Pulse Shape Analysis Research Articles

Evaluation of different LSC methods for 222Rn determination in waters

Monitoring of 222Rn in drinking or surface waters, as well as in groundwater has been performed regularly in connection with geological, hydrogeological and hydrological surveys and health hazard studies. Liquid scintillation counting (LSC) is often preferred analytical method for 222Rn measurements in waters as it allows multiple-sample automatic analysis. LSC method implies mixing of water samples with organic scintillation cocktail, which triggers radon diffusion from the aqueous into an organic phase for which it has a much greater affinity, eliminating the possibility of radon emanation in that manner.The main aim of this paper is calibration of the liquid scintillation counter Qunatulus 1220™ for measuring of radon in water and evaluation of two different methods (one-phase and two-phase) in order to obtain the most suitable LSC technique for radon in water measurement. In this study four different scintillation cocktails were tested: one miscible (Ultima Gold AB) and three immiscible (High Efficiency Mineral Oil Scintillator, Opti-Fluor O and Ultima Gold F). Evaluation of presented methods was based on obtained detection efficiency and achieved Minimal Detectable Activity (MDA) values. Comparison of presented methods, accuracy and precision, as well as different scintillation cocktail's performance, was considered from results of measurements of 226Ra spiked water samples with known activity and environmental samples. LSC results were compared with the results of radon in water measurement obtained by alpha spectrometer RAD7. Calibration was done as a dependence of calibration factor (CF) from Pulse Shape Analysis (PSA).According to the obtained results, with proper adjustment of calibration parameters, both methods could be used for radon in water measurements. The obtained MDA values for all four scintillation cocktails are very low, less than 0.1 Bq l−1 for measuring time of 300 min.

New methods to identify low energy 3He with Silicon-based detectors

Methods to discriminate low energy mass-3 particles using Silicon detectors are reviewed. The time-of-flight technique based on analog electronics and measuring time between a reference signal and the charge signal from the Silicon detector does not allow to discriminate 3He from 3H. One method consists in adding a thin layer of Silicon (typically of 20μm) to recover the standard discrimination by ΔE-E identification matrix. Strong inhomogeneities in thickness are observed for these thin detectors. Difficulties in handling such detectors have led to investigate numerical approaches using reverse-mounted neutron transmutation doped Silicon detectors. First, the pulse shape analysis (PSA) technique has been investigated on the current and charge signals. PSA enables the discrimination of tritons and 3He and also 3He and 4He with good figures of merit. Secondly, the time of flight between two digitized signals (a reference signal from the beam pulse and the current or the charge signal) is presented. Both numerical techniques give promising results for the identification of light particles with Silicon detectors.

Evaluation of Eu:LiCAF for neutron detection utilizing SiPMs and portable electronics

With the increasing cost and decreasing availability of 3He, there have been many efforts to find alternative neutron detection materials. Lithium calcium aluminum fluoride (LiCAF) enriched to 95% 6Li doped with europium was evaluated here as a replacement material for 3He. Wafers 0.5 cm thick, consisting of LiCAF crystals in a rubberized matrix, were embedded with wavelength shifting fibers (WSF) and mated to silicon photo-multipliers (SiPMs) to measure the photon response in a flux of neutrons from a DD neutron generator. Excellent discrimination was realized between neutrons and gammas, and both pulse-height discrimination and pulse-shape analysis were explored. A Figure of Merit (FoM) of 1.03 was achieved. By applying pulse-shape analysis, a simple neutron count output was generated by utilizing a low-pass filter to suppress fast pulses from the SiPM output and subsequently applying a threshold to the remaining signal. Custom electronics were built to bias the SiPMs, then amplify, filter, discriminate, and digitize the LiCAF/WSF scintillation photons, resulting in a digital pulse that can easily be counted with any microcontroller or field programmable gate array. A significant advantage of LiCAF is that it can be fabricated into any shape/size (when embedded in a rubberized matrix), and the light output and transparency is sufficient to allow for thicker scintillators which enable detection of both thermal and epithermal neutrons. This work demonstrated that Eu:LiCAF is capable of discriminating gammas from neutrons and is a potential replacement material for 3He, especially for nuclear security applications and neutron spectroscopy.

