Range Of Magnetic Fields Research Articles

Coupled circularly polarized electromagnetic soliton states in magnetized plasmas

The interaction between two co-propagating electromagnetic pulses in a magnetized plasma is considered, from first principles, relying on a fluid-Maxwell model. Two circularly polarized wavepackets by same group velocities are considered, characterized by opposite circular polarization, to be identified as left-hand- or right hand circularly polarized (i.e. LCP or RCP, respectively). A multiscale perturbative technique is adopted, leading to a pair of coupled nonlinear Schrödinger-type (NLS) equations for the modulated amplitudes of the respective vector potentials associated with the two pulses. Systematic analysis reveals the existence, in certain frequency bands, of three different types of vector soliton modes: an LCP-bright/RCP-bright coupled soliton pair state, an LCP-bright/RCP-dark soliton pair, and an LCP-dark/RCP-bright soliton pair. The value of the magnetic field plays a critical role since it determines the type of vector solitons that may occur in certain frequency bands and, on the other hand, it affects the width of those frequency bands that are characterized by a specific type of vector soliton (type). The magnetic field (strength) thus arises as an order parameter, affecting the existence conditions of each type of solution (in the form of an envelope soliton pair). An exhaustive parametric investigation is presented in terms of frequency bands and in a wide range of magnetic field (strength) values, leading to results that may be applicable in beam-plasma interaction scenarios as well as in space plasmas and in the ionosphere.

Alloying Driven Antiferromagnetic Skyrmions on NiPS3 Monolayer: A First-Principles Calculation.

Topological magnetic states are promising information carriers for ultrahigh-density and high-efficiency magnetic storage. Recent advances in two-dimensional (2D) magnets provide powerful platforms for stabilizing various nanometer-size topological spin textures within a wide range of magnetic field and temperature. However, non-centrosymmetric 2D magnets with broken inversion symmetry are scarce in nature, making direct observations of the chiral spin structure difficult, especially for antiferromagnetic (AFM) skyrmions. In this work, it is theoretically predicted that intrinsic AFM skyrmions can be easily triggered in XY-type honeycomb magnet NiPS3 monolayer by alloying of Cr atoms, due to the presence of a sizable Dzyaloshinskii-Moriya interaction. More interestingly, the diameter of the AFM skyrmions in Ni3/4Cr1/4PS3 decreases from 12 to 4.4nm as the external magnetic field increases and the skyrmion phases remain stable up to an external magnetic field of 4 T. These results highlight an effective strategy to generate and modulate the topological spin texture in 2D magnets by alloying with magnetic element.

All-solid highly sensitive fiber-tip magnetic field sensor based on a Fabry-Perot interferometer with a breakpoint structure.

An all-solid fiber-tip Fabry-Perot interferometer (FPI) coated with a nickel film is proposed and experimentally verified for magnetic field sensing with high sensitivity. It is fabricated by splicing a segment of a thin-wall capillary tube to a standard single-mode fiber (SMF), then inserting a tiny segment of fiber with a smaller diameter into the capillary tube, and creating an ultra-narrow air-gap at the SMF end to form an FPI. When the device is exposed to magnetic field, the capillary tube is strained due to the magnetostrictive effect of the nickel film coated on its outer surface. In addition, owing to the unique breakpoint sensitivity-enhancement structure of the air-gap FPI, the elongation of the capillary tube whose length is over 100 times longer than the air-gap width is entirely transferred to the cavity length change of the FPI, and the sensor is extremely sensitive to the magnetic field as proved by our experiments, achieving a high sensitivity of up to 2.236 nm/mT for a linear magnetic field range from 40 to 60 mT, as well as a low-temperature cross-sensitivity of 56µT/°C. The all-solid stable structure, compact size (total length of ∼3.0 mm), and reflective working mode with high magnetic field sensitivity indicate that this sensor has good application prospects.

