Enhanced Quantum Coherence Research Articles

Enhanced quantum coherence of plasmonic resonances with a chiral exceptional points

Enhanced quantum coherence of plasmonic resonances with a chiral exceptional points

Protecting the Quantum Coherence of Two Atoms Inside an Optical Cavity by Quantum Feedback Control Combined with Noise-Assisted Preparation

We propose a theoretical scheme to enhance quantum coherence and obtain steady-state coherence by combining quantum feedback control and noise-assisted preparation. We investigate the effects of quantum-jump-based feedback control and noise field on the quantum coherence and excited-state population between two atoms inside an optical cavity where a noise field drives one, and the other is under quantum feedback control. It is found that steady quantum coherence can be achieved by adding an external noise field, and the quantum feedback can prolong the coherence time with partial suppression of the spontaneous emission of atoms. In addition, we study the influence of the joint action of quantum feedback and noise-assisted preparation on quantum coherence and show that the combined action of feedback control and noise-assisted preparation is more effective in enhancing steady coherence. The findings of our research offer some general guidelines for improving the steady-state coherence of coupled qubit systems and have the potential to be applied in the realm of quantum information technology.

Quantum enhancement of qutrit dynamics of a three-level giant atom coupling to a one-dimensional waveguide

Dynamics of quantum coherence and non-Markovianity of a three-level giant atom coupling to a one-dimensional waveguide and a classical field are investigated theoretically. The time delay of the photo propagation in the waveguide is taken into account and our aim is to access the collective impact of a waveguide and classical control of the system on the time evolution of coherence and non-Markovianity. For a giant atom, we find that the various values of the accumulated phase and time delay does not make much difference for the coherence evolution but there exists non-Markovian behavior for the vast majority of the chosen parameter values. With regard to the initial relative phase, the quantum coherence takes a monotonic behavior for a small atom but decreases with oscillations for a giant atom with majority values of the initial relative phase. Quantum coherence of a small atom decreases monotonically with regardless of the Rabi frequency and the atom’s detuning to a large extent but a large Rabi frequency or a large atom’s detuning will induce non-Markovian behavior for a giant atom. With a comparative analysis, the coherence evolution is enhanced significantly in that there is non-Markovian behavior for the dynamics of quantum coherence in a much larger range of scaled time for a giant atom than that for a small atom. Our study provide clues to preserve and to enhance quantum coherence in qutrit systems.

Enhancing quantum coherence of a fluxonium qubit by employing flux modulation with tunable-complex-amplitude

We propose to protect fluxonium qubits that are away from half flux quantum against environmental noises, especially flux noise, by adopting a modulated flux with tunable-complex-amplitude. Using open-system Floquet theory, we derive a Lindblad equation and extract decoherent rates for pure-dephasing, excitation and relaxation. After examining intrinsic attributes of the flux driven fluxonium qubit, we put forward an analytic manner to locate dynamical sweet spots for fast and weak driving. Continuous families of dynamical sweet spots are found in the parameter plane of relative amplitude factor and relative phase. Around a family of dynamical sweet spots or between two families of dynamical sweet spots, there exist continuous regions with long coherent times that exceed . Taking advantage of the two noise-insensitive channels: relative amplitude factor and relative phase, a flux driven fluxonium qubit can become immune to flux noises from both the dc and ac flux amplitudes. And the optimal driving amplitudes are no longer isolated at a certain driving frequency, but become continuous. This is in sharp contrast to the usual schemes based on flux modulation with real-amplitude. As a result, there are plenty of manipulating flexibility in our flux driving scheme with tunable-complex-amplitude, which may be useful in logical operations among flux driven fluxonium qubits or other flux qubits.

Binding Sites, Vibrations and Spin-Lattice Relaxation Times in Europium(II)-Based Metallofullerene Spin Qubits.

