Tribovoltaic nanogenerators (TVNGs) based on tribovoltaic effect can output DC current directly, and has the advantages of high output current density and low internal resistance. While TVNGs have been restricted by its low output voltage and power. Herein, we have developed a metal-polymer film with a micro-uneven structure on the surface, much higher corrosion resistance and wear resistance than metal. On this basis, a centimeter-level sliding structure metal-EP/GaN-TVNG has been fabricated, which shows a high and stable long-term DC electrical output (a maximized power output of 4.19 W/m2 when matched with a 0.07 MΩ resistor, a stable output current of 2.25 A/m2 and a peak Voc of 27 V). Further, a TVNG vehicle travelling intelligent sensor and system which can integrate electrical signals collected by TVNG into digital signal processing algorithms and then feed backing to the driving system, has been designed and manufactured. As an effective method for deep analysis of signals, Ensemble Empirical Mode Decomposition (EEMD) has been used for the first time for deep processing of nanogenerator signals in this work. This work provides a new model of further development of high output TVNG and a new deep signal processing methods of TVNG/TENG signal.