Distribution Of Aerosol Optical Depth Research Articles

Sustainable data-driven insights: Statistical analysis and artificial intelligence-driven modelling of aerosol concentrations in Hyderabad district, India

Air pollution stands as a pressing issue in contemporary times, leading to the loss of millions of lives and exerting detrimental effects on the economy. The aerosols especially particulate matter, which are dispersions of matter in air medium play an important role in manipulating the climatological variables in an area. The current study was developed in response to the need to study aerosols and particulates on annual levels using 20-year (2002–2021) daily mean Aerosol Optical Depth (AOD) product released by Moderate Resolution Imaging Spectrometer (MODIS) sensors, and to generate prediction models for AOD using artificial intelligence (AI) techniques for Hyderabad district in India. The results of daily mean analysis revealed a rising trend in the number of days with severe AOD (> 1). Yearly mean AOD distribution showed a percentage increase of 45.31 % from 2002 to 2021. Furthermore, factor analysis was carried out to check for correlations of AOD and PM2.5 with various meteorological and pollutant variables. It was observed that both PM2.5 and AOD had significant weak to moderate (p < 0.05; r < 0.5) correlations with both pollutants and meteorological variables. The hybrid deep learning-based CNN-LSTM was identified as the best-fit model to predict AOD, outperforming MLP – ARIMA and MLP models. CNN – LSTM showed an R2 of 0.70, MAE of 0.08, MSE of 0.02 and RMSE of 0.14.

Hemispherically symmetric strategies for stratospheric aerosol injection

Abstract. Stratospheric aerosol injection (SAI) comes with a wide range of possible design choices, such as the location and timing of the injection. Different stratospheric aerosol injection strategies can yield different climate responses; therefore, understanding the range of possible climate outcomes is crucial to making informed future decisions on SAI, along with the consideration of other factors. Yet, to date, there has been no systematic exploration of a broad range of SAI strategies. This limits the ability to determine which effects are robust across different strategies and which depend on specific injection choices. This study systematically explores how the choice of SAI strategy affects climate responses in one climate model. Here, we introduce four hemispherically symmetric injection strategies, all of which are designed to maintain the same global mean surface temperature: an annual injection at the Equator (EQ), an annual injection of equal amounts of SO2 at 15° N and 15° S (15N+15S), an annual injection of equal amounts of SO2 at 30° N and 30° S (30N+30S), and a polar injection strategy that injects equal amounts of SO2 at 60° N and 60° S only during spring in each hemisphere (60N+60S). We compare these four hemispherically symmetric SAI strategies with a more complex injection strategy that injects different quantities of SO2 at 30° N, 15° N, 15° S, and 30° S in order to maintain not only the global mean surface temperature but also its large-scale horizontal gradients. All five strategies are simulated using version 2 of the Community Earth System Model with the middle atmosphere version of the Whole Atmosphere Community Climate model, version 6, as the atmospheric component, CESM2(WACCM6-MA), with the global warming scenario, Shared Socioeconomic Pathway (SSP)2-4.5. We find that the choice of SAI strategy affects the spatial distribution of aerosol optical depths, injection efficiency, and various surface climate responses. In addition, injecting in the subtropics produces more global cooling per unit injection, with the EQ and the 60N+60S cases requiring, respectively, 59 % and 50 % more injection than the 30N+30S case to meet the same global mean temperature target. Injecting at higher latitudes results in larger Equator-to-pole temperature gradients. While all five strategies restore Arctic September sea ice, the high-latitude injection strategy is more effective due to the SAI-induced cooling occurring preferentially at higher latitudes. These results suggest trade-offs wherein different strategies appear better or worse, depending on which metrics are deemed important.

Retrieval of aerosol optical depth over the Arctic cryosphere during spring and summer using satellite observations

