Fermi Liquid Research Articles

Theory of confined high Tc superconductivity in monovalent metals

Monovalent nontransition metals are robust Fermi liquids. They defy superconductivity even at lowest temperatures (Li is a minor exception: [Formula: see text] mK). However, Thapa, Pandey, Ghosh and collaborators 8 have reported, from 2018, signals for transient and unstable granular superconductivity at ambient temperatures in Ag nanoparticles embedded in Au matrix. We develop a theory, where competing superconducing, CDW and SDW orders lose and get confined (go off-shell). They leave behind a robust Fermi liquid on-shell. A single half filled band crossing the Fermi level provides a number of special k-space regions for singlet stabilizing umklapp pair scattering and superconductivity stabilizing repulsive pair scattering. Carefully designed perturbations could deconfine a confined superconductivity. We suggest that electron transfer (doping) from Ag nanoparticles to Au matrix (with a higher electronegativity), quasi 2D structural reconstructions (e.g., 9R structure), electronically decoupled 2D patches and 1D segments expose confined superconductivity. Beneath a calm Fermi sea, strong supercurrents may exist in several metals.

Dielectric catastrophe at the Wigner-Mott transition in a moiré superlattice

The bandwidth-tuned Wigner-Mott transition is an interaction-driven phase transition from a generalized Wigner crystal to a Fermi liquid. Because the transition is generally accompanied by both magnetic and charge-order instabilities, it remains unclear if a continuous Wigner-Mott transition exists. Here, we demonstrate bandwidth-tuned metal-insulator transitions at fixed fractional fillings of a MoSe2/WS2 moiré superlattice. The bandwidth is controlled by an out-of-plane electric field. The dielectric response is probed optically with the 2s exciton in a remote WSe2 sensor layer. The exciton spectral weight is negligible for the metallic state with a large negative dielectric constant. It continuously vanishes when the transition is approached from the insulating side, corresponding to a diverging dielectric constant or a ‘dielectric catastrophe’ driven by the critical charge dynamics near the transition. Our results support the scenario of continuous Wigner-Mott transitions in two-dimensional triangular lattices and stimulate future explorations of exotic quantum phases in their vicinities.

Extremely correlated Fermi liquid theory for the U=∞, d=∞ Hubbard model to O(λ3)

We present the $O({\ensuremath{\lambda}}^{3})$ results from the $\ensuremath{\lambda}$ expansion in the extremely correlated Fermi-liquid theory applied to the infinite-dimensional $t\ensuremath{-}J$ model (with $J=0$) and compare the results with the earlier $O({\ensuremath{\lambda}}^{2})$ results as well as the results from the dynamical mean-field theory. We focus attention on the $T$ dependence of the resistivity $\ensuremath{\rho}(T)$, the Dyson self-energy, and the quasiparticle weight $Z$ at various densities. The comparison shows that all the methods display quadratic-in-$T$ resistivity followed by a quasilinear-in-$T$ resistivity characterizing a strange metal and gives an estimate of the different scales of these variables relative to the exact results.

Zero sound and plasmon modes for non-Fermi liquids

We derive the quantum Boltzmann equation (QBE) by using generalized Landau-interaction parameters, obtained through the nonequilibrium Green's function technique. This is a generalization of the usual QBE formalism to non-Fermi liquid (NFL) systems, which do not have well-defined quasiparticles. We apply this framework to a controlled low-energy effective field theory for the Ising-nematic quantum critical point, in order to find the collective excitations of the critical Fermi surface in the collisionless regime. We also compute the nature of the dispersion after the addition of weak Coulomb interactions. The zero angular momentum longitudinal vibrations of the Fermi surface show a linear-in-wavenumber dispersion, which corresponds to the zero sound of Landau's Fermi liquid theory. The Coulomb interaction modifies it to a plasmon mode in the long-wavelength limit, which disperses as the square-root of the wavenumber. Remarkably, our results show that the zero sound and plasmon modes exhibit the same behaviour as in a Fermi liquid, although an NFL is fundamentally different from the former.

