Interdigitated Electrodes Research Articles

Conductometric immunosensor for specific Escherichia coli O157:H7 detection on chemically funcationalizaed interdigitated aptasensor

Escherichia coli O157:H7 is a strain of Escherichia coli known for causing foodborne illness through the consumption of contaminated or raw food. To detect this pathogen, a conductometric immunosensor was developed using a conductometric sensing approach. The sensor was constructed on an interdigitated electrode and modified with a monoclonal anti-Escherichia coli O157:H7 aptamer. A total of 200 electrode pairs were fabricated and modified to bind to the target molecule replica. The binding replica, acting as the bio-recognizer, was linked to the electrode surface using 3-Aminopropyl triethoxysilane. The sensor exhibited excellent performance, detecting Escherichia coli O157:H7 in a short time frame and demonstrating a wide detection range of 1 fM to 1 nM. Concentrations of Escherichia coli O157:H7 were detected within this range, with a minimum detection limit of 1 fM. This innovative sensor offers simplicity, speed, high sensitivity, selectivity, and the potential for rapid sample processing. The potential of this proposed biosensor is particularly beneficial in applications such as drug screening, environmental monitoring, and disease diagnosis, where real-time information on biomolecular interactions is crucial for timely decision-making and where cross-reactivity or interference may compromise the accuracy of the analysis.

Using a protrusion sapphire substrate to synthesize ZnO nanoflower arrays and application of Cu decorated ZnO nanoflower arrays as a H2 and CO gas sensor

In this study, a straightforward method is proposed to grow ZnO nanoflower arrays, which will be utilized as gas sensors for detecting H2 and CO gases. The process involves using the sol–gel method to create the ZnO thin films on a sapphire substrate with protrusion structure. These thin films are then annealed to serve as the seed layer for the subsequent growth of ZnO nanorods. For the synthesis of the ZnO nanorods, a 0.3[Formula: see text]M solution containing C6H12N4 and Zn(CH3COO)2 − 2H2O was employed as the precursor, and the hydrothermal method was used at 90∘C for a synthesis time of 60[Formula: see text]min. Due to the unique protrusion structure of the ZnO seed layer, the ZnO nanorods grew perpendicular to it, resulting in the formation of the ZnO nanoflowers. Furthermore, the ZnO seed layer’s matrix structure enables the growth of the ZnO nanoflowers in an orderly array pattern. For the further enhancement of the sensing properties of the gas sensor, a deposition method was used to decorate the Cu nanomaterials on the ZnO nanoflower arrays. The undecorated and Cu-decorated ZnO nanoflower arrays were proceeded to fabricate devices utilizing complemented by an interdigital upper electrode. Subsequently, the gas-sensing performance of both sensor types was compared concerning their ability to detect H2 and CO gases. The findings in this research conclusively indicate that sensors fabricated using the Cu-decorated ZnO nanoflower arrays exhibited a remarkable enhancement in gas-sensing properties when compared to the device using the undecorated ZnO nanoflower arrays, particularly for detecting H2 and CO gases. These results demonstrated that the Cu-decorated sensors had substantially higher response rates and faster response times during the gas-detecting processes.

Analysis of human epidermal growth factor receptor 2 interaction on aptamer-probed interdigitated electrode for breast cancer diagnosis.

Breast cancer has been reported to be high in its incidence with women, and early identification of breast cancer helps to improve and provide an effective treatment. Tumor markers are active substances; in particular, human epidermal growth factor receptor 2 (HER2) is over-expressed at the level of 20%-30%. This research work developed a highly sensitive HER2 biosensor on the interdigitated electrode (IDE) by using aptamer as a detection probe. To enhance the analytical performances, aptamer was attached to the gold nanoparticle and immobilized on the IDE through a chemical linker [(3-aminopropyl)triethoxysilane]. On the aptamer conjugation, HER2 was quantified through current-volt measurements, and the limit of detection of HER2 was calculated as 1pg/mL on a linear range from 0.1 to 3000pg/mL at an R2 (regression coefficient) of 0.9657. Further, a selective performance with human serum increased the current responses by increasing HER2 concentrations. Specific experiments with control protein and complementary aptamer sequence failed to enhance the current responses. This HER2 biosensor reflects the occurrence of breast cancer at its lower abundance and helps to identify the associated complications.

