Hard X-ray Imaging Research Articles

Hitomi X-ray observation of the pulsar wind nebula G21.5−0.9

Abstract We present results from the Hitomi X-ray observation of a young composite-type supernova remnant (SNR) G21.5−0.9, whose emission is dominated by the pulsar wind nebula (PWN) contribution. The X-ray spectra in the 0.8–80 keV range obtained with the Soft X-ray Spectrometer (SXS), Soft X-ray Imager, and Hard X-ray Imager (HXI) show a significant break in the continuum as previously found with the NuSTAR observation. After taking into account all known emissions from the SNR other than the PWN itself, we find that the Hitomi spectra can be fitted with a broken power law with photon indices of Γ1 = 1.74 ± 0.02 and Γ2 = 2.14 ± 0.01 below and above the break at 7.1 ± 0.3 keV, which is significantly lower than the NuSTAR result (∼9.0 keV). The spectral break cannot be reproduced by time-dependent particle injection one-zone spectral energy distribution models, which strongly indicates that a more complex emission model is needed, as suggested by recent theoretical models. We also search for narrow emission or absorption lines with the SXS, and perform a timing analysis of PSR J1833−1034 with the HXI and the Soft Gamma-ray Detector. No significant pulsation is found from the pulsar. However, unexpectedly, narrow absorption line features are detected in the SXS data at 4.2345 keV and 9.296 keV with a significance of 3.65 σ. While the origin of these features is not understood, their mere detection opens up a new field of research and was only possible with the high resolution, sensitivity, and ability to measure extended sources provided by an X-ray microcalorimeter.

Advances in indirect detector systems for ultra high-speed hard X-ray imaging with synchrotron light

We report on indirect X-ray detector systems for various full-field, ultra high-speed X-ray imaging methodologies, such as X-ray phase-contrast radiography, diffraction topography, grating interferometry and speckle-based imaging performed at the hard X-ray imaging beamline ID19 of the European Synchrotron—ESRF. Our work highlights the versatility of indirect X-ray detectors to multiple goals such as single synchrotron pulse isolation, multiple-frame recording up to millions frames per second, high efficiency, and high spatial resolution. Besides the technical advancements, potential applications are briefly introduced and discussed.

In-orbit performance and calibration of the Hard X-ray Imager onboard Hitomi (ASTRO-H)

The Hard X-ray Imager (HXI) onboard Hitomi (ASTRO-H) is an imaging spectrometer covering hard X-ray energies of 5-80 keV. Combined with the hard X-ray telescope, it enables imaging spectroscopy with an angular resolution of $1^\prime.7$ half-power diameter, in a field of view of $9^\prime\times9^\prime$. The main imager is composed of 4 layers of Si detectors and 1 layer of CdTe detector, stacked to cover wide energy band up to 80 keV, surrounded by an active shield made of BGO scintillator to reduce the background. The HXI started observations 12 days before the Hitomi loss, and successfully obtained data from G21.5$-$0.9, Crab and blank sky. Utilizing these data, we calibrate the detector response and study properties of in-orbit background. The observed Crab spectra agree well with a powerlaw model convolved with the detector response, within 5% accuracy. We find that albedo electrons in specified orbit strongly affect the background of Si top layer, and establish a screening method to reduce it. The background level over the full field of view after all the processing and screening is as low as the pre-flight requirement of $1$-$3\times10^{-4}$ counts s$^{-1}$ cm$^{-2}$ keV$^{-1}$.

In-flight performance of the Canadian Astro-H Metrology System

The Canadian Astro-H Metrology System (CAMS) on the Hitomi X-ray satellite is a laser alignment system that measures the lateral displacement (X/Y) of the extensible optical bench (EOB) along the optical axis of the hard X-ray telescopes (HXTs). The CAMS consists of two identical units that together can be used to discern translation and rotation of the deployable element along the axis. This paper presents the results of in-flight usage of the CAMS during deployment of the EOB and during two observations (Crab and G21.5-0.9) with the HXTs. The CAMS was extremely important during the deployment operation by providing real-time positioning information of the EOB with micrometer scale resolution. In this work, we show how the CAMS improves data quality coming from the hard X-ray imagers. Moreover, we demonstrate that a metrology system is even more important as the angular resolution of the telescope increases. Such a metrology system will be an indispensable tool for future high resolution X-ray imaging missions.

