Magnetization Reversal Research Articles

Three-dimensional crescent-shaped ion velocity distributions created by magnetic reconnection in the presence of a guide field

By means of theory and particle simulations, crescent-shaped ion velocity distributions in the outflow region of symmetric magnetic reconnection in the presence of a guide magnetic field are investigated. Assuming a spatial one-dimensional electromagnetic field, a theoretical model accounting for the shape of crescents is derived. First, following the earlier theoretical models suggested by Bessho et al. [Geophys. Res. Lett. 43, 1828–1836 (2016)] and Zenitani et al. [J. Geophys. Res.: Space Phys. 122, 7396–7413 (2017)], we derive a theoretical model for 2D velocity distributions based on the conservation of the canonical momentum and the energy. The 2D theoretical model exhibits a two-dimensional structure of crescent-shaped velocity distributions and further demonstrates that no magnetic field reversal is required in the formation of crescents, although many researchers have considered that magnetic field reversal plays an essential role. Next, we construct a theoretical model for 3D velocity distributions based not only on the conservation of the canonical momentum in two directions and the energy but also on the conservation of the magnetic moment and the kinetic energy in the moving frame with the reconnection outflow speed, which are applied when the guide field ratio is high. The 3D theoretical model derives a three-dimensional structure of crescents by combination of an antiparallel magnetic field and a guide magnetic field comparable to or greater than the reconnection field. Both of the 2D and 3D theoretical models are consistent with ion velocity distributions found in our particle simulations.

Magnetization reversal via domain wall motion in vertical high-aspect-ratio nanopillar with two magnetic junctions

A vertical ferromagnetic (FM) nanopillar can be used as magnetic memory owing to characteristics such as its high storage capacity and high thermal stability. The perpendicular shape anisotropy (PSA) of the pillar enables its magnetization direction to be stabilized. A pillar with a high aspect ratio exhibits both strong PSA and magnetization with high thermal stability. Reversing the magnetization direction of such a pillar using the current flowing through it is a significant challenge in spintronics. However, spin injection from another FM layer alone cannot reverse the magnetization of pillars of which the length exceeds 100 nm. This motivated us to propose a magnetic junction (MJ) consisting of a high-aspect-ratio FM nanopillar with two thin FM layers. Using micromagnetic simulation, we demonstrate the magnetization reversal of a 150 nm-long pillar with a diameter of 15 nm. The simulation revealed that the magnetization of the pillar reverses because of the spin transfer torque induced by the spin injection from the two thin FM layers and the spin-polarized current (SPC) flowing in the pillar in the longitudinal direction. During the magnetization reversal process, a domain wall (DW) first forms at one end of the pillar due to the spin injection. Then, driven by the SPC, the DW moves to the other end of the pillar, and the magnetization is reversed. The magnetization direction of the pillar, controlled by changing the direction of the current flowing through the pillar, can be evaluated from the respective magnetoresistance values of the two MJs. Alternatively, by pinning the DW in the pillar, a three-value magnetic memory can be developed. In addition, multi-bit and analog memories can be developed by controlling the pinning position of the DW. The high-aspect-ratio pillar-writing scheme is foreseen to pave the way for the practical development of next-generation spintronic devices.

A computational approach to predict and enhance the sensitivity of X-ray resonant magnetic reflectometry to the magnetic behavior of deeply buried interfaces

In the present work a computational approach is applied to model and predict the results of X-ray resonant magnetic reflectometry – a non-destructive synchrotron-based technique to probe chemical composition, crystallographic environment and magnetization in multilayer epitaxial heterostructures with nanoscale depth resolution. The discussed 2D mapping approach is a step forward with respect to conventional resonant X-ray reflectometry and consists of collecting a fine step array of reflected intensity as a function of grazing angle and photon energy across the absorption edge of a particular chemical element. With the use of circularly polarized photons the method can be extended to magnetic systems to produce a map of dichroic reflectance directly related to the magnetization profile of the heterostructure. Studying the magnetic field dependence of dichroic reflectance maps can provide valuable information on the magnetization reversal of individual sublayers of a multilayer heterostructure. In the present paper modeling is performed for a bilayer system mimicking the behavior of a 30 nm ɛ-Fe2O3 thin film that is known to exhibit a pronounced two-component magnetic hysteresis. A technique to find optimal energy/angle combinations in order to sense magnetization of individual sublayers is proposed. Also discussed is the advantage of heavy-element capping, which leads to a substantial increase of the dichroic intensity oscillation contrast in the pre-edge region where the sensitivity to the magnetic behavior of the deeply buried interfaces is most pronounced.

