Fermi Liquid Research Articles

Correlation of preparation conditions of SrRuO<sub>3</sub> ultrathin films with topological Hall effect

As one of the magnetic transition metal oxides, SrRuO<sub>3</sub> (SRO) has received much attention in recent years, which is mainly due to its unique itinerate ferromagnetism and the unusual electrical transport properties–behaving as Fermi liquid at low temperature and bad metal at high temperature. In the growth of SRO thin films, there are many factors that can affect the quality of thin films. In this work, we study various factors affecting the growth and quality of SRO thin films by using laser molecular beam epitaxy (laser MBE), including laser energy density, substrate temperature and target surface conditions, and explore their influences on the topological Hall effect (THE) in SRO. For thin films grown at high laser energy density and high temperature, we found that there are large trenches at the edge of steps, which deteriorate the transport properties of the thin films. When using low laser energy density, extra SrO may exist in the films, which also suppresses the conductivity. Films grown at low temperature tend to have poor crystallinity while films grown at high temperature exhibit island structures. The ablation degree of the target surface increases the decomposition of SRO to SrO, Ru and volatile RuO<sub>4</sub>, resulting in Ru defects in the grown thin film. The SRO thin film grown under the optimal conditions (1.75 J·cm<sup>–2</sup>, 670 ℃, fresh target surface) exhibits the optimal conductivity and the strongest THE. For non-optimal growth conditions that favors thickness inhomogeneity or Ru defects in the film, THE becomes weaker or even disappears. Therefore, we believe that the THE is due to the Dzyaloshinskii-Moriya interaction (DMI) resulting from the interfacial inversion asymmetry and the associated chiral spin structures.

Unconventional exciton evolution from the pseudogap to superconducting phases in cuprates

Electron quasiparticles play a crucial role in simplifying the description of many-body physics in solids with surprising success. Conventional Landau’s Fermi-liquid and quasiparticle theories for high-temperature superconducting cuprates have, however, received skepticism from various angles. A path-breaking framework of electron fractionalization has been established to replace the Fermi-liquid theory for systems that show the fractional quantum Hall effect and the Mott insulating phenomena; whether it captures the essential physics of the pseudogap and superconducting phases of cuprates is still an open issue. Here, we show that excitonic excitation of optimally doped Bi2Sr2CaCu2O8+δ with energy far above the superconducting-gap energy scale, about 1 eV or even higher, is unusually enhanced by the onset of superconductivity. Our finding proves the involvement of such high-energy excitons in superconductivity. Therefore, the observed enhancement in the spectral weight of excitons imposes a crucial constraint on theories for the pseudogap and superconducting mechanisms. A simple two-component fermion model which embodies electron fractionalization in the pseudogap state provides a possible mechanism of this enhancement, pointing toward a novel route for understanding the electronic structure of superconducting cuprates.

Thermal conductivity and heat diffusion in the two-dimensional Hubbard model

We study the electronic thermal conductivity $\kappa_\textrm{el}$ and the thermal diffusion constant $D_\textrm{Q,el}$ in the square lattice Hubbard model using the finite-temperature Lanczos method. We exploit the Nernst-Einstein relation for thermal transport and interpret the strong non-monotonous temperature dependence of $\kappa_\textrm{el}$ in terms of that of $D_\textrm{Q,el}$ and the electronic specific heat $c_\textrm{el}$. We present also the results for the Heisenberg model on a square lattice and ladder geometries. We study the effects of doping and consider the doped case also with the dynamical mean-field theory. We show that $\kappa_\textrm{el}$ is below the corresponding Mott-Ioffe-Regel value in almost all calculated regimes, while the mean free path is typically above or close to lattice spacing. We discuss the opposite effect of quasi-particle renormalization on charge and heat diffusion constants. We calculate the Lorenz ratio and show that it differs from the Sommerfeld value. We discuss our results in relation to experiments on cuprates. Additionally, we calculate the thermal conductivity of overdoped cuprates within the anisotropic marginal Fermi liquid phenomenological approach.

Multicomponent odd-parity superconductivity in UAu2 at high pressure

We report that high-quality single crystals of the hexagonal heavy fermion material uranium diauride (UAu2) become superconducting at pressures above 3.2 GPa, the pressure at which an unusual antiferromagnetic state is suppressed. The antiferromagnetic state hosts a marginal fermi liquid and the pressure evolution of the resistivity within this state is found to be very different from that approaching a standard quantum phase transition. The superconductivity that appears above this transition survives in high magnetic fields with a large critical field for all field directions. The critical field also has an unusual angle dependence suggesting that the superconductivity may have an order parameter with multiple components. An order parameter consistent with these observations is predicted to host half-quantum vortices (HQVs). Such vortices can be topologically entangled and have potential applications in quantum computing.