Glimpse of the highly obscured HMXB IGR J16318−4848 with Hitomi

Abstract We report on a Hitomi observation of IGR J16318−4848, a high-mass X-ray binary system with an extremely strong absorption of NH ∼ 1024 cm−2. Previous X-ray studies revealed that its spectrum is dominated by strong fluorescence lines of Fe as well as continuum emission lines. For physical and geometrical insight into the nature of the reprocessing material, we utilized the high spectroscopic resolving power of the X-ray microcalorimeter (the soft X-ray spectrometer: SXS) and the wide-band sensitivity by the soft and hard X-ray imagers (SXI and HXI) aboard Hitomi. Even though the photon counts are limited due to unintended off-axis pointing, the SXS spectrum resolves Fe Kα1 and Kα2 lines and puts strong constraints on the line centroid and line width. The line width corresponds to a velocity of 160$^{+300}_{-70}$ km s−1. This represents the most accurate, and smallest, width measurement of this line made so far from the any X-ray binary, much less than the Doppler broadening and Doppler shift expected from speeds that are characteristic of similar systems. Combined with the K-shell edge energy measured by the SXI and HXI spectra, the ionization state of Fe is estimated to be in the range of Fe i–iv. Considering the estimated ionization parameter and the distance between the X-ray source and the absorber, the density and thickness of the materials are estimated. The extraordinarily strong absorption and the absence of a Compton shoulder component have been confirmed. These characteristics suggest reprocessing materials that are distributed in a narrow solid angle or scattering, primarily by warm free electrons or neutral hydrogen. This measurement was achieved using the SXS detection of 19 photons. It provides strong motivation for follow-up observations of this and other X-ray binaries using the X-ray Astrophysics Recovery Mission and other comparable future instruments.

Multimodal hard x-ray imaging with resolution approaching 10 nm for studies in material science

We report multimodal scanning hard x-ray imaging with spatial resolution approaching 10 nm and its application to contemporary studies in the field of material science. The high spatial resolution is achieved by focusing hard x-rays with two crossed multilayer Laue lenses and raster-scanning a sample with respect to the nanofocusing optics. Various techniques are used to characterize and verify the achieved focus size and imaging resolution. The multimodal imaging is realized by utilizing simultaneously absorption-, phase-, and fluorescence-contrast mechanisms. The combination of high spatial resolution and multimodal imaging enables a comprehensive study of a sample on a very fine length scale. In this work, the unique multimodal imaging capability was used to investigate a mixed ionic-electronic conducting ceramic-based membrane material employed in solid oxide fuel cells and membrane separations (compound of Ce0.8Gd0.2O2−x and CoFe2O4) which revealed the existence of an emergent material phase and quantified the chemical complexity at the nanoscale.

Inorbit performance of the Hard X-ray Telescope (HXT) on board the Hitomi (ASTRO-H) satellite

Hitomi (ASTRO-H) carries two Hard X-ray Telescopes (HXTs) that can focus X-rays up to 80 keV. Combined with the Hard X-ray Imagers (HXIs) that detect the focused X-rays, imaging spectroscopy in the high-energy band from 5 keV to 80 keV is made possible. We studied characteristics of HXTs after the launch such as the encircled energy function (EEF) and the effective area using the data of a Crab observation. The half power diameters (HPDs) in the 5--80 keV band evaluated from the EEFs are 1.59 arcmin for HXT-1 and 1.65 arcmin for HXT-2. Those are consistent with the HPDs measured with ground experiments when uncertainties are taken into account. We can conclude that there is no significant change in the characteristics of the HXTs before and after the launch. The off-axis angle of the aim point from the optical axis is evaluated to be less than 0.5 arcmin for both HXT-1 and HXT-2. The best-fit parameters for the Crab spectrum obtained with the HXT-HXI system are consistent with the canonical values.

Modeling of proton-induced radioactivation background in hard X-ray telescopes: Geant4-based simulation and its demonstration by Hitomi’s measurement in a low Earth orbit

