Low Beam Currents Research Articles

Application of 2D correlation methods to the analysis of XPS spectra of ion irradiated poly (ether ether ketone)

The effects of ion irradiation conditions on poly (ether ether ketone) (PEEK) was probed by X-ray photoelectron (XPS) and two-dimensional correlation (2D-COS) spectroscopies. XPS data were reorganized according to the absorbed dose and penetration of X-ray radiation into PEEK. Subsequently, generalized and hybrid 2D-COS techniques were used to explore the effects of ion irradiation energy, type, and beam current on the chemistry of PEEK. The carbon peak at 284.4 eV changed on opposite direction on irradiation with the two different ions, i.e. proton and helium, or by increasing the dose rate. The reduction in the peak at 286.3 eV on helium irradiation implied the formation of three-dimensional structures involving C-C bonding via the H-link mechanism. The carbon peaks shifted to higher binding energy on irradiation with low beam current, and the opposite was true using high beam current. The former indicated oxidation reactions, and the latter indicated cross-linking formation. Changing the ions used on irradiating polymer not only control cross-linking extent but also produced different cross-linking structures. XPS combined with 2D-COS techniques provides a powerful tool to investigate the mechanism of complicated reactions such those occurring in the ion irradiation of PEEK.

Anomalous effects in the aluminum oxide sputtering yield

The sputtering yield of aluminum oxide during reactive magnetron sputtering has been quantified by a new and fast method. The method is based on the meticulous determination of the reactive gas consumption during reactive DC magnetron sputtering and has been deployed to determine the sputtering yield of aluminum oxide. The accuracy of the proposed method is demonstrated by comparing its results to the common weight loss method excluding secondary effects such as redeposition. Both methods exhibit a decrease in sputtering yield with increasing discharge current. This feature of the aluminum oxide sputtering yield is described for the first time. It resembles the discrepancy between published high sputtering yield values determined by low current ion beams and the low deposition rate in the poisoned mode during reactive magnetron sputtering. Moreover, the usefulness of the new method arises from its time-resolved capabilities. The evolution of the alumina sputtering yield can now be measured up to a resolution of seconds. This reveals the complex dynamical behavior of the sputtering yield. A plausible explanation of the observed anomalies seems to originate from the balance between retention and out-diffusion of implanted gas atoms, while other possible causes are commented.

Characterization and application of in-vacuum PIXE/EBS system for the direct elemental analysis of thick solid biological samples

Utilization of combined particle-induced X-ray emission (PIXE) and elastic backscattering (EBS) spectrometry for the direct elemental analysis of thick solid biological samples was thoroughly discussed. Powdered samples pressed as pellets were directly analyzed. Combination of applying low ion beam currents, random scanning of the sample across the beam during data acquisition, and using special sample holder enabled effective minimization of local ion beam heating. This subsequently inhibited potential element loss during ion beam irradiation. Matrix elements were determined from multiple EBS spectra, which were acquired using three different ion beam energies. Subsequently, averaging of the elemental concentrations obtained was achieved using novel MultiSIMNRA software. Moreover, combined EBS spectrometry, nuclear reaction analysis (NRA), and elastic recoil detection analysis (ERDA) measurements were used to overcome the limitations of using EBS separately and subsequently obtain accurate matrix element concentrations. The validity of the PIXE/EBS system for the direct elemental analysis of thick biological samples was comprehensively evaluated. The obtained concentration values demonstrated reliable results for most investigated elements (5–15%), starting from sodium onwards. The non-satisfying results were evaluated and justified.

THz-pump and X-ray-probe sources based on an electron linac.

We describe a compact THz-pump and X-ray-probe beamline, based on an electron linac, for ultrafast time-resolved diffraction applications. Two high-energy electron (γ > 50) bunches, 5 ns apart, impinge upon a single-foil or multifoil radiator and generate THz radiation and X-rays simultaneously. The THz pulse from the first bunch is synchronized to the X-ray beam of the second bunch by using an adjustable optical delay of a THz pulse. The peak power of THz radiation from the multifoil radiator is estimated to be 0.14 GW for a 200 pC well-optimized electron bunch. GEANT4 simulations show that a carbon foil with a thickness of 0.5-1.0 mm has the highest yield of 10-20 keV hard X-rays for a 25 MeV beam, which is approximately 103 photons/(keV pC-electrons) within a few degrees of the polar angle. A carbon multifoil radiator with 35 foils (25 μm thick each) can generate close to 103 hard X-rays/(keV pC-electrons) within a 2° acceptance angle. With 200 pC charge and a 100 Hz repetition rate, we can generate 107 X-rays per 1 keV energy bin per second or 105 X-rays per 1 keV energy bin per pulse. The longitudinal time profile of an X-ray pulse ranges from 400 to 600 fs depending on the acceptance angle. The broadening of the time duration of an X-ray pulse is observed owing to its diverging effect. A double-crystal monochromator will be used to select and transport the desired X-rays to the sample. The heating of the radiators by an electron beam is negligible because of the low beam current.