To design molecular spin qubits with enhanced quantum coherence, a control of the coupling between the local vibrations and the spin states is crucial, which could be realized in principle by engineering molecular structures via coordination chemistry. To this end, understanding the underlying structural factors that govern the spin relaxation is a central topic. Here, we report the investigation of the spin dynamics in a series of chemically designed europium(II)‐based endohedral metallofullerenes (EMFs). By introducing a unique structural difference, i. e. metal‐cage binding site, while keeping other molecular parameters constant between different complexes, these manifest the key role of the three low‐energy metal‐displacing vibrations in mediating the spin‐lattice relaxation times (T 1). The temperature dependence of T 1 can thus be normalized by the frequencies of these low energy vibrations to show an unprecedentedly universal behavior for EMFs in frozen CS2 solution. Our theoretical analysis indicates that this structural difference determines not only the vibrational rigidity but also spin‐vibration coupling in these EMF‐based qubit candidates.

Zero-Bias Conductance Peaks Effectively Tuned by Gating-Controlled Rashba Spin-Orbit Coupling.

Zero-bias conductance peaks (ZBCPs) can manifest a number of notable physical phenomena and thus provide critical characteristics to the underlying electronic systems. Here, we report observations of pronounced ZBCPs in hybrid junctions composed of an oxide heterostructure LaAlO_{3}/SrTiO_{3} and an elemental superconductor Nb, where the two-dimensional electron system (2DES) at the LaAlO_{3}/SrTiO_{3} interface is known to accommodate gate-tunable Rashba spin-orbit coupling (SOC). Remarkably, the ZBCPs exhibit a domelike dependence on the gate voltage, which correlates strongly with the nonmonotonic gate dependence of the Rashba SOC in the 2DES. The origin of the observed ZBCPs can be attributed to the reflectionless tunneling effect of electrons that undergo phase-coherent multiple Andreev reflection, and their gate dependence can be explained by the enhanced quantum coherence time of electrons in the 2DES with increased momentum separation due to SOC. We further demonstrate theoretically that, in the presence of a substantial proximity effect, the Rashba SOC can directly enhance the overall Andreev conductance in the 2DES-barrier-superconductor junctions. These findings not only highlight nontrivial interplay between electron spin and superconductivity revealed by ZBCPs, but also set forward the study of superconducting hybrid structures by means of controllable SOC, which has significant implications in various research fronts from superconducting spintronics to topological superconductivity.

Evolution of quantum coherence induced by band gaps and initial-state preparation measurements

The evolution of quantum coherence in a qubit is analyzed, over short and long times, in case the qubit interacts with a bosonic environment. The distribution of the frequency modes exhibits a low-frequency band gap. The initial conditions under study of the qubit and the bosonic environment are factorized or prepared with selective or nonselective measurements. The modulus of the coherence term of the reduced density matrix of the qubit evolves algebraically over short times and, due to the band gap, tends to the nonvanishing asymptotic value with damped oscillations. Depending on the measurement scheme, the nonselective preparation measurement can enhance quantum coherence or accelerate the decoherence process, over short times, according to dominant linear laws. Over long times, the nonselective preparation measurement produces the slowest-decaying envelope of the damped oscillations among the decoherence processes under study. Similar short- and long-time evolution is exhibited by the trace distance measure of two general states of the qubit.

Decoherence of a two-qubit system interacting with initially correlated random telegraph noises

Decoherence of a two-qubit system is studied in terms of an exactly solvable dephasing model. In this model, the two qubits are influenced by the random telegraph noises (RTNs) which are dynamically independent but initially correlated, where the initial correlation means that joint probability of the two RTNs is not factorizable at an initial time. It is shown that the purely classical initial correlation between the RTNs can create interesting effects on the time evolution of the two-qubit system. For this purpose, two-qubit coherence, entanglement and other correlations are investigated in detail. It is found that the initial correlation can suppress the decoherence of the two-qubit system. The most important result is that the time evolution of the two-qubit system can become non-Markovian in the presence of the initial correlation, even if it is Markovian in the absence of the initial correlation. Furthermore, it is shown that the initial correlation between the RTNs can enhance quantum coherence and correlation of the two-qubit system.

Enhanced quantum coherence in exchange coupled spins via singlet-triplet transitions.