Abstract. The climate in the Arctic has warmed much more quickly in the last 2 to 3 decades than at the mid-latitudes, i.e., during the Arctic amplification (AA) period. Radiative forcing in the Arctic is influenced both directly and indirectly by aerosols. However, their observation from ground or airborne instruments is challenging, and thus measurements are sparse. In this study, total aerosol optical depth (AOD) is determined from top-of-atmosphere reflectance measurements by the Advanced Along-Track Scanning Radiometer (AATSR) on board ENVISAT over snow and ice in the Arctic using a retrieval called AEROSNOW for the period 2003 to 2011. AEROSNOW incorporates an existing aerosol retrieval algorithm with a cloud-masking algorithm, alongside a novel quality-flagging methodology specifically designed for implementation in the high Arctic region (≥ 72∘ N). We use the dual-viewing capability of the AATSR instrument to accurately determine the contribution of aerosol to the reflection at the top of the atmosphere for observations over the bright surfaces of the cryosphere in the Arctic. The AOD is retrieved assuming that the surface reflectance observed by the satellite can be well parameterized by a bidirectional snow reflectance distribution function (BRDF). The spatial distribution of AOD shows that high values in spring (March, April, May) and lower values in summer (June, July, August) are observed. The AEROSNOW AOD values are consistent with those from collocated Aerosol Robotic Network (AERONET) measurements, with no systematic bias found as a function of time. The AEROSNOW AOD in the high Arctic was validated by comparison with ground-based measurements at the PEARL, OPAL, Hornsund, and Thule stations. The AEROSNOW AOD value is less than 0.15 on average, and the linear regression of AEROSNOW and AERONET total AOD yields a slope of 0.98, a Pearson correlation coefficient of R=0.86, and a root mean square error (RMSE) of =0.01 for the monthly scale in both spring and summer. The AEROSNOW observation of increased AOD values over the high Arctic cryosphere during spring confirms clearly that Arctic haze events were well captured by this dataset. In addition, the AEROSNOW AOD results provide a novel and unique total AOD data product for the springtime and summertime from 2003 to 2011. These AOD values, retrieved from spaceborne observation, provide a unique insight into the high Arctic cryospheric region at high spatial resolution and temporal coverage.

Quantitative assessment of the potential of optimal estimation for aerosol retrieval from geostationary weather satellites in the frame of the iAERUS‐GEO algorithm

AbstractSatellite remote sensing enables the study of atmospheric aerosols at large spatial scales, with geostationary platforms making this possible at sub‐daily frequencies. High‐temporal‐resolution aerosol observations can be made from geostationary data by using robust numerical inversion methods such as the widely‐used optimal estimation (OE) theory. This is the case of the instantaneous Aerosol and surfacE Retrieval Using Satellites in GEOstationary orbit (iAERUS‐GEO) algorithm, which successfully retrieves aerosol optical depth (AOD) maps from the Meteosat Second Generation weather satellite based on a simple implementation of the OE approach combined with the Levenberg–Marquardt method. However, the exact gain in inversion performances that can be obtained from the multiple and more advanced possibilities offered by OE is not well documented in the current literature. Against this background, this article presents the quantitative assessment of OE for the future improvement of the iAERUS‐GEO algorithm. To this end, we use a series of comprehensive experiments based on AOD maps retrieved by iAERUS‐GEO using different OE implementations, and ground‐based observations used as reference data. First, we assess the varying importance in the inversion process of satellite observations and a priori information according to the content of satellite aerosol information. Second, we quantify the gain of AOD estimation in log space versus linear space in terms of accuracy, AOD distribution and number of successful retrievals. Finally, we evaluate the accuracy improvement of simultaneous AOD and surface reflectance retrieval as a function of the regions covered by the Meteosat Earth's disk.

Estimation of hourly one square kilometer fine particulate matter concentration over Thailand using aerosol optical depth

In the recent years, concentration of fine particulate matter that are 2.5 microns or less in diameter (PM2.5) in Thailand has consistently exceeded the national ambient air quality standard. Currently, the measurement of PM2.5 concentration relies on air quality monitoring stations operated by the Pollution Control Department of Thailand (PCD). However, these stations are insufficient, particularly in rural areas, where agricultural open burning are major sources of pollution after harvesting period. This study aims to enhance the monitoring of PM2.5 concentration by leveraging cost-effective technologies. We propose the integration of satellite data, specifically Aerosol Optical Depth (AOD) from Multi-Angle Atmospheric Correction (MAIAC) product and Himawari-8 satellites, with the Weather Research and Forecasting Model (WRF) data, to provide supplementary data to the ground-based monitoring. Hourly 5 × 5 km2 AOD data from Himawari-8 were downscaled to a high-resolution of 1 × 1 km2, leveraging the AOD distribution pattern of the concurrent MAIAC product using eXtreme Gradient Boosting (XGBoost) model. Notably, during Thailand’s rainy season (May to August), the study observed a relative reduction in the training model’s R-square value. This phenomenon is attributed to temporal discrepancies between Himawari-8 and the MAIAC products during this period. The predictive models of PM2.5 concentrations with the identification of pertinent variables through Pearson’s correlation analysis and recursive feature elimination, driven by the robust XGBoost model. Subsequently, the downscaled AOD, wind speed, temperature, and pressure were identified as predictors for the estimation of hourly PM2.5 concentration. This comprehensive approach enabled the projection of PM2.5 levels across Thailand, encompassing over 600,000 grids at 1 × 1 km2 resolution. The developed models, thus, offer a valuable tool for robust and high-resolution PM2.5 concentration estimation, presenting significant implications for air quality monitoring and management in Thailand.