Neutron background measurements with a hybrid neutron detector at the Kuo-Sheng Reactor Neutrino Laboratory

We report in situ neutron background measurements at the Kuo-Sheng Reactor Neutrino Laboratory (KSNL) by a hybrid neutron detector (HND) with a data size of 33.8 days under identical shielding configurations as during the neutrino physics data taking. The HND consists of BC-501A liquid and BC-702 phosphor powder scintillation neutron detectors, which is sensitive to both fast and thermal neutrons, respectively. Neutron-induced events for the two channels are identified and differentiated by pulse shape analysis, such that background of both are simultaneously measured. The fast neutron fluxes are derived by an iterative unfolding algorithm. Neutron induced background in the germanium detector under the same fluxes, both due to cosmic-rays and ambient radioactivity, are derived and compared with the measurements. The results are valuable to background understanding of the neutrino data at the KSNL. In particular, neutron-induced background events due to ambient radioactivity as well as from reactor operation are negligible compared to intrinsic cosmogenic activity and ambient $\gamma$-activity. The detector concept and analysis procedures are applicable to neutron background characterization in similar rare-event experiments.

Multilayer phoswich scintillators for neutron / gamma discrimination

MultiLayer Phoswich (MLP) scintillators have been studied for fission neutron detection by Monte-Carlo simulations and experimental tests. n/γ discrimination behavior of these systems and their angular dependencies have been characterized. The possibility to carry on a neutron counting system based of such an approach has been proven, and according to the results, an optimal thickness of layers for fission neutron counting was found around [100–150] μm. But, contrary to current liquid or solid-state discrimination scintillators, it appears that MLP-based neutron counting systems cannot directly classify neutron and gamma-ray interaction events from pulse shape analysis. To operate properly, it is therefore required to implement a compensation algorithm in the system readout.

Fast screening of operational aqueous samples by gross alpha and beta counting with LSC systems

At nuclear installations a large number of samples is used to control operational tasks and health physics parameters. A fast screening process can be applied to provide immediate indication on possible contamination, and liquid scintillation counting (LSC) is the preferred method. Many LSC systems, which do not perform pulse shape analysis, are still in use. A screening procedure for these systems is presented based on three windows analysis. It may greatly reduce work and time, compared to using a proportional counter system, besides providing more accurate results.

Separation of gamma-ray and neutron events with CsI(Tl) pulse shape analysis

Separation of gamma-ray and neutron events with CsI(Tl) pulse shape analysis

Improving sensitivity of a BEGe-based high-purity germanium spectrometer through pulse shape analysis

We performed Pulse Shape Analysis to separate single-scattered gamma energy deposition events from multiple-scattered photons in a high-sensitivity gamma -ray spectrometer. The spectrometer is based on a Broad Energy High Purity Germanium detector and the developed technique uses multivariate analysis by an application of the Multi-Layer Perceptron Neural Network. A very good separation of the single-site- and multi-site events was achieved leading to a significant reduction of the background level of the investigated spectrometer – the double escape peak, rich in single-site events, was reduced by 95%, while the full energy peaks lost at most 25% of their counts. The peak to Compton ratio, calculated for the 2614.5 keV gamma line from ^{208}Tl, was improved by 114.3%.

Testing of a sCVD diamond detection system in the CROCUS reactor

The paper describes the testing of the NEUTON detection system into CROCUS, the zero-power reactor of the Ecole Polytechnique Federale de Lausanne (EPFL). NEUTON is composed of a $4 {\rm mm} \times 4$ mm sCVD diamond detector with a 6Li converter and the associated acquisition electronics. It is developed by CIVIDEC Instrumentation GmbH. The use of a diamond detector with converter in the mixed radiation field of a nuclear reactor is challenging because these detectors are sensitive to gamma-rays, fast neutrons and thermal neutrons through conversion in 6Li . In NEUTON, the rejection of gamma-rays is achieved in real time, via the analysis of the signal pulse shape from the detector. To do so, a few signal characteristics (amplitude, area and FWHM) are recorded in the integrated Field Programmable Gate Arrays (FPGA) of the system. This treatment does not induce any dead time. Measurements in CROCUS demonstrated for the first time the capability of a system like NEUTON to detect and separate fast neutrons, thermal neutrons, and gamma-rays. The system response was shown to be linear with respect to the reactor power (up to 35W) and its thermal sensitivity was found to be $(3.5\pm 0.2)\times 10^{-5}$ cps/nv.