Evaluation of Upscaling the Selective Electrophoretic Deposition of Reduced Graphene Oxide on Miniaturized Au Interdigital Electrodes from Chip-to Wafer-Level

Today’s novel materials challenge the research industry to enhance the performance and to reduce the power consumption of microchips as well as to develop new sensor principles. All this applies pressure on the investigation of new economical mass production technologies for the integration into standard process sequences or on top of state-of-the-art CMOS devices. Since the discovery of graphene in 2004, many different variations have been investigated, thus the number of publications of graphene-based content grew from a few in 2004 exponential to 1.2 million only in 2019, according to Google Scholar analysis. The deposition of graphene-based materials at wafer-level is still difficult to do economically on standard SEMI wafers up to 8” diameter. In this publication, the selective electrophoretic deposition (EPD) of reduced graphene oxide flakes (rGO) will be shown. This technique is a very promising deposition method for large scale fabrication. The EPD of rGO particles is the only known way to create 3D surface topologies for an enhanced sensing area of electrochemical sensor applications e.g. biosensors. The electrical and chemical properties of this novel material provides a broad range of applications for possible sensor solutions [1, 2]. Firstly, the deposition will be shown on chip scale to gain optimum parameters in suspension preparation and EPD deposition time/voltage for a uniform particle deposition over the sensor area. Shortcuts from particles between the transmission lines or co-deposition on reference electrodes have to be avoided. This leads to a high selectivity in rGO particle deposition on Au-structures. Afterwards designs and experiments have been made on array level and a proof of concept wafer-level deposition with a low volume suspension is demonstrated. In previous work, the adhesion of rGO on Au structures in electrochemical sensors with a liquid flow, showed a migration of the deposited particles with the friction of the liquid [3]. Therefore, standard separation of particle agglomeration or splitting of primary particles with ultra sonic sonotrodes are not sufficient to gain highly concentrated suspensions with homogenous target particle distributions (< 0,5µm ≤ 1µm ≥ 5µm). For this reason, a novel particle crushing preparation by ball milling is introduced and enhanced selectivity with an improved adhesion is demonstrated. A full process of the preparation of the colloidal suspension with the definition of target particle sizes with an optimum zeta potential will be provided and the cathodic electrophoretic deposition shown [4, 5]. For the evaluation of the deposition experiments, stereo microscopy is used to reveal the selectivity on the interdigital electrode (IDE) structures (sensor area) and scanning electron microscopy (SEM) analysis is used to characterize particle sizes and 3D topography, in terms of primary and secondary particles (agglomerates). For this study, IDE structures with 15 different geometry variations (3µm to 15µm lines and spaces) are used that were manufactured [6] to evaluate the rGO deposition on chip level. A novel multisensory array design with eight sensing areas are presented, combined with wafer-level deposition as a proof of concept on a 200mm wafer.

ZnO Decorated Graphene-Based NFC Tag for Personal NO2 Exposure Monitoring during a Workday.

This paper presents the integration of a sensing layer over interdigitated electrodes and an electronic circuit on the same flexible printed circuit board. This integration provides an effective technique to use this design as a wearable gas measuring system in a target application, exhibiting high performance, low power consumption, and being lightweight for on-site monitoring. The wearable system proves the concept of using an NFC tag combined with a chemoresistive gas sensor as a cumulative gas sensor, having the possibility of holding the data for a working day, and completely capturing the exposure of a person to NO2 concentrations. Three different types of sensors were tested, depositing the sensing layers on gold electrodes over Kapton substrate: bare graphene, graphene decorated with 5 wt.% zinc oxide nanoflowers, or nanopillars. The deposited layers were characterized using FESEM, EDX, XRD, and Raman spectroscopy to determine their crystalline structure, morphological and chemical compositions. The gas sensing performance of the sensors was analyzed against NO2 (dry and humid conditions) and other interfering species (dry conditions) to check their sensitivity and selectivity. The resultant-built wearable NFC tag system accumulates the data in a non-volatile memory every minute and has an average low power consumption of 24.9 µW in dynamic operation. Also, it can be easily attached to a work vest.

Study and fabrication of rain triboelectric nanogenerator based on laser-induced graphene interdigital electrode

In this work, a rain triboelectric nanogenerator (R-TENG) based on a laser-induced graphene (LIG) interdigital electrode was developed to harvest rain energy. The R-TENG comprises a LIG interdigital electrode on a polymer substrate with a hydrophobic Polydimethylsiloxane (PDMS) layer as a protective layer. When raindrops fall onto the surface of the PDMS layer and move between two adjacent interdigital electrodes, the accumulated charges move back and forth, resulting in the generation of alternating current. The LIG pattern design and the energy collection efficiency were studied by altering the production parameters of the LIG electrode and measuring the droplet diameter on the PDMS surface. A R-TENG with an electrode width of 3 mm produces a laser power of 2.1 W, and an output voltage of 2.46 V is generated. The R-TENG could be applied as an additional energy source to harvest rain energy for agricultural IoT sensors.