Kondo breakdown transitions and phase-separation tendencies in valence-fluctuating heavy-fermion metals

The breakdown of the lattice Kondo effect in local-moment metals can lead to nontrivial forms of quantum criticality and a variety of non-Fermi-liquid phases. Given indications that Kondo breakdown transitions involve criticality not only in the spin but also in the charge sector, we investigate the interplay of Kondo breakdown and strong valence fluctuations in generalized Anderson lattice models. We employ a parton mean-field theory to describe the transitions between deconfined fractionalized Fermi liquids and various confined phases. We find that rapid valence changes near Kondo breakdown can render the quantum transition first order. This leads to phase-separation tendencies which, upon inclusion of longer-range Coulomb interactions, will produce intrinsically inhomogeneous states near Kondo breakdown transitions. We connect our findings to unsolved aspects of experimental data.

Tuning the Fermi liquid crossover in Sr2RuO4 with uniaxial stress

We perform nuclear magnetic resonance (NMR) measurements of the oxygen-17 Knight shifts for Sr2RuO4, while subjected to uniaxial stress applied along [100] direction. The resulting strain is associated with a strong variation of the temperature and magnetic field dependence of the inferred magnetic response. A quasiparticle description based on density-functional theory calculations, supplemented by many-body renormalizations, is found to reproduce our experimental results, and highlights the key role of a van-Hove singularity. The Fermi-liquid coherence scale is shown to be tunable by strain, and driven to low values as the associated Lifshitz transition is approached.

Bonding and Electronic Nature of the Anionic Framework in LaPd3S4

Double Dirac materials are a topological phase of matter in which a non-symmorphic symmetry enforces greater electronic degeneracy than normally expected – up to eightfold. The cubic palladium bronzes NaPd3O4 and LaPd3S4 are built of Pd3X4 (X = O, S) anionic frameworks that are ionically bonded to A cations (A = Na, La). These materials were recently identified computationally as harboring eightfold fermions. Here we report the preparation of single crystals and electronic properties of LaPd3S4. Measurements down to T = 0.45 K and in magnetic fields up to μ0H = 65 T are consistent with normal Fermi liquid physics of a Dirac metal in the presence of dilute magnetic impurities. This interpretation is further confirmed by analysis of specific heat, magnetization measurements and comparison to density functional theory (DFT) calculations. Through a bonding analysis of the DFT electronic structure of NaPd3O4 and LaPd3S4, we identify the origin of the stability of the anionic Pd3X4 framework at higher electron counts for X = S than X = O, and propose chemical tuning strategies to enable shifting the 8-fold fermion points to the Fermi level.

Superconductivity in TlBi2 with a large Kadowaki-Woods ratio

In this article, the superconducting and normal state properties of TlBi$_2$ with the AlB$_2$-type structure were studied by the resistivity, magnetization and specific heat measurements. It was found that bulk superconductivity with $T_{C}$ = 6.2 K emerges in TlBi$_2$, which is a phonon-mediated $s$-wave superconductor with a strong electron-phonon coupling ($\lambda$$_{ep}$ = 1.38) and a large superconducting gap ($\Delta_{0}$/$k_{B}T_{C}$ = 2.25). We found that the $\rho$($T$) exhibits an unusual $T$-linear dependence above 50 K, and can be well described by the Fermi-liquid theory below 20 K. Interestingly, its Kadowaki-Woods ratio $A/\gamma^{2}$ [9.2$\times$10$^{-5}$ $\mu\Omega$ cm(mol K$^{2}$/mJ)$^{2}$] is unexpectedly one order of magnitude larger than that obtained in many heavy Fermi compounds, although the electron correlation is not so strong.

Colloquium : Planckian dissipation in metals

Relaxational processes for conduction electrons in metals come with characteristic temperature dependences; classic examples at low temperatures are the $1/{T}^{2}$ law for the relaxation time in a Fermi liquid, and the Bloch $1/{T}^{5}$ law for electron-phonon scattering. The strange metal phase of cuprate superconductors is governed instead by the Planckian time, which is given in terms of fundamental constants only. This Colloquium discusses the concept of such a fundamental timescale and the degree to which it provides a lower bound for relaxation times, and illustrates these ideas with examples from conventional and unconventional metals.