A theoretical analysis of superconducting pairing in correlated metallic systems

We have introduced a Coulomb correlated normal state to study the superconducting pairing within a Fermi liquid (FL)-like background in a 3-dimensional system. The role of the Coulomb correlation has been actively incorporated by means of the Gutzwiller projection scheme, in the presence of phonon mediated attractive electron–electron (AEE) interaction throughout the entire regime of its applicability. We variationally modulate the Coulomb correlation strength from the weak to the strong regime in our calculational procedure. The main highlight of our results is the appearance of a ‘2-gap-like’ structure in the superconducting phase, arising out of the two-body interacting matrix elements, calculated in the presence of the active Coulomb correlation. We have made use of the ‘two-square well model’ potential to evaluate the superconducting pairing gaps at zero temperature. Our Calculational scheme has been applied to a simple cubic lattice system for a physical realization. All the consequences are elaborated and discussed.

Soft modes in Fermi liquids at arbitrary temperatures

We use kinetic-theory methods to analyze Landau Fermi-liquid theory, and in particular to investigate the number and nature of modes in Fermi liquids that are soft in the long-wavelength limit, both in the hydrodynamic and the collisionless regimes. In the hydrodynamic regime we show that Fermi-liquid theory is consistent with Navier-Stokes hydrodynamics at all temperatures, as expected. The soft modes are the ones familiar from classical hydrodynamics that are controlled by the five conservation laws; namely, two first-sound modes, two shear diffusion modes, and one heat diffusion mode. These modes have a particle-like spectrum and are soft, or scale invariant, at all temperatures. In the collisionless regime we show that the entire single-particle distribution function is soft with a continuous part of the spectrum. This continuous soft mode, which is well known but often not emphasized, has important physical consequences, e.g., for certain quantum phase transitions. In addition, there are the well-known soft zero-sound excitations that describe angular fluctuations of the Fermi surface; their spectra are particle-like. They are unrelated to conservation laws, acquire a mass at any nonzero temperature, and their number depends on the strength of the quasiparticle interaction. We also discuss the fates of these two families of soft modes as the temperature changes. With increasing temperature the size of the collisionless regime shrinks, the damping of the modes grows, and eventually all of the collisionless modes become overdamped. In their stead the five hydrodynamic modes appear in the hydrodynamic regime at asymptotically low frequencies. The two families of soft modes are unrelated and have very different physical origins. In charged Fermi liquids the first-sound modes in the hydrodynamic regime and the $\ensuremath{\ell}=0$ zero-sound modes in the collisionless regime get replaced by plasmons, all other modes remain soft.

Fluctuating quantum kinetic theory

We consider a quantum Langevin kinetic equation for a system of fermions. We first derive the Langevin force noise correlation functions in Landau's Fermi-liquid kinetic theory from general considerations. We then use the resulting equation to calculate the equilibrium dynamic structure factor in the collisionless regime at low temperatures. The result is in agreement with the conventional many-body result. We then use the theory to derive both the fluctuating Navier-Stokes equations for a quantum fluid and the fluctuating hydrodynamic equations for fermions in the presence of quenched disorder. We also discuss the modifications needed for the fluctuating hydrodynamic equations to describe an electron fluid with long-ranged interactions, and we prove an $H$ theorem for the nonlinear Landau kinetic equation.

On the dynamic distinguishability of nodal quasi-particles in overdoped cuprates

La_{1.67}1.67Sr_{0.33}0.33CuO_44 is not a superconductor and its resistivity follows a purely T^22 temperature dependence at very low temperatures. La_{1.71}1.71Sr_{0.29}0.29CuO_44, on the other hand, has a superconducting ground state together with a T-Linear term in its resistivity. The concomitant emergence of these two features below a critical doping is mystifying. Here, I notice that the electron-electron collision rate in the Fermi liquid above the doping threshold is unusually large. The scattering time of nodal quasi-particles expressed in a dimensionless parameter \zetaζ is very close to what has been found in liquid ^33He at its melting pressure. In the latter case, fermionic particles become dynamically distinguishable by excess of interaction. Ceasing to be dynamically indistinguishable, nodal electrons will be excluded from the Fermi sea. Such non-degenerate carriers will then scatter the degenerate ones within a phase space growing linearly with temperature.

