Graphene Plasmons Research Articles

Electrically tunable graded photonic crystal lens based on graphene plasmons.

Controlling the nonlinear relationship between surface plasmon polariton (SPP) mode index and chemical potential of graphene can be used in the field of active transformation optics. Here, we propose an electrically tunable 2D Graded Photonic Crystal (GPC) lens based on graphene SPP platform. Our platform comprises a graphene monolayer integrated into a back-gated structure with nano-patterned gate insulators. When the chemical potential of the graphene surface is designed to operate in the nonlinear region, the designed GPC lens can be continuously transformed between a Maxwell's fish-eye lens and a Luneburg lens by tuning the gate voltage. The range of the lens background chemical potential for allowing this transformation is systematically studied. To compensate for the significant errors inherent in the conventional effective medium theory (EMT) during the homogenization of photonic crystals (PCs), we propose a generalized effective medium theory (GEMT). The validity and accuracy of this approach are verified through comparisons with true values (based on rigorous eigenvalue solutions) and EMT values. Due to its advantages of on-site controls and easy fabrication characteristics, the proposed graphene GPC provides a new way for practical on-chip light manipulation.

Giant Enhancement of Negative Friction by Resonant Coupling Between Localized Surface Phonon Polaritons and Graphene Plasmonics

Abstract Negative friction refers to a frictional force that acts in the same direction as the motion of an object, which has been predicted in terahertz (THz) gain systems [Phys. Rev. B 108 (4), 045406(2023)]. In this work, we investigate the enhancement of the negative friction experienced by nanospheres placed near a graphene substrate. We find that the magnitude of negative friction is related to the resonant coupling between the surface plasmon polaritons (SPPs) of the graphene and localized surface phonon-polaritons (LSPhP) of nanospheres. We exam nanospheres consisted of several different materials, including SiO2, SiC, ZnSe, NaCl, lnSb. Our results suggest that the LSPhP of NaCl nanospheres match effectively with the amplified SPPs of graphene sheets. The negative friction for NaCl nanospheres can be enhanced about one-to-two orders of magnitude compared to that of silica (SiO2) nanospheres. At the resonant peak of negative friction, the required quasi-Fermi energy of graphene is lower for NaCl nanospheres. Our finds hold great prospects for the mechanical manipulations of nanoscale particles.

The combination of graphene plasmons and surface plasmons in a crystalline Ge2Sb1.5Bi0.5Te5 metasurface structure for laser mode-locking

The combination of graphene plasmons and surface plasmons in a crystalline Ge2Sb1.5Bi0.5Te5 metasurface structure for laser mode-locking

Analogical atomic effects of graphene nanostructure induced by nonlinearity.

A scheme to construct analogical atoms using graphene nanostructures via quantum nonlinearity is proposed. Due to the strong field localization capability of graphene plasmons and the significant intrinsic nonlinearity of graphene, a strong nonlinear optical response can be realized even with single-photon excitation. In this process, the quantum vacuum localized plasmonic mode plays a crucial role in achieving the third-order multi-photon nonlinear effect. The eigenfrequency of the nanostructure can shift by an amount tens of times larger than the decay rate, causing the nanostructure cavity to exhibit atomic-like behaviors. Furthermore, multilevel atoms can be constructed through the interaction of composite graphene nanostructures. The parameters of these atoms can be manipulated by adjusting the nanostructure size, Fermi energy, and other parameters. This research holds significant potential for applications in highly integrated, controllable nanophotonics.

Surface plasmon-mediated photoluminescence boost in graphene-covered CsPbBr3 quantum dots

