AbstractThe airborne electromagnetic (AEM) method is becoming an effective means for subsurface electrical property reconstruction with the merits of terrain adaptability and acquisition efficiency. However, instantaneous inversion of time‐domain AEM data is still a challenge, owing to the huge amount of data. Inspired by Google's neural machine translation system, we develop a fast inversion operator guided by deep learning to translate time‐domain AEM measurements directly into subsurface resistivity structures. Trained by synthetic data, our system shows impressive adaptability to field observations and strong robustness against noise disturbance. Applied to the AEM data set acquired by the U.S. Geological Survey in Leach Lake Basin, CA, USA, our system successfully delivers results in seconds for a common PC from more than 740,000 AEM soundings. The inverted structures clearly delineate the geometries of the lake, surrounding mountains and faults. The inversion operator can support instantaneous subsurface resistivity reconstruction for AEM observations.