Quantum fidelity of the Aubry-André model and the exponential orthogonality catastrophe

Advances in experimental tools allow to study quantum fidelity in unprecedented controlled settings. While the fidelity in metals, when adding a local impurity, is well known to show the Anderson orthogonality catastrophe (AOC), there remain outstanding questions in other quantum phases and settings. Here, we aim to tackle these by exploring systematically the ground-state fidelity of the Fermi liquid in the (extended) Aubry-Andr\'e (AA) model, which allows to explore the AOC in both localized extended and critical phases. We discover that the AOC is typically exponential in the critical regime of the AA model and at the mobility edge of the extended AA model for an extended impurity, while it decays in the AA model with a power law for a weak single-site impurity. We explain this in terms of critical correlations and multipoint correlations. The OC is found to be exponential in the insulating regime, due to a fundamentally different, statistical mechanism, which is explained in detail. Furthermore, we consider a parametric perturbation to the AA model, and find an exponential OC numerically, in agreement with an analytical derivation which we provide here.

Ultracold spin-balanced fermionic quantum liquids with renormalized P -wave interactions

We consider a spin-balanced degenerate gas of spin-1/2 fermions whose dynamics is governed by low-energy $P$-wave interactions, characterized by the scattering volume $a_1$ and effective momentum $r_1$. The energy per particle $\bar{\cal{E}}$ in the many-body system is calculated by resumming the ladder diagrams comprising both particle-particle and hole-hole intermediate states, following the novel advances recently developed by us in Ann.Phys. 437,168741(2022). This allows to obtain a renormalized result for $\bar{\cal{E}}$ within generic cutoff regularization schemes, with $\bar{\cal{E}}$ directly expressed in terms of the scattering parameters $a_1$ and $r_1$, once the cut off is sent to infinity. The whole set of possible values of $a_1$ and $r_1$ is explored for the first time in the literature looking for minima in the energy per particle with $\bar{\cal{E}}$ given as described. They are actually found, but a further inspection reveals that the associated scattering parameters give rise to resonance poles in the complex momentum-plane with positive imaginary part, which is at odds with the Hermiticity of the Hamiltonian. We also determine that these conflictive poles, with a pole-position momentum that is smaller in absolute value than the Fermi momentum of the system, clearly impact the calculation of $\bar{\cal{E}}$. As a result, we conclude that unpolarized spin-1/2 fermionic normal matter interacting in $P$-wave is not stable. We also study three universal parameters around the unitary limit. Finally, the whole set of values for the parameters $a_1$, $r_1$ is characterized according to whether they give rise to unallowed poles and, if so, by attending to their pole positions relative to the Fermi momentum of the system explored.

Collective modes in interacting two-dimensional tomographic Fermi liquids

We develop an analytically solvable model for interacting two-dimensional Fermi liquids with separate collisional relaxation rates for parity-odd and parity-even Fermi surface deformations. Such a disparity of collisional lifetimes exists whenever scattering is restricted to inversion-symmetric Fermi surfaces, and should thus be a generic feature of two-dimensional Fermi liquids. It implies an additional unanticipated "tomographic" transport regime (in between the standard collisionless and hydrodynamic regimes) in which even-parity modes are overdamped while odd-parity modes are collisionless. We derive expressions for both the longitudinal and the transverse conductivity and discuss the collective mode spectrum along the collisionless-tomographic-hydrodynamic crossover. Longitudinal modes cross over from zero sound in the collisionless regime to hydrodynamic first sound in the tomographic and hydrodynamic regime, where odd-parity damping appears as a subleading correction to the lifetime. In charged Fermi liquids with long-range Coulomb coupling, these modes reduce to plasmons with a strongly suppressed odd-parity correction to the damping. The transverse response, by contrast, has a specific tomographic transport regime with two imaginary odd-parity modes, one of which requires a finite repulsive interaction, distinct from both the shear sound in the collisionless regime and an overdamped diffusive current mode in the hydrodynamic limit. Our work demonstrates that there are deep many-body aspects of interacting Fermi liquids, which are often thought to be well understood theoretically, remaining unexplored.