Long-Term MERRA-2 Reanalysis Data Indicate Atmospheric Environmental Changes for Three Major Concentrating-Solar-Power-Plant Project Areas in Xinjiang, China

The characteristics, distributions, and trends of the aerosol optical depth (AOD) and dust aerosol optical depth (DAOD) of three major concentrating solar power (CSP)-plant project areas (Hami, Turpan, and Ruoqiang) in Xinjiang, China were investigated and analyzed during 1980–2022 using the Modern-Era Retrospective analysis for Research and Applications Version 2 (MERRA-2) reanalysis products. The monthly variation, seasonal variation, inter-annual variation, distributions of AOD and DAOD, and proportions of dust in the aerosols in these three CSP-plant project areas were computed and analyzed. Overall, the annual mean AOD at 550 nm in the Turpan project area was the highest (0.20–0.36), while Ruoqiang had the lowest annual mean AOD at 550 nm (0.13–0.30), and the annual mean AOD at 550 nm in Hami was distributed between 0.17 and 0.33. After 2010, the change in the rate of the annual mean AOD showed an overall downward trend in Hami and Ruoqiang, indicating that the atmospheric environmental changes in both areas were more favorable for the operation of CSP plants. In the project areas of Hami, Turpan, and Ruoqiang, more than 90% of the AOD values were mainly in ranges 0.10–0.30, 0.10–0.35, and 0.05–0.30, respectively. As expected, the AOD values in spring and summer were significantly higher than those in autumn and winter in the three study areas. In spring, the dust contents (i.e., ratios of DAOD to AOD) were the highest, accounting for 64% (Hami), 67% (Turpan), and 69% (Ruoqiang) of the total aerosol contents. In all three areas, the proportions of dust in aerosols in spring have shown an increasing trend since 2000, suggesting that the negative impact of the dust on the power generation efficiency in these areas has gradually been increasing. Therefore, it is recommended that the CSP plants in Hami, Turpan, and Ruoqiang develop a strategy for cleaning heliostats, especially in spring, to reduce the impact of dust adhesion on the efficiency of the CSP plants.

Comprehensive Evaluation of Spatial Distribution and Temporal Trend of NO2, SO2 and AOD Using Satellite Observations over South and East Asia from 2011 to 2021

The past decade has witnessed remarkable economic development, marked by rapid industrialization and urbanization across Asian regions. This surge in economic activity has led to significant emissions, resulting in alarming levels of air pollution. Our study comprehensively assessed the spatial and temporal trends of key pollutants, namely nitrogen dioxide (NO2), sulfur dioxide (SO2), and aerosol (using aerosol optical depth (AOD) at 550 nm as an indicator), from 2011 to 2021. The data sources utilized include OMI onboard the Aura satellite for NO2 and SO2, as well as MODIS onboard Terra and Aqua satellites for AOD. The results from spatial and temporal trend analyses of the three parameters show that there is a clear declining trend over China and Republic of Korea (e.g., NO2 is declining with an overall rate of −7.8 × 1012 molecules/cm2/year over China) due to the strict implementation of air pollution control policies. However, it is essential to note that both countries still grapple with substantial pollution levels, with proportions exceeding 0.5, indicating that air quality is improving but has not yet reached a safe threshold. In contrast, South Asian regions, including Bangladesh, Pakistan, and India, are experiencing an increasing trend (e.g., NO2 is increasing with an overall rate of 1.2 × 1012 molecules/cm2/year in Bangladesh), primarily due to the lack of rigorous air pollution control policies. The average emissions of NO2 and SO2 were remarkably higher in winter than in summer. Notably, the identified hotspots are statistically significant and predominantly coincide with densely populated areas, such as the North China Plain (NCP). Furthermore, this study underscores the pivotal role of sector-wise emissions in air quality monitoring and improvement. Different cities are primarily influenced by emissions from specific sectors, emphasizing the need for targeted pollution control measures. The findings presented in this research contribute valuable insights to the air quality monitoring and improvement efforts in East and South Asian regions.

