Intense Neutron Research Articles

DONES EVO: Risk mitigation for the IFMIF-DONES facility

The International Fusion Materials Irradiation Facility- DEMO Oriented Neutron Source (IFMIF-DONES) is a scientific infrastructure aimed to provide an intense neutron source for the qualification of materials to be used in future fusion power reactors. Its implementation is critical for the construction of the fusion DEMOnstration Power Plant (DEMO).IFMIF-DONES is a unique facility requiring a broad set of technologies. Although most of the necessary technologies have already been validated, there are still some aspects that introduce risks in the evolution of the project.In order to mitigate these risks, a consortium of companies, with the support of research centres and the funding of the CDTI (Centre for the Development of Industrial Technology and Innovation), has launched the DONES EVO Programme, which comprises six lines of research:•Improvement of signal transmission and integrity (planning and integration risks)•Optimisation of RF conditioning processes (planning and reliability risks)•Development of a reliable beam extraction device (reliability risks)•Development of technologies for the production of medical isotopes (reliability risks)•Improvement of critical parts of the lithium purification system (safety and reliability risks)•Validation of the manufacture of critical components with special materials (reliability risk).DONES EVO will focus on developing the appropriate response to the risks identified in the IFMIF-DONES project through research and prototyping around the associated technologies.This contribution will present a discussion of the risks, the proposed response to them and the evolution of the technologies involved, following selected experiments carried out throughout the project.

Response of silicon solar cells to neutrons in post-detonation monitoring

In this study, we evaluated the feasibility of using solar photovoltaic (PV) panels for the detection of prompt neutrons from a nuclear denotation. Monte Carlo (MC) simulations were performed to evaluate the response of silicon (Si) solar cells (SCs) to neutrons and support the experiments. The response of Si SCs to fission spectrum neutrons was measured experimentally using the fast neutron beam of a research reactor. Steady-state neutron measurements indicated a clear response of the Si SCs, which correlated with changes in the neutron intensity. Time-modulated neutron measurements performed using a neutron chopper demonstrated a clear transient response of Si SCs to neutrons, which was observed in the signal power spectral density plots containing peaks corresponding to frequencies of neutron pulses produced by the chopper. The resulting signal was found to be small, which was attributed to the extremely small active neutron interaction volume inside the SCs. In a real detonation scenario, the transient neutron flux is expected to be higher, and the effective neutron interaction volume of large area solar PV panels is much larger, which could significantly boost the signal. The study, overall, demonstrated the potential of large area solar PV panels or a solar farm for prompt detection and identification of a nuclear detonation.

Technical Note: Revisiting the general calibration of cosmic-ray neutron sensors to estimate soil water content

Abstract. Cosmic-ray neutron sensing (CRNS) is becoming increasingly popular for monitoring soil water content (SWC). To retrieve SWC from observed neutron intensities, local measurements of SWC are typically required to calibrate a location-specific parameter, N0, in the corresponding transfer function. In this study, we develop a generalized conversion function that explicitly takes into account the different factors that govern local neutron intensity. Thus, the parameter N0 becomes location independent, i.e. generally applicable. We demonstrate the feasibility of such a “general calibration function” by analysing 75 CRNS sites from four recently published datasets. Given the choice between the two calibration strategies – local or general – users will wonder which one is preferable. To answer this question, we estimated the resulting uncertainty in the SWC by means of error propagation. While the uncertainty in the local calibration depends on both the local reference SWC itself and its error, the uncertainty in the general calibration is mainly governed by the errors in vegetation biomass and soil bulk density. Our results suggest that a local calibration – generally considered best practice – might often not be the best option. In order to support the decision which calibration strategy – local or general – is actually preferable in the user-specific application context, we provide an interactive online tool that assesses the uncertainty in both options (https://cosmic-sense.github.io/local-or-global, last access: 23 February 2024).