Three-dimensional carbon interdigitated ring array nanofibers for electrochemical detection of dopamine neurotransmitter

Dopamine (DA) neurotransmitter is a prominent component of the central nervous system and its deficiency contributes to several diseases, such as Parkinson’s disease and schizophrenia, which significantly influence the quality of life of affected individuals. This paper introduces a circular interdigitated ring electrode, the three-dimensional carbon interdigitated ring array nanofibers (3D C-IDRA NFs), for the detection of DA using amperometric detection. The study utilized cyclic voltammetry and chronoamperometry to investigate DA. The integration of carbon nanofibers (CNFs) with 3D C-IDRA demonstrated enhanced surface area, increased current peak, and superior performance compared to the standalone 3D C-IDRA electrode, as evidenced by a redox amplification factor of 2.94 and a collection efficiency of 81.1%. The results highlight that integrating CNFs with 3D C-IDRA improves the electrochemical performance in detecting DA neurotransmitter. Thus, this discovery elucidates the advantageous potential of the 3D C-IDRA NF electrode in a wide range of applications.

Laser etching of on-chip ultra-high stability flexible micro MnO2//Zn batteries

Micro zinc batteries have great potential in fields such as smart clothing, wearable devices, and implantable medical devices, due to their high-energy density and biocompatibility, etc. However, the side reactions in Zn anode have limited their lifespan. Here we design a high stable fork-finger-shaped electrode using laser etching to obtain MnO2//Zn flexible miniature zinc ion batteries. And then, a carbon slurry is introduced to inhibit hydrogen evolution to suppress the detachment of the zinc anode. Compared with Au/PET interface, the PET/C interface had lower water retention and higher hydrogen evolution production barrier based on first-principles calculation. The interdigital electrode based on PET/C/Au had good stability. The micro MnO2–Zn flexible battery showed high specific capacity of 0.091 mAh/cm2 at 0.1 mA. After 5000 cycles at 0.5 mA, the capacity retention rate reached 83.6%. This study of interdigital electrode by laser etching brings an inspired universal pathway to fabricate a reversible Zn anode for micro-zinc storage systems.

Facile, cost-effective NO2 gas sensors based on polymer intercalated graphene/ reduced graphene oxide materials

BackgroundThe increasing severity of air pollution has driven the demand for efficient and cost-effective NO2 gas sensors. This report aims to develop a miniaturized NO2 gas sensor based on polymer intercalated graphene and reduced graphene oxide and investigate their adsorption mechanisms. MethodsThe fabrication of sensors is realized by depositing the graphene materials via a surfactant assisted two-step dipping onto laser-patterned interdigitated electrodes. The characterization of the graphene materials is carried out using various microscopic/spectroscopic techniques and the sensing performance is evaluated using a potentiostat. Significant findingsThe study reveals that the sensor based on reduced graphene oxide outperforms the graphene sensor, exhibiting a doubled response. Moreover, Langmuir adsorption isotherm also suggests the enhanced performance is attributable to the additional adsorption sites created by oxygen defects.

Fully Printed Cellulose Nanofiber-Ag Nanoparticle Composite for High-Performance Humidity Sensor.

This paper reports a high-performance humidity sensor made using a novel cellulose nanofiber (CNF)-silver nanoparticle (AgNP) sensing material. The interdigital electrode pattern was printed via reverse-offset printing using Ag nano-ink, and the sensing layer on the printed interdigitated electrode (IDE) was formed by depositing the CNF-AgNP composite via inkjet printing. The structure and morphology of the CNF-AgNP layer are characterized using ultraviolet-visible spectroscopy, an X-ray diffractometer, field emission scanning electron microscopy, energy-dispersive X-ray analysis, and transmission electron microscopy. The humidity-sensing performance of the prepared sensors is evaluated by measuring the impedance changes under the relative humidity variation between 10 and 90% relative humidity. The CNF-AgNP sensor exhibited very sensitive and fast humidity-sensing responses compared to the CNF sensor. The electrode distance effect and the response and recovery times are investigated. The enhanced humidity-sensing performance is reflected in the increased conductivity of the Ag nanoparticles and the adsorption of free water molecules associated with the porous characteristics of the CNF layer. The CNF-AgNP composite enables the development of highly sensitive, fast-responding, reproducible, flexible, and inexpensive humidity sensors.