Interaction of nitrogen-vacancy centers in diamond with a dense ensemble of carbon-13

The nitrogen-vacancy center in diamond attracts a lot of attention in sensing applications, mainly for temperature, magnetic field, and rotation measurements. Nuclear spins of carbon-13 surrounding the nitrogen-vacancy center can be used as a memory or sensing element. In the current work, a diamond plate with a relatively large concentration of carbon-13 was synthesized and examined. The spectrum of optically detected magnetic resonance was recorded and analyzed in a magnetic field range of 5–200 G. A strain-independent measurement technique of carbon-13 isotope concentration based on the analysis of magnetic resonance spectra was developed. Additionally, narrow features in the spectrum were detected and understood.

Highly sensitive surface acoustic wave magnetic field sensor based on the loss mechanism

Currently, the surface acoustic wave (SAW) magnetic field sensing technique utilises the SAW velocity/frequency mechanism of magnetoacoustic interaction as an indicator of the magnetic sensitivity mechanism. However, this method has low sensitivity and poor stability. To address this problem, a dynamic magnetoelastic coupling theoretical model is constructed to theoretically simulate the influence of the ΔE effect of magnetically sensitive thin films on SAW propagation attenuation. This study describes a high-sensitivity SAW magnetic field sensing mechanism based on magnetoacoustic attenuation. The simulation results show a clear relationship between the acoustic propagation loss and external magnetic field, indicating a structure-property relationship. An amorphous soft magnetic material (Fe90Co10)78Si12B10 was used as a magnetically sensitive thin film due to its high permeability, low coercivity (Hc), low hysteresis, ease of magnetisation and demagnetisation. SAW magnetosensitive device operating on a frequency of 200 MHz has been experimentally developed using a standard semiconductor photolithography process. A SiO2 layer was deposited on a 36° YX-LiTaO3 substrate as a waveguide, and a (Fe90Co10)78Si12B10 layer was on the top of the propagation area as a magnetosensitive film. The experimental results showed that the acoustic loss change due to the magnetic field variation was 4.63 dB within a magnetic field range of 0 Oe to ±10 Oe, which agreed with the theoretical results. The sensor had a sensitivity of 0.7546 dB Oe−1 within the range of 0–4 Oe and the lower detection limit of magnetic fields was 0.272 Oe, low hysteresis error of 0.54%, multiple repeatability error of 0.13%, excellent repeatability and stability were achieved in the experiments from the developed sensing device.

Influences of divalent ion substitution on the magnetic and dielectric properties of W-type barium ferrite

Abstract Saturation magnetization, magneto-crystalline anisotropy field and dielectric properties are closely related to microwave devices applied at different frequencies. For regulating the magnetic and dielectric properties of W-type barium ferrites, single-phase BaMe 2Fe16O27 (Me = Fe, Mn, Zn, Ni, Co) with different Me ions were synthesized by the high-temperature solid-state method. The saturation magnetization (M s) range from 47.77 emu/g to 95.34 emu/g and the magnetic anisotropy field (H a) range from 10700.60 Oe to 13739.57 Oe, depending on the type of cation substitution in the hexagonal lattice. The dielectric permittivity and dielectric loss decrease with increasing frequency of the AC electric field in the low-frequency region, while they almost remain constant in the high-frequency region. The characteristics of easy regulation and preparation make it a potential candidate for use in microwave device applications.

Comprehensive theoretical and experimental study of plasma plume dynamics across magnetic field

Dynamics of laser-produced plasma plume in the presence of magnetic field has been investigated theoretically and experimentally. A mathematical model has been proposed to estimate the time variation of axial dimension, expansion velocity and effective deceleration of the plasma plume across the magnetic field. The numerical solutions are also verified with analytical solutions. In order to validate the theoretical model, two directional, time-resolved images of laser-produced nickel and tungsten plasmas have been recorded in different magnetic field. The simulated plasma dynamics is compared with experimental data for significantly different atomic masses of ablated species, expand in wide range of magnetic field, ranging from 0.1 to 0.5 T. Most of the dynamical features for the both, diamagnetic and beyond the diamagnetic region e.g., temporal variation of plume dimension, characteristic time duration of diamagnetic behaviour, bubble radius and plasma instability are well captured by theoretical model with reasonable agreement with experimental observations.