Peculiar Physics of Heavy-Fermion Metals: Theory versus Experiment

This review considers the topological fermion condensation quantum phase transition (FCQPT) that leads to flat bands and allows the elucidation of the special behavior of heavy-fermion (HF) metals that is not exhibited by common metals described within the framework of the Landau Fermi liquid (LFL) theory. We bring together theoretical consideration within the framework of the fermion condensation theory based on the FCQPT with experimental data collected on HF metals. We show that very different HF metals demonstrate universal behavior induced by the FCQPT and demonstrate that Fermi systems near the FCQPT are controlled by the Fermi quasiparticles with the effective mass M* strongly depending on temperature T, magnetic field B, pressure P, etc. Within the framework of our analysis, the experimental data regarding the thermodynamic, transport and relaxation properties of HF metal are naturally described. Based on the theory, we explain a number of experimental data and show that the considered HF metals exhibit peculiar properties such as: (1) the universal T/B scaling behavior; (2) the linear dependence of the resistivity on T, ρ(T)∝A1T (with A1 is a temperature-independent coefficient), and the negative magnetoresistance; (3) asymmetrical dependence of the tunneling differential conductivity (resistivity) on the bias voltage; (4) in the case of a flat band, the superconducting critical temperature Tc∝g with g being the coupling constant, while the M* becomes finite; (5) we show that the so called Planckian limit exhibited by HF metals with ρ(T)∝T is defined by the presence of flat bands.

Dynamical Mean-Field Theory of Moiré Bilayer Transition Metal Dichalcogenides: Phase Diagram, Resistivity, and Quantum Criticality

We present a comprehensive dynamical mean field study of the triangular moir\'e Hubbard model, which is believed to represent the physics of moir\'e bilayer transition metal dichalcogenides. In these materials, important aspects of the band structure including the bandwidth and the order and location of van Hove singularities can be tuned by varying the interlayer potential. We present a magnetic and metal-insulator phase diagram and a detailed study of the dependence of the resistivity on temperature, band filling and interlayer potential. We find that transport displays Fermi liquid, strange metal and quantum critical behaviors in distinct regions of the phase diagram. We show how magnetic order affects the resistivity. Our results elucidate the physics of the correlated states and the metal-insulator continuous transition recently observed in twisted homobilayer WSe$_2$ and heterobilayer MoTe$_2$/WSe$_2$ experiments.

Superconductivity in monolayer FeSe enhanced by quantum geometry

We formulate the superfluid weight in unconventional superconductors with $\mathbit{k}$-dependent Cooper pair potentials based on the geometric properties of Bloch electrons. We apply the formula to a model of monolayer FeSe obtained by first-principles calculation. Our numerical calculations point to a significant enhancement of the Berezinskii-Kosterlitz-Thouless transition temperature due to the geometric contribution to the superfluid weight, which is not included in the Fermi liquid theory. The $\mathbit{k}$ dependence of the gap function also stabilizes the superconducting state. Our results reveal that the geometric properties of Bloch electrons play an essential role in superconducting materials and pave the way for clarifying hidden aspects of superconductivity from the viewpoint of quantum geometry.

Entanglement of Skeletal Regions.

The entanglement entropy (EE) encodes key properties of quantum many-body systems. It is usually calculated for subregions of finite volume (or area in 2D). Here, we study the EE of skeletal regions that have no volume, such as a line in 2D. We show that skeletal entanglement displays new behavior compared with its bulk counterpart, and leads to distinct universal quantities. We provide nonperturbative bounds for the skeletal area-law coefficient of a large family of quantum states. We then explore skeletal scaling for the toric code, conformal bosons and Dirac fermions, Lifshitz critical points, and Fermi liquids. We discover signatures including skeletal topological EE, novel corner terms, and strict area-law scaling for metals. These findings suggest that skeletal entropy serves as a measure for the range of entanglement. Finally, we outline open questions relating to other systems and measures such as the logarithmic negativity.

Solvable theory of a strange metal at the breakdown of a heavy Fermi liquid

We introduce an effective theory for quantum critical points (QCPs) in heavy fermion systems, involving a change in carrier density without symmetry breaking. Our new theory captures a strongly coupled metallic QCP, leading to robust marginal Fermi liquid transport phenomenology, and associated linear in temperature ($T$) "strange metal" resistivity, all within a controlled large $N$ limit. In the parameter regime of strong damping of emergent bosonic excitations, the QCP also displays a near-universal "Planckian" transport lifetime, $\tau_{\mathrm{tr}}\sim\hbar/(k_BT)$. This is contrasted with the conventional so-called "slave boson" theory of the Kondo breakdown, where the large $N$ limit describes a weak coupling fixed point and non-trivial transport behavior may only be obtained through uncontrolled $1/N$ corrections. We also compute the weak-field Hall coefficient within the effective model as the system is tuned across the transition. We further find that between the two plateaus, reflecting the different carrier densities in the two Fermi liquid phases, the Hall coefficient can develop a peak in the critical crossover regime, like in recent experimental findings, in the parameter regime of weak boson damping.

