Fly ash and multiwalled carbon nanotubes (MWCNT) reinforced multiphase polyurethane (PU) composite sheets have been fabricated by using a solution casting technique. Utilization of fly ash was the prime objective in order to reduce environmental pollution and to enhance the shielding properties of PU polymer. Our study proves that fly ash particles with MWCNTs in a PU matrix leads to novel hybrid high performance electromagnetic shielding interference material. Scanning electron microscopy confirms the existence of fly ash particles along with MWCNTs in a PU matrix. This multiphase composite shows total shielding effectiveness of 35.8 dB (>99.99% attenuation) in the Ku-band (12.4–18 GHz) frequency range. This is attributed to high dielectric losses of reinforcement present in the polymers matrix. The Nicolson–Ross–Weir algorithm has been applied to calculate the electromagnetic attributes and dielectric parameters of the PU samples by using scattering parameters (S11, S22, S12, S21). The synthesized multiphase composites were further characterized by using x-ray diffraction, Fourier transform infrared spectroscopy, and thermo gravimetric analysis.
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