Cesium-mediated electron redistribution and electron-electron interaction in high-pressure metallic CsPbI3

Electron-phonon coupling was believed to govern the carrier transport in halide perovskites and related phases. Here we demonstrate that electron-electron interaction enhanced by Cs-involved electron redistribution plays a direct and prominent role in the low-temperature electrical transport of compressed CsPbI3 and renders Fermi liquid (FL)-like behavior. By compressing δ-CsPbI3 to 80 GPa, an insulator-semimetal-metal transition occurs, concomitant with the completion of a slow structural transition from the one-dimensional Pnma (δ) phase to a three-dimensional Pmn21 (ε) phase. Deviation from FL behavior is observed upon CsPbI3 entering the metallic ε phase, which progressively evolves into a FL-like state at 186 GPa. First-principles density functional theory calculations reveal that the enhanced electron-electron coupling results from the sudden increase of the 5d state occupation in Cs and I atoms. Our study presents a promising strategy of cationic manipulation for tuning the electronic structure and carrier scattering of halide perovskites at high pressure.

Interlayer Electron-Hole Friction in Tunable Twisted Bilayer Graphene Semimetal.

Charge-neutral conducting systems represent a class of materials with unusual properties governed by electron-hole (e-h) interactions. Depending on the quasiparticle statistics, band structure, and device geometry these semimetallic phases of matter can feature unconventional responses to external fields that often defy simple interpretations in terms of single-particle physics. Here we show that small-angle twisted bilayer graphene (SA TBG) offers a highly tunable system in which to explore interactions-limited electron conduction. By employing a dual-gated device architecture we tune our devices from a nondegenerate charge-neutral Dirac fluid to a compensated two-component e-h Fermi liquid where spatially separated electrons and holes experience strong mutual friction. This friction is revealed through the T^{2} resistivity that accurately follows the e-h drag theory we develop. Our results provide a textbook illustration of a smooth transition between different interaction-limited transport regimes and clarify the conduction mechanisms in charge-neutral SA TBG.

Violation of Luttinger's theorem in the simplest doped Mott insulator: Falicov-Kimball model in the strong-correlation limit

The Luttinger's theorem has long been taken as the key feature of Landau's Fermi liquid, which signals the presence of quasiparticles. Here, by the unbiased Monte Carlo method, violation of Luttinger's theorem is clearly revealed in the Falicov-Kimball (FK) model, indicating the robust correlation-driven non-Fermi liquid characteristic under any electron density. Introducing hole carriers to the half-filled FK leads to Mott insulator-metal transition, where the Mott quantum criticality manifests unconventional scaling behavior in transport properties. Further insight on the violation of the Luttinger's theorem is examined by combining Hubbard-I approximation with a composite fermion picture, which emphasizes the importance of a mixed excitation of the itinerant electron and the composite fermion. Interestingly, when compared FK model with a binary disorder system, it suggests that the two-peak band structure discovered by Monte Carlo and Hubbard-I approaches is underlying the violation of Luttinger's theorem.

Coulomb drag between two strange metals

We study the Coulomb drag between two strange-metal layers using the Einstein-Maxwell-Dilaton model from holography. We show that the low-temperature dependence of the drag resistivity is $\rho_D \propto T^4$, which strongly deviates from the quadratic dependence of Fermi liquids. We also present numerical results at room temperature, using typical parameters of the cuprates, to provide an estimate of the magnitude of this effect for future experiments. We find that the drag resistivity is enhanced by the plasmons characteristic of the two-layer system.

Tuning Quantum Phase Transitions at Half Filling in 3L−MoTe2/WSe2 Moiré Superlattices