A new dataset of erodibility in dust source for WRF-Chem model based on remote sensing and soil texture - Application and Validation

The erodibility factor is an essential parameter in the WRF-Chem model that determines the amount of dust emission. However, current models that use erodibility data are assumed static and lack sufficient characterization of dust source regions' highly heterogeneous and dynamic nature. This results in significant errors and uncertainties in the dust simulation. To address this issue, we propose a new approach that involves developing a physically based erodibility dataset using soil moisture, vegetation coverage, soil texture, and land use data. This new dataset covers the entire globe with a 1 km resolution, which can represent dust sources in finer detail. The results of the dust simulations indicated that the new dataset considerably improved the model's overall performance. The evaluation results showed that the root-mean-square error (RMSE) of PM10 simulated with the new erodibility data was reduced by 32.4%, and the correlation coefficient (R) was increased by 82.4% compared to the default data. Additionally, the simulated spatial distribution of aerosol optical depth (AOD) is closer to that of the satellite AOD product. Our new data provide a more accurate description of the erodibility of dust source regions, refine the parameterization of dust emissions in the model, and ultimately improve dust prediction.

Uvsq-Sat NG, a New CubeSat Pathfinder for Monitoring Earth Outgoing Energy and Greenhouse Gases

Climate change is undeniably one of the most pressing and critical challenges facing humanity in the 21st century. In this context, monitoring the Earth’s Energy Imbalance (EEI) is fundamental in conjunction with greenhouse gases (GHGs) in order to comprehensively understand and address climate change. The French Uvsq-Sat NG pathfinder mission addresses this issue through the implementation of a Six-Unit CubeSat, which has dimensions of 111.3 × 36.6 × 38.8 cm in its unstowed configuration. Uvsq-Sat NG is a satellite mission spearheaded by the Laboratoire Atmosphères, Observations Spatiales (LATMOS), and supported by the International Satellite Program in Research and Education (INSPIRE). The launch of this mission is planned for 2025. One of the Uvsq-Sat NG objectives is to ensure the smooth continuity of the Earth Radiation Budget (ERB) initiated via the Uvsq-Sat and Inspire-Sat satellites. Uvsq-Sat NG seeks to achieve broadband ERB measurements using state-of-the-art yet straightforward technologies. Another goal of the Uvsq-Sat NG mission is to conduct precise and comprehensive monitoring of atmospheric gas concentrations (CO2 and CH4) on a global scale and to investigate its correlation with Earth’s Outgoing Longwave Radiation (OLR). Uvsq-Sat NG carries several payloads, including Earth Radiative Sensors (ERSs) for monitoring incoming solar radiation and outgoing terrestrial radiation. A Near-Infrared (NIR) Spectrometer is onboard to assess GHGs’ atmospheric concentrations through observations in the wavelength range of 1200 to 2000 nm. Uvsq-Sat NG also includes a high-definition camera (NanoCam) designed to capture images of the Earth in the visible range. The NanoCam will facilitate data post-processing acquired via the spectrometer by ensuring accurate geolocation of the observed scenes. It will also offer the capability of observing the Earth’s limb, thus providing the opportunity to roughly estimate the vertical temperature profile of the atmosphere. We present here the scientific objectives of the Uvsq-Sat NG mission, along with a comprehensive overview of the CubeSat platform’s concepts and payload properties as well as the mission’s current status. Furthermore, we also describe a method for the retrieval of atmospheric gas columns (CO2, CH4, O2, H2O) from the Uvsq-Sat NG NIR Spectrometer data. The retrieval is based on spectra simulated for a range of environmental conditions (surface pressure, surface reflectance, vertical temperature profile, mixing ratios of primary gases, water vapor, other trace gases, cloud and aerosol optical depth distributions) as well as spectrometer characteristics (Signal-to-Noise Ratio (SNR) and spectral resolution from 1 to 6 nm).

