Uranium In Groundwater Research Articles

Assessment of chemical risk associated with naturally occurring uranium in groundwater from East Khandesh, India

Assessment of chemical risk associated with naturally occurring uranium in groundwater from East Khandesh, India

Uranium in groundwaters of North Kazakhstan

Relevance. The need to dentify the characteristics of the distribution of radioactive elements in the groundwater of Northern Kazakhstan. Aim. Generalization of available data on the geochemistry of groundwater and uranium and radon distribution in them using the example of the northern regions of the Republic of Kazakhstan. Methods. Generalization of long-term hydrogeochemical research and compilation of an electronic data bank on the territory of Northern Kazakhstan. A laboratory study of the chemical composition of groundwater was carried out at the Research Laboratory of Hydrogeochemistry of the School of Natural Resources Engineering of Tomsk Polytechnic University. Measurements of 222Rn contents in waters were carried out using the Alfarad Plus complex in the Laboratory of Hydrogeology of Sedimentary Basins of Siberia, Institute of Geology and Geography, Siberian Branch, Russian Academy of Sciences. Results. The groundwater of aquifers of different ages, distributed in the territory of Northern Kazakhstan (North Kazakhstan uranium province), was studied. Two geochemical sets of groundwater were identified. The first is characterized by the dominance of HCO3– and Mg2+ in the water composition, and the second by Cl– and Na+. A change in composition and an increase in the value of total mineralization from 0,1 to 49 g/dm3, in the direction from north to south, indicate the development of continental salinization. In natural waters of the first group, uranium content varies from 0.065 to 16000 μg/dm3 and radon activity from 4 to 3885 Bq/dm3. For sodium chloride waters of the second set, concentrations can reach 32500 μg/dm3, and radon activity is 6–59 Bq/dm3, since the emanating reservoir (granitoids) is located to the north – at a distance of 80–100 km. Naturally, granitoid massifs of the studied region are sources of uranium. Their drainage by the river network leads to its removal and concentration on geochemical barriers in the groundwater of the Neogene-Quaternary aquifer. This distribution of radioactive elements is associated with the high migration ability of uranium in solution in the form of uranyl ion in oxidizing geochemical conditions.

Uranium and Radium in Groundwater and Incidence of Colorectal Cancer in Georgia Counties, USA: An Ecologic Study.

Colorectal cancer (CRC) is the third most commonly occurring cancer in the United States, with higher incidence rates among Black populations. Groundwater concentrations of natural radionuclides uranium and radium have seldom been investigated in relation to CRC despite their known carcinogenicity. We investigate spatial patterns of CRC by race, and in relation to groundwater concentrations of uranium and radium, testing the hypothesis that uranium and radium in groundwater might differentially contribute to incident CRC in Black and White populations in counties of Georgia, USA. Black populations showed a higher incidence of CRC than White populations; the median incident rate difference was 9.23 cases per 100,000 (95% CI: 2.14, 19.40). Spatial cluster analysis showed high incidence clusters of CRC in similar regions for Black and White populations. Linear regression indicated there are, on average, 1-2 additional cases of colorectal cancer in counties with higher levels of radium in their groundwater, irrespective of race. Uranium was not associated with CRC. This ecologic study suggests that radium in groundwater may be linked with increased incidence of CRC, although it did not explain higher CRC incidence rates in Black populations. Further studies are needed to verify this association given the inherent limitations in the ecologic study design and the crude exposure assessment.

Isotope characterisation of groundwater resources in uranium impacted Fazilka, Punjab

AbstractGroundwater is the most reliable source for freshwater supplies in India and abroad. Population rise has affected the groundwater resources both in terms of quality and quantity. Punjab, being an agrarian state, is highly dependent on groundwater resources for both irrigation and drinking purposes. Recent studies have indicated presence of uranium in groundwater especially in southwestern parts of Punjab. In this research, water samples were collected from Fazilka district of Punjab for evaluating the water quality focussing uranium and identifying source and recharge processes of groundwater. Uranium concentration was found in both shallow and deep groundwater samples. Inter-ionic correlations signify that alkalinity and electrical conductivity of the water samples control the uranium mobilization from the aquifer matrix. Isotopic systematics demonstrate that groundwater recharge is mainly through rainwater infiltration.