Many sought-after exotic states of matter are known to emerge close to quantum phase transitions, such as quantum spin liquids and unconventional superconductivity. It is, thus, desirable to experimentally explore systems that can be continuously tuned across these transitions. Here, we demonstrate such tunability and the electronic correlation effects in triangular moiré superlattices formed between trilayer MoTe2 and monolayer WSe2 (3L−MoTe2/WSe2). Through transport measurements, we observe an electronic analog of the Pomeranchuk effect at half filling of the first moiré subband, where increasing temperature paradoxically enhances charge localization. At low temperatures the system exhibits the characteristic of a Fermi liquid with strongly renormalized effective mass, suggesting a correlated metal state. The state is highly susceptible to out-of-plane electric and magnetic fields, which induce a Lifshitz transition and a metal-insulator transition (MIT), respectively. It enables identification of a tricritical point in the quantum phase diagram at the base temperature. We explain the Lifshitz transition in terms of interlayer charge transfer under the vertical electric field, which leads to the emergence of a new Fermi surface and immediate suppression of the Pomeranchuk effect. The existence of quantum criticality in the magnetic-field-induced MIT is supported by scaling behaviors of the resistance. Our work shows the 3L−MoTe2/WSe2 lies in the vicinity to the MIT point of the triangular lattice Hubbard model, rendering it a unique system to manifest the rich correlation effects at an intermediate interaction strength.Received 27 February 2022Revised 10 August 2022Accepted 14 September 2022DOI:https://doi.org/10.1103/PhysRevX.12.041015Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article’s title, journal citation, and DOI.Published by the American Physical SocietyPhysics Subject Headings (PhySH)Research AreasCritical phenomenaDensity of statesElectrical conductivityFermi surfaceHall effectLandau levelsMagnetotransportPhase diagramsQuantum phase transitionsQuantum transportTransport phenomenaCondensed Matter, Materials & Applied Physics

Pasta Phases in Neutron Star Mantle: Extended Thomas–Fermi vs. Compressible Liquid Drop Approaches

Nuclear pasta phases in the neutron stars mantle can affect the mechanical and transport properties of superdense matter, thus playing an important role in the dynamics and evolution of neutron stars. In this paper, we compare results obtained by the Extended Thomas–Fermi (ETF) method with the compressible liquid drop model (CLDM), based on the thermodynamically consistent description of the surface properties calculated for the two-phase plane interface and the same energy-density functional (for numerical illustration, we applied the Skyrme-type functional SLy4). Our ETF calculations found that pasta phases in cylindrical form cover a significant crustal region (both normal and inverse phases, aka spaghetti and bucatini are presented). Meanwhile, within the applied CLDM framework, which includes the thermodynamically required effect of neutron adsorption on the cluster’s surface but neglects curvature corrections, only the spaghetti phase was found to be energetically favorable in the small density range prior to crust–core transition. On the other hand, the recent CLDM of Dinh Thi et al., 2021, which, on the contrary, accounts for curvature term but neglects neutron adsorption, predicts pasta phase onset in better agreement with the ETF. This fact highlights the importance of the curvature effects and allows counting on the potential validity of the CLDMs as a convenient, transparent and accurate tool for investigation of the pasta-phase properties.

Tuning the many-body interactions in a helical Luttinger liquid

In one-dimensional (1D) systems, electronic interactions lead to a breakdown of Fermi liquid theory and the formation of a Tomonaga-Luttinger Liquid (TLL). The strength of its many-body correlations can be quantified by a single dimensionless parameter, the Luttinger parameter K, characterising the competition between the electrons’ kinetic and electrostatic energies. Recently, signatures of a TLL have been reported for the topological edge states of quantum spin Hall (QSH) insulators, strictly 1D electronic structures with linear (Dirac) dispersion and spin-momentum locking. Here we show that the many-body interactions in such helical Luttinger Liquid can be effectively controlled by the edge state’s dielectric environment. This is reflected in a tunability of the Luttinger parameter K, distinct on different edges of the crystal, and extracted to high accuracy from the statistics of tunnelling spectra at tens of tunnelling points. The interplay of topology and many-body correlations in 1D helical systems has been suggested as a potential avenue towards realising non-Abelian parafermions.

Spin chain on a metallic surface: Dissipation-induced order versus Kondo entanglement

We explore the physics of a spin-1/2 Heisenberg chain with Kondo interaction, $J_k$, to a two-dimensional electron gas. At weak $J_k$ the problem maps onto a Heisenberg chain locally coupled to a dissipative Ohmic bath. At the decoupled fixed point, the dissipation is a marginally relevant perturbation and drives long-range antiferromagnetic order along the chain. In the dynamical spin structure factor we observe a quadratic low-energy dispersion akin to Landau-damped Goldstone modes. At large $J_k$ Kondo screening dominates, and the spin correlations of the chain inherit the power law of the host metal, akin to a paramagnetic heavy Fermi liquid. In both phases we observe heavy bands near the Fermi energy in the composite-fermion spectral function. Our results, obtained from auxiliary-field quantum Monte Carlo simulations, provide a unique negative-sign-free realization of a quantum transition between an antiferromagnetic metal and a heavy-fermion metal. We discuss the relevance of our results in the context of scanning tunneling spectroscopy experiments of magnetic adatom chains on metallic surfaces.