Natural fiber-reinforced hybrids are a new topic of study in supramolecular chemistry. Such natural fabrics are low-cost fibers exhibiting good specific characteristics and low density. The tribological and mechanical properties of handwoven sisal/twill glass fabric reinforced polymer blends were scientifically investigated. Hand lay-up lamination specimens were created in a mould and dried under mild pressure at atmospheric conditions for 24 h. Each of the hybrid composites had four layers, with the quantity and location of glass layers varying to provide five distinct layering patterns. A group of any and all sisal lamination, on the other hand, had been created. ASTM standards were followed for sample preparation and evaluation. The results revealed that incorporating twill E-glass fiber with polymer composites may considerably improve the characteristics of the sisal combination. S5 hybrid composites reached maximum tensile and bending strengths of 74.26 MPa and 161.25 MPa, respectively. The wear of the S3 series laminated hybrid is lower (0.84 × 10–4) than that of the other hybrid compound and plain polymer material. The layering arrangement has a stronger impact on hybrid composites in terms of both mechanical and tribological characteristics. The results show how layering affects the mechanical and tribological properties of these new natural fiber-reinforced combinations. This presents exciting new opportunities for many material research and engineering applications, such as making strong, portable car parts.
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