Scale-up of high specific activity 186gRe production using graphite-encased thick 186W targets and demonstration of an efficient target recycling process

Abstract Production of high specific activity 186gRe is of interest for development of theranostic radiopharmaceuticals. Previous studies have shown that high specific activity 186gRe can be obtained by cyclotron irradiation of enriched 186W via the 186W(d,2n)186gRe reaction, but most irradiations were conducted at low beam currents and for short durations. In this investigation, enriched 186W metal targets were irradiated at high incident deuteron beam currents to demonstrate production rates and contaminants produced when using thick targets. Full-stopping thick targets, as determined using SRIM, were prepared by uniaxial pressing of powdered natural abundance W metal or 96.86% enriched 186W metal encased between two layers of graphite flakes for target material stabilization. An assessment of structural integrity was made on each target preparation. To assess the performance of graphite-encased thick 186W metal targets, along with the impact of encasing on the separation chemistry, targets were first irradiated using a 22 MeV deuteron beam for 10 min at 10, 20, and 27 μA, with an estimated nominal deuteron energy of 18.7 MeV on the 186W target material (after energy degradation correction from top graphite layer). Gamma-ray spectrometry was performed post EOB on all targets to assess production yields and radionuclidic byproducts. The investigation also evaluated a method to recover and recycle enriched target material from a column isolation procedure. Material composition analyses of target materials, pass-through/wash solutions and recycling process isolates were conducted with SEM, FTIR, XRD, EDS and ICP-MS spectrometry. To demonstrate scaled-up production, a graphite-encased 186W target made from recycled 186W was irradiated for ~2 h with 18.7 MeV deuterons at a beam current of 27 μA to provide 0.90 GBq (24.3 mCi) of 186gRe, decay-corrected to the end of bombardment. ICP-MS analysis of the isolated 186gRe solution provided data that indicated the specific activity of 186gRe in this scaled-up production run was 2.6±0.5 GBq/μg (70±10 Ci/mg).

High-efficiency detector of secondary and backscattered electrons for low-dose imaging in the ESEM

A new Combined System for high-efficiency detection of Secondary and Backscattered Electrons (CSSBE) in the ESEM consists of three detectors: an ionisation SE detector, an improved scintillation BSE detector, and a new Ionisation Secondary Electron Detector with an electrostatic Separator (ISEDS). The ISEDS optimizes conditions for electron-gas ionisation phenomena in the ESEM to achieve a strongly amplified signal from the secondary electrons with a minimal contribution from backscattered and beam electrons. For this purpose, it is originally equipped with an electrostatic separator, which focuses signal electrons towards a detection electrode and controls the concentration of positive ions above the sample. The working principle of the ISEDS is explained by simulations of signal electron trajectories in gas using the EOD program with our Monte Carlo module. The ability to detect the signal electrons in a selected range of energies is described with Geant4 Monte Carlo simulations of electron-solid interactions and proven by experimental results. High-efficiency detection of the ISEDS is demonstrated by imaging a low atomic number sample under a reduced beam energy of 5 keV, very low beam currents of up to 0.2 pA, and gas pressure of hundreds of Pa.

Design and manufacture of the RF power supply and RF transmission line for SANAEM project Prometheus

A 1–5 MeV proton beamline is being built by the Turkish Atomic Energy Authority in collaboration with a number of graduate students from different universities. The primary goal of the project, is to acquire the design ability and manufacturing capability of all the components locally. SPP will be an accelerator and beam diagnostics test facility and it will also serve the detector development community with its low beam current. This paper discusses the design and construction of the RF power supply and the RF transmission line components such as its waveguide converters and its circulator. Additionally low and high power RF test results are presented to compare the performances of the locally produced components to the commercially available ones.