Manipulation of spin states at the single-atom scale underlies spin-based quantum information processing and spintronic devices. These applications require protection of the spin states against quantum decoherence due to interactions with the environment. While a single spin is easily disrupted, a coupled-spin system can resist decoherence by using a subspace of states that is immune to magnetic field fluctuations. Here, we engineered the magnetic interactions between the electron spins of two spin-1/2 atoms to create a "clock transition" and thus enhance their spin coherence. To construct and electrically access the desired spin structures, we use atom manipulation combined with electron spin resonance (ESR) in a scanning tunneling microscope. We show that a two-level system composed of a singlet state and a triplet state is insensitive to local and global magnetic field noise, resulting in much longer spin coherence times compared with individual atoms. Moreover, the spin decoherence resulting from the interaction with tunneling electrons is markedly reduced by a homodyne readout of ESR. These results demonstrate that atomically precise spin structures can be designed and assembled to yield enhanced quantum coherence.

Frozen Condition of Quantum Coherence for Atoms on a Stationary Trajectory.

The quantum coherence (QC) of two comoving atoms on a stationary trajectory is investigated. We develop a formalism to characterize the properties of atoms on a stationary trajectory. We give a criterion under which QC is frozen to a nonzero value. The frozen condition that vanishing super- or subradiant decay rate is not so sensitive to the initial condition of state. We show that enhanced QC and a subradiant state can be gained from the initial state.

Photon catalysis acting as noiseless linear amplification and its application in coherence enhancement

Photon catalysis is an intriguing quantum mechanical operation during which no photon is added to or subtracted from the relevant optical system. However, we prove that photon catalysis is in essence equivalent to the simpler but more efficient noiseless linear amplifier. This provides a simple and zero-energy-input method for enhancing quantum coherence. We show that the coherence enhancement holds both for a coherent state and a two-mode squeezed vacuum (TMSV) state. For the TMSV state, biside photon catalysis is shown to be equivalent to two times the single-side photon catalysis, and two times the photon catalysis does not provide a substantial enhancement of quantum coherence compared with single-side catalysis. We further extend our investigation to the performance of coherence enhancement with a more realistic photon catalysis scheme where a heralded approximated single-photon state and an on-off detector are exploited. Moreover, we investigate the influence of an imperfect photon detector and the result shows that the amplification effect of photon catalysis is insensitive to the detector inefficiency. Finally, we apply the coherence measure to quantum illumination and see the same trend of performance improvement as coherence enhancement is identified in practical quantum target detection.

Enhancing Coherent Light-Matter Interactions through Microcavity-Engineered Plasmonic Resonances.

Quantum manipulation is challenging in localized-surface plasmon resonances (LSPRs) due to strong dissipations. To enhance quantum coherence, here we propose to engineer the electromagnetic environment of LSPRs by placing metallic nanoparticles (MNPs) in optical microcavities. An analytical quantum model is first built to describe the LSPR-microcavity interaction, revealing the significantly enhanced coherent radiation and the reduced incoherent dissipation. Furthermore, when a quantum emitter interacts with the LSPRs in the cavity-engineered environment, its quantum yield is enhanced over 40 times and the radiative power over one order of magnitude, compared to those in the vacuum environment. Importantly, the cavity-engineered MNP-emitter system can enter the strong coupling regime of cavity quantum electrodynamics, providing a promising platform for the study of quantum plasmonics, quantum information processing, precise sensing, and spectroscopy.

Substantially Enhancing Quantum Coherence of Electrons in Graphene via Electron-Plasmon Coupling.

The interplays between different quasiparticles in solids lay the foundation for a wide spectrum of intriguing quantum effects, yet how the collective plasmon excitations affect the quantum transport of electrons remains largely unexplored. Here we provide the first demonstration that when the electron-plasmon coupling is introduced, the quantum coherence of electrons in graphene is substantially enhanced with the quantum coherence length almost tripled. We further develop a microscopic model to interpret the striking observations, emphasizing the vital role of the graphene plasmons in suppressing electron-electron dephasing. The novel and transformative concept of plasmon-enhanced quantum coherence sheds new insight into interquasiparticle interactions, and further extends a new dimension to exploit nontrivial quantum phenomena and devices in solid systems.