Charge trapping-induced current–voltage hysteresis in a squaraine nanowire mesh enables synaptic memristive functionality

Nanowires (NWs) composed of 2,4-bis[(4-diethylamino)-2-hydroxyphenyl] squaraine were prepared by evaporation-induced self-assembly (EISA). NWs were ∼560 nm wide (aspect ratios: 10–90). X-ray diffraction analysis indicated polymorphism (monoclinic/triclinic). Optical data reported the triclinic phase with energetic disorder. Given the favorable alignment of the Au work function and squaraine HOMO energy, symmetric, unipolar metal–insulator–metal devices were formed by the EISA of NW meshes on inter-digitated Au electrodes. Room temperature DC I–V characteristics displayed hysteretic I–V loops, indicating memristive behavior. At low bias, data indicated Ohmic transport with carrier extraction facilitated by thermionic emission. At high biases, devices exhibited space-charge-limited conduction in the presence of shallow traps. At 77 K, data indicated Ohmic transport at low bias with carrier extraction by thermionic emission while, at high biases, trap-limited space-charge-limited conduction in the presence of traps distributed in energy, with carrier extraction by Fowler–Nordheim tunneling, was observed. The I–V hysteresis was eliminated at 77 K and attenuated by fast scan rates at room temperature, suggesting that carrier trapping/de-trapping underpinned the hysteresis. In impedance measurements, the device response fitted a Randles equivalent circuit indicating purely electronic conduction. By applying voltage waveforms, I–V hysteresis and analog resistive switching (memristive) functionality were observed. Device conductance could be increased sweep by sweep, giving conductance tuning through distinct states, with wait time- or voltage-erase options, consistent with trap filling/emptying effects. Repeated erase–write–read of multiple distinct states over many voltage cycles during continuous use in air was demonstrated. Finally, synaptic functions, e.g., pulse-dependent plasticity, and short- to long-term memory transition, were successfully emulated.

Boosting Photoresponse of Self‐Powered Photoelectrochemical Photodetectors via Planar Interdigital Electrodes

AbstractUnderwater optical communications (UOC) and light imaging have aroused tremendous attention due to the ever‐growing exploration of marine resources. Photoelectrochemical‐type photodetectors (PEC PDs) have good application potential in underwater optoelectronic devices because of their intrinsic aqueous operation characteristics with a self‐powered function and high sensitivity. However, most of the currently reported PEC PDs consist of sandwich‐like device structures, increasing the weight, volume, and complexity of the devices. Here, a planar interdigital electrode (IE) structure for high‐performance self‐powered PEC PDs for the first time is proposed. The CuO‐based IE PEC PDs achieve good photoresponse in the wide region of 365–850 nm with a high responsivity of 21.86 mA W−1 (455 nm irradiation), a fast response time (0.02/0.17 s), and good stability in artificial seawater. The good photoresponse is attributed to the promotion of interfacial electrochemical reaction kinetics and the accelerated charge transport by IE structure. Moreover, the CuO‐based IE PEC PDs show good UOC and underwater light imaging capability. Furthermore, the IE structure successfully applies in p‐Se and CuSe PEC PDs, demonstrating its good universality. The simpler structure and good photoresponse demonstrate that IE structure provides a new perspective for designing high‐performance, low‐cost, and self‐powered PEC PDs.

Foam Pressure Mapping with Optimized Electrodes

Nano-composite piezo-responsive foam (NCPF) is an inexpensive foam that can be used to measure a static load while still providing a comfortable interface. The purpose of this study was to create a modularized foam-based pressure measurement system. A measurement system was developed that uses an interdigitated electrode applied to the NCPF. Applied pressure changes the impedance of the NCPF, which, in turn, is converted into a voltage using a voltage divider. A modular measurement system is described that uses an ATtiny 1627 microcontroller to measure the pressure at nine electrodes. The nine electrode modules are controlled by an ESP32 microcontroller that aggregates the data and wirelessly transmits the data to a tablet. The modular system was demonstrated with 1008 individual electrodes. The characterization of the electrode combined with the NCPF is presented, along with optimization of the electrode geometry.

