206Bi was implanted into iron and nickel at T<0.2 K and room temperature. In all cases nuclear magnetic resonance of oriented206Bi was observed. Nuclear orientation data are compatible with nearly 100 per cent of the206Bi nuclei experiencing the hyperfine interaction corresponding to the resonance frequency but strength and shape of the resonance depend on the sample preparation which is discussed in detail. Nuclear orientation experiments with122,124SbZn and206BiZn show a sizably smaller average quadrupole interaction frequency immediately after on-line implantation than after annealing at room temperature.