Atomically Thin Al2O3 Films for Tunnel Junctions

Metal-Insulator-Metal tunnel junctions (MIMTJ) are common throughout the microelectronics industry. The industry standard AlOx tunnel barrier, formed through oxygen diffusion into an Al wetting layer, is plagued by internal defects and pinholes which prevent the realization of atomically-thin barriers demanded for enhanced quantum coherence. In this work, we employed in situ scanning tunneling spectroscopy (STS) along with molecular dynamics simulations to understand and control the growth of atomically thin Al2O3 tunnel barriers using atomic layer deposition (ALD). We found that a carefully tuned initial H2O pulse hydroxylated the Al surface and enabled the creation of an atomically-thin Al2O3 tunnel barrier with a high quality M-I interface and a significantly enhanced barrier height compared to thermal AlOx. These properties, corroborated by fabricated Josephson Junctions, show that ALD Al2O3 is a dense, leak-free tunnel barrier with a low defect density which can be a key component for the next-generation of MIMTJs.

Enhancing quantum coherence and quantum Fisher information by quantum partially collapsing measurements

We consider the enhancement effect of quantum partially collapsing measurements, i.e., weak measurement and quantum measurement reversal, on quantum coherence and quantum Fisher information, both of which are transmitted through a spin-chain channel. For the state parameter lying in the region $$(\pi /2,\ \pi )$$(?/2,?), weak measurement can enhance quantum coherence and quantum Fisher information. For the state parameter lying in the region $$(0,\ \pi /2)$$(0,?/2), quantum coherence and quantum Fisher information can be enhanced by quantum measurement reversal combined with weak measurement. We assume the probabilistic nature of the method should be responsible for the enhancement.

Spin Dynamics and Low Energy Vibrations: Insights from Vanadyl-Based Potential Molecular Qubits.

Here we report the investigation of the magnetization dynamics of a vanadyl complex with diethyldithiocarbamate (Et2dtc-) ligands, namely [VO(Et2dtc)2] (1), in both solid-state and frozen solution. This showed an anomalous and unprecedentedly observed field dependence of the relaxation time, which was modeled with three contributions to the relaxation mechanism. The temperature dependence of the weight of the two processes dominating at low fields was found to well correlate with the low energy vibrations as determined by THz spectroscopy. This detailed experimental comparative study represents a fundamental step to understand the spin dynamics of potential molecular quantum bits, and enriches the guidelines to design molecule-based systems with enhanced quantum coherence.

Enhancing quantum coherence with short-range correlated disorder

We introduce a two-dimensional short-range correlated disorder that is the natural generalization of the well-known one-dimensional dual random dimer model [Phys. Rev. Lett 65, 88 (1990)]. We demonstrate that, as in one dimension, this model induces a localization-delocalization transition in the single-particle spectrum. Moreover we show that the effect of such a disorder on a weakly-interacting boson gas is to enhance the condensate spatial homogeneity and delocalisation, and to increase the condensate fraction around an effective resonance of the two-dimensional dual dimers. This study proves that short-range correlations of a disordered potential can enhance the quantum coherence of a weakly-interacting many-body system.

Enhanced quantum coherence in graphene caused by Pd cluster deposition

We report on the unexpected increase in the dephasing lengths of a graphene sheet caused by the deposition of Pd nanoclusters, as demonstrated by weak localization measurements. The dephasing lengths reached saturated values at low temperatures. Theoretical calculations indicate the p-type charge transfer from the Pd clusters, which contributes more carriers. The saturated values of dephasing lengths often depend on both the carrier concentration and mean free path. Although some impurities are increased as revealed by decreased mobilities, the intense charge transfer leads to the improved saturated values and subsequent improved dephasing lengths.

Molecular spin qubits based on lanthanide ions encapsulated in cubic polyoxopalladates: design criteria to enhance quantum coherence

Axial compression and a magnetic field can help to get coherent spin qubits.

Investigating Leggett-Garg inequality for a two level system under decoherence in a non-Markovian dephasing environment.

Leggett-Garg inequalities (LGI) test the correlations of a single system measured at different times. Violation of LGI implies either the absence of a realistic description of the system or the impossibility of measuring the system without disturbing it. We investigate the violation of the Leggett-Garg inequality for a two level system under decoherence in a non-Markovian dephasing environment. We discuss the non-Markovian dynamics of the violation of LGI at zero temperature and also at finite temperature for different structured environments. An enhanced quantum coherence is shown through the violation of Leggett-Garg inequality in the strong non-Markovian regime of the environment.