The optical properties of graphene (Gr)-covered CsPbBr3 quantum dots (QDs) were investigated using micro-photoluminescence spectroscopy, revealing a remarkable three orders of magnitude enhancement in photoluminescence (PL) intensity compared to bare CsPbBr3 QDs. To elucidate the underlying mechanisms, we combined experimental techniques with density functional theory (DFT) calculations. DFT simulations showed that the graphene layer generates interfacial electrostatic potential barriers when in contact with the CsPbBr3 surface, impeding carrier leakage from perovskite to graphene and enhancing radiative recombination. Additionally, graphene passivates CsPbBr3 surface defect states, suppressing nonradiative recombination of photo-generated carriers. Our study also revealed that graphene becomes n-doped upon contact with CsPbBr3 QDs, activating its plasmon mode. This mode resonantly couples with photo-generated excitons in the perovskite. The momentum mismatch between graphene plasmons and free-space photons is resolved through plasmon scattering at Gr/CsPbBr3 interface corrugations, facilitating the observed super-bright emission. These findings highlight the critical role of graphene as a top contact in dramatically enhancing CsPbBr3 QDs’ PL. Our work advances the understanding of graphene-perovskite interfaces and opens new avenues for designing high-efficiency optoelectronic devices. The multifaceted enhancement mechanisms uncovered provide valuable insights for future research in nanophotonics and materials science, potentially leading to breakthroughs in light-emitting technologies.

Polarization-dependent near-field coupling and far-field harmonic modulation in a graphene-based plasmonic nanostructure

The interplay between light and matter has fostered innovative research in surface plasmons, specifically in graphene, due to its tunable Fermi energy and reduced losses in the infrared and terahertz spectra. This study explores the anisotropic coupling of nonlocalized surface plasmons in graphene with localized magnetic polaritons (MP) in a silicon carbide (SiC) array. By adjusting graphene’s Fermi energy and polarization angle, we successfully achieved hybrid coupling, giving rise to three clearly distinguishable hybridized states. Using the coupled oscillator model as a framework, we conducted an analysis of the intricate multimode coupling and accurately ascertained the weighting efficiencies of the individual modes comprising the hybrids. By integrating the design principles of space-time coding metasurfaces, we successfully broadened the scope of the application, extending its reach from the near-field to the far-field. These novel discoveries pave new paths for advancements in thermal emitters, photonic systems, energy conversion technologies, and the creation of cutting-edge plasmonic devices.

Multidimensional dynamic control of optical skyrmions in graphene–chiral–graphene multilayers

Abstract Optical skyrmions are topological quasiparticles with a complex vectorial field structure. Their associated characteristics of ultra-small, ultra-fast and topological protection have great application prospects in high density data storage, light matter interaction and optical communication. At present, the research of optical skyrmions is still in its infancy, where the construction and flexible regulation of different topological textures are current research hotspot. Here, we combine the twist degree of freedom of materials and optical skyrmions. Based on graphene–chiral–graphene multilayers structure, we demonstrate the field mode symmetry and hybridization to form Bloch-type graphene plasmons skyrmion lattice. At the same time, by changing chirality parameter, the Fermi energy of graphene and the phase of incident light, multidimensional control of Bloch-type optical skyrmions can be realized. Our work demonstrated that the properties of materials provide the additional dimensions to regulate the topological states, and the combination of different materials structures provides the possibility for dynamic construction and manipulation of multiple topological states, which is expected to find applications in integrated nanophotonics devices.

Efficient excitation of acoustic graphene plasmons for sub-nanoscale infrared sensing

Acoustic graphene plasmons (AGPs) exhibit extremely spatial confinement and near-field enhancement, holding great potential for sub-nanoscale infrared sensing. However, the efficient excitation of AGPs is challenging due to the large momentum mismatch between AGPs and the incident light. Here, we numerically demonstrate an efficient AGP launcher consisting of a monolayer graphene (MG)/graphene nanoantenna (GNA) array/gold reflector hybrid structure. The resonant GNA array, which is in close proximity to MG, excites ultra-confined AGPs between the GNA array and MG, as well as confined GPs in MG. Moreover, the excitation efficiency of AGPs is significantly enhanced due to the constructive interference. Benefiting from the ultra-confined near fields and gate-tunable resonance frequency of AGPs, the characteristic vibrational signals of the sub-nanoscale (0.8 nm) polyethylene layer and A/G-IgG protein layer can be distinctly observed in the absorption spectra of hybrid structure. The efficient AGP launcher provides a highly compact platform for subwavelength optics and sub-nanoscale sensing.

