Multiphoton States Research Articles

Formation of Non-Classical Multiphoton States of Light with Squeezed Quantum Fluctuations in Bismuth-Modified Tellurite Glass Fibers

Formation of Non-Classical Multiphoton States of Light with Squeezed Quantum Fluctuations in Bismuth-Modified Tellurite Glass Fibers

Integrable high-efficiency generation of three-photon entangled states by a single incident photon

Generation of multi-photon entangled states with high efficiency in integrated photonic quantum systems is still a big challenge. The usual three-photon generation efficiency based on the third-order nonlinear effect is extremely low. Here, we propose a scheme to generate three-photon correlated states, which are entangled states in frequency space and bound states in real space, with high efficiency. This method relies on two crucial processes. On one hand, by employing a Sagnac interferometer, an incident photon can be transformed into a symmetric superposition of the clockwise and counterclockwise modes of the Sagnac loop, which can then be perfectly absorbed by the emitter. On the other hand, the coupling strengths of the two transition paths of the emitter to the Sagnac loop are set to be equal, under which the absorbed photon can be emitted completely from the cascaded transition path due to quantum interference. By adjusting the coupling strengths among the three transition paths of the emitter and the waveguide modes, we can control the spectral entanglement and spatial separation among the three photons. Our proposal can be used to generate three-photon entangled states on demand, and the efficiency can be higher than 90% with some practical parameters, which can find important applications in integrated quantum information processing.

Linear quantum systems: A tutorial

The purpose of this tutorial is to give a brief introduction to linear quantum control systems. The mathematical model of linear quantum control systems is presented first, then some fundamental control-theoretic notions such as stability, controllability and observability are given, which are closely related to several important concepts in quantum information science such as decoherence-free subsystems, quantum non-demolition variables, and back-action evasion measurements. After that, quantum Gaussian states are introduced, in particular, an information-theoretic uncertainty relation is presented which often gives a better bound for mixed Gaussian states than the well-known Heisenberg uncertainty relation. The quantum Kalman filter is presented for quantum linear systems, which is the quantum analogy of the Kalman filter for classical (namely, non-quantum-mechanical) linear systems. The quantum Kalman canonical decomposition for quantum linear systems is recorded, and its application is illustrated by means of a recent experiment. As single- and multi-photon states are useful resources in quantum information technology, the response of quantum linear systems to these types of input is presented. Finally, coherent feedback control of quantum linear systems is briefly introduced, and a recent experiment is used to demonstrate the effectiveness of quantum linear systems and networks theory.

Формирование неклассических многофотонных состояний света со сжатыми квантовыми флуктуациями в волокнах из модифицированного висмутом теллуритного стекла

An optical fiber with a high Kerr nonlinearity coefficient is proposed and produced from a bismuth-modified tellurite glass for creation of nonclassical multiphoton states of light. Specifically, we propose to use those fibers to squeeze the quantum fluctuations of one of the quadratures of light in the 20 W signal significantly below -10 dB compared to the standard quantum noise limit, which is important for various practical applications. Using numerical modeling based on stochastic nonlinear Schrodinger equation, we demonstrate noise squeezing stronger than -16 dB for lengths of tellurite fiber 6-14 m, while squeezing of -14 dB is expected in silica fibers for lengths of 120-300 m. Analytical formulas were used to analyse the physical factors which limit the squeezing achievable.

Sending-or-not-sending twin-field quantum key distribution with multiphoton states

The twin-field quantum key distribution (TF-QKD) protocol has led to extensive investigation for its capacity of overcoming the rate-distance limit. One variant for TF-QKD named sending-or-not-sending (SNS) TF-QKD has also been proposed. The SNS-TF-QKD encodes the classical keys 0 and 1 in sending or not sending the phase-randomized coherent states, which helps it to tolerate large misalignment errors due to optical phase fluctuations. Nevertheless, the original SNS-TF-QKD scheme utilizes only single-photon interference in generating secret keys, which seems quite different from other TF-QKD protocols. In this paper, we prove that multiphoton interference in the SNS TF-QKD protocol can also contribute to key generation. Accordingly, an improved SNS-TF-QKD scheme with higher key rate is proposed, where events of not only single-photon but also two-photon emissions are considered as effective events.