Spatio-temporal variations of aerosol optical depth over Ukraine under the Russia-Ukraine war

The ongoing Russia-Ukraine war has an impact on air quality in the contested region, but it is difficult to assess it during the war and to distinguish between weather conditions and anthropogenic impacts on air pollution. Aerosol optical depth (AOD) might be a way to indicate the regional air quality remotely. In this study, we analyze satellite-based MODIS Multi-Angle Implementation of Atmospheric Correction (MAIAC) AOD products to compare monthly mean AOD values before and during the war. By examining the spatial-temporal distribution of AOD in 2022 and comparing it with a baseline period from 2012 to 2021, we aim to assess the impact of the conflict. Our analysis employs a time series algorithm that decomposes long-term trends and seasonal variations, enabling us to identify AOD changes associated with the war-induced artificial perturbations. Additionally, we utilize satellite-based tropospheric NO2 data and nighttime lighting data as auxiliary sources to support the analysis of abnormal AOD changes resulting from the war. Furthermore, four parameters from Aerosol Robotic Network (AERONET) measurements in the Kyiv site, including angstrom exponent (AE), single scattering albedo (SSA), refractive index (RI), fine mode fraction (FMF) were exclusively discussed to explore the possible changes of aerosol physical-optical properties over Ukraine during the war. Results showed that air quality in Ukraine has been affected by the war in contradictory ways at different levels. At the national level, atmospheric pollution has dropped across Ukraine due to a decrease in the sources of air pollution emissions as a result of the suppression of economic and agricultural activities. Meanwhile, atmospheric air quality has deteriorated at the local scale where war is intense due to the large amounts of air pollutants emitted by explosions. Specifically, a significant decrease in AOD of 22.46% compared to the baseline period was observed across Ukraine in January and February 2022 before the war. Additionally, there was a column density reduction of over 10% for tropospheric NO2 compared to the same period in the previous year. Following the outbreak of the war on February 24, significant increases in AOD were observed in March when compared to the baseline period. Eastern Ukraine experienced a significant increase of 40.14%, while northern Ukraine and central Ukraine saw rises of 34.15% and 45.78%, respectively. In April, a wider distribution of areas with significantly high AOD values across Ukraine was observed compared to March. In July, widespread areas with anomalous low AOD appeared in northern and western Ukraine, likely due to a decrease in post-harvest agricultural burning caused by the war. In August, anomalous high AOD areas were observed in central Ukraine, possibly attributed to continued Russian long-range strikes and a new round of bombardments.

Evaluation and Comparison of Multi-Satellite Aerosol Optical Depth Products over East Asia Ocean.

The atmosphere over the ocean is an important research field that involves multiple aspects such as climate change, atmospheric pollution, weather forecasting, and marine ecosystems. It is of great significance for global sustainable development. Satellites provide a wide range of measurements of marine aerosol optical properties and are very important to the study of aerosol characteristics over the ocean. In this study, aerosol optical depth (AOD) data from seventeen AERONET (Aerosol Robotic Network) stations were used as benchmark data to comprehensively evaluate the data accuracy of six aerosol optical thickness products from 2013 to 2020, including MODIS (Moderate-resolution Imaging Spectrometer), VIIRS (Visible Infrared Imaging Radiometer Suite), MISR (Multi-Angle Imaging Spectrometer), OMAERO (OMI/Aura Multi-wavelength algorithm), OMAERUV (OMI/Aura Near UV algorithm), and CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) in the East Asian Ocean. In the East Asia Sea, VIIRS AOD products generally have a higher correlation coefficient (R), expected error within ratio (EE within), lower root mean square error (RMSE), and median bias (MB) than MODIS AOD products. The retrieval accuracy of AOD data from VIIRS is the highest in spring. MISR showed a higher EE than other products in the East Asian Ocean but also exhibited systematic underestimation. In most cases, the OMAERUV AOD product data are of better quality than OMAERO, and OMAERO overestimates AOD throughout the year. The CALIPSO AOD product showed an apparent underestimation of the AOD in different seasons (EE Below = 58.98%), but when the AOD range is small (0 < AOD < 0.1), the CALIPSO data accuracy is higher compared with other satellite products under small AOD range. In the South China Sea, VIIRS has higher data accuracy than MISR, while in the Bohai-Yellow Sea, East China Sea, Sea of Japan, and the western Pacific Ocean, MISR has the best data accuracy. MODIS and VIIRS show similar trends in R, EE within, MB, and RMSE under the influence of AOD, Angstrom exponent (AE), and precipitable water. The study on the temporal and spatial distribution of AOD in the East Asian Ocean shows that the annual variation of AOD is different in different sea areas, and the ocean in the coastal area is greatly affected by land-based pollution. In contrast, the AOD values in the offshore areas are lower, and the aerosol type is mainly clean marine type aerosol. These findings can help researchers in the East Asian Ocean choose the most accurate and reliable satellite AOD data product to better study atmospheric aerosols' impact and trends.