Energy Barriers for the Spontaneous Magnetization Reversal of Atomic Co Chains on the Surface Pt(664) in the Model of Dzyaloshinskii–Moriya Interaction

Energy Barriers for the Spontaneous Magnetization Reversal of Atomic Co Chains on the Surface Pt(664) in the Model of Dzyaloshinskii–Moriya Interaction

Computational modelling of a triaxial vibrating sample magnetometer

Magnetic Field Assisted Additive Manufacturing (MFAAM) enables 3D printing of magnetic materials of various shapes which exhibit a complex anisotropy energy surface containing contributions generated from different origins such as sample, particle, and agglomerate shape anisotropy, flow and field induced anisotropy, and particle crystal anisotropy. These novel magnet shapes require the need to measure the x, y, and z components of the magnetic dipole moment simultaneously to fully understand the magnetic reversal mechanism and unravel the complex magnetic anisotropy energy surface of 3D printed magnetic composites. This work aims to develop a triaxial vibrating sample magnetometer (VSM) by adding a z-coil set to a pre-existing biaxial VSM employing a modified Mallison coil set. The optimum size and location of the sensing coils were determined by modeling the sensitivity matrix of the z-coil set. The designed coil set was implemented using 3D printed spools, a manual coil winder, and gauge 38 copper wire. A 3D printed strontium ferrite nylon composite sample was used to estimate the sensitivity of the z-coils (50 mV/emu). The results herein are applicable for any VSM using a modified Mallison biaxial coil configuration allowing for a quick implementation on pre-existing systems.

Nonadiabatic effects in the electron-optical system of a relativistic millimeter-wave gyrotron

Gyrotrons based on relativistic electron flows generated by thermionic magnetron injection guns are promising pulsed sources of millimeter and submillimeter radiation with multi-megawatt output power. Obviously, to increase the output power of such devices, it is necessary to provide a high beam current of more than 100 A. At the selected emission density, this forces the use of an emitter with a sufficiently large area. As is well known, wide emitters produce beams with a large velocity spread, which reduces the efficiency of the electron-wave interaction. Therefore, it is necessary to increase the diameter and, accordingly, increase the distance from the cathode to the gyrotron cavity, which leads to an increase in the magnetization reversal coefficient. Thus, the magnetic field in the region of beam formation becomes weak, and the Larmor radius and the turn pitch of the electron trajectory become large compared to the geometry of the surrounding electrodes, which can cause nonadiabatic effects. In this work, we consider one of these effects, which consists in the emergence of a range of anode voltage values in which the monotonic growth of the pitch factor stops. The results of trajectory analysis using current tube and discrete source methods based on the ANGEL software package are presented, as well as an assessment of the influence of a magnetic lens on the properties of an electron beam based on a simple analytical model.

Analysis on coercivity enhancement mechanism of grain-boundary-diffused and Dual-alloyed Nd-Fe-B Magnets

With the rapid development of application fields, such as the green energy industry, has resulted in increased demand for magnetic characteristics, especially the coercivity (Hcj). In this paper, two types of (Nd, Dy)-Fe-B magnets with comparable Hcj values were prepared using by grain boundary diffusion (GBD) method and dual alloy (DA) method. The composition, microstructure, domain structure, and magnetization reversal process of GBD and DA magnets were subjected to comparison. Additionally, an analysis of the specific coercivity mechanism was also conducted by fitting the Brown's equation. The results of composition and microstructure analysis revealed the formation of core-shell structural grains were formed in both GBD and DA methods. Specifically, the GBD method exhibited a higher concentration of Dy in the shell, constituting 26.8 % of the total rare earth (RE) content. In contrast the DA magnets had Dy accounting for 15.8 % of the total RE content in the shell. This discrepancy was identified as the primary factor contributing to the superior efficiency in enhancing the coercivity (Hcj) observed in the GBD method. The fitting results showed that GBD magnets were more inclined to nucleate in the core region in grain, whereas DA magnets nucleate at the edge of the grain shell layer. Both the observation of magnetic domains and magnetization reversal processes analysis revealed that the demagnetization process in GBD magnets is more uniform, which leads to better squareness. Our finding can provide theoretical and experimental basis for the preparation of high-performance Nd-Fe-B magnets.