The high-speed after-pulse measurement system for PMT

A system employing a desktop FADC has been developed to investigate the features of 8-inch Hamamatsu PMT R5912. The system stands out for its high-speed and informative results as a consequence of adopting fast waveform sampling technology. Recording the full waveforms allows us to perform pulse shape analysis. High-precision after-pulse time and charge distribution results are presented in this manuscript. Other characteristics of the photomultiplier tube, such as the gain of charge, dark rate and transit time spread, can be also obtained by this system.

Separation of gamma-ray and neutron events with CsI(Tl) pulse shape analysis

Fast neutrons are a large background to measurements of gamma-rays emitted from excited nuclei, such that detectors which can efficiently distinguish between the two are essential. In this paper we describe the separation of gamma-rays from neutrons with the pulse shape information of the CsI(Tl) scintillator, using a fast neutron beam and several gamma-ray sources. We find that a figure of merit optimized for this separation takes on large and stable values (nearly 4) between 5 and 10 MeV of electron equivalent deposited energy, the region of most interest to the study of nuclear de-excitation gamma-rays. Accordingly this work demonstrates the ability of CsI(Tl) scintillators to reject neutron backgrounds to gamma-ray measurements at these energies.

Particle identification using digital pulse shape discrimination in a nTD silicon detector with a 1 GHz sampling digitizer

In beam test experiments have been carried out for particle identification using digital pulse shape analysis in a 500 μm thick Neutron Transmutation Doped (nTD) silicon detector with an indigenously developed FPGA based 12 bit resolution, 1 GHz sampling digitizer. The nTD Si detector was used in a low-field injection setup to detect light heavy-ions produced in reactions of ∼ 5 MeV/A 7Li and 12C beams on different targets. Pulse height, rise time and current maximum have been obtained from the digitized charge output of a high bandwidth charge and current sensitive pre-amplifier. Good isotopic separation have been achieved using only the digitized charge output in case of light heavy-ions. The setup can be used for charged particle spectroscopy in nuclear reactions involving light heavy-ions around the Coulomb barrier energies.

Position resolution simulations for the inverted-coaxial germanium detector, SIGMA

The SIGMA Germanium detector has the potential to revolutionise γ-ray spectroscopy, providing superior energy and position resolving capabilities compared with current large volume state-of-the-art Germanium detectors. The theoretical position resolution of the detector as a function of γ-ray interaction position has been studied using simulated detector signals. A study of the effects of RMS noise at various energies has been presented with the position resolution ranging from 0.33 mm FWHM at Eγ=1MeV, to 0.41 mm at Eγ=150 keV. An additional investigation into the effects pulse alignment have on pulse shape analysis and in turn, position resolution has been performed. The theoretical performance of SIGMA operating in an experimental setting is presented for use as a standalone detector and as part of an ancillary system.

DarkSide-20k: A 20 tonne two-phase LAr TPC for direct dark matter detection at LNGS