LED fluorimetric analysis of uranium in potable groundwater and associated health concerns

LED fluorimetric analysis of uranium in potable groundwater and associated health concerns

Dose assessment from exposure to uranium and radon in groundwater in Safi province, Morocco

ABSTRACT In this study we evaluate the uranium and radon concentrations in groundwater from the Province of Safi. The samples were collected from 58 wells across five communes and analyzed using the LR-115 type II detector. Results indicate that uranium concentrations ranged from the Limit of Detection (LLD) to 3.73 µg/l, with a mean of 0.72 µg/l, well below the World Health Organization’s safe limit of 30 µg/l. Radon levels varied from LLD to 2.39 Bq/l, with an average of 0.60 Bq/l, also below the United States Environmental Protection Agency’s limit of 11 Bq/l. The estimated total annual effective dose due to uranium and radon ranged from 3.47 to 18.84 µSv/y, with an average of 7.54 µSv/y, which is significantly lower than the European Commission’s recommended limit of 100 µSv/y. This investigation represents the first study of uranium and radon levels in groundwater in the Province of Safi, providing valuable data for future research and public health.

A coupling numerical model for simulating groundwater uranium removal in coupling device of electric field and PRB

The remediation of groundwater uranium pollution has been successfully researched and implemented. However, the cost-effectiveness remains challenging to evaluate. Numerical modeling presents a potential solution, while the coupling of multi-physics in uranium pollution remediation has been a global challenge. This study developed a multi-physics coupled model to simulate the evolution of groundwater uranium plumes in composite remediation system, which was composed of permeable reactive barrier (PRB) and electrokinetic remediation (EKR). Meanwhile, pH changes are also taken into account. The research revolved around sandbox dynamic migration experiments, where key parameters were measured for model building. Based on this, a mathematical model for achieving multi field coupling has been proposed. Substitute equations were used to unify the calculation of flow field and electric field into the same dimension. The results showed that the pH variations induced by electrolysis propagate towards the center of the electric field. Medium adsorption of uranium reached its peak when the pH was between 4 and 5. The driving force of groundwater flow in the coupled field was about 3.5 times that of electroosmosis, occupying a dominant position. Electric fields can serve as auxiliary means to delay the migration of uranium. Under ensuring the effective operation of the system for 360 days, the system can save 25 % of PRB thickness with the EKR assistance. The model can not only predict evolution of uranium plume in groundwater, but also calculate the performance and lifespan of composite remediation systems, providing guidance and recommendations for the design of real-site remediation systems.

Radiation dose due to uranium in groundwater to the population of Chamarajanagar district, Karnataka, India.

This paper presents the concentration of uranium in 67 groundwater samples of Chamarajanagar district, Karnataka, India, estimated using an LED fluorimeter. The age-dependent ingestion dose to the population of the district is also studied. The concentration of uranium in groundwater varied from 0.20 to 57.50μgL-1 with an average of 4.40μgL-1. The annual ingestion dose due to uranium varies from 0.18 to 142.68μSvy-1, with an average of 7.11μSvy-1. The ingestion dose received by the population in the study area is less than the recommended level of 100μSvy-1 by the World Health Organization (2011).

Natural Attenuation of Groundwater Uranium in Post-Neutral-Mining Sites Evidenced from Multiple Isotopes and Dissolved Organic Matter.

Although natural attenuation is an economic remediation strategy for uranium (U) contamination, the role of organic molecules in driving U natural attenuation in postmining aquifers is not well-understood. Groundwaters were sampled to investigate the chemical, isotopic, and dissolved organic matter (DOM) compositions and their relationships to U natural attenuation from production wells and postmining wells in a typical U deposit (the Qianjiadian U deposit) mined by neutral in situ leaching. Results showed that Fe(II) concentrations and δ34SSO4 and δ18OSO4 values increased, but U concentrations decreased significantly from production wells to postmining wells, indicating that Fe(III) reduction and sulfate reduction were the predominant processes contributing to U natural attenuation. Microbial humic-like and protein-like components mediated the reduction of Fe(III) and sulfate, respectively. Organic molecules with H/C > 1.5 were conducive to microbe-mediated reduction of Fe(III) and sulfate and facilitated the natural attenuation of dissolved U. The average U attenuation rate was -1.07 mg/L/yr, with which the U-contaminated groundwater would be naturally attenuated in approximately 11.2 years. The study highlights the specific organic molecules regulating the natural attenuation of groundwater U via the reduction of Fe(III) and sulfate.