Magnetization reversal and domain wall pinning in nanowires with nonlinear modulation of diameter

Micromagnetic simulation of magnetization reversal is studied on cylindrical tapered nanowire with radii 50nm and 10nm at wider and narrower end respectively. The radius decreases from wider end to the narrower end non-linearly as R-βzδ where δ is the degree of non-linearity. Value of δ is either an integer (n) or reciprocal of integer (1/n). At remanence, a vortex and flower state at the wider and narrower extremes respectively are exhibited combined with ferromagnetic ordering in the majority of volume. When δ is below 1/2, pinning and depinning of domain wall drives the hysteresis following a Modified Kondorsky model. Otherwise, the magnetization reversal proceeds with nucleation and propagation of vortex domain wall according to Kondorsky model. The propagation of domain wall is dependent upon the value of δ which suggests tunability of magnetic characteristics with modulation of diameter. For instance, large values of coercivity is observed for wires that have strong domain wall pinning which is considerably reduced when depinning and propagation of domain wall takes over. A large range (20kA/m to 130kA/m) of coercivity can be obtained by changing the modulation.

Understanding of magnetization reversal mechanism of precipitation-hardening samarium-cobalt magnets from micromagnetic simulation

The precipitation-hardening Sm-Co magnets not only have irreplaceable applications under extreme conditions such as high temperatures, but are also the most typical magnets with pinning-controlled magnetization reversal mechanism. However, there have always been two views on this type of pinning, attractive or repulsive. In this article, the modification of the parallel interface to the titled interface, led to occurrence of quasi-repulsive and quasi-attractive pinning modes, by employing micromagnetic simulation methods. The corresponding domain wall energy relationship between the pinning phase and main phase was analyzed for different pinning modes, according to the morphology of domain wall from the simulation results. The analysis results indicated that relatively small difference in domain wall energy between the two phases led to quasi-repetitive and quasi-attractive pinning modes. Our findings can provide a reference for further understanding of the magnetization reversal mechanism of precipitation-hardening Sm-Co magnets. The emphasis on the influence of 1:5/2:17 interface orientation on pinning also provided a perspective on the magnetization reversal mechanism of other nanostructured permanent magnet materials.

Magnetic Properties and THz Emission from Co/CoO/Pt and Ni/NiO/Pt Trilayers.

THz radiation emitted by ferromagnetic/non-magnetic bilayers is a new emergent field in ultra-fast spin physics phenomena with a lot of potential for technological applications in the terahertz (THz) region of the electromagnetic spectrum. The role of antiferromagnetic layers in the THz emission process is being heavily investigated at the moment. In this work, we fabricate trilayers in the form of Co/CoO/Pt and Ni/NiO/Pt with the aim of studying the magnetic properties and probing the role of very thin antiferromagnetic interlayers like NiO and CoO in transporting ultrafast spin current. First, we reveal the static magnetic properties of the samples by using temperature-dependent Squid magnetometry and then we quantify the dynamic properties with the help of ferromagnetic resonance spectroscopy. We show magnetization reversal that has large exchange bias values and we extract enhanced damping values for the trilayers. THz time-domain spectroscopy examines the influence of the antiferromagnetic interlayer in the THz emission, showing that the NiO interlayer in particular is able to transport spin current.