Dzyaloshinskii-Moriya interactions, Néel skyrmions and V4 magnetic clusters in multiferroic lacunar spinel GaV4S8

Using ab initio density functional theory with static mean-field correlations, we calculate the Heisenberg and Dzyaloshinskii-Moriya interactions (DMI) for an atomistic spin Hamiltonian for the lacunar spinel, GaV4S8. The parameters describing these interactions are used in atomistic spin dynamics and micromagnetic simulations. The magnetic properties of the lacunar spinel GaV4S8, a material well-known from experiment to host magnetic skyrmions of Néel character, are simulated with these ab initio calculated parameters. The Dzyaloshinskii-Moriya contribution to the micromagnetic energy is a sum of two Lifshitz invariants, supporting the formation of Néel skyrmions and its symmetry agrees with what is usually expected for C3ν-symmetric systems. There are several conclusions one may draw from this work. One concerns the quantum nature of the magnetism, where we show that the precise magnetic state of the V4 cluster is crucial for understanding quantitatively the magnetic phase diagram. In particular, we demonstrate that a distributed-moment state of each V4 cluster explains well a variety of properties of GaV4S8, such as the band gap, observed Curie temperature and especially the stability of Néel skyrmions in the experimentally relevant temperature and magnetic-field range. In addition, we find that electronic correlations change visibly the calculated value of the DMI.

1H Spin-Lattice Relaxation Processes in Solutions of H2N-Fe3O4 Nanoparticles: Insights from NMR Relaxometry.

1H spin-lattice relaxation experiments have been performed for water and glycerol/water solutions of H2N-Fe3O4 superparamagnetic nanoparticles (NPs) of about 7 nm diameter. The experiments encompass a broad frequency range covering 3 orders of magnitude, from 10 kHz to 10 MHz (referring to 1H resonance frequency), and have been performed in the temperature range from 298 to 313 K, varying the concentration of the superparamagnetic species. This extensive dataset has been used for twofold purposes. The first one is to serve as a challenge for thorough tests of theoretical models describing nuclear relaxation in solutions of superparamagnetic NPs, depending on their magnetic properties and dynamics of the solvent molecules. The challenge is posed by the wish to reproduce the data in a broad range of magnetic fields (not only at high fields) and by the need to explain the differences in the relaxation scenarios for water and glycerol/water solutions by varying only the solvent parameters. The second purpose is to get insights into the magnetic properties (electronic relaxation properties) of the nanoparticles due to their high applicational potential.

Dynamics of quantum coherence and nonlocality of a two-spin system in the chemical compass.

In this paper a system consisting of two electron spins has been prepared initially in a singlet state using the chemical compass model is considered. It is assumed that each electron spin interacts symmetrically and/or asymmetrically with its respective private nuclear environment in the presence of an external magnetic field. We discussed the effect of the interaction parameters and the external magnetic field on some quantifiers of quantum correlations as entanglement, coherence, Bell inequality, as well as the steerability inequality. It is shown that within a certain range of external magnetic fields, the quantum coherence and entanglement behave similarly. The Bell and the steerable inequalities predicted a similar behavior for symmetric and asymmetric interactions. Moreover, as one increases the external magnetic field, the lower bounds of both inequalities have improved. The usefulness of using the spin state as quantum channel to teleport a two-qubit system has examined where the Bell inequality could be above its classical bounds by controlling the interaction parameters. It is shown that by tuning the coupling parameters the fidelity of the teleported state exceeds the classical bounds, as well as the long-lived stationary fidelity could be achieved during the interaction time.

On semiconductor–metal transition in FeSi induced by ultrahigh magnetic field

At low temperatures, iron monosilicide is a strongly correlated narrow-gap semiconductor. A first order transition to metal state induced by magnetic field was observed for the first time at 355 T in Ref. [Yu. B. Kudasov et al., JETP Lett. 68 (1998) 350]. However, recently a smooth transition from 230 T to 270 T was found under similar conditions in Ref. [D. Nakamura et al., Phys. Rev. Lett. 127 (2021) 156601]. This discrepancy goes far beyond experimental errors and deserves a careful study. A methodological analysis of inductive and RF techniques of conductivity measurements shows that the difference of these critical magnetic field estimations stems from a divergence in dynamic ranges of the techniques. In fact, the above mentioned methods supplement each other. The semiconductor-metal transition under magnetic field in FeSi is a complex phenomenon which occurs at the wide range of magnetic fields.