Spatiotemporal Variations of Aerosol Optical Depth and the Spatial Heterogeneity Relationship of Potential Factors Based on the Multi-Scale Geographically Weighted Regression Model in Chinese National-Level Urban Agglomerations

Investigating the spatiotemporal variation characteristics of aerosol optical depth (AOD) and its driving factors is essential for assessing atmospheric environmental quality and alleviating air pollution. Based on a 22-year high-resolution AOD dataset, the spatiotemporal variations of AOD in mainland China and ten national urban agglomerations were explored based on the Mann–Kendall trend test and Theil–Sen median method. Random forest (RF) and multiscale geographically weighted regression (MGWR) were combined to identify the main driving factors of AOD in urban agglomerations and to reveal the spatial heterogeneity of influencing factors. The results showed that areas with high annual average AOD concentrations were mainly concentrated in the Chengdu–Chongqing, Central Plains, Shandong Peninsula, and Middle Yangtze River urban agglomerations. Southern Beijing–Tianjin–Hebei and its surrounding areas revealed the highest AOD pollution during summer, whereas the worst pollution during the remaining three seasons occurred in the Chengdu–Chongqing urban agglomeration. Temporally, except for the Ha-Chang and Mid-Southern Liaoning urban agglomerations, where the average annual AOD increased, the other urban agglomerations showed a decreasing trend. Among them, the Central Plains, Middle Yangtze River, Guanzhong Plain, and Yangtze River Delta urban agglomerations all exhibited a decline greater than 20%. According to the spatial trends, most urban agglomerations encompassed much larger areas of decreasing AOD values than areas of increasing AOD values, indicating that the air quality in most areas has recently improved. RF analysis revealed that PM2.5 was the dominant factor in most urban clusters, followed by meteorological factors. MGWR results show that the influencing factors have different spatial scale effects on AOD in urban agglomerations. The socioeconomic factors and PM2.5 showed strong spatial non-stationarity with regard to the spatial distribution of AOD. This study can provide a comprehensive understanding of AOD differences among urban agglomerations, and it has important theoretical and practical implications for improving the ecological environment and promoting sustainable development.

Spatiotemporal changes of aerosol optical depth and its response to urbanization: a case study of Jinan City, China, 2009-2018.

With the insidiously growing impact of urban development on the environment, the issue of air quality has attracted extensive attention nationally and globally. It is of great significance to study the influence of urbanization on air quality for the rational development of cities. MODIS-MAIAC (Moderate Resolution Imaging Spectroradiometer-Multi-Angle Implementation of Atmospheric Correction) Aerosol optical depth (AOD) product, DMSP/OLS (Defense Meteorological Satellite Program/Operational Linescan System) and NPP/VIIRS (Suomi National Polar-orbiting Partnership/Visible Infrared Imaging Radiometer Suite) night-light were used to explore the spatiotemporal variation and correlation between AOD and urbanization development before and after the promulgation of environmental governance policies in Jinan City from 2009 to 2018. Results show that (1) the spatial distribution of AOD in Jinan had the characteristics of high in the north and low in the south, high in the west and low in the east, and low in some parts of the central region; there was a significant seasonal variation in time, with the highest AOD in summer and the lowest in winter. During 2009-2013, the annual average variation of AOD increased by 20.6%, while during 2014-2018, it decreased by 35.3%; (2) The distribution of night-light in Jinan City has progressively expanded, mirroring the city's ongoing development. The spatial distribution of aerosols in urban areas was relatively low compared to the surrounding areas of the city. (3) From 2009 to 2013, there existed a significant positive correlation between the spatial and temporal distribution of AOD and night-light. However, from 2014 to 2018, with the implementation of environmental governance policies, this relationship shifted to a significant negative correlation between the spatial and temporal distribution of AOD and night-light. Through an analysis of the correlation between urban development and aerosol depth in Jinan City over the past decade, it can be concluded that urban development does not inevitably result in elevated AOD levels. Notably, the Jinan government has achieved remarkable results in controlling the atmospheric environment, as evidenced by recent years' improvements.