Giant Enhancement of Unconventional Photon Blockade in a Dimer Chain.

Unconventional photon blockade refers to the suppression of multiphoton states in weakly nonlinear optical resonators via the destructive interference of different excitation pathways. It has been studied in a pair of coupled nonlinear resonators and other few-mode systems. Here, we show that unconventional photon blockade can be greatly enhanced in a chain of coupled resonators. The strength of the nonlinearity in each resonator needed to achieve unconventional photon blockade is suppressed exponentially with lattice size. The analytic derivation, based on a weak drive approximation, is validated by wave function MonteCarlo simulations. These findings show that customized lattices of coupled resonators can be powerful tools for controlling multiphoton quantum states.

Fidelity of time-bin-entangled multiphoton states from a quantum emitter

We devise a mathematical framework for assessing the fidelity of multi-photon entangled states generated by a single solid-state quantum emitter, such as a quantum dot or a nitrogen-vacancy center. Within this formalism, we theoretically study the role of imperfections present in real systems on the generation of time-bin encoded Greenberger-Horne-Zeilinger and one-dimensional cluster states. We consider both fundamental limitations, such as the effect of phonon-induced dephasing, interaction with the nuclear spin bath, and second-order emissions, as well as technological imperfections, such as branching effects, non-perfect filtering, and photon losses. In a companion paper, we consider a particular physical implementation based on a quantum dot emitter embedded in a photonic crystal waveguide and apply our theoretical formalism to assess the fidelities achievable with current technologies.

Heralded path-entangled NOON states generation from a reconfigurable photonic chip

Maximal multi-photon entangled states, known as NOON states, play an essential role in quantum metrology. With the number of photons growing, NOON states are becoming increasingly powerful and advantageous for obtaining supersensitive and super-resolved measurements. In this paper, we propose a universal scheme for generating three- and four-photon path-entangled NOON states on a reconfigurable photonic chip via photons subtracted from pairs and detected by heralding counters. Our method is postselection free, enabling phase supersensitive measurements and sensing at the Heisenberg limit. Our NOON-state generator allows for integration of quantum light sources as well as practical and portable precision phase-related measurements.

Periodic Cavity State Revivals from Atomic Frequency Combs.

Spin ensembles with a comb-shaped spectrum have shown exciting properties as efficient quantum memories. Here, we present a rigorous theoretical study of such atomic frequency combs in the strong coupling limit of cavity QED, based on a full quantum treatment using tensor-network methods. Our results demonstrate that arbitrary multiphoton states in the cavity are almost perfectly absorbed by the spin ensemble and reemitted as parity-flipped states at periodic time intervals. Fidelity values near unity are achieved in these revived states by compensating for energy shifts induced by the strong spin-cavity coupling through adjustments of individual coupling values of the teeth in the atomic frequency comb.

Conflict-free collective stochastic decision making by orbital angular momentum of photons through quantum interference

In recent cross-disciplinary studies involving both optics and computing, single-photon-based decision-making has been demonstrated by utilizing the wave-particle duality of light to solve multi-armed bandit problems. Furthermore, entangled-photon-based decision-making has managed to solve a competitive multi-armed bandit problem in such a way that conflicts of decisions among players are avoided while ensuring equality. However, as these studies are based on the polarization of light, the number of available choices is limited to two, corresponding to two orthogonal polarization states. Here we propose a scalable principle to solve competitive decision-making situations by using the orbital angular momentum of photons based on its high dimensionality, which theoretically allows an unlimited number of arms. Moreover, by extending the Hong-Ou-Mandel effect to more than two states, we theoretically establish an experimental configuration able to generate multi-photon states with orbital angular momentum and conditions that provide conflict-free selections at every turn. We numerically examine total rewards regarding three-armed bandit problems, for which the proposed strategy accomplishes almost the theoretical maximum, which is greater than a conventional mixed strategy intending to realize Nash equilibrium. This is thanks to the quantum interference effect that achieves no-conflict selections, even in the exploring phase to find the best arms.

