.01 s. The peak value diminishes with increasing depth. Both the settlement and dynamic vertical soil pressure are dependent on impact energy, increasing as impact energy rises. The center-to-center spacing between the two tampers has a minimal effect on the maximum settlement and peak dynamic soil pressure along the centerline of each tamper. However, it significantly affects the maximum settlement and peak dynamic soil pressure along the centerline between the two tampers. As the spacing increases, the maximum settlement and peak dynamic soil pressure along the centerline between the two tampers decrease due to the attenuation of interaction between the two tampers.