As space science advances, the significance of space robotics research escalates, particularly in control methodologies. Addressing the work efficiency requirements during the mission of the in-cabin robot, it is necessary to develop a fast and robust position and attitude coupling controller for in-cabin robots. This paper presents a predefined-time sliding mode position and attitude coupling control method, employing the SE(3) frame description. The first, the dynamic model of the in-cabin robot is developed within the SE(3) framework. Then, the predefined-time position and attitude coupling sliding mode controller is designed with a sliding surface based on the dynamic error model, and a hyperbolic tangent function is used to suppress system chattering. In addition, the stability of the proposed control method is rigorously confirmed using the Lyapunov theorem, ensuring that the convergence time is accurately predefined. Finally, simulation results are provided to demonstrate the effectiveness of this novel control strategy. A comparative analysis with fixed-time sliding mode control highlights its superior performance.