Hydrogeochemical characteristics and enrichment regularities of groundwater uranium in the Erlian basin, China

Groundwater is a key medium for the migration and enrichment of elements into ore bodies in sandstone-type uranium deposits, with anomalies of uranium elements and their associated components in water serving as indicators for exploring such deposits. The Erlian Basin, located in central-northern Inner Mongolia, is a crucial production area for sandstone-type uranium deposits in China. The groundwater flow system in the basin plays a significant role in the formation of uranium deposits. To study the hydrogeochemical characteristics and enrichment regularities of groundwater uranium in the Erlian Basin, 269 groundwater samples were collected. Hydrogeochemical analysis methods, such as Piper diagrams, Gibbs diagrams, and contour maps, were employed to determine the distribution characteristics and occurrence forms of groundwater uranium in the study area. The primary water chemistry types in the study area were HCO3–Ca•Na, HCO3–Na, HCO3•SO4–Na, and SO4•HCO3–Na•Ca. The distribution range of uranium content in groundwater in the study area was 0.1–453 μg/L (average of 53.08 μg/L). A comprehensive analysis, based on the direction of groundwater flow and changes in the redox environment, suggested that the higher uranium values in groundwater were distributed in the runoff and discharge areas, with uranium anomaly points existing in areas with alternating oxidation and reduction zones. These uranium anomaly points were in good agreement with the known large uranium deposits of Nuheting, Qiharigetu, Daoersu, and others, thereby predicting six other uranium hydrochemical anomaly points as prospective areas for uranium mineralization. The pH value distribution range in the study area's groundwater was 6.8–9.1, and the redox potential (Eh) value range was -126–52 mV, indicating that uranium exists in groundwater in the form of UO2(CO3)34− and UO2(CO3)22−. An increase in bicarbonate (HCO3−) is conducive to uranium dissolution. The enrichment and occurrence forms of uranium in groundwater are influenced by the concentrations of Fe and (Ca2++Mg2+), with uranium precipitation and enrichment occurring as the groundwater evolves and changes in the redox environment. The uranium content in deep wells is higher than in nearby shallow wells, indicating that deep water circulation is beneficial for mineralization. The pH, Eh, HCO3−, Fe, and other hydrogeochemical indicators are indicative of uranium enrichment; thus, they can be considered as reference bases when exploring for potential uranium resources.

Decoding uranium variation over the Indian peninsula through leveraging standardized precipitation evapotranspiration indices and groundwater level fluctuations

The present study aims to predict the concentration of uranium (U) in groundwater in India by utilizing water quantity indicators, such as Standardised Precipitation Index (SPI), Standardised Precipitation Evapotranspiration Index (SPEI), and Gravity Recovery and Climate Experiment (GRACE) based groundwater levels. The study adopts a multi-scale approach, ranging from state-level to agroclimatic zones. The findings indicate that the highest levels of U (101–500 μg.L−1), which surpass the World Health Organization (WHO) prescribed limit of 30 μg.L−1 for drinking water, are primarily concentrated in India's plateau and hills regions. The GRACE data map portrays a downward trend in groundwater levels throughout India, with the mid-Gangetic plains experiencing the most significant decline. The meteorological aspect of the study, as indicated by SPI and SPEI, reveals that the plateau and hills region is experiencing a decline in rainfall. The SPEI further underscores the grim picture of decreasing precipitation in northern India. Additionally, the study employs cluster analysis to cluster states according to the division of agro-climatic zones. Lastly, the study employs a random forest algorithm to assess the relative importance of each predictor and predict U concentration under the trinity of precipitation, extraction, and evaporation. The most significant contribution of this work is to identify the hotspots in India that require the most attention in terms of U toxicity owing to groundwater decline. Overall, this study highlights the need for immediate attention to mitigate the adverse impacts of U contamination and aims at sensitizing the stakeholders towards the compelling need to fulfil SDG-3 (health aspects due to U hazard) and SDG-6 (groundwater over-exploitation and deteriorating water quality).