An Ultrasensitive Room-Temperature H2 Sensor Based on a TiO2 Rutile–Anatase Homojunction

Metal oxide semiconductor hetero- and homojunctions are commonly constructed to improve the performance of hydrogen sensors at room temperature. In this study, a simple two-step hydrothermal method was employed to prepare TiO2 films with homojunctions of rutile and anatase phases (denoted as TiO2-R/A). Then, the microstructure of anatase-phase TiO2 was altered by controlling the amount of hydrochloric acid to realize a more favorable porous structure for charge transport and a larger surface area for contact with H2. The sensor used a Pt interdigital electrode. At an optimal HCl dosage (25 mL), anatase-phase TiO2 uniformly covered rutile-phase TiO2 nanorods, resulting in a greater response to H2 at 2500 ppm compared with that of a rutile TiO2 nanorod sensor by a factor of 1153. The response time was 21 s, mainly because the homojunction formed by the TiO2 rutile and anatase phases increased the synergistic effect of the charge transfer and potential barrier between the two phases, resulting in the formation of more superoxide (O2−) free radicals on the surface. Furthermore, the porous structure increased the surface area for H2 adsorption. The TiO2-R/A-based sensor exhibited high selectivity, long-term stability, and a fast response. This study provides new insights into the design of commercially competitive hydrogen sensors.

Enhancing cell separation in a hybrid spiral dielectrophoretic microchannel: Numerical insights and optimal operating conditions.

Reliable separation of circulating tumor cells from blood cells is crucial for early cancer diagnosis and prognosis. Many conventional microfluidic platforms take advantage of the size difference between particles for their separation, which renders them impractical for sorting overlapping-sized cells. To address this concern, a hybrid inertial-dielectrophoretic microfluidic chip is proposed in this work for continuous and single-stage separation of lung cancer cell line A549 cells from white blood cells of overlapping size. The working mechanism of the proposed spiral microchannel embedded with planar interdigitated electrodes is validated against the experimental results. A numerical investigation is carried out over a range of flow conditions and electric field intensity to determine the separation efficiency and migration characteristics of the cell mixture. The results demonstrate the unique capability of the proposed microchannel to achieve high-throughput separation of cells at low applied voltages in both vertical and lateral directions. A significant lateral separation distance between the CTCs and the WBCs has been achieved, which allows for high-resolution and effective separation of cells. The separation resolution can be controlled by adjusting the strength of the applied electric field. Furthermore, the results demonstrate that the lateral separation distance is maximum at a voltage termed the critical voltage, which increases with the increase in the flow rate. The proposed microchannel and the developed technique can provide valuable insight into the development of a tunable and robust medical device for effective and high-throughput separation of cancer cells from the WBCs.

Understanding of ammonium salts under-deposit corrosion: Electrochemical and AIMD investigations

In-situ electrochemical experiments and ab initio molecular dynamics (AIMD) simulations are combined to investigate the under-deposit corrosion and hygroscopicity of ammonium salts on SAE 1020 steel interdigital electrodes. The findings indicate that the hygroscopicity of ammonium salts influences the evolution of the interface and the accumulation of the product film. The corresponding simulations reveal that the hydrolysis of NH4+ leads to the generation of a proton transfer chain, resulting in an elevation of H+ concentration. This hydrolysis behavior is effectively catalyzed on the Fe(1 0 0) surface, promoting the occurrence of anodic adsorption and cathodic hydrogen evolution reaction, thereby inducing corrosion.

Transforming scalable synthesis of graphene aerosol gel material toward highly flexible and wide-temperature tolerant printed micro-supercapacitors

The ever-growing demand for portable, bendable, twistable, and wearable microelectronics operating in a wide temperature range has stimulated an immense interest in the development of solid-state flexible energy storage devices using scalable fabrication technology. Herein, we developed additively manufactured graphene aerosol gel-based all-solid-state micro-supercapacitors (MSCs) via inkjet printing with functioning temperature in the range from −15 to +70 °C and exhibiting a super-stable and reliable electrochemical performance using interdigitated finger electrodes and PVA/H3PO4 solid-state electrolyte. The graphene aerosol gel was obtained using a scalable single step synthesis method from a gas phase precursor using a detonation process, producing a nanoscale shell type structure. The fabricated graphene aerosol gel-based solid-state MSC achieved a volumetric capacitance of 376.63 mF cm−3 (areal capacitance of 76.23 μF cm−2) at a constant current of 0.25 μA and demonstrated exceptional cyclic stability (∼99.6% of capacitance retention) over 10 000 cycles. To exploit the mechanical strength of the as-fabricated graphene aerosol gel-based solid-state MSC, its supercapacitive performance was scrutinized under various bending and twisting angles and the results showed excellent mechanical flexibility. Furthermore, to study the electrochemical performance of the as-fabricated graphene aerosol gel solid-state MSC in stringent surroundings, a broad temperature dependent supercapacitive analysis was performed as stated above. The electrochemical results of the as-fabricated graphene aerosol gel based all-solid-state MSC exhibit a highly potential route to develop scalable and authentic future miniaturized energy storage devices for IoT based smart electronic appliances.