Hard X-ray astronomical observatories in orbit suffer from a significant amount of background due to radioactivation induced by cosmic-ray protons and/or geomagnetically trapped protons. Within the framework of a full Monte Carlo simulation, we present modeling of in-orbit instrumental background which is dominated by radioactivation. To reduce the computation time required by straightforward simulations of delayed emissions from activated isotopes, we insert a semi-analytical calculation that converts production probabilities of radioactive isotopes by interaction of the primary protons into decay rates at measurement time of all secondary isotopes. Therefore, our simulation method is separated into three steps: (1) simulation of isotope production, (2) semi-analytical conversion to decay rates, and (3) simulation of decays of the isotopes at measurement time. This method is verified by a simple setup that has a CdTe semiconductor detector, and shows a 100-fold improvement in efficiency over the straightforward simulation. To demonstrate its experimental performance, the simulation framework was tested against data measured with a CdTe sensor in the Hard X-ray Imager onboard the Hitomi X-ray Astronomy Satellite, which was put into a low Earth orbit with an altitude of 570 km and an inclination of 31°, and thus experienced a large amount of irradiation from geomagnetically trapped protons during its passages through the South Atlantic Anomaly. The simulation is able to treat full histories of the proton irradiation and multiple measurement windows. The simulation results agree very well with the measured data, showing that the measured background is well described by the combination of proton-induced radioactivation of the CdTe detector itself and thick Bi4Ge3O12 scintillator shields, leakage of cosmic X-ray background and albedo gamma-ray radiation, and emissions from naturally contaminated isotopes in the detector system.

Design and characterization of a 12-bit 10MS/s 10mW pipelined SAR ADC for CZT-based hard X-ray imager

This paper presents a 12-bit pipelined successive approximation register (SAR) ADC for CZT-based hard X-ray Imager. The proposed ADC is comprised of a first-stage 6-bit SAR-based Multiplying Digital Analog Converter (MDAC) and a second-stage 8-bit SAR ADC. A novel MDAC architecture using Vcm-based Switching method is employed to maximize the energy efficiency and improve the linearity of the ADC. Moreover, the unit-capacitor array instead of the binary-weighted capacitor array is adopted to improve the conversion speed and linearity of the ADC in the first-stage MDAC. In addition, a new layout design method for the binary-weighted capacitor array is proposed to reduce the capacitor mismatches and make the routing become easier and less-time-consuming. Finally, several radiation-hardened-by-design technologies are adopted in the layout design against space radiation effects. The prototype chip was fabricated in 0.18 μm mixed-signal 1.8V/3.3V process and operated at 1.8 V supply. The chip occupies a core area of only 0.58 mm2. The proposed pipelined SAR ADC achieves a peak signal-to-noise-and-distortion ratio (SNDR) of 66.7 dB and a peak spurious-free dynamic range (SFDR) of 78.6 dB at 10 MS/s sampling rate and consumes 10 mW. The figure of merit (FOM) of the proposed ADC is 0.56 pJ/conversion-step.

Laser processing quality monitoring by combining acoustic emission and machine learning: a high-speed X-ray imaging approach

In situ and real-time monitoring of laser processes are very challenging due to complex dynamics of the laser-matter interactions. Acoustic emission (AE) technique is often used as non-destructive monitoring of many kinds of processes. However, acoustic emission is not industrialized for laser processing for two reasons. First, the signals are too sensitive to the environmental noises. Second, a correlation of the acoustic emission signal with the real events is very difficult to realize despite being of utmost importance. To overcome these difficulties, we combined fast hard X-ray imaging with acoustic sensors and state-of-the-art machine learning.

A compact imaging system with a CdTe double-sided strip detector for non-destructive analysis using negative muonic X-rays

A CdTe double-sided strip detector (CdTe-DSD) is an ideal device for imaging and spectroscopic measurements in the hard X-ray range above 10 keV. Recent development enables us to realize an imager with a detection area of ∼10 cm2. An energy resolution of 1–2 keV (FWHM) and a position resolution of a few hundred μm are available from the detector. This type of imager has been long awaited for non-destructive elemental analysis, especially by using negative muons, because energies of characteristic X-rays from muonic atoms are about 200 time higher than those from normal atoms. With the method that uses negative muons, hard X-ray information gives the spatial distribution of elements in samples at a certain depth defined by the initial momentum of the muon beam. In order to study three-dimensional imaging capability of the method, we have developed a compact imaging system based on CdTe-DSD and a ϕ 3 mm pinhole collimator as the first prototype. We conducted experiments with samples which consist of layers of Al, BN and LiF irradiated by negative muon beams in MUSE/J-PARC and successfully reconstruct hard X-ray images of muonic X-rays from B, N and F at various depths.