Health risk assessment due to uranium contamination in groundwater: MATLAB based Monte-Carlo simulations

ABSTRACT Uranium contamination is a growing concern due to its inherent toxicity, which poses a significant threat to human health. The health risk assessment due to uranium contamination in groundwater of Mansa district, Punjab (India) is investigated. The LED LF-2a Fluorimeter model by Quantalase (Indore) was used for measurement of uranium concentration in groundwater collected in October 2021 from twenty-six locations. A comparison is conducted between the deterministic and probabilistic approaches since the deterministic approach might either underestimate or exaggerate the risk estimation. Monte-Carlo simulations are used to curtail the associated uncertainties in the data. The simulations are carried out in MATLAB for risk assessment and sensitivity analysis. The deterministic and probabilistic approaches are used to calculate hazard quotient, excess cancer risk and annual effective dose. Using probabilistic approach, the hazard quotient for male and female at 5th percentile is 4.36 and 3.81, respectively. Similarly, the hazard quotient for male and female at 95th percentile is 38.95 and 34.26, respectively. The mean hazard quotient is 18.45 and 15.68 for male and female, respectively, using deterministic approach. The hazard quotient is greater than 1 for both genders (male and female) and excess cancer risk is also higher than 10−4 using both deterministic and probabilistic approaches. The annual effective dose using deterministic approach is 0.23 mSv year−1 whereas using probabilistic approach, the 5th and 95th percentile is 0.56 mSv year−1 and 4.33 mSv year−1, respectively. The sensitivity analysis indicated that the overall risk is more sensitive to concentration of uranium in groundwater and the exposure frequency. This study emphasises on the hazards posed to humans by the ingestion of uranium contaminated groundwater, hence stressing the urgency for taking actions to protect the population of the study area.

Geo-spatial epidemiology of gallbladder cancer in Bihar, India

Recently, a substantial increase in gallbladder cancer (GBC) cases has been reported in Bihar, India. The region's groundwater can naturally contain harmful concentrations of arsenic, which appears to be epidemiologically linked to the unusually high incidence. However, the root causes remain largely unexplored. Recent findings of uranium in the state's groundwater may also have associations. This study investigates the geo-spatial epidemiology of GBC in Bihar, India—with a focus on the correlation between environmental carcinogens, particularly arsenic and uranium in groundwater, and the incidence of GBC. Utilizing data from 8460 GBC patients' registration records over an 11-year period at a single health center, the research employs Semi-parametric Geographically Weighted Poisson Regression (S-GWPR) to account for non-stationarity associations and explores significant factors contributing to GBC prevalence at a subdistrict level. The S-GWPR model outperformed the standard Poisson regression model. The estimates suggest that arsenic and uranium concentrations in groundwater did not present significant associations; however, this could be due to the lower resolution of this data at the district level, necessitating higher resolution data for accurate estimates. Other socio-environmental factors included demonstrated significant regional heterogeneity in their association with GBC prevalence. Notably, each 1 % increase in the coverage of well- and canal-irrigated areas is associated with a maximum of 3.0 % and 5.2 % rise in the GBC incidence rate, respectively, likely attributable to carcinogen exposure from irrigation water. Moreover, distance to the health center and domestic electricity connections appear to influence the number of reported GBC cases. The latter suggests that access to electricity might have facilitated the use of groundwater pumps—increasing exposure to carcinogens. The results underscore the necessity for targeted health policies and interventions based on fine-resolution spatial analysis, as well as ongoing environmental monitoring and research to better understand the multifaceted risk factors contributing to GBC.

Evaluation of the toxicological effects of uranium on human health in Chandrapur, Maharashtra, with reference to the water quality index

Groundwater is an important resource and approximate 80% of the world’s population depends solely on it to satisfy their needs. In the present investigation groundwater quality was assessed using WQI. For the same parameters viz, temperature, pH, conductivity, DO, alkalinity, TDS, sulphate, fluoride, bicarbonate, chloride, uranium, total hardness, calcium and magnesium hardness were assessed during post monsoon period in November 2021 in the Chandrapur region. For conducting this research total 116 groundwater samples were collected from different hydrological stations for the assessment of WQI. WQI is an important tool to assess quality of water for drinking and is classified as excellent to unsafe, i.e., 0-100 score. In this investigation WQI was found to be in the range between 27.63-674.56 exceeding both minimum and maximum score. The results of the present investigation showed that only 5.17% of water is safe for drinking,18% of water indicated poor water quality, 15% of water has very poor water quality and 77% of water is unsuitable for drinking purpose and proper treatment is required before use. During this investigation uranium in groundwater was also assessed considering its chemotoxical and radiological effects on human health. The chemotoxical and radiological effects were analyzed adopting standard equations given by USEPA. The radiological risk of mortality and morbidity was found to be 1.37E-05-1.47E-05, respectively. Thus, presence of uranium was noted and radiological risk was found to be below the permissible limit of AERB standard. The chemical toxicity of average value of Lifetime Average Daily Dose (LADD) and Hazard Quotient (HQ) was observed 0.315 and 0.00571, respectively and chemical toxicity of LADD was found to be in 8.62% sample population and above the permissible limits which can affect human health and can have kidney toxicity, bone and lung toxicity.