Contribution of the Magnetic Subsystem to the Generation of Longitudinal Acoustic Waves during Domain Wall Motion in Yttrium Orthoferrite

Purpose. Modern technologies in their development are increasingly in need of increasing the speed of processing and recording information. An alternative to semiconductor methods is magnetic memory based on changing magnetic moments. The speed of magnetization reversal is determined by the speed of motion of domain walls. The speed is maximum in weak ferromagnets. The purpose of this work is to study the effect of a magnetic wave generated by a moving domain wall on a longitudinal acoustic wave, taking into account the absorption of a magnetic wave in yttrium orthoferrite.Methods. The equation describing the effect of a magnetic wave generated by a moving domain wall on a longitudinal acoustic wave is solved using the following methods: the slowly varying amplitude method, the perturbation theory method, and the Lagrange method.Results. For an orthoferrite crystal, the contribution of the magnetic wave accompanying the motion of the domain wall in yttrium orthoferrite to the deformation of the amplitude of the longitudinal acoustic wave is calculated. This contribution in a bounded crystal, without taking into account the absorption of magnetic waves in the absence of the influence of acoustic waves on them, is of the order of 10-6 cm. In an unbounded crystal, the corresponding contribution, taking into account the absorption of magnetic waves, into the generation of longitudinal acoustic waves is of the order of magnitude 10-10 cm with a theoretical thickness of the domain wall D3 ≈ 10-6 cm.Conclusion. To study the mechanisms of the influence of a magnetic wave generated by a moving DW on a longitudinal acoustic wave, yttrium orthoferrite was taken. Since a weak ferromagnet is characterized by a significant increase in the magnetoelastic coupling when it overcomes the sound barrier. It is this circumstance that made it possible to experimentally observe the generation of elastic displacements by a moving domain wall. To develop devices for recording and processing information based on weak ferromagnets, it is necessary to fully investigate the mechanisms that affect the dynamics of a domain wall during its motion. Such a factor is the interaction of magnetic and acoustic waves with the domain wall, which can affect the quality of information processing. The evaluation of the contributions of these mechanisms can be used to develop the element base of devices for recording and processing information based on the magnetic memory of weak ferromagnets.

Interfacial engineering to manipulate the effective spin Hall angle of perpendicularly magnetized systems

The spin current can be generated by passing an electric current through a heavy metal. The spin current generation depends on the spin Hall angle (θsh) of the material. To manipulate the effective θsh, a thin layer of Au has been introduced at the bottom Pt/Co and the top Co/Pt interfaces in Ta/Pt/Co/Pt based perpendicularly magnetic anisotropy systems, and current-induced magnetization reversal of Co has been studied to estimate Jc. The introduction of the Au layer at the top Co/Pt interface (Ta/Pt/Co/Au/Pt) did not produce any significant reduction in the Jc. However, a significant reduction of Jc (∼34%) has been observed, while the Au layer has been deposited at the bottom Pt/Co interface (Ta/Pt/Au/Co/Pt), indicating an enhancement in the value of θsh. We also performed a micromagnetic simulation to understand the qualitative change of the θsh. Micromagnetic simulation suggested that the θsh becomes 0.07 in Ta/Pt/Au/Co/Pt multilayer compared to θsh=0.05 of the Ta/Pt/Co/Pt system. Pt/Co/Au/Co/Au exhibits a reduction in Jc up to ∼30% and corresponds to θsh=0.09. A Ta capping layer has been introduced to inject more spin current into the Co layer since Pt and Ta have opposite spin Hall angles. The Jc lowers up to ∼58% in Ta/Pt/Au/Co/Pt/Ta multilayer, corresponding to θsh=0.23. We also achieved field-free switching at Jc=1.55×1011 by depositing an in-plane magnetized layer of Co in Ta/Pt/Au/Co/Pt/Ta/Co/Pt multilayer.

Spin–Orbit Torque and Current‐Driven Switching in Pt100‐yTby/Co/AlOx Trilayers

AbstractTo decrease the energy consumption for the electrical manipulation of magnetization, the enhancement of the spin Hall effect through alloying is widely investigated, but the use of rare earth elements is rarely mentioned. This work reports the modification of the spin Hall effect on Pt by doping rare earth Tb atoms. The spin–orbit torque (SOT) performance is significantly enhanced in Pt100‐yTby alloyed heavy metal (HM) layer. Compared with the Tb‐free sample, the damping‐like effective field per unit current density increases to 1.9 times in the samples with Tb content between 5% and 10%. The critical current density for magnetization reversal is greatly reduced by 65% in a device with Pt87Tb13 HM layer and the in‐plane assistant field as small as ±20 Oe is sufficient for the deterministic switching in the same device. By magneto‐optical Kerr effect imaging, it is confirmed that the increased in‐plane field can effectively compensate the Dzyaloshinskii–Moriya interaction (DMI), which not only helps to reduce the critical current, but also facilitates the domain wall motion and is beneficial for the switching process. All results show that the Pt‐Tb alloy is a competitive candidate for low‐power spintronic devices.