Building on the successful experience in operating the DarkSide-50 detector, the DarkSide Collaboration is going to construct DarkSide-20k, a direct WIMP search detector using a two-phase Liquid Argon Time Projection Chamber (LArTPC) with an active (fiducial) mass of 23 t (20 t). The DarkSide-20k LArTPC will be deployed within a shield/veto with a spherical Liquid Scintillator Veto (LSV) inside a cylindrical Water Cherenkov Veto (WCV). Operation of DarkSide-50 demonstrated a major reduction in the dominant $^{39}$Ar background when using argon extracted from an underground source, before applying pulse shape analysis. Data from DarkSide-50, in combination with MC simulation and analytical modeling, shows that a rejection factor for discrimination between electron and nuclear recoils of $\gt3\times10^9$ is achievable. This, along with the use of the veto system, is the key to unlocking the path to large LArTPC detector masses, while maintaining an "instrumental background-free" experiment, an experiment in which less than 0.1 events (other than $\nu$-induced nuclear recoils) is expected to occur within the WIMP search region during the planned exposure. DarkSide-20k will have ultra-low backgrounds than can be measured in situ. This will give sensitivity to WIMP-nucleon cross sections of $1.2\times10^{-47}$ cm$^2$ ($1.1\times10^{-46}$ cm$^2$) for WIMPs of $1$ TeV$/c^2$ ($10$ TeV$/c^2$) mass, to be achieved during a 5 yr run producing an exposure of 100 t yr free from any instrumental background. DarkSide-20k could then extend its operation to a decade, increasing the exposure to 200 t yr, reaching a sensitivity of $7.4\times10^{-48}$ cm$^2$ ($6.9\times10^{-47}$ cm$^2$) for WIMPs of $1$ TeV$/c^2$ ($10$ TeV$/c^2$) mass.

Digital fast pulse shape and height analysis on cadmium-zinc-telluride arrays for high-flux energy-resolved X-ray imaging.

Cadmium-zinc-telluride (CZT) arrays with photon-counting and energy-resolving capabilities are widely proposed for next-generation X-ray imaging systems. This work presents the performance of a 2 mm-thick CZT pixel detector, with pixel pitches of 500 and 250 µm, dc coupled to a fast and low-noise ASIC (PIXIE ASIC), characterized only by the preamplifier stage. A custom 16-channel digital readout electronics was used, able to digitize and process continuously the signals from each output ASIC channel. The digital system performs on-line fast pulse shape and height analysis, with a low dead-time and reasonable energy resolution at both low and high fluxes. The spectroscopic response of the system to photon energies below (109Cd source) and above (241Am source) the K-shell absorption energy of the CZT material was investigated, with particular attention to the mitigation of charge sharing and pile-up. The detector allows high bias voltage operation (>5000 V cm-1) and good energy resolution at moderate cooling (3.5% and 5% FWHM at 59.5 keV for the 500 and 250 µm arrays, respectively) by using fast pulse shaping with a low dead-time (300 ns). Charge-sharing investigations were performed using a fine time coincidence analysis (TCA), with very short coincidence time windows up to 10 ns. For the 500 µm pitch array (250 µm pitch array), sharing percentages of 36% (52%) and 60% (82%) at 22.1 and 59.5 keV, respectively, were measured. The potential of the pulse shape analysis technique for charge-sharing detection for corner/border pixels and at high rate conditions (250 kcps pixel-1), where the TCA fails, is also shown. Measurements demonstrated that significant amounts of charge are lost for interactions occurring in the volume of the inter-pixel gap. This charge loss must be accounted for in the correction of shared events. These activities are within the framework of an international collaboration on the development of energy-resolved photon-counting systems for high-flux energy-resolved X-ray imaging (1-140 keV).

Temperature quenching in LAB based liquid scintillator

The effect of temperature changes on the light output of LAB based liquid scintillator is investigated in a range from -5 to 30,^{circ }C with alpha -particles and electrons in a small scale setup. Two PMTs observe the scintillator liquid inside a cylindrically shaped aluminum cuvette that is heated or cooled and the temperature dependent PMT sensitivity is monitored and corrected. The alpha -emitting isotopes in dissolved radon gas and in natural Samarium (bound to a LAB solution) excite the liquid scintillator mixtures and changes in light output with temperature variation are observed by fitting light output spectra. Furthermore, also changes in light output by compton electrons, which are generated from external calibration gamma -ray sources, is analysed with varying temperature. Assuming a linear behaviour, a combined negative temperature coefficient of {(-0.29 pm 0.01)}{,%/^{circ }}hbox {C} is found. Considering hints for a particle type dependency, electrons show {(-0.17 pm 0.02)}{,%/^{circ }}hbox {C}, whereas the temperature dependency seems stronger for alpha -particles, with {(-0.35 pm 0.03)}{,%/^{circ }}hbox {C}. Due to a high sampling rate, a pulse shape analysis can be performed and shows an enhanced slow decay component at lower temperatures, pointing to reduced non-radiative triplet state de-excitations.