Activated corrosion product contamination assessments of DEMO WCLL breeding blanket primary heat transport system

In water-cooled fusion reactors, the assessment of the primary system contamination is essential for waste management, machine availability, occupational radiation exposure, and radiological hazard determination. The primary cooling water is not only directly activated by the intense neutron field but is a contamination vector for a significant variety of gamma emitters with short to long decay half-lives. Corrosion products can be activated in those regions under neutron flux of the primary circuit and then released in the cooling water.In the EU-DEMO fusion power plant equipped with the Water-Cooled Lithium Lead Breeding Blanket (WCLL-BB) concept, the primary coolant undergoes intense neutron fields in the first wall and the breeding zone regions of the blanket. Activated Corrosion Products (ACPs) are then formed, released into the water, transported in the cooling loop and finally deposited onto the ex -vessel surfaces of the Primary Heat Transport System (PHTS), where working personnel are susceptible to being radiologically exposed.This work addresses the complete assessment of ACPs in the WCLL-BB PHTS of EU-DEMO. The simultaneous and multi-physical processes behind the ACP formation are tackled using the OSCAR-Fusion code, a comprehensive tool developed by the CEA (France) to assess contamination in fusion nuclear reactors. The whole system is modelled with zero-dimensional nodes with assigned geometrical, thermal-hydraulics, material and chemical parameters. Activation reaction rates integrated over the whole spectrum and calculated with MCNP are given to those regions exposed to the neutron flux. Results are provided in terms of mass and activity inventories of ACPs as deposit and inner oxide layers of components (pipes, heat exchangers, pumps...), ions in solution, particles in suspension, and filters and resins trapping.Mobilizable inventories such as ions, particles and deposits are important source terms in accidental scenario evolutions, while the whole activity inventory constitutes the main long-term gamma emitting source for dose rate maps determination in the tokamak building rooms housing the main PHTS equipment.

Potential of Radioactive Isotopes Production in DEMO for Commercial Use

There is widespread use of nuclear radiation for medical imagery and treatments. Worldwide, almost 40 million treatments are performed per year. There are also applications of radiation sources in other commercial fields, e.g., for weld inspection or steelmaking processes, in consumer products, in the food industry, and in agriculture. The large number of neutrons generated in a fusion reactor such as DEMO could potentially contribute to the production of the required radioactive isotopes. The associated commercial value of these isotopes could mitigate the capital investments and operating costs of a large fusion plant. The potential of producing various radioactive isotopes was studied from material pieces arranged inside a DEMO equatorial port plug. In this location, they are exposed to an intensive neutron spectrum suitable for a high isotope production rate. For this purpose, the full 3D geometry of one DEMO toroidal sector with an irradiation chamber in the equatorial port plug was modeled with an MCNP code to perform neutron transport simulations. Subsequent activation calculations provide detailed information on the quality and composition of the produced radioactive isotopes. The technical feasibility and the commercial potential of the production of various isotopes in the DEMO port are reported.

Employing NDVI as vegetation correction variable to improve soil moisture measurements of mobile cosmic-ray neutron sensor near the Qilian Mountains

Cosmic-ray neutron sensors (CRNS) are a powerful tool for measuring soil moisture on a hectometer scale, and mobile cosmic-ray neutron technology holds significant importance for upscaling soil moisture. However, vegetation strongly affects with CRNS soil moisture measurements. Variations in vegetation over time change how the CRNS is affected, which is more challenging than a stable vegetation cover, particularly during CRNS roving, where one crosses many vegetation covers. To correct vegetation, we hypothesized that Normalized Difference Vegetation Index (NDVI) can representvegetation hydrogen pools. From 2020 to 2023, at the 74 plots with varying vegetation cover near the Qilian Mountains, the experiments for soil moisture measurements were conducted in shrubs, forests, deserts, farmlands, and grasslands using a Cosmic-ray Neutron Rover. The measured neutron intensity clearly varied across different landscapes, and the calibrated parameter N0 differed among 74 plots. The variations in vegetation cover resulted in low measurement accuracy for CRNS. All three NDVI vegetation correction methods (NDVI-θNDVI method, NDVI-NDVIave method, and NDVI-N0 method) offered by the study could improve accuracy of soil moisture measurements. In the optimal NDVI-N0 method, the relationship between NDVI and N0 was established using a power function y = 373.9 (x + 0.015)−0.136 (R2 = 0.77), which had the capability to decrease the root mean square error between oven-dried and measured soil moisture from 0.093 to 0.032 g g−1 in our study area. Employing NDVI instead of biomass for CRNS vegetation correction can substantially reduce workload and effectively enhance CRNS soil moisture measurements, showing the potential for upscaling soil moisture.