Pulsed magnetization reversal in Ni nanowire

Pulsed magnetic field-induced magnetization reversal in Ni nanowires is investigated using micromagnetic simulation. The pulse amplitude, duration, and size of the nanowire are proven to have substantial impacts on the magnetization reversal process. Increasing pulse amplitude and duration leads to faster magnetization reversal for 10 nm-diameter nanowires. But for 40 nm-diameter nanowires with the same aspect ratio, the pulse parameters have a complicated influence on the magnetization reversal process due to the formation and propagation of magnetic domain walls. Further investigations reveal that applying a pulsed field at a certain angle from the long axis of the nanowire or raising the temperature can significantly accelerate the magnetization reversal process.

Comparison of driven equilibrium and standard spin-echo sequence in MR microscopy: Analysis of signal dependence on RF pulse imperfection and diffusion

Rapid MR imaging of slowly relaxing samples is often challenging. The most commonly used solutions are found in multi spin-echo (RARE) sequences or gradient-echo (GE) sequences, which allow faster imaging of such samples with multiple acquisitions of k-space lines per excitation or imaging with very short repetition times (TRs). Another solution is the use of a spin-echo (SE) sequence superimposed with a driven equilibrium Fourier transform (DEFT) method. Such a (DE-SE) imaging sequence has two refocusing RF pulses that produce two spin-echoes. In the first echo, the signal is acquired from the k-space line, and in the second echo, a 90° RF pulse is applied, typically 180° out of phase with respect to the excitation RF pulse. This last RF pulse allows almost complete magnetization reversal back to the longitudinal orientation with minimal magnetization loss. The DE-SE sequence and its RARE variant are widely used in clinical imaging, but its use in MR microscopy has some peculiarities related to the usually less perfect RF pulse flip angles and diffusion. In this study, their effects are first theoretically analyzed and later verified by experiments on test samples performed on a 9.4 T system for MR microscopy. Experiments on a water-filled tube for TE = 3.4 ms and TR = 25–200 ms showed that the DE-SE sequence produces about 10 times more signal than the SE sequence in this TR range. Finally, the performance of the DE-SE sequence compared to the SE sequence was demonstrated on a biological sample. The presented DE-SE sequence has been shown to be effective for rapid imaging of samples with long T1 relaxation times in MR microscopy and can also be considered as a suitable method for rapid proton density weighed imaging of materials.

The effect of roughness in reverse magnetization process of [Co/Cu]2 multilayers

The effect of roughness in reverse magnetization process of [Co/Cu]2 multilayers

“Tailoring thermal stability and in-plane magnetic anisotropy of CoFeB alloy thin films via growth conditions engineering”

The present work investigates the influence of growth conditions on the magneto-structural properties of magnetron-sputtered CoFeB alloy thin films. Films grown at room temperature (RT) are soft magnetic (coercivity <9 Oe), show amorphous microstructure, and possess a distinct uniaxial magnetic anisotropy (UMA) in the film plane. The amorphous microstructure and UMA persist up to a growth temperature (Ts) of 300 °C. CoFeB film grown at Si (100) substrate shows amorphous to crystalline phase transformation at Ts = 500 °C. In contrast, under the same growth conditions, the CoFeB film prepared on the SiO2 substrate maintains an amorphous structure up to Ts = 500 °C. The difference in the microstructures was explained in terms of the out-diffusion of B to the interfacial layer and segregation near the substrate for the films having crystalline and amorphous structure, respectively. On both the substrates Addition of W buffer layer facilitated the growth of smooth and nanocrystalline CoFeB films at Ts ∼300 °C. Upon crystallization, UMA evolution with a simultaneous increase in the coercive field is interpreted in terms of joint effect of random anisotropy model and surface/interface roughness-induced magnetization reversal mechanism. Unlike post-annealing, the CoFeB films prepared at high temperature shows superior thermal stability against crystallization. The relationship between the soft magnetic performance, UMA evolution, and thermal stability of CoFeB films with the growth conditions is established. The study reveals the role of growth condition engineering, to obtain CoFeB thin films with controlled microstructure and magnetic performance, which is crucial for designing the spintronics devices.