Characterization of the aerosol vertical distributions and their impacts on warm clouds based on multi-year ARM observations

Aerosol vertical distribution plays a crucial role in cloud development and thus precipitation since both aerosol indirect and semi-direct effects significantly depend on the relative position of aerosol layer in reference to cloud, but its precise influence on cloud remains unclear. In this study, we integrated multi-year Raman Lidar measurements of aerosol vertical profiles from the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) facility with available Value-Added Products of cloud features to characterize aerosol vertical distributions and their impacts on warm clouds over the continental and marine ARM atmospheric observatories, i.e., Southern Great Plains (SGP) and Eastern North Atlantic (ENA). A unimodal seasonal distribution of aerosol optical depths (AODs) with a peak in summer is found at upper boundary layer over SGP, while a bimodal distribution is observed at ENA for the AODs at lower levels with a major winter-spring maximum. The diurnal mean of upper-level AOD at SGP shows a maximum in the early evening. According to the relative positions of aerosol layers to clouds we further identify three primary types of aerosol vertical distribution, including Random, Decreasing, and Bottom. It is found that the impacts of aerosols on cloud may or may not vary with aerosol vertical distribution depending on environmental conditions, as reflected by the wide variations of the relations between AOD and cloud properties. For example, as AOD increases, the liquid water paths (LWPs) tend to be reduced at SGP but enhanced at ENA. The relations of cloud droplet effective radius with AOD largely depend on aerosol vertical distributions, particularly showing positive values in the Random type under low-LWP condition (<50 g m−2). The distinct features of aerosol-cloud interactions in relation to aerosol vertical distribution are likely attributed to the continental-marine contrast in thermodynamic environments and aerosol conditions between SGP and ENA.

Spatial distribution of aerosols burden and evaluation of changes in aerosol optical depth using multi-approach observations in tropical region

Understanding of Aerosol optical depth (AOD) parameter is important for air quality assessment. This study aims to evaluate and validate AOD measurements from combine datasets to improve air quality for a period 2005–2020 using Aerosol Robotic Network (AERONET) at Ilorin site (8.320° N, 4.340° E) in Nigeria. AOD outputs from Community Atmosphere Model Version 6 with chemistry (CAM6-chem) at 1° horizontal resolution and Modern-Era Retrospective analysis for Research and Applications (MERRA-2) are investigated in addition to validation of two satellites AOD retrievals: Moderate Resolution Imaging Spectroradiometer (MODIS) and Multi-angle Imaging Spectroradiometer (MISR). Result of spatial distribution of AOD shows high values > 1 in the North and Western Sahara compared to Central Africa. Desert dust shows largest contribution in the North and Western Africa that is up to 2 magnitude larger than other aerosol types. Primary organic matter (POM) and secondary organic aerosols (SOAs) both presents high burdens with later been dominant at around 10° band, and black carbon (BC) largest burden (2.6 × 10 − 5 kgm − 2) is seen in the model from oil and gas exploration site in Nigeria. Inter-comparison of MERRA/MISR/MODIS and AERONET AOD using linear correlation of the seasonal dependence demonstrated high correlation (r = 0.864 − 0.973) subjected to Root Mean Square Error (RMSE = 0.069 − 0.211), suggesting good agreement between the datasets. When compared to seasonal mean maximum AERONET AOD value of 0.978 MERRA is ∼5%, MISR ∼28% and MODIS ∼29% lower with stronger correlations observed in the wet and pre-harmattan seasons. Similarly, MODEL AOD at 550 nm and dust burden were found to be ∼34% and ∼67% lower in context to AERONET AOD annual mean value of 0.627. Positive relationships that indicate an upward slope exist between all the computed datasets with moderate value of AERONET/CAM-chem spearman partial correlation, and MERRA/MODIS and MODIS/MISR showing strong and significant relationship with p-value less than 0.05. Low variance is observed with all measurements except in MERRA.