A novel comparison of Møller and Compton electron-beam polarimeters

We have performed a novel comparison between electron-beam polarimeters based on M{\o}ller and Compton scattering. A sequence of electron-beam polarization measurements were performed at low beam currents ($<$ 5 $\mu$A) during the $Q_{\rm weak}$ experiment in Hall C at Jefferson Lab. These low current measurements were bracketed by the regular high current (180 $\mu$A) operation of the Compton polarimeter. All measurements were found to be consistent within experimental uncertainties of 1% or less, demonstrating that electron polarization does not depend significantly on the beam current. This result lends confidence to the common practice of applying M{\o}ller measurements made at low beam currents to physics experiments performed at higher beam currents. The agreement between two polarimetry techniques based on independent physical processes sets an important benchmark for future precision asymmetry measurements that require sub-1% precision in polarimetry.

Prompt Gamma Rays Detected With a BGO Block Compton Camera Reveal Range Deviations of Therapeutic Proton Beams

The dose deposition profile of protons is interesting for tumour treatment due to the increased ionization density at the end of their track. However, the inaccurate knowledge of the proton stopping point limits the precision of the therapy. Prompt gamma rays, a by-product of the irradiation, are candidates for an indirect measurement of the particle range. Compton cameras have been proposed for prompt gamma ray imaging, but struggle with high trigger rates and low coincident efficiency. The feasibility in a clinical environment has yet to be proved. At Universitats Protonen Therapie Dresden, two bismuth germanate (BGO) block detectors arranged face-to-face are deployed for imaging tests with a homogeneous target irradiated by a proton pencil beam. Shifts of the target, increase of its thickness and beam energy variation experiments are conducted. Each measurement lasts about 15 minutes at a low proton beam current. The effect of one centimetre proton range deviations on the backprojected images is analysed. The number of valid Compton events as well as the trigger rate expected in a realistic treatment plan with pencil beam scanning are estimated. The results support the use of a high density material despite its moderate energy resolution, in order to maximize the coincident efficiency. Nevertheless, they discourage the applicability of a two-plane Compton camera in a clinical scenario with usual beam currents.

ION SOURCE FOR A SINGLE PARTICLE ACCELERATOR

This paper proposes a method to obtain very low beam current on the injection side of an particle accelerator. By using a combination of a well known ion source type and a short photo-emissive laser pulse, very low amount of ions can be created. The method could be used in the ion source of various types of the accelerators, where very low beam current is essential. The design is adapted to build a compact internal ion source and the dimensions of the device are adjusted to fit central region of the cyclotron U-120M. The functional parameters of the device are discussed and the ammount of the produced ions is estimated.

Nanomanufacturing Concerns about Measurements Made in the SEM Part V: Dealing with Noise.

Scanning electron microscopes (SEM) are used extensively in research and advanced manufacturing for materials characterization, metrology and process control. Unfortunately, noise can limit the specimen-specific detail and the information that can be acquired in any SEM micrograph, or measurement made from those data. The majority of SEM measurements are done at low primary electron beam currents and fast imaging mode resulting in rather noisy signals - often too noisy. The amount and the type of the noise and the steps taken to deal with it are critical to the quality and amount of the information gathered. This fifth presentation, in this series of SEM dimensional metrology tutorial papers, discusses some of the various causes of measurement uncertainty in scanned particle beam instruments specifically dealing with signal-to-noise (SNR) and its contribution to measurement imprecision.

Development of the Radiofrequency Section of a Ku-band Multiple-Beam Klystron

ABSTRACTThe multiple-beam klystrons (MBKs) are well known for some distinct performance advantages over their single-beam versions. The advantages of the MBKs include higher average power, relatively lower operating voltages, higher bandwidth, and low individual beam current. However, the design of the MBKs is more extensive and requires thorough and careful three-dimensional electromagnetic simulations and analysis. In this article, design of a four-beam klystron compatible with a predesigned electron gun is reported. Starting with simple analytical approach, detailed design and electromagnetic simulation results of the radiofrequency (RF) cavities are presented. Uniformity of the RF coupling between the external circuitry and the cavity RF field has been investigated in detail with the help of commercially available three-dimensional electromagnetic design code. A cold-test model of the RF cavity has been fabricated and its resonant frequency has been characterized experimentally. Design of the individual cavities, electromagnetic analysis of the same, simulation results of the beam-wave interaction, as well as the experimental frequency characterization of a fabricated cavity is presented in this paper.