Light funneling into localized acoustic graphene plasmons for extreme infrared and terahertz field enhancement and confinement

Enhancing light-matter interaction through deep subwavelength-scale confinement is crucial for numerous applications like molecular sensing, optoelectronic devices, and non-linear optics. Here, we report the excitation of localized acoustic graphene plasmons (LAGPs) confined in a sub-micro- wide, nanometer-thick layer using a metal slit antenna. This approach enables light funneling in the infrared and terahertz regimes, leading to strong field enhancement and confinement. LAGPs exhibit broad-band excitation characteristics, with the number of excited modes adjustable via the symmetry of the relative positioning between graphene and the metal slit. Detailed analysis indicates that the local field intensities of LAGPs are critically influenced by both the periodicity of the device structure and the electron relaxation time of graphene. These findings are effectively elucidated using temporal coupled mode theory. In comparison to conventional non-localized acoustic graphene plasmons, LAGPs demonstrate significantly improved field confinement and enhancement attributed to the funneling effect. Our study presents a promising avenue for achieving robust light-matter interaction and holds potential for various applications in the infrared and terahertz domains.

Valley-polarized edge plasmons in graphene p–n junctions with pseudomagnetic fields

Abstract Owing to the inherent characteristics of collective excitations in graphene, electrical control of edge plasmons is highly desirable for nanoplasmonic applications. This study investigates valley-polarized edge pseudomagneplasmons in a graphene p–n junction subjected to a strain-induced pseudomagnetic field. A four-component hydrodynamic model is employed and solved via the Wiener–Hopf method, revealing the coexistence of three plasmon modes, including counterpropagating acoustic edge modes, gapless topological edge states, and zero modes. The valley polarization, as determined from the numerically exact solution, is stronger than that predicted by the approximate models. Notably, the confinement of edge plasmons at the graphene p–n junction significantly exceeds that at the graphene/vacuum interface, possibly because of the electron–hole attraction. Furthermore, gate-controlled subwavelength confinement is successfully achieved by applying an appropriate gate voltage, thereby highlighting a unique and promising attribute of edge pseudomagnetoplasmons in graphene p–n junctions.

REFRACTIVE INDEX BASED DETECTION WITH A HIGH SENSITIVITY BIOSENSOR ENHANCED BY GRAPHENE

Over the past decade, optical sensors have made significant advances. An optical sensor examines the environmental impact through the change of an optical signal and offers advantages such as low cost and label-free detection. In this study, a sensor consisting of a single graphene layer and a slit positioned on the substrate is proposed. The strip gap made to improve the excitation of graphene plasmons allowed to achieve 96.2% high transmission resonance mode. This demonstrates the ability of the sensor surface to detect changing environmental conditions. The results show that the sensitivity of the sensor is 6282 nm/RIU when the sensor surface is exposed to analytes with different refractive indices. The use of a single graphene sheet eliminates the need for a metal resonator and achieves a higher sensitivity compared to some experiments recently published in the literature. Thus, the disadvantage of significant ohmic losses in metal resonators is avoided. Furthermore, a thorough discussion of various factors, including the modification of the strip gap width on the graphene layer and electrical tunability, led to the achievement of optimal sensitivity.

A tunable graphene dual mode absorber for efficient terahertz radiation absorption and sensing applications

This paper presents a novel plasmonic graphene absorber designed for the terahertz frequency range, utilizing a dual mode optical filter configuration. The absorber consists of a layered periodic array comprising gold, SiO₂ and graphene. Key components include a graphene disk and four strategically positioned graphene stripes on a SiO₂ substrate. An underlying gold layer enhances the absorption efficiency by serving as a reflector. The structure is numerically simulated using the 3D finite difference time domain (FDTD) method. A comprehensive parametric study has been conducted to optimize the absorber's performance. The simulation results demonstrate near perfect absorption at 4.16 THz and 5.88 THz. This innovative design enables efficient absorption of terahertz radiation due to the plasmonic resonance effects of the graphene components. Additionally, the absorption frequency can be dynamically adjusted by altering the chemical potential of graphene through applying an external bias voltage. The tailored geometry and material composition result in a compact absorber with high absorption values and tunability. Detailed performance analysis through numerical simulations demonstrates the absorber's potential for applications in sensing, imaging, and communication systems operating in the terahertz frequency range.