Array of Interdigitated Bipolar Electrodes for Selective Capture and Analysis of Melanoma Cells

AbstractWe report a method for dielectrophoretic capture of melanoma cells and their electrochemical analysis for tumor‐specific markers, using a microfluidic device composed of microwells overlying an array of interdigitated bipolar electrodes (IDBPEs). In this device, cells are captured on each IDBPE by dielectrophoresis, and microfabricated wells allow for retention of the cells to enable their subsequent electrochemical analysis. This advancement is significant because it addresses a need for cancer diagnostics with few‐ to single‐cell resolution amenable to use in low‐resource settings. Specifically, this approach combines the selectivity of dielectrophoresis for cell phenotype, the low cost of electrochemical methods, and the ability of BPEs to be arrayed, with the sensitivity afforded by interdigitation. The IDBPE detects a redox‐active species produced by an enzyme‐linked antibody targeted to a cell surface antigen, and reports the current by electrochemiluminescence. In this work, we first characterize cell capture by dielectrophoresis at the IDBPE array. Second, the retention of cells in the microwells and their viability is demonstrated. Then, the sensitivity of the IDBPE for the redox‐active species is quantified. Finally, we demonstrate capture and analysis of melanoma cells at the IDBPE array, which underscores the ability of the IDBPE to achieve biologically relevant detection limits.

Surface Acoustic Waves (SAW) Sensors: Tone-Burst Sensing for Lab-on-a-Chip Devices.

The article presents the design concept of a surface acoustic wave (SAW)-based lab-on-a-chip sensor with multifrequency and multidirectional sensitivity. The conventional SAW sensors use delay lines that suffer from multiple signal losses such as insertion, reflection, transmission losses, etc. Most delay lines are designed to transmit and receive continuous signal at a fixed frequency. Thus, the delay lines are limited to only a few features, like frequency shift and change in wave velocity, during the signal analysis. These facts lead to limited sensitivity and a lack of opportunity to utilize the multi-directional variability of the sensing platform at different frequencies. Motivated by these facts, a guided wave sensing platform that utilizes simultaneous tone burst-based excitation in multiple directions is proposed in this article. The design incorporates a five-count tone burst signal for the omnidirectional actuation. This helps the acquisition of sensitive long part of the coda wave (CW) signals from multiple directions, which is hypothesized to enhance sensitivity through improved signal analysis. In this article, the design methodology and implementation of unique tone burst interdigitated electrodes (TB-IDT) are presented. Sensing using TB-IDT enables accessing multiple frequencies simultaneously. This results in a wider frequency spectrum and allows better scope for the detection of different target analytes. The novel design process utilized guided wave analysis of the substrate, and selective directional focused interdigitated electrodes (F-IDT) were implemented. The article demonstrates computational simulation along with experimental results with validation of multifrequency and multidirectional sensing capability.

Recent Progress in Electric‐field Enhanced 3D Graphene Electrodes using Laser Scribing for In‐plane Microsupercapacitors

AbstractThe increasing demand for miniature, flexible electronic devices have fueled the need for compact and high‐performing energy storage solutions. Microsupercapacitors (mSCs) with reduced dimension and novel electrode design have gained prominence. This concept paper summarizes and views the recent advancements in mSCs with a focus on 3D graphene electrodes and their novel electrode design to increase energy performance of the devices. Especially, we focus on these 3D graphene structures fabricated using a laser‐scribing method which offer an efficient, cost‐effective approach for enhanced mSC performance. Further, this work delves into the vital link between the electrical field effect and geometrically engineered interdigitated electrodes, which is pivotal for maximizing the ion transport and mSC energy storage performance. The insights presented here are promising for meeting the power requirements of future miniature electronics.