Diagrammatic approach to scattering of multiphoton states in waveguide QED

We give an exposure to diagrammatic techniques in waveguide QED systems. A particular emphasis is placed on the systems with delayed coherent quantum feedback. Specifically, we show that the $N$-photon scattering matrices in single-qubit waveguide QED systems, within the rotating wave approximation, admit for a parametrization in terms of $N-1$-photon effective vertex functions and provide a detailed derivation of a closed hierarchy of generalized Bethe-Salpeter equations satisfied by these vertex functions. The advantage of this method is that the above mentioned integral equations hold independently of the number of radiation channels, their bandwidth, the dispersion of the modes they are supporting, and the structure of the radiation-qubit coupling interaction, thus enabling one to study multi-photon scattering problems beyond the Born-Markov approximation. Further, we generalize the diagrammatic techniques to the systems containing more than a single emitter by presenting an exact set of equations governing the generic two and three-photon scattering operators. The above described theoretical machinery is then showcased on the example of a three-photon scattering on a giant acoustic atom, recently studied experimentally [Nat. Phys. 15, 1123 (2019)].

All-optical long-distance quantum communication with Gottesman-Kitaev-Preskill qubits

Quantum repeaters are a promising platform for realizing long-distance quantum communication and thus could form the backbone of a secure quantum internet, a scalable quantum network, or a distributed quantum computer. Repeater protocols that encode information in single- or multi-photon states are limited by transmission losses and the cost of implementing entangling gates or Bell measurements. In this work, we consider implementing a quantum repeater protocol using Gottesman-Kitaev-Preskill (GKP) qubits. These qubits are natural elements for quantum repeater protocols, because they allow for deterministic Gaussian entangling operations and Bell measurements, which can be implemented at room temperature. The GKP encoding is also capable of correcting small displacement errors. At the cost of additional Gaussian noise, photon loss can be converted into a random displacement error channel by applying a phase-insensitive amplifier. Here we show that a similar conversion can be achieved in two-way repeater protocols by using phase-sensitive amplification applied in the post-processing of the measurement data, resulting in less overall Gaussian noise per (sufficiently short) repeater segment. We also investigate concatenating the GKP code with higher level qubit codes while leveraging analog syndrome data, post-selection, and path-selection techniques to boost the rate of communication. We compute the secure key rates and find that GKP repeaters can achieve a comparative performance relative to methods based on photonic qubits while using orders-of-magnitude fewer qubits.

Linear dichroism in few-photon ionization of laser-dressed helium

Ionization of laser-dressed atomic helium is investigated with focus on photoelectron angular distributions stemming from two-color multi-photon excited states. The experiment combines extreme ultraviolet (XUV) with infrared (IR) radiation, while the relative polarization and the temporal delay between the pulses can be varied. By means of an XUV photon energy scan over several electronvolts, we get access to excited states in the dressed atom exhibiting various binding energies, angular momenta, and magnetic quantum numbers. Furthermore, varying the relative polarization is employed as a handle to switch on and off the population of certain states that are only accessible by two-photon excitation. In this way, photoemission can be suppressed for specific XUV photon energies. Additionally, we investigate the dependence of the photoelectron angular distributions on the IR laser intensity. At our higher IR intensities, we start leaving the simple multi-photon ionization regime. The interpretation of the experimental results is supported by numerically solving the time-dependent Schrödinger equation in a single-active-electron approximation.Graphic abstract

Passive PT -symmetric Floquet coupler

Based on a Liouville-space formulation of open systems, we present a solution to the quantum master equation of two coupled optical waveguides with varying loss. The periodic modulation of the Markovian loss of one of them yields a passive $\mathcal{PT}$-symmetric Floquet system that, at resonance, shows a strong reduction of the required loss for the $\mathcal{PT}$ symmetry to be broken. We showcase this transition for a multi-photon state, and we show how to physically implement the modulated loss with reservoir engineering of a set of bath modes.