Magnetic field dependence of the para-ortho conversion rate of molecular hydrogen in SABRE experiments

The use of parahydrogen – the isomer of molecular hydrogen with zero nuclear spin – is important for promising and actively developing methods for spin hyperpolarization of nuclei called parahydrogen induced polarization (PHIP). However, the dissolved parahydrogen in PHIP experiments quickly loses its spin order, resulting in the formation of orthohydrogen and reduction of the overall nuclear polarization of the substrate. This process is due to the difference of chemical shifts of hydride protons, as well as spin–spin couplings between nuclei, in the intermediate catalytic complexes, and it has not been rigorously explained so far. We proposed a new experimental technique based on magnetic field cycling for measuring the rate of molecular hydrogen para–ortho conversion in solution and applied it for non-hydrogenative PHIP Signal Amplification By Reversible Exchange (SABRE) experiments. The para–ortho conversion rate was measured over a wide range of magnetic field from 0.5 mT to 9.4 T. It was found that the conversion rate strongly depends on the magnetic field in which the reaction occurs, as well as on the concentrations of reactants. The rate decreases with increasing the concentration of pyridine ligand and increases with increasing the concentration of iridium catalyst. The model, which takes into account the reversible exchange of molecular hydrogen with the catalyst, nuclear spin–spin interaction of hydride protons with nuclei of ligands within catalytic complex and nuclear Zeeman interactions, qualitatively describes the experimental data. Two types of complexes with different spin system symmetry contribute to the molecular hydrogen conversion. In asymmetric complexes possessing hydride protons with different chemical shifts due to the presence of chlorine anion ligand the para–ortho conversion rate increases with magnetic field, while for symmetric complexes this mechanism is not operable. In the magnetic field where level anti-crossing occurs the resonant feature for the rate of para–ortho conversion is found. The results of this work can be utilized for finding the optimal conditions for obtaining the maximum hyperpolarization in the experiments employing parahydrogen.

Barkhausen noise in disordered striplike ferromagnets: Experiment versus simulations.

In this work, we present a systematic comparison of the results obtained from the low-frequency Barkhausen noise recordings in nanocrystalline samples with those from the numerical simulations of the random-field Ising model systems. We performed measurements at room temperature on a field-driven metallic glass stripe made of VITROPERM 800R, a nanocrystalline iron-based material with an excellent combination of soft and magnetic properties, making it a cutting-edge material for a wide range of applications. Given that the Barkhausen noise emissions emerging along a hysteresis curve are stochastic and depend in general on a variety of factors (such as distribution of disorder due to impurities or defects, varied size of crystal grains, type of domain structure, driving rate of the external magnetic field, sample shape and temperature, etc.), adequate theoretical modeling is essential for their interpretation and prediction. Here the Random field Ising model, specifically its athermal nonequilibrium version with the finite driving rate, stands out as an appropriate choice due to the material's nanocrystalline structure and high Curie temperature. We performed a systematic analysis of the signal properties and magnetization avalanches comparing the outcomes of the numerical model and experiments carried out in a two-decade-wide range of the external magnetic field driving rates. Our results reveal that with a suitable choice of parameters, a considerable match with the experimental results is achieved, indicating that this model can accurately describe the Barkhausen noise features in nanocrystalline samples.

Cryogenic calibration for Hall probes

A superconducting undulator (SCU) prototype with a magnet length of 4m is being developed for the SHINE (Shanghai High Repetition Rate XFEL and Extreme Light Facility) project. The period length of the undulator is 16mm, the period number is 250, and the pole gap is 5mm. A point measurement system with three Hall probes will be used to measure the magnetic fields in the gap. The Hall probes fixed on a sledge will experience temperatures of about 4.2K to 50K when they move through the undulator gap. A temperature-dependent calibration system for these hall probes is necessary. The paper introduces the configuration of the cryogenic calibration system, and the result for the sensitivity and nonlinearity of one Hall probe from 2.8K to 300K over a magnetic field range of ±1.9T.

Observation of Topological Hall Effect in a Chemically Complex Alloy.