Shielding NSLS-II light source: Importance of geometry for calculating radiation levels from beam losses

Third generation high brightness light sources are designed to have low emittance and high current beams, which contribute to higher beam loss rates that will be compensated by Top-Off injection. Shielding for these higher loss rates will be critical to protect the projected higher occupancy factors for the users. Top-Off injection requires a full energy injector, which will demand greater consideration of the potential abnormal beam miss-steering and localized losses that could occur. The high energy electron injection beam produces significantly higher neutron component dose to the experimental floor than a lower energy beam injection and ramped operations. Minimizing this dose will require adequate knowledge of where the miss-steered beam can occur and sufficient EM shielding close to the loss point, in order to attenuate the energy of the particles in the EM shower below the neutron production threshold (<10MeV), which will spread the incident energy on the bulk shield walls and thereby the dose penetrating the shield walls. Designing supplemental shielding near the loss point using the analytic shielding model is shown to be inadequate because of its lack of geometry specification for the EM shower process. To predict the dose rates outside the tunnel requires detailed description of the geometry and materials that the beam losses will encounter inside the tunnel. Modern radiation shielding Monte-Carlo codes, like FLUKA, can handle this geometric description of the radiation transport process in sufficient detail, allowing accurate predictions of the dose rates expected and the ability to show weaknesses in the design before a high radiation incident occurs. The effort required to adequately define the accelerator geometry for these codes has been greatly reduced with the implementation of the graphical interface of FLAIR to FLUKA. This made the effective shielding process for NSLS-II quite accurate and reliable. The principles used to provide supplemental shielding to the NSLS-II accelerators and the lessons learned from this process are presented.

Electrostatic-focusing image sensor with volcano-structured Spindt-type field emitter array

The authors have developed a highly sensitive, compact image sensor comprising a field emitter array (FEA) and a high-gain avalanche rushing amorphous photoconductor (HARP) target with the ultimate aim of developing an ultrahigh sensitivity, compact, high-definition television camera. Double-gated field emitters have the advantage of a compact electron beam focusing system; however, image intensities reproduced by a sensor with the double-gated, Spindt-type field emitter array with the focusing electrode stacked 1.5 μm above the gate electrode were nonuniform owing to low electron beam current. The minimum required electron beam current extracted from the double-gated field emitter array is considered for possible use with the sensor. Furthermore, a suitable field emitter array pitch to balance the electron beam current and the electrostatic-focusing lens strength was simulated. For the sensor's design guidelines, a field emitter array pitch of approximately 3 μm would be reasonable in the case of employing the volcano-structured, double-gated, Spindt-type field emitter array with the focusing electrode placed 0.2 μm below the gate electrode hole. Based on simulation results, an image sensor with the volcano-structured, Spindt-type, 3.1-μm-pitch FEA with the focusing electrode placed 0.2 μm below the gate electrode hole was fabricated. It was confirmed that the minimum electron beam current extracted from the volcano-structured FEA was approximately 2 μA/pix, and the sensor could obtain images with improved image intensity uniformity by utilizing the electrostatic-focusing effect. These results indicate that the volcano-structured, double-gated, Spindt-type FEA is potentially suitable for high-definition television FEA-HARP image sensors.

Low Starting Electron Beam Current in Degenerate Band Edge Oscillators

We propose a new principle of operation in vacuum electron-beam-based oscillators that leads to a low beam current for starting oscillations. The principle is based on super synchronous operation of an electron beam interacting with four degenerate electromagnetic modes in a slow-wave structure (SWS). The four mode super synchronous regime is associated with a very special degeneracy condition in the dispersion diagram of a cold periodic SWS called degenerate band edge (DBE). This regime features a giant group delay in the finitelength SWS and low starting-oscillation beam current. The starting beam current is at least an order of magnitude smaller compared to a conventional backward wave oscillator (BWO) of the same length. As a representative example we consider a SWS conceived by a periodically-loaded metallic waveguide supporting a DBE, and investigate starting-oscillation conditions using Pierce theory generalized to coupled transmission lines (CTL). The proposed super synchronism regime can be straightforwardly adapted to waveguide geometries others than the periodically-loaded waveguide considered here since DBE is a general property that can be realized in a variety of structures.

