Plastic anisotropy is a key factor that affects the formability and performance of Al-Mg alloys. In this study, the effects of Mg content and strain path shifting from unidirectional rolling (UDR) to cross rolling processes (CR) on plastic anisotropy in Al-Mg alloys were investigated. Al-6 and 9Mg alloys were heat-treated and rolled in two different ways: the first was a UDR process, and the other was a CR process at room temperature. The rolled specimens were analyzed by electron backscattered diffraction method and tensile test. High Mg content suppresses the formation of texture that strengthens the plastic anisotropy in both UDR and CR processes. CR significantly reduces the rolling texture area fraction, leading to greater texture randomness compared to UDR. CR promotes the formation of low-angle deformation bands, which low-angle bands appear to have a weaker impact on deformation resistance and may contribute to the reduced anisotropy in CR-processed materials. CR results in a more uniform distribution of stored energy. R-value which represents plastic anisotropy decreases by shifting from UDR to CR, and by increment of Mg content. Overall, this study demonstrates that CR is a promising approach for improving the formability and performance of Al-Mg alloys by effectively controlling plastic anisotropy.