Radiation effect assessment on spent fuel transport CASK by aircraft sabotage attack

The purpose of this study is to evaluate the radiation effects depending on the size of the damage of cask when the outer shield of a spent nuclear fuel transportation cask is damaged by impact due to sabotage. Neutron and gamma-ray intensities and spectra were calculated using the ORIGEN module of the SCALE 6.2.4 code package (W. A. Wieselquist et al., 2020), and the equivalent dose rates were calculated using the MCNP6.2 code (C. J Werner, et al., 2017).The ABAQUS code was used to assess the degree of the opening of the cask lid due to external impact, and in the case of radiation source leakage, the dose assessment was performed by assuming a maximum of 6% damage to the nuclear fuel assemblies based on overseas experimental cases.

Principles, Recent Developmentsand Perspectives in Boron NeutronCapture Therapy (BNCT)

For decades, BNCT was seen as an attractive concept and an intellectual challenge with no prospect of widespread clinical application. This situation has changed fundamentally in just a few years with the progress in accelerator technology. Low-energy, high-intensity neutron sources can now be integrated into hospitals and are therefore directly available for patient treatment. A pioneer in this field is the development in Japan, where patients are already being treated in three hospitals, using in-house accelerator-based systems. Furthermore, the costs associated with the BNCT treatment of recurrent tumors in the head and neck area are already covered by the healthcare system. It is time to keep up to date with this technology and work to make it available to patients in high-tech medicine in other countries, especially in Europe and North America. This short article summarizes the main principles of BNCT, outlines some aspects of its history and mentions ongoing projects as well as some hurdles that need to be overcome, as well as the scientific questions that need to be addressed for wider availability of the method.

Actinide targets for the synthesis of superheavy nuclei

The use of heavy actinide targets, including 243Am, 240,242,244Pu, 245,248Cm, 249Bk, and 249Cf, irradiated by intense heavy ion beams of 48Ca has resulted in a significant expansion of the periodic table since 2000, including the discovery of five new heaviest elements and more than 50 new isotopes. These actinide materials can only be produced by intense neutron irradiation in very high flux reactors followed by chemical processing and purification in specialized hot cell facilities available in only a few locations worldwide. This paper reviews the reactor production of heavy actinides, the recovery and chemical separation of actinide materials, and the preparation of actinide targets for superheavy element experiments. The focus is on 248Cm, 249Bk, mixed 249−251Cf, and 254Es, including current availabilities and new production processes. The impacts of new facilities, including the Superheavy Element Factory at Dubna, accelerator and separator upgrades at RIKEN, and proposed upgrades to the High Flux Isotope Reactor at Oak Ridge are also described. Examples of recent superheavy element research are discussed as well as future opportunities for superheavy research using actinide targets.

Neutron/gamma scintillation detector for status monitoring of accelerator-driven neutron source IREN

This paper presents a neutron/gamma detector based on a micropixel avalanche photodiode and a plastic scintillator that monitors the status of the accelerator-driven intense resonance neutron source (IREN) facility by measuring the neutron/gamma intensity in the target hall. The electronics of the neutron/gamma detector has been designed and developed. The size of the plastic scintillator was selected to be 3.7 × 3.7 × 30 mm3 due to the sensitive area of the MAPD. The experimental results demonstrated a dependence between the count rate of the detector and the frequency of the accelerator. The detector is sensitive to intermediate and fast neutrons. The minimum detectable energy was determined to be 200 keV using Cs-137 point gamma source. The maximum counting rate of the detector from TTL out is about 2.2·106 counts/sec, but for analogue output it is about 2·107 counts/sec. The detector can not allow discriminating neutrons and gamma rays by charge integration method.