Superconductivity near a nematoelastic quantum critical point

We study the pairing instability of a two-dimensional metallic system induced by Ising-nematic quantum fluctuations in the presence of an unavoidable relevant coupling of the nematic order parameter to the elastic modes (acoustic phonons) of the lattice. We find that this nematoelastic coupling $\lambda_\mathrm{latt}$ leads to a decrease of both the superconducting (SC) critical temperature $T_c$ and the gap function $\Delta$, regardless of the gap symmetry. Interestingly, we show that $\lambda_\mathrm{latt}$ provides a knob that allows us to investigate the emergence of the SC phase at low temperatures, as an instability from either a non-Fermi liquid or a Fermi liquid normal state. The phase transitions between the SC and these normal states are characterized by different critical exponents, which may also vary for each gap symmetry. Finally, we argue that these results might explain the dependence of $T_c$ in the vicinity of the nematic quantum critical point exhibited by the compound FeSe$_{1 - x}$S$_x$.

Ab-initio Study of Interacting Fermions at Finite Temperature with Neural Canonical Transformation

We present a variational density matrix approach to the thermal properties of interacting fermions in the continuum. The variational density matrix is parametrized by a permutation equivariant many-body unitary transformation together with a discrete probabilistic model. The unitary transformation is implemented as a quantum counterpart of neural canonical transformation, which incorporates correlation effects via a flow of fermion coordinates. As the first application, we study electrons in a two-dimensional quantum dot with an interaction-induced crossover from Fermi liquid to Wigner molecule. The present approach provides accurate results in the low-temperature regime, where conventional quantum Monte Carlo methods face severe difficulties due to the fermion sign problem. The approach is general and flexible for further extensions, thus holds the promise to deliver new physical results on strongly correlated fermions in the context of ultracold quantum gases, condensed matter, and warm dense matter physics.

Strongly Correlated Quantum Spin Liquids versus Heavy Fermion Metals: A Review.

This review considers the topological fermion condensation quantum phase transition (FCQPT) that explains the complex behavior of strongly correlated Fermi systems, such as frustrated insulators with quantum spin liquid and heavy fermion metals. The review contrasts theoretical consideration with recent experimental data collected on both heavy fermion metals (HF) and frustrated insulators. Such a method allows to understand experimental data. We also consider experimental data collected on quantum spin liquid in and quasi-one dimensional (1D) quantum spin liquid in both and with the aim to establish a sound theoretical explanation for the observed scaling laws, Landau Fermi liquid (LFL) and non-Fermi-liquid (NFL) behavior exhibited by these frustrated insulators. The recent experimental data on the heavy-fermion metal , with , and on its sister compounds and , carried out under the application of magnetic field as a control parameter are analyzed. We show that the thermodynamic and transport properties as well as the empirical scaling laws follow from the fermion condensation theory. We explain how both the similarity and the difference in the thermodynamic and transport properties of and in its sister compounds and emerge, as well as establish connection of these (HF) metals with insulators , and . We demonstrate that the universal LFL and NFL behavior emerge because the HF compounds and the frustrated insulators are located near the topological FCQPT or are driven by the application of magnetic fields.

Transport and spectroscopic signatures of a disorder-stabilized metal in two-dimensional frustrated Mott insulators

Frustrated Mott insulators such as transition metal dichalcogenides present an ideal platform for the experimental realization of externally tuned insulator-metal transition. In this paper, we present the first nonperturbative numerical investigation of the disorder-induced insulator-metal transition in a two-dimensional frustrated Mott insulator. Our approach is generic and captures the essential physics of Mott insulator-metal transition in geometrically frustrated lattices. For concreteness, we have compared our results with the experimental observations on copper (Cu) intercalated 1T-TaS2. Based on the magnetic, spectroscopic, and transport signatures, we have mapped out the thermal phase diagram of Cu intercalated 1T-TaS2 and established that over a regime of moderate disorder strength this material hosts an antiferromagnetic metal. Moreover, the insulator-metal transition in this system is not tied to the loss of magnetic correlations, thereby giving rise to two quantum critical points. The emergent non-Fermi liquid metal is governed by resilient quasiparticles, that survive as the relevant low energy excitations even after the break down of the Fermi liquid description. The transport and spectroscopic signatures discussed in this paper are expected to serve as important benchmarks for future experiments on this and related class of materials.