Characterisation of Redlen high-flux CdZnTe

CdZnTe is a promising material for the current generation of free electron laser light sources and future laser-driven γ-ray sources which require detectors capable of high flux imaging at X-ray and γ-ray energies (> 10 keV) . However, at high fluxes CdZnTe has been shown to polarise due to hole trapping, leading to poor performance. Novel Redlen CdZnTe material with improved hole transport properties has been designed for high flux applications. Small pixel CdZnTe detectors were fabricated by Redlen Technologies and flip-chip bonded to PIXIE ASICs. An XIA Digital Gamma Finder PIXIE-16 system was used to digitise each of the nine analogue signals with a timing resolution of 10 ns. Pulse shape analysis was used to extract the rise times and amplitude of signals. These were measured as a function of applied bias voltage and used to calculate the mobility (μ) and mobility-lifetime (μτ) of electrons and holes in the material for three identical detectors. The measured values of the transport properties of electrons in the high-flux-capable material was lower than previously reported for Redlen CdZnTe material (μeτe ∼ 1 × 10−3 cm2V−1 and μe ∼ 1000 cm2V−1s−1) while the hole transport properties were found to have improved (μhτh ∼ 3 × 10−4 cm2V−1 and μh ∼ 100 cm2V−1s−1).

Calibration and optimization of alpha-beta separation procedures for determination of radium/radon in single- and two-phase liquid scintillation systems

Liquid scintillation alpha beta discrimination technique based on pulse shape analysis (PSA) was evaluated for determination of 226Ra and 222Rn in water samples. In view of the significance of calibration, for the reliable and precise determination of 226Ra and 222Rn concentrations in water samples, calibration procedures were standardized for single and two phase systems using Quantulus 1220 liquid scintillation counter. PSA optimization and efficiency calibrations were performed using 226Ra standard rather than conventionally used pure alpha and beta standards and substantiated by measuring the activity concentrations of 226Ra and 222Rn in the spiked water samples.

Optimisation of pulse shape discrimination using EJ299-33 for high energy neutron detection in proton beam therapy

It is widely understood that proton beam therapy has considerable clinical benefits over photon therapy for treating certain types of tumours. Protons deposit most of their energy in a very localised area, the so-called Bragg peak, sparing surrounding healthy tissue and critical organs from radiation. However, secondary neutrons and gamma rays are generated in the beam nozzle and inside the patient. Clinically, it is highly desirable to monitor the neutron dose the patient is exposed to, and this requires a neutron detector sensitive to high energies. EJ299-33 is a solid plastic scintillator capable of discriminating neutrons from gamma rays using pulse shape analysis of scintillation light. EJ299-33 has the potential to detect neutrons with energies up to 100 MeV and does not present leakage and flammability hazards generally associated with liquid scintillators. Experimental measurements with 60Co, 137Cs and 241AmBe sources were performed to calibrate and optimise pulse shape discrimination parameters. We also performed experimental measurements at the Clatterbridge Cancer Centre in a 60 MeV passive scattered beam to detect high energy neutrons.

Suppression of alpha-induced lateral surface events in the COBRA experiment using CdZnTe detectors with an instrumented guard-ring electrode

The COBRA collaboration searches for neutrinoless double beta-decay (0νββ-decay) using CdZnTe semiconductor detectors with a coplanar-grid readout and a surrounding guard-ring structure. The operation of the COBRA demonstrator at the Gran Sasso underground laboratory (LNGS) indicates that alpha-induced lateral surface events are the dominant source of background events. By instrumenting the guard-ring electrode it is possible to suppress this type of background. In laboratory measurements this method achieved a suppression factor of alpha-induced lateral surface events of 5300+2660−1380, while retaining (85.3 ±0.1%) of gamma events occurring in the entire detector volume. This suppression is superior to the pulse-shape analysis methods used so far in COBRA by three orders of magnitude.