The topological Hall effect (THE) is the transport response of chiral spin textures and thus can serve as a powerful probe for detecting and understanding these unconventional magnetic orders. So far, the THE is only observed in either noncentrosymmetric systems where spin chirality is stabilized by Dzyaloshinskii-Moriya interactions, or triangular-lattice magnets with Ruderman-Kittel-Kasuya-Yosida-type interactions. Here, a pronounced THE is observed in a Fe-Co-Ni-Mn chemically complex alloy with a simple face-centered cubic (fcc) structure across a wide range of temperatures and magnetic fields. The alloy is shown to have a strong magnetic frustration owing to the random occupation of magnetic atoms on the close-packed fcc lattice and the direct Heisenberg exchange interaction among atoms, as evidenced by the appearance of a reentrant spin glass state in the low-temperature regime and the first principles calculations. Consequently, THE is attributed to the nonvanishing spin chirality created by strong spin frustration under the external magnetic field, which is distinct from the mechanism responsible for the skyrmion systems, as well as geometrically frustrated magnets.

Snap-through instability of a high arch of magneto elastomers with a giant magnetic actuation

In our previous work [Chen et al., Int. J. Solids Struct. 246–247, 111607 (2022)], we designed a flat arch structure for hard magnetic soft material. It used snap-through instability for remote actuation and large deformation in a small magnetic field range (25–170 Oe). The ratio of the magnetic-driven deflection to the arch length was about 0.05. To improve this ratio, we designed a high arch of magneto elastomers, which expanded the range of ratio from 0.05 to 0.5, increasing it by an order of magnitude. However, raising the arch height extended the driving range while unintentionally increasing the critical magnetic field for snap-through. To overcome this challenge, we reduced the bending stiffness of the arch-shaped structure, effectively lowering the critical magnetic field. Our goal is to optimize the structure of hard magnetic soft materials to achieve a broader driving range under quasi-static applied magnetic field conditions. This is accomplished by adjusting the arch height and structural stiffness to balance different performance requirements. Our research could have a significant impact on applications and devices that utilize magnetic materials.

Quantitative measurements of reactive oxygen species partitioning in electron transfer flavoenzyme magnetic field sensing.

Biological magnetic field sensing that gives rise to physiological responses is of considerable importance in quantum biology. The radical pair mechanism (RPM) is a fundamental quantum process that can explain some of the observed biological magnetic effects. In magnetically sensitive radical pair (RP) reactions, coherent spin dynamics between singlet and triplet pairs are modulated by weak magnetic fields. The resulting singlet and triplet reaction products lead to distinct biological signaling channels and cellular outcomes. A prevalent RP in biology is between flavin semiquinone and superoxide (O2 •-) in the biological activation of molecular oxygen. This RP can result in a partitioning of reactive oxygen species (ROS) products to form either O2 •- or hydrogen peroxide (H2O2). Here, we examine magnetic sensing of recombinant human electron transfer flavoenzyme (ETF) reoxidation by selectively measuring O2 •- and H2O2 product distributions. ROS partitioning was observed between two static magnetic fields at 20nT and 50μT, with a 13% decrease in H2O2 singlet products and a 10% increase in O2 •- triplet products relative to 50µT. RPM product yields were calculated for a realistic flavin/superoxide RP across the range of static magnetic fields, in agreement with experimental results. For a triplet born RP, the RPM also predicts about three times more O2 •- than H2O2, with experimental results exhibiting about four time more O2 •- produced by ETF. The method presented here illustrates the potential of a novel magnetic flavoprotein biological sensor that is directly linked to mitochondria bioenergetics and can be used as a target to study cell physiology.

Investigation on a high-power V-band transit-time oscillator under a low guiding magnetic field with a focusing cathode

Low guiding magnetic fields are favored for high-power microwave sources in practical applications for the sake of compactness and miniaturization, especially for permanent magnet packaging to replace the bulky and heavy solenoid system. A novel focusing cathode is proposed in a V-band transit-time oscillator to reduce the requirement for guiding magnetic fields. Particle-in-cell simulation results indicate that in the diode region, the radial electric field and electron beam current are reduced with the focusing cathode, further leading to improved transmission of the electron beam under a low guiding magnetic field. With an input of diode voltage of 393 kV, a beam current of 5.25 kA, and a low guiding magnetic field of 0.6 T, the transit-time oscillator outputs a microwave with an average power of 566 MW and a frequency of 58.6 GHz, resulting in a conversion efficiency of 27.3%. The proposed V-band transit-time oscillator with a focusing cathode can also stably work under a large range of input voltage and magnetic field, desired for further research with permanent magnet packaging.