A high-resolution CdTe imaging detector with multi-pinhole optics for in-vivo molecular imaging

High-resolution CdTe semiconductor detectors with both fine position resolution and high energy resolution hold great promise to improve measurement in various hard X-ray and gamma-ray imaging experiments. In the field of in-vivo molecular imaging, where the molecules labeled with radioisotopes are injected into a small animal and their distribution in a body is detected by gamma-ray imaging detectors externally, a large detection area is also required to obtain a number of projections from multiple pinholes. We have developed a prototype imaging system consisting of a 32 mm-wide CdTe double-sided strip detector equipped with multi-pinhole optics. We describe its imaging capability, as studied through experiments with radioisotopes for medical use (125I and 111In) and a 3D phantom.

NuSTAR Hard X-Ray Observation of a Sub-A Class Solar Flare

Abstract We report a Nuclear Spectroscopic Telescope Array (NuSTAR) observation of a solar microflare, SOL2015-09-01T04. Although it was too faint to be observed by the GOES X-ray Sensor, we estimate the event to be an A0.1 class flare in brightness. This microflare, with only ∼5 counts s−1 detector−1 observed by the Reuven Ramaty High Energy Solar Spectroscopic Imager (RHESSI), is fainter than any hard X-ray (HXR) flare in the existing literature. The microflare occurred during a solar pointing by the highly sensitive NuSTAR astrophysical observatory, which used its direct focusing optics to produce detailed HXR microflare spectra and images. The microflare exhibits HXR properties commonly observed in larger flares, including a fast rise and more gradual decay, earlier peak time with higher energy, spatial dimensions similar to the RHESSI microflares, and a high-energy excess beyond an isothermal spectral component during the impulsive phase. The microflare is small in emission measure, temperature, and energy, though not in physical size; observations are consistent with an origin via the interaction of at least two magnetic loops. We estimate the increase in thermal energy at the time of the microflare to be 2.4 × 1027 erg. The observation suggests that flares do indeed scale down to extremely small energies and retain what we customarily think of as “flare-like” properties.

Three-Dimensional Imaging of Biological Tissue by Cryo X-Ray Ptychography

High-throughput three-dimensional cryogenic imaging of thick biological specimens is valuable for identifying biologically- or pathologically-relevant features of interest, especially for subsequent correlative studies. Unfortunately, high-resolution imaging techniques at cryogenic conditions often require sample reduction through sequential physical milling or sectioning for sufficient penetration to generate each image of the 3-D stack. This study represents the first demonstration of using ptychographic hard X-ray tomography at cryogenic temperatures for imaging thick biological tissue in a chemically-fixed, frozen-hydrated state without heavy metal staining and organic solvents. Applied to mammalian brain, this label-free cryogenic imaging method allows visualization of myelinated axons and sub-cellular features such as age-related pigmented cellular inclusions at a spatial resolution of ~100 nanometers and thicknesses approaching 100 microns. Because our approach does not require dehydration, staining or reduction of the sample, we introduce the possibility for subsequent analysis of the same tissue using orthogonal approaches that are expected to yield direct complementary insight to the biological features of interest.

Real-time monitoring of laser powder bed fusion process using high-speed X-ray imaging and diffraction

We employ the high-speed synchrotron hard X-ray imaging and diffraction techniques to monitor the laser powder bed fusion (LPBF) process of Ti-6Al-4V in situ and in real time. We demonstrate that many scientifically and technologically significant phenomena in LPBF, including melt pool dynamics, powder ejection, rapid solidification, and phase transformation, can be probed with unprecedented spatial and temporal resolutions. In particular, the keyhole pore formation is experimentally revealed with high spatial and temporal resolutions. The solidification rate is quantitatively measured, and the slowly decrease in solidification rate during the relatively steady state could be a manifestation of the recalescence phenomenon. The high-speed diffraction enables a reasonable estimation of the cooling rate and phase transformation rate, and the diffusionless transformation from β to α’ phase is evident. The data present here will facilitate the understanding of dynamics and kinetics in metal LPBF process, and the experiment platform established will undoubtedly become a new paradigm for future research and development of metal additive manufacturing.

MMX-I: A data-processing software for multi-modal X-ray imaging and tomography

Scanning hard X-ray imaging allows simultaneous acquisition of multimodal information, including X-ray fluorescence, absorption, phase and dark-field contrasts, providing structural and chemical details of the samples. Combining these scanning techniques with the infrastructure developed for fast data acquisition at Synchrotron Soleil permits to perform multimodal imaging and tomography during routine user experiments at the Nanoscopium beamline. A main challenge of such imaging techniques is the online processing and analysis of the generated very large volume (several hundreds of Giga Bytes) multimodal data-sets. This is especially important for the wide user community foreseen at the user oriented Nanoscopium beamline (e.g. from the fields of Biology, Life Sciences, Geology, Geobiology), having no experience in such data-handling. MMX-I is a new multi-platform open-source freeware for the processing and reconstruction of scanning multi-technique X-ray imaging and tomographic datasets. The MMX-I project aims to offer, both expert users and beginners, the possibility of processing and analysing raw data, either on-site or off-site. Therefore we have developed a multi-platform (Mac, Windows and Linux 64bit) data processing tool, which is easy to install, comprehensive, intuitive, extendable and user-friendly. MMX-I is now routinely used by the Nanoscopium user community and has demonstrated its performance in treating big data.