Experimental study on Compton camera for boron neutron capture therapy applications

Boron neutron capture therapy (BNCT) is a high-dose-intensive radiation therapy that has gained popularity due to advancements in accelerator neutron sources. To determine the dose for BNCT, it is necessary to know the difficult-to-determine boron concentration and neutron fluence. To estimate this dose, we propose a method of measuring the prompt γ-rays (PGs) from the boron neutron capture reaction (BNCR) using a Compton camera. We performed a fundamental experiment to verify basic imaging performance and the ability to discern the PGs from 511 keV annihilation γ-rays. A Si/CdTe Compton camera was used to image the BNCR and showed an energy peak of 478 keV PGs, separate from the annihilation γ-ray peak. The Compton camera could visualize the boron target with low neutron intensity and high boron concentration. This study experimentally confirms the ability of Si/CdTe Compton cameras to image BNCRs.

Recent H- ion source research and development at the Oak Ridge National Laboratory* *This manuscript has been authored by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the US Department of Energy (DOE). This research was supported by the DOE Office ofScience, Basic Energy Science, Scientific User Facilities. The US government retains and thepublisher, by accepting the article for publication, acknowledges that

The U.S. Spallation Neutron Source (SNS) is a state-of-the-art neutron scattering facility delivering the world's most intense pulsed neutron beams to a wide array of instruments which are used to conduct investigations in many fields of science and engineering. Neutrons are produced from spallation of liquid Hg by bombardment of short (∼1 μs), intense (∼35 A) pulses of protons delivered at 60 Hz by a storage ring which is fed by a high-intensity, ∼1 GeV H- LINAC. This facility has operated almost continuously since 2006, with ion source performance increasing over those years, and currently providing 50–60 mA of H- ions with a duty-factor of 6% for maintenance-free runs of several months with near 100% availability. Ion source research and development at ORNL has played a key role in enabling and supporting this success: this report provides an update on some of the ongoing ion source research and development efforts which have been undertaken since the previous Negative Ion Beams and Sources (NIBS) conference in 2020. These include significant improvements to H- beam current by extraction from a larger source outlet aperture and improvements to the electron dumping system which should eliminate the gradual loss of electrode voltage over the course of a run which has occasionally impacted SNS operations. Improvement and simplification of the plasma ignition system for the external antenna ion source, a long-standing problem, was also realized. Lastly, RF coupling efficiency was measured for both the SNS internal and external antenna ion sources.

Unveiling the structural phase transition and magnetic structure of ternary boride PrIr3B2

We present a comprehensive study of PrIr3B2, which includes a detailed investigation of its crystal and magnetic structure using neutron diffraction. AC and DC magnetization and heat capacity data reveal antiferromagnetic ordering at T N = 10 K. The heat capacity measurements further exhibit a broad peak near 270 K which is related to a structural transition from P6/mmm to C2/m seen in low temperature x-ray diffraction and neutron diffraction. High intensity neutron diffraction data confirm the long-range ordering of Pr3+ spins, with no apparent magnetic moment on either of the Iridium sites. Two possible magnetic structures with either k 1 = [1,0,0] or k 2 = [½,½,0] fit nearly equally well the neutron diffraction data. However, based on previous magnetization studies on a single crystalline sample it is argued that the second solution with k 2 corresponds to the appropriate magnetic structure of PrIr3B2 below 10 K. In this magnetic structure, the Pr3+ moments are oriented at ∼45° to both the a and b axes, with the c-axis being the hard axis of magnetization. Overall, our results provide new insights into the magnetic and structural properties of PrIr3B2.

Application of cosmic‐ray neutron probes for measuring soil moisture in rocky areas of the Taihang Mountains, North China

AbstractThe cosmic‐ray neutron probe (CRNP) is a mesoscale and noninvasive method for measuring soil moisture and has been widely studied and applied. However, studies of its applicability in rocky mountainous areas are still challenging in complex topography and high gravel content. In this study, a field experiment was carried out to assess the applicability of the CRNP for measuring soil moisture in rocky areas of Taihang Mountains of North China. The results showed that the Pearson correlation coefficient and the root mean square error between the soil moisture from CRNP and the drying method are 0.911 and 0.025 m3 m−3, respectively, indicating that the CRNP can estimate the average soil moisture well in the study area. Compared with the capacitive sensor, the CRNP overestimated soil moisture when small rainfall events occurred, which was caused by the interception of canopy and litter. The nonlinear weighting method performed better than the linear weighting method in representing average soil moisture within the CRNP footprint. The high gravel content that contained high lattice water content reduced the penetration depth of CRNP. Biomass reduces the accuracy of the CRNP by affecting the neutron intensity. In summary, CRNP can measure soil moisture accurately in rocky areas of the Taihang Mountains, especially in dry environments with low biomass.