Design and Analysis of a Plasmonic Metasurface-Based Graphene Sensor for Highly Sensitive and Label-Free Detection of COVID-19 Biomarkers

Design and Analysis of a Plasmonic Metasurface-Based Graphene Sensor for Highly Sensitive and Label-Free Detection of COVID-19 Biomarkers

Theory of intrinsic acoustic plasmons in twisted bilayer graphene

Theory of intrinsic acoustic plasmons in twisted bilayer graphene

On-chip transfer of ultrashort graphene plasmon wave packets using terahertz electronics

On-chip transfer of ultrashort graphene plasmon wave packets using terahertz electronics

Beamforming of Electrically Tunable Plasmonic Graphene Strip Nanoantennas in the Terahertz, Far-Infrared, and Mid-Infrared Ranges

Beamforming of Electrically Tunable Plasmonic Graphene Strip Nanoantennas in the Terahertz, Far-Infrared, and Mid-Infrared Ranges

Memristive Thermal Radiator by Highly Tunable Graphene Plasmon

AbstractThe dynamic regulation of thermal radiation in the mid‐infrared region is technologically important in diverse applications such as thermal management and camouflage. However, there is a notable lack of research on the combination of infrared radiators and memristors, which can maintain previous states or modes without extra power consumption. Here, a memristive mid‐infrared radiator, where graphene nanoribbon grating serves simultaneously as a floating gate for charge storage and a tunable infrared nanoantenna for thermal radiation is proposed. This design enables precise and fast modulation, low power consumption, and scalability. Even a small change of one attocoulomb in the stored charge can produce a 1‐µm peak shift in the absorption peak. This work provides a platform for a memristive infrared thermal radiator that can be further exploited for electrochromic glazing or on‐chip radiative cooling.

Highly Confined Hybridized Polaritons in Scalable van der Waals Heterostructure Resonators.

The optimization of nanoscale optical devices and structures will enable the exquisite control of planar optical fields. Polariton manipulation is the primary strategy in play. In two-dimensional heterostructures, the ability to excite mixed optical modes offers an additional control in device design. Phonon polaritons in hexagonal boron nitride have been a common system explored for the control of near-infrared radiation. Their hybridization with graphene plasmons makes these mixed phonon polariton modes in hexagonal boron nitride more appealing in terms of enabling active control of electrodynamic properties with a reduction of propagation losses. Optical resonators can be added to confine these hybridized plasmon-phonon polaritons deeply into the subwavelength regime, with these structures featuring high quality factors. Here, we show a scalable approach for the design and fabrication of heterostructure nanodisc resonators patterned in chemical vapor deposition-grown monolayer graphene and h-BN sheets. Real-space mid-infrared nanoimaging reveals the nature of hybridized polaritons in the heterostructures. We simulate and experimentally demonstrate localized hybridized polariton modes in heterostructure nanodisc resonators and demonstrate that those nanodiscs can collectively couple to the waveguide. High quality factors for the nanodiscs are measured with nanoscale Fourier transform infrared spectroscopy. Our results offer practical strategies to realize scalable nanophotonic devices utilizing low-loss hybridized polaritons for applications such as on-chip optical components.

Topological valley plasmons in twisted monolayer-bilayer graphene moiré superlattices

Topological valley plasmons in twisted monolayer-bilayer graphene moiré superlattices

Ultrasensitive acoustic graphene plasmons in a graphene-transition metal dichalcogenide heterostructure: Strong plasmon–phonon coupling and wavelength sensitivity enhanced by a metal screen

Acoustic plasmons in graphene exhibit strong confinement induced by a proximate metal surface and hybridize with phonons of transition metal dichalcogenides (TMDs) when these materials are combined in a van der Waals heterostructure, thus forming screened graphene plasmon–phonon polaritons (SGPPPs), a type of acoustic mode. While SGPPPs are shown to be very sensitive to the dielectric properties of the environment, enhancing the SGPPPs coupling strength in realistic heterostructures is still challenging. Here we employ the quantum electrostatic heterostructure model, which builds upon the density functional theory calculations for monolayers, to show that the use of a metal as a substrate for graphene-TMD heterostructures (i) vigorously enhances the coupling strength between acoustic plasmons and the TMD phonons, and (ii) markedly improves the sensitivity of the plasmon wavelength on the structural details of the host platform in real space, thus allowing one to use the effect of environmental screening on acoustic plasmons to probe the structure and composition of a van der Waals heterostructure down to the monolayer resolution.