In this article, the synchronization of multiple fractional-order neural networks with unbounded time-varying delays (FNNUDs) is investigated. By introducing a pinning linear control, sufficient conditions are provided for achieving the synchronization of multiple FNNUDs via an extended Halanay inequality. Moreover, a new effective adaptive control which applies to the fractional differential equations with unbounded time-varying delays is designed, under which sufficient criteria are presented to ensure the synchronization of multiple FNNUDs. The introduced control in this article is also workable in traditional integer-order neural networks. Finally, the validity of obtained results is demonstrated by a numerical example.