Microbial removal of uranyl from aqueous solution by Leifsonia sp. in the presence of different forms of iron oxides

Immobilization of uranyl by indigenous microorganisms has been proposed as an economic and clean in-situ approach for removal of uranium, but the potential mechanisms of the process and the stability of precipitated uranium in the presence of widespread Fe(III) (hydr)oxides remain elusive. The potential of iron to serve as a reductant and/or an oxidant of uranium indicates that bioemediation strategies which mainly rely on the reduction of highly soluble U(VI) to poorly soluble U(IV) minerals to retard uranium transport in groundwater may be enhanced or hindered under different environmental conditions. This study purposes to determine the effect of ubiquitous Fe(III) (hydr)oxides (two-line ferrihydrite, hematite and goethite) on the removal of U(VI) by Leifsonia sp. isolated from an acidic tailings pond in China. The removal mechanism was elucidated via SEM-EDS, XPS and Mössbauer. The results show that the removal of U(VI) was retarded by Fe(III) (hydr)oxides when the initial concentration of U(VI) was 10 mg/L, pH was 6, temperature was 25 °C. Particularly, the retardatory effect of hematite on U(VI) removal was blindingly obvious. Also, it is worth noting that the U(VI) in the precipitate slow-released in the Fe(III) (hydrodr) oxide treatment groups, accompanied by an increase in Fe(II) concentration. SEM-EDS results demonstrated that the ferrihydrite converted to goethite may be the reason for U(VI) release in the process of 15 days culture. Mössbauer spectra fitting results further imply that the metastable iron oxides were transformed into stable Fe3O4 state. XPS measurements results showed that uranium product is most likely a mixture of Iron-U(IV) and Iron-U(VI), which indicated that the hexavalent uranium was converted into tetravalent uranium. These observations imply that the stability of the uranium in groundwater may be impacted on the prevailing environmental conditions, especially the solid-phase Fe(III) (hydr)oxide in groundwater or sediment.

Water-rock interactions of uranium deposits: A field investigation and laboratory batch experiment

Interactions between bedrock and groundwater in the far-field of a deep geological repository (DGR) for high-level radioactive waste significantly affect the transport of uranium, which is the major radionuclide in a DGR. Therefore, the present study evaluated the geochemical behavior of uranium by assessing the hydrogeochemical characteristics of groundwater, surface water, mine water, and quarry runoff water in the Okcheon metamorphic belt, which represents a natural analogue study site in Korea. A batch experiment was also conducted to further elucidate the interactions between the uranium-containing rock and groundwater in the study area. The results of the field investigation indicated that uranium in groundwater formed aqueous complexes in the form of calcium uranyl tricarbonate. The concentrations of uranium in groundwater were low, at less than 1 μg L−1, which seems to be attributable to the dissolutions of uraninite, coffinite, UO2(am), and U4O9(c) under the moderately reduced condition and subsequent control by co-precipitation with iron (hydr)oxides. The results of the batch experiment showed that uranium concentrations may be controlled by adsorption or surface complexation with iron oxides. The field study demonstrates the equilibrium state maintained in the current geochemical conditions at the study site, while the batch experiment provides implications regarding the reaction processes over time. Overall, this study showed that uranium forms complexes with carbonate and sulfate under the geochemical conditions of the study site, and that its mobility could be restricted through co-precipitation or adsorption/surface complexation. This study is expected to contribute to a comprehensive understanding of how the behavior of uranium is affected by the evolution of geochemical conditions around the DGR.

A bidirectional kinetic reaction model to predict uranium distribution in permeable reactive bio-barrier with high-sulfate environment