Double-Gated, Spindt-Type Field Emitter With Improved Electron Beam Extraction

We have developed a highly sensitive, compact image sensor that comprises a field emitter array (FEA) and a high-gain avalanche-rushing amorphous photoconductor target, with the ultimate aim of developing an ultrahighly sensitive, compact, high-definition television camera. Double-gated FEs have an advantage of having a compact electron beam focusing system; however, image intensities reproduced by the sensor were nonuniform due to low electron beam current. Furthermore, the simulated electron beam current disagreed with the measured current. The electron beam current characteristics of two types of double-gated, Spindt-type FEs (both with improved electron beam current extraction) are discussed for possible use within the sensor: convex-structured and volcano-structured. A highly accurate simulation model of the image sensor using a double-gated, Spindt-type FE has been examined; the simulated electron beam currents extracted from the double-gated, Spindt-type FE are in agreement with the measured electron beam currents when the initial electron velocity is assumed, thus suggesting that the simulated anode current–anode voltage characteristic conforms to the measured one. For example, the electron beam currents extracted from the convex-structured and volcano-structured FEs when the focusing electrode is placed 0.2 $\mu \text{m}$ below the gate electrode opening at a focusing electrode voltage of 15 V are, respectively, 1.8 and 1.9 times larger than that extracted from the previously used FEs when the focusing electrode is stacked 1.5 $\mu \text{m}$ above the gate electrode. The results show potential for reducing the degradation of the uniformity of the reproduced image’s intensity, and show that the highly accurate simulation model of the sensor is valid to design the double-gated FEAs for the sensor.

Shielding synchrotron light sources: Advantages of circular shield walls tunnels

Third generation high brightness light sources are designed to have low emittance and high current beams, which contribute to higher beam loss rates that will be compensated by Top-Off injection. Shielding for these higher loss rates will be critical to protect the projected higher occupancy factors for the users. Top-Off injection requires a full energy injector, which will demand greater consideration of the potential abnormal beam miss-steering and localized losses that could occur. The high energy electron injection beam produce significantly higher neutron component dose to the experimental floor than lower energy injection and ramped operations. High energy neutrons produced in the forward direction from thin target beam losses are a major component of the dose rate outside the shield walls of the tunnel. The convention has been to provide thicker 90° ratchet walls to reduce this dose to the beam line users. We present an alternate circular shield wall design, which naturally and cost effectively increases the path length for this forward radiation in the shield wall and thereby substantially decreasing the dose rate for these beam losses. This shield wall design will greatly reduce the dose rate to the users working near the front end optical components but will challenge the beam line designers to effectively utilize the longer length of beam line penetration in the shield wall. Additional advantages of the circular shield wall tunnel are that it's simpler to construct, allows greater access to the insertion devices and the upstream in tunnel beam line components, as well as reducing the volume of concrete and therefore the cost of the shield wall.

Accelerator and detector physics at the Bern medical cyclotron and its beam transport line

Abstract The cyclotron laboratory for radioisotope production and multi-disciplinary research at the Bern University Hospital (Inselspital) is based on an 18-MeV proton accelerator, equipped with a specifically conceived 6-m long external beam line, ending in a separate bunker. This facility allows performing daily positron emission tomography (PET) radioisotope production and research activities running in parallel. Some of the latest developments on accelerator and detector physics are reported. They encompass novel detectors for beam monitoring and studies of low current beams.

Far-reaching geometrical artefacts due to thermal decomposition of polymeric coatings around focused ion beam milled pigment particles.

Focused ion beam and scanning electron microscope (FIB-SEM) instruments are extensively used to characterize nanoscale composition of composite materials, however, their application to analysis of organic corrosion barrier coatings has been limited. The primary concern that arises with use of FIB to mill organic materials is the possibility of severe thermal damage that occurs in close proximity to the ion beam impact. Recent research has shown that such localized artefacts can be mitigated for a number of polymers through cryogenic cooling of the sample as well as low current milling and intelligent ion beam control. Here we report unexpected nonlocalized artefacts that occur during FIB milling of composite organic coatings with pigment particles. Specifically, we show that FIB milling of pigmented polysiloxane coating can lead to formation of multiple microscopic voids within the substrate as far as 5 μm away from the ion beam impact. We use further experimentation and modelling to show that void formation occurs via ion beam heating of the pigment particles that leads to decomposition and vaporization of the surrounding polysiloxane. We also identify FIB milling conditions that mitigate this issue.

Characterizing the response of a scintillator-based detector to single electrons

Here we report the response of a high angle annular dark field scintillator-based detector to single electrons. We demonstrate that care must be taken when determining the single electron intensity as significant discrepancies can occur when quantifying STEM images with different methods. To account for the detector response, we first image the detector using very low beam currents (∼8fA), and subsequently model the interval between consecutive single electrons events. We find that single electrons striking the detector present a wide distribution of intensities, which we show is not described by a simple function. Further, we present a method to accurately account for the electrons within the incident probe when conducting quantitative imaging. The role detector settings play on determining the single electron intensity is also explored. Finally, we extend our analysis to describe the response of the detector to multiple electron events within the dwell interval of each pixel.