Adiabatic transition from a BCS superconductor to a Fermi liquid and phase dynamics

We investigate the physics of an adiabatic transition from a BCS superconductor to a Fermi liquid for an exponentially slow decreasing pairing interaction. We show that, depending on the order of the thermodynamic limit and large times, a situation can arise in which the Fermi liquid keeps a memory of the parent BCS state. Furthermore, a time inversion of the interaction, supplemented by a manipulation analogous to a spin-/photon-echo experiment, allows us to recover the parent BCS state. Moreover, we study the evolution of the order parameter phase $\ensuremath{\phi}$ in transforming the BCS superconductor to a conventional metal. Since the global phase is the conjugate variable of the density, we explicitly show how to use the dynamics of $\ensuremath{\phi}$ together with gauge invariance to build up the noninteracting chemical potential away from particle-hole symmetry. We further analyze the role of $\ensuremath{\phi}$ in restoring the gauge-invariant current response when the noninteracting Fermi liquid is approached starting from a BCS superconductor in the presence of an external vector field.

Dielectric response of electrons with strong local correlations and long-ranged Coulomb interactions

Motivated by recent experiments, we append long ranged Coulomb interactions to dominant strong local correlations and study the resulting t-J-VC model for the 2-dimensional cuprate materials. This model includes the effect of short ranged Hubbard–Gutzwiller–Kanamori type correlations and long ranged Coulomb interactions on tight binding electrons. We calculate the {q→,ω} dependent charge density fluctuations in this model using the extremely correlated Fermi liquid theory characterized by quasiparticles with very small weight Z. We develop a novel set of formulae to represent the dynamical charge susceptibility and the dielectric function, using a version of the charge-current continuity equation for a band system, valid for arbitrary q→. Combining these ingredients, we present results for the irreducible dynamical charge susceptibility χ˜ρρ(q→,ω), (longitudinal) dielectric function ɛ(q→,ω), current susceptibility χ˜JJ(q→,ω), conductivity σ(q→,ω), and the plasma frequency for any q→. We also present calculations for the first moment of the structure function and discuss a characteristic energy scale Ωp(q→) which locates a peak in Imχ˜ρρ(q→,ω).

Thermodynamics of an exactly solvable model for superconductivity in a doped Mott insulator

Computing superconducting properties starting from an exactly solvable model for a doped Mott insulator stands as a grand challenge. We have recently shown that this can be done starting from the Hatsugai-Kohmoto (HK) model which can be understood generally as the minimal model that breaks the non-local $\mathbb Z_2$ symmetry of a Fermi liquid, thereby constituting a new quartic fixed point for Mott physics [Phillips et al., Nature Physics 16, 1175 (2020); Huang et al., Nature Physics (2022)]. In the current work, we compute the thermodynamics, condensation energy, and electronic properties such as the NMR relaxation rate $1/T_1$ and ultrasonic attenuation rate. Key differences arise with the standard BCS analysis from a Fermi liquid: 1) the free energy exhibits a local minimum at $T_p$ where the pairing gap turns on discontinuously above a critical value of the repulsive HK interaction, thereby indicating a first-order transition, 2) a tri-critical point emerges, thereby demarcating the boundary between the standard second-order superconducting transition and the novel first-order regime, 3) Mottness changes the sign of the quartic coefficient in the Landau-Ginzburg free-energy fuctional relative to that in BCS, 4) as this obtains in the strongly interacting regime, it is Mott physics that underlies the generic first-order transition, 5) the condensation energy exceeds that in BCS theory suggesting that multiple Mott bands might be a way of enhancing superconducting, 6) the heat-capacity jump is non-universal and increases with the Mott scale, 7) Mottness destroys the Hebel-Slichter peak in NMR, and 8) Mottness enhances the fall-off of the ultrasonic attenuation at the pairing temperature $T_p$. As several of these properties are observed in the cuprates, our analysis here points a way forward in computing superconducting properties of strongly correlated electron matter.