Shubnikov–de Haas oscillations of biaxial-strain-tuned superconductors in pulsed magnetic field up to 60 T

Two-dimensional (2D) materials have gained increasing prominence not only in fundamental research but also in daily applications. However, to fully harness their potential, it is crucial to optimize their properties with an external parameter and track the electronic structure simultaneously. Magnetotransport over a wide magnetic field range is a powerful method to probe the electronic structure and, for metallic 2D materials, quantum oscillations superimposed on the transport signals encode Fermi surface parameters. In this manuscript, we utilize biaxial strain as an external tuning parameter and investigate the effects of strain on the electronic properties of two quasi-2D superconductors, MoTe2 and RbV3Sb5, by measuring their magnetoresistance in pulsed magnetic fields up to 60 T. With a careful selection of insulating substrates, we demonstrate the possibility of both the compressive and tensile biaxial strains imposed on MoTe2 and RbV3Sb5, respectively. For both systems, the applied strain has led to superconducting critical temperature enhancement compared to their free-standing counterparts, proving the effectiveness of this biaxial strain method at cryogenic temperatures. Clear quantum oscillations in the magnetoresistance—the Shubnikov–de Haas (SdH) effect—are obtained in both samples. In strained MoTe2, the magnetoresistance exhibits a nearly quadratic dependence on the magnetic field and remains non-saturating even at the highest field, whereas in strained RbV3Sb5, two SdH frequencies showed a substantial enhancement in effective mass values, hinting at a possible enhancement of charge fluctuations. Our results demonstrate that combining biaxial strain and pulsed magnetic field paves the way for studying 2D materials under unprecedented conditions.

Separating the contributions of the magnetic subsystems in antiferromagnetic ferrihydrite nanoparticles by analyzing the magnetization in fields of up to 250 kOe

Contributions of different magnetic subsystems formed in the systems of synthetic ferrihydrite nanoparticles (characterized previously) with an average size of < d>≈2.7 nm coated with polysaccharide arabinogalactan in different degrees have been separated by measuring the dependences of their magnetization M on magnetic field H of up to 250kOe on vibrating sample and pulsed magnetometers. The use of a wide measuring magnetic field range has been dictated by the ambiguity in identifying a linear M(H) portion for such antiferromagnetic nanoparticle systems within the conventional field range of 60–90 kOe. The thorough analysis of the magnetization curves in the temperature range of 100–250 K has allowed the verification of the contributions of (i) uncompensated magnetic moments µun in the superparamagnetic subsystem, (ii) the subsystem of surface spins with the paramagnetic behavior, and (iii) the antiferromagnetic susceptibility of the antiferromagnetically ordered ferrihydrite particle core. As a result, a model of the magnetic state of ferrihydrite nanoparticles has been proposed and the numbers of spins corresponding to magnetic subsystems (i)–(iii) have been estimated. An average magnetic moment μunof ∼ 145μB (μB is the Bohr magneton) per particle corresponds approximately to 30 decompensated spins of iron atoms in a particle (about 3 % of all iron atoms), which, according to the Néel’s hypothesis μun∼<d>3/2, are localized both on the surface and in the bulk of an antiferromagnetically ordered particle. The fraction of free (paramagnetic) spins is minimal in the sample without arabinogalactan coating of the nanoparticle surface (7 %) and is attained 20 % of all iron atoms in the sample with the highest degree of spatial separation of particles. According to this estimation, paramagnetic spins are located mainly on the edges and protruding areas of particles. Most magnetic moments of iron atoms are ordered antiferromagnetically and the corresponding magnetic susceptibility of this subsystem behaves as in an antiferromagnet with the randomly distributed crystallographic axes, i.e., increases with temperature.