Writing temperature and thickness dependence of perpendicular magnetic-dot magnetization reversal probability

Investigation is necessary to figure out magnetization dynamics at high temperatures due to the low power requirement for heat-assisted magnetic recording technology. The Landau-Lifshitz-Gilbert equation was employed to assess the dynamic of magnetization in perpendicular magnetic-dots at elevated temperatures, considering the thermal contribution to the effective field. The simulated perpendicular magnetic-dot has a 50×50 nm2 surface area with thicknesses of 10 nm, 50 nm, and 100 nm. This study reveals that the probability of magnetization reversal and the threshold field in the thermally-assisted magnetic reversal process of a magnetic dot is influenced by the thickness and writing temperature. Below the Curie point, as sample thickness increases, demagnetization energy increases, requiring a larger external magnetic field for magnetization reversal. For the thicker sample, the magnitude of the writing field decreases as the temperature increases, which corresponds to temperature-dependent magnetization. Meanwhile, the optimum writing field is obtained below the Curie point. The magnetic-dot with 100 nm of thickness has an effective writing temperature of 739.7 K with a corresponding writing field is 250 Oe while its reversal probability at zero magnetic field is up to 0.2. Magnetic-dot thickness affects magnetization reversal probability due to domain wall propagation mechanisms during magnetic switching that result from the demagnetization factor. Moreover, as the temperature approaches the Curie temperature, the probability of zero-field magnetization reversal in the absence of an external magnetic field is observed to escalate which has a direct impact on the writing field magnitude. It was found that the effective writing temperature is below the Curie temperature, which allows several hundred Oersted of the writing field.

Coercivity mechanism of La–Nd–Fe–B films with Y spacer layer

The effect of the Y spacer layer on the phase composition, coercivity, and magnetization reversal processes of La–Nd–Fe–B films has been investigated. The addition of a 10 nm Y spacer layer increases the coercivity of the film to 1.36 T at 300 K and remains 0.938 T at 380 K. As the thickness of the Y spacer layer increases, Y participates in the formation of the main phase in the film, and further regulates the formation of La–B phases. The results of the first-order reversal curve (FORC) and micromagnetic fitting show that the coercivity of all the films is dominated by nucleation mechanism. The c-axis preferred orientation, good magnetic microstructure parameters and the largest dipole interaction enhance the coercivity. Therefore, the introduction of the Y spacer layer can be an effective way to improve the coercivity of La–Nd–Fe–B film over a wide temperature range of 150 K–380 K.

Controlled Growth of Submillimeter-Scale Cr5Te8 Nanosheets and the Domain Wall Nucleation Governed Magnetization Reversal Process.

Two-dimensional (2D) ferromagnets have attracted widespread attention for promising applications in compact spintronic devices. However, the controlled synthesis of high-quality, large-sized, and ultrathin 2D magnets via facile, economical method remains challenging. Herein, we develop a hydrogen-tailored chemical vapor deposition approach to fabricating 2D Cr5Te8 ferromagnetic nanosheets. Interestingly, the time period of introducing hydrogen was found to be crucial for controlling the lateral size, and a Cr5Te8 single-crystalline nanosheet of lateral size up to ∼360 μm with single-unit-cell thickness has been obtained. These samples exhibit a leading role of domain wall nucleation in governing the magnetization reversal process, providing important references for optimizing the performances of associated devices. The nanosheets also show notable magnetotransport response, including nonmonotonous magnetic-field-dependent magnetoresistance and sizable anomalous Hall resistivity, demonstrating Cr5Te8 as a promising material for constructing high-performance magnetoelectronic devices. This study presents a breakthrough of large-sized CVD-grown 2D magnetic materials, which is indispensable for constructing 2D spintronic devices.