The use of permeable reactive bio-barriers (Bio-PRBs) is a developing method for remediation of uranium groundwater pollution. However, some remediation effects are difficult to estimate when because of the subsurface environment. Advanced knowledge of uranium migration and reactions in Bio-PRBs is crucial for successful practical application. In this study, a bidirectional kinetic reaction model was developed for predicting uranium reduction in a Bio-PRB system. The research demonstrates that the model is able to predict the uranium migration and rapidly evaluate the Bio-PRBs performance. The results show that contact period and microbial growth are the key factors that affect the remediation performance of Bio-PRBs. Microbial growth could lead to a decrease in hydraulic conductivity (K). The hydraulic conductivity loss in the free microorganisms (FM) group was 0.8–2.3 m/d, which was significantly smaller than the immobilized microorganism (IM) group (0.8–5.2 m/d). Compared to the IM group, the simulation results reveal that longer contact reaction period improves the remediation performance of SO42− and uranium by 32.6% and 21.7%, respectively. The bidirectional reaction between microorganisms and pollutants leads to a decrease in the remediation efficiency. In addition, the model can be used to design standard Bio-PRBs for real field of uranium contanminated groundwater. To meet the remediation goal of groundwater, the width of IM group needs to be increased to 250 cm while 500 cm for FM group. Therefore, IM-PRBs save costs significantly. The model has successfully optimized Bio-PRBs and predicted uranium contaminant-plume evolution and microbial growth inhibition in different Bio-PRBs.

A correlational study of uranium in groundwater with other physicochemical parameters using GIS mapping in Godda district of Jharkhand, India.

The present research concentrates on the cumulative use of GPS and GIS technologies, which are excellent resources for analyzing and monitoring divergent physicochemical parameters in groundwater, including pH, TDS, EC, ORP, Ca+2, Mg+2, NO3-, F-, SO4-2, Cl- and PO4-3 with explicit regard to uranium. Garmin GPS is used to record the locations of the sampling points in the Godda study area. The research aims to offer a thorough understanding of the relationship between soil and water, its impact on public health and the extent to which water can be used in various ways based on its quality. Utilizing the inverse distance weighted (IDW) technique, it is examined how these groundwater parameters and the Water Quality Index(WQI) can be estimated spatially. Additionally, a correlation analysis of the water quality parameters is computed to estimate the local population's cancer risk living in the study area. Except for calcium and magnesium, which are present in excess concentrations throughout the study area with the highest values of 325 and 406mg/l, respectively at Amedihaand Meherma, the results showed that the maximum concentration parameters are within limits with the standard. The main reason might be the area's predominance of Alfisol soil type. The radioactive element uranium is found to be in a limited range. Chemo-toxicity and radiological risk assessment of the whole area lie far below the restricted cancer risk limit i.e., 30ppb with the highest concentration of 14ppb in the 'Sunderpahari' region, following the results obtained. The WQIfor the area ranges from 'good' to 'very poor.' The results were favorable but a few sites such as 'Boarijor' and its surroundings, require additional attention to enhance groundwater quality. Given uranium's low availability in groundwater the region's cancer risk assessment is below average.

Mapping of uranium in groundwater of Mysuru district, Karnataka, India and radiation dose to the population

Uranium in ground and surface water may pose significant health hazards, if they are ingested via drinking pathway because of its radiological and chemical toxicities. Higher uranium concentration in drinking water can lead to serious diseases like leukemia, kidney cancer, stomach cancer and renal damages etc. In the present investigation, uranium concentration in groundwater samples of Mysuru district has been studied using an LED fluorimeter. About 350 water samples have been collected covering all the areas of Mysuru district and the uranium concentration varied from 0.34 to 242.93 µg l−1. The age depended dose due to uranium in drinking water has been estimated to evaluate the health hazards. The annual ingestion dose varied from 0.51 to 95.76 µSv y−1. The radiological and chemical toxicity risk to the population due to uranium in water was estimated. The Excess Cancer Risk varied from 1.22 × 10−6 to 102.63 × 10−6. The mean value of Hazard Quotient 0.07 indicates that the populations are less prone to adverse health effects of uranium contamination in water.

Estimation of radiation dose due to U and 222Rn in groundwater to the population of Kodagu district, Karnataka, India

Abstract Systematic studies on natural radioactivity in the groundwater of Kodagu district, India were carried out. LED fluorimetric technique to measure uranium activity and emanometric technique to measure 222Rn activity in groundwater samples were used. The concentration of U and 222Rn in the water samples was observed to vary from 0.44 to 8.81 μg L−l with a geometric mean of 2.04 μg L−l and 1.54 to 9.61 Bq L−1 with a geometric mean of 3.59 Bq L−1, respectively. The estimated concentrations of uranium and radon in groundwater were within the recommended standard limits. The radiation dose due to U and 222Rn in groundwater was estimated and the total dose due to these radionuclides was found to vary from 4.51 to 30.28 μSv y−1 which was below the prescribed safe limit of 0.1 mSv y−1 by the WHO.