Mesoscale soil moisture survey by mobile cosmic-ray neutron sensor across various landscapes in the Heihe River Basin

The cosmic-ray neutron technology is a novel method for upscaling soil moisture, holding significant importance in drought monitoring, soil water storage estimation, calibration of remote sensing products, and data assimilation of land surface models. However, most studies conducted soil moisture measurement experiments using static Cosmic-Ray Neutron Sensors (CRNS) and are often limited to a single landscape, lacking in-situ measurement for the cosmic-ray neutron rover across various landscapes. This study carried out soil moisture observation experiments using a cosmic-ray neutron rover in nine grassland plots, nine farmland plots, and nine desert plots of the Heihe River Basin, Northwest China. The neutron counts displayed clear variations among different plots, and an equation could represent the relationship between neutron intensity and multiple variables near the ground. The parameter N0 was the smallest for grassland and greatest for desert, and there was a significant negative correlation between Normalized Difference Vegetation Index and N0 (P <0.05). Furthermore, the performance of CRNS notably improved after considering soil lattice water and soil organic matter. The Root Mean Square Error (RMSE) between the measured and oven-dried soil moisture increased with radius. Soil moisture measured by CRNS strongly supported the 100 m diameter footprint assumption (RMSE <0.044 g/g). The study offers valuable insights into the application and promotion of cosmic-ray neutron technology across various landscapes within a basin.

Time-of-flight spectroscopy of ultracold neutrons at the PSI UCN source

The ultracold neutron (UCN) source at the Paul Scherrer Institute (PSI) provides high intensities of storable neutrons for fundamental physics experiments. The neutron velocity spectrum parallel to the beamline axis was determined by time-of-flight spectroscopy using a neutron chopper. In particular, the temporal evolution of the spectrum during neutron production and UCN storage in the source storage volume was investigated and compared to Monte Carlo simulation results. A softening of the measured spectrum from a mean velocity of 7.7(1)–5.1(1) hbox {m s}^{-1} occurred within the first 30 hbox {s} after the proton beam pulse had impinged on the spallation target. A spectral hardening was observed over longer time scales of one measurement day, consistent with the effect of surface degradation of the solid deuterium moderator.

A Novel, Rapid Response Renewable Biopolymer Neutron and Gamma Radiation Solid-State Detector for Dosimetry and Nuclear Reactor Flux-Power Mapping

A novel solid-state neutron and gamma radiation monitor-dosimeter based on biopolymer polylactic acid (PLA) is presented. The resulting detector (PLAD) technology takes advantage of property changes of the renewable PLA resin when subject to ionizing nuclear radiation. A simple yet rapid and accurate (±10%) low-cost (&lt;$0.01/detector) mass loss upon dissolution (MLD) technique was successfully developed; MLD is based on a simple mass balance for discerning neutron and/or gamma doses using small (40 mg, ~4 mm diameter) ultra-low-cost (&lt;$0.01) resin beads via dissolution in acetone. The GammaCellTM Co-60 irradiator, and the PUR-1 12 kW fission nuclear research reactor were utilized, respectively. Irradiation absorbed doses ranged from 1 to 100 kGy. Acetone bath temperature was varied from ~40 °C to ~54 °C. Results revealed a strong dependence of MLD on acetone bath temperature between neutron and gamma photon dose components; this allowed for the unique ability of PLAD to potentially perform as both a neutron-cum-gamma or as a gamma or neutron radiation dosimeter and intensity level detector. A linear trend is found for combined neutron and gamma radiation doses from 0 to 40 kGy when dissolution is conducted above 50 °C. The important potential ability to distinguish neutron from gamma radiation fields was scoped and found to be feasible by determining MLD at 45 °C. The potential was studied for simultaneous use as an in-core neutron and gamma monitor of an operating 3 GWt light-water reactor (LWR). Scoping tests were conducted with the pre-irradiated (@ 20 °C) PLAD resin beads followed by heating to in-core LWR coolant (300 °C) conditions for ~30 s corresponding to the time to reach ~40 kGy total doses in a typical 3 GWt LWR. MLD results were unaffected, indicating the exciting and unique potential for in situ (low-cost, accurate and rapid) simultaneous mapping of neutron and gamma radiation fluxes, related dosimetry, and fission power level monitoring.