CORONAS-F observation of gamma-ray emission from the solar flare on 2003 October 29

Appreciable hard X-ray (HXR) and gamma-ray emissions in the 0.04–150MeV energy range associated with the 2003 October 29 solar flare (X10/3B) were observed at 20:38–20:58 UT by the SONG instrument onboard the CORONAS-F mission. To restore flare gamma-ray spectra we fitted the SONG energy loss spectra with a three-component model of the incident spectrum: (1) a power law in energy, assumed to be due to electron bremsstrahlung; (2) a broad continuum produced by prompt nuclear de-excitation gamma-lines; and (3) a broad gamma-line generated from pion-decay. We also restored spectra from the RHESSI data, compared them with the SONG spectra and found a reasonable agreement between these spectra in the 0.1–10MeV energy range. The pion-decay emission was observed from 20:44:20 UT and had its maximum at 20:48–20:51 UT. The power-law spectral index of accelerated protons estimated from the ratio between intensities of different components of gamma rays changed with time. The hardest spectrum with a power-law index S =−3.5–3.6 was observed at 20:48–20:51 UT. Time histories of the pion-decay emission and proton spectrum were compared with changes of the locations of flare energy release as shown by RHESSI hard X-ray images and remote and remote Hα brightenings. An apparent temporal correlation between processes of particle acceleration and restructuring of flare magnetic field was found. In particular, the protons were accelerated to subrelativistic energies after radical change of the character of footpoint motion from a converging motion to a separation motion.

Imaging at an x-ray absorption edge using free electron laser pulses for interface dynamics in high energy density systems.

Tuning the energy of an x-ray probe to an absorption line or edge can provide material-specific measurements that are particularly useful for interfaces. Simulated hard x-ray images above the Fe K-edge are presented to examine ion diffusion across an interface between Fe2O3 and SiO2 aerogel foam materials. The simulations demonstrate the feasibility of such a technique for measurements of density scale lengths near the interface with submicron spatial resolution. A proof-of-principle experiment is designed and performed at the Linac coherent light source facility. Preliminary data show the change of the interface after shock compression and heating with simultaneous fluorescence spectra for temperature determination. The results provide the first demonstration of using x-ray imaging at an absorption edge as a diagnostic to detect ultrafast phenomena for interface physics in high-energy-density systems.

Hard x-ray scanning imaging achieved with bonded multilayer Laue lenses.

We report scanning hard x-ray imaging with a monolithic focusing optic consisting of two multilayer Laue lenses (MLLs) bonded together. With optics pre-characterization and accurate control of the bonding process, we show that a common focal plane for both MLLs can be realized at 9.317 keV. Using bonded MLLs, we obtained a scanning transmission image of a star test pattern with a resolution of 50 × 50 nm2. By applying a ptychography algorithm, we obtained a probe size of 17 × 38 nm2 and an object image with a resolution of 13 × 13 nm2. The significant reduction in alignment complexity for bonded MLLs will greatly extend the application range in both scanning and full-field x-ray microscopies.

Interlaced zone plate optics for hard X-ray imaging in the 10\u2009nm range

Multi-keV X-ray microscopy has been particularly successful in bridging the resolution gap between optical and electron microscopy. However, resolutions below 20 nm are still considered challenging, as high throughput direct imaging methods are limited by the availability of suitable optical elements. In order to bridge this gap, we present a new type of Fresnel zone plate lenses aimed at the sub-20 and the sub-10 nm resolution range. By extending the concept of double-sided zone plate stacking, we demonstrate the doubling of the effective line density and thus the resolution and provide large aperture, singlechip optical devices with 15 and 7 nm smallest zone widths. The detailed characterization of these lenses shows excellent optical properties with focal spots down to 7.8 nm. Beyond wave front characterization, the zone plates also excel in typical imaging scenarios, verifying their resolution close to their diffraction limited optical performance.