Mapping wave packet bifurcation at a conical intersection in CH3I by attosecond XUV transient absorption spectroscopy

Extreme ultraviolet (XUV) transient absorption spectroscopy has emerged as a sensitive tool for mapping the real-time structural and electronic evolution of molecules. Here, attosecond XUV transient absorption is used to track dynamics in the A-band of methyl iodide (CH3I). Gaseous CH3I molecules are excited to the A-band by a UV pump (277nm, ∼20fs) and probed by attosecond XUV pulses targeting iodine I(4d) core-to-valence transitions. Owing to the excellent temporal resolution of the technique, passage through a conical intersection is mapped through spectral signatures of nonadiabatic wave packet bifurcation observed to occur at 15 ± 4fs following UV photoexcitation. The observed XUV signatures and time dynamics are in agreement with previous simulations [H. Wang, M. Odelius, and D. Prendergast, J. Chem. Phys. 151, 124106 (2019)]. Due to the short duration of the UV pump pulse, coherent vibrational motion in the CH3I ground state along the C-I stretch mode (538 ± 7cm-1) launched by resonant impulsive stimulated Raman scattering and dynamics in multiphoton excited states of CH3I are also detected.

Quantum simulations with multiphoton Fock states

Quantum simulations are becoming an essential tool for studying complex phenomena, e.g. quantum topology, quantum information transfer and relativistic wave equations, beyond the limitations of analytical computations and experimental observations. To date, the primary resources used in proof-of-principle experiments are collections of qubits, coherent states or multiple single-particle Fock states. Here we show a quantum simulation performed using genuine higher-order Fock states, with two or more indistinguishable particles occupying the same bosonic mode. This was implemented by interfering pairs of Fock states with up to five photons on an interferometer, and measuring the output states with photon-number-resolving detectors. Already this resource-efficient demonstration reveals topological matter, simulates non-linear systems and elucidates a perfect quantum transfer mechanism which can be used to transport Majorana fermions.

Interface between Trapped-Ion Qubits and Traveling Photons with Close-to-Optimal Efficiency

A near optimum system for entangled photon collection and absorption in a single trapped ion is experimentally achieved: High-efficiency is further demonstrated by the generation of multi-photon states with up to 15 photons.

Photonic quantum data locking

Quantum data locking is a quantum phenomenon that allows us to encrypt a long message with a small secret key with information-theoretic security. This is in sharp contrast with classical information theory where, according to Shannon, the secret key needs to be at least as long as the message. Here we explore photonic architectures for quantum data locking, where information is encoded in multi-photon states and processed using multi-mode linear optics and photo-detection, with the goal of extending an initial secret key into a longer one. The secret key consumption depends on the number of modes and photons employed. In the no-collision limit, where the likelihood of photon bunching is suppressed, the key consumption is shown to be logarithmic in the dimensions of the system. Our protocol can be viewed as an application of the physics of Boson Sampling to quantum cryptography. Experimental realisations are challenging but feasible with state-of-the-art technology, as techniques recently used to demonstrate Boson Sampling can be adapted to our scheme (e.g., Phys. Rev. Lett. 123, 250503, 2019).

Single-mode multiphoton polarization states under random Pauli noises

We investigate behaviors of single-mode multiphoton polarization states under lossless random Pauli noises, where ``single-mode'' means that all the photons are in the same spatiotemporal mode and cannot be distinguished by any degree of freedom. We characterize the different decoherence effects of multiphoton and single-photon polarization states via the normalized linear entropy. Our results show that, contrary to single-photon states, multiphoton states cannot always evolve to the maximally mixed states. In particular, decoherence-free states and subspaces are found for the random Pauli noises. We reveal that the distinct behaviors result from the bosonic bunching effect and permutation symmetry, and hence our study may be generalized to other photon degrees of freedom and even some other bosonic systems.

A Novel Quantum Voting Scheme Based on BB84-State

BB84-state is the non-orthogonal single-photon state which has the advantage of easy implementation compared with the quantum multi-photon entanglement states. In this paper, based on BB84-state, by introducing a trusted third-party voting center, a quantum voting scheme is proposed. In this scheme, by performing corresponding unitary operation on BB84-state, all voters send their voting information to the tallyman Charlie, then Charlie counts all votes under the supervision of voting management center Bob, which ensures that the protocol can resist inside attacks. Moreover, by utilizing the decoy particles, our scheme can efficiently prevent outside attacks. Compared with other related quantum voting protocols, our protocol has higher qubit efficiency and fewer interactive times.