Retrieving soil moisture using cosmic-ray neutron technology based on COSMIC model in the desert-oasis region.

Cosmic-ray neutron technology could estimate average soil moisture on scale of hectometers by monitoring the neutron intensity near the ground, which has been successfully applied in forest, grassland, farmland, and other ecosystems. To verify the reliability of Cosmic-ray Soil Moisture Interaction Code (COSMIC) model for retrieving mesoscale soil moisture in arid regions, we carried out soil moisture observation experiment by using the cosmic-ray neutron rover in the desert-oasis region of the middle reaches of Heihe River. The results showed that the fast neutron intensity in the desert-oasis region were 350-715 counts·(30 s)-1, and the calibrated high energy neutron intensity (Ncosmic) were (38.5±2.2) counts·(30 s)-1, which was affected by land surface characteristics. Both COSMIC model (root mean square error=0.019 g·g-1) and N0 equation (root mean square error=0.018 g·g-1) could well assess the mesoscale soil moisture, with the accuracy of soil moisture being higher considering soil lattice water. The average penetration depth was 19 cm in the oasis region and 36 cm in the desert region during the experiment. COSMIC model could be used to retrieve soil moisture by cosmic ray neutron in the desert-oasis regions, which had great potential to realize data assimilation of surface meteorological-hydrological-ecological variables by combining with land surface models.

Monte Carlo simulations of LUOSHU: a new 46-meter small-angle neutron scattering instrument in China

The LUOSHU small-angle neutron scattering spectrometer is one of the neutron scattering instruments under construction at China Mianyang Research Reactor. Quantitative characterization of nanoparticles is now in a higher demand for research interests in material science, physics, chemistry, biology. Therefore, as a general-purpose small-angle scattering spectrometer, LUOSHU is aimed to provide a large accessible Q range, flexible resolution and sufficient neutron flux. Monte Carlo simulations have been performed on LUOSHU from the neutron source to sample platform to optimize the parameters of the bender part, collimation system, and the velocity selector. And the instrument layout is optimized base on the simulation results. Finally, the maximum neutron intensity of the neutron beam at the sample stage can reach 1.01 × 107 N·s-1·cm-2 and its divergence is 0.63.

A change in perspective: downhole cosmic-ray neutron sensing for the estimation of soil moisture

Abstract. Above-ground cosmic-ray neutron sensing (CRNS) allows for the non-invasive estimation of the field-scale soil moisture content in the upper decimetres of the soil. However, large parts of the deeper vadose zone remain outside of its observational window. Retrieving soil moisture information from these deeper layers requires extrapolation, modelling or other methods, all of which come with methodological challenges. Against this background, we investigate CRNS for downhole soil moisture measurements in deeper layers of the vadose zone. To render calibration with in situ soil moisture measurements unnecessary, we rescaled neutron intensities observed below the terrain surface with intensities measured above a waterbody. An experimental set-up with a CRNS sensor deployed at different depths of up to 10 m below the surface in a groundwater observation well combined with particle transport simulations revealed the response of downhole thermal neutron intensities to changes in the soil moisture content at the depth of the downhole neutron detector as well as in the layers above it. The simulation results suggest that the sensitive measurement radius of several decimetres, which depends on soil moisture and soil bulk density, exceeds that of a standard active neutron probe (which is only about 30 cm). We derived transfer functions to estimate downhole neutron signals from soil moisture information, and we describe approaches for using these transfer functions in an inverse way to derive soil moisture from the observed neutron signals. The in situ neutron and soil moisture observations confirm the applicability of these functions and prove the concept of passive downhole soil moisture estimation, even at larger depths, using cosmic-ray neutron sensing.