Analysis and Validation of the Aerosol Optical Depth of MODIS Products in Gansu Province, Northwest China

The accurate determination of aerosol optical depth (AOD) is of great importance for climate change research and environmental monitoring. To understand the applicability of the MODIS aerosol product inversion algorithm in Gansu Province, this work uses ground-based solar photometer AOD observation data to validate the MODIS C6 version of the AOD product. Additionally, the retrieval accuracy of MODIS C6 Deep Blue (DB) algorithm AOD products and Deep Blue and Dark Target Fusion (DB–DT combined) algorithm AOD products for Gansu Province when setting different spatial sampling windows is compared and analyzed. Meanwhile, the monitoring effects of these two AOD algorithms in typical polluted atmospheric conditions in Gansu Province are compared. The results show that (1) the correlation between the MODIS AOD products of the two algorithms and the ground-based observation data decreases with an increasing spatial sampling window size. When the spatial sampling window of the two algorithms is set at 30 km × 30 km, it is more representative of the AOD value in Gansu Province, thus reflecting local characteristics. (2) When the spatial sampling window is set at 30 km × 30 km, the inversion effect of the DB algorithm AOD is better than that of the DB–DT combined algorithm AOD on different underlying surfaces. (3) The seasonal variability in the inversion accuracy of the DB algorithm AOD is less than that of the DB–DT combined algorithm, and it has inversion advantages in spring, autumn and winter, while the DB–DT combined algorithm outperforms the DB algorithm only in winter. The inversion effect of the two algorithms on AOD is influenced by the spatial sampling window setting. (4) Both the DB algorithm AOD and the DB–DT combined algorithm AOD can monitor the distribution of AOD in the central and western regions of Gansu, especially for high values of AOD under polluted atmospheric conditions, which represents a good monitoring effect. However, the two algorithms perform poorly in monitoring the southeast region of Gansu, while there is a discontinuous AOD distribution in the northwest region of Gansu. Overall, the MODIS DB algorithm AOD product has higher applicability in Gansu Province. This work provides a good reference for local air pollution and climate prediction.

Long-term spatiotemporal variation in atmospheric aerosol properties over Türkiye based on MERRA-2 reanalysis data: aerosol classification based on city type.

Due to their complex aerosol characteristics, it is crucial to analyze the trends and properties of atmospheric aerosols over the eastern Mediterranean countries. This study comprehensively evaluates Aerosol Optical Depth (AOD) and Angström Exponent (AE) trends and aerosol classification over Türkiye, using the MERRA-2 reanalysis data from 1980 to 2019. The spatial distributions of AOD and AE were determined across various temporal scales, including multiannual, 5-year intervals, seasonal, and monthly periods. The analysis of the spatial distribution of AOD values revealed that the mean values in the northwestern areas, ranging from 0.20 to 0.25, were comparatively higher than those observed in the eastern regions, which ranged from 0.10 to 0.15. Between 1980 and 1994, the AOD values gradually increased, followed by a subsequent decline from 1995 to 2019. Based on 5-year intervals between 1980 and 2019, the coastal regions exhibited higher AOD values than the inland areas. Specifically, higher AOD values were noted between May and August, whereas lower values were observed during autumn and winter. Additionally, higher AE values were detected over the northwestern region, while the southeastern region had the lowest AE values, particularly during spring, attributed to the frequent occurrence of dust transport events in this area. The AOD and AE values were also examined in different city types, using the population thresholds of the European Commission. The global city category consisting only of Istanbul showed the highest AOD values across all seasons, while the category of very small cities, which includes 12 cities, had the lowest AOD values. Furthermore, this study investigated the contributions of dominant aerosol categories across various city types based on multiannual and seasonal variations of AOD and AE. The results showed that mixed and continental aerosols had higher portions across all city types. However, biomass burning/industrial and mixed aerosol categories were more prominent in global and large cities. Overall, this study provides a comprehensive overview of the atmospheric aerosol properties in Türkiye and can serve as a useful guide for researchers intending to conduct future studies utilizing AOD and AE data obtained through MERRA-2 aerosol diagnosis.

High-Resolution Aerosol Optical Depth Retrieval in Urban Areas Based on Sentinel-2

In this paper, an improved aerosol optical depth (AOD ) retrieval algorithm is proposed based on Sentinel-2 and AErosol RObotic NETwork (AERONET ) data. The surface reflectance for AOD retrieval was estimated from the image that had minimal aerosol contamination in a temporal window determined by AERONET data. Validation of the Sentinel-2 AOD retrievals was conducted against four Aerosol Robotic Network (AERONET ) sites located in Beijing. The results show that the Sentinel-2 AOD retrievals are highly consistent with the AERONET AOD measurements (R = 0.942), with 85.56% falling within the expected error. The mean absolute error and the root-mean-square error are 0.0688 and 0.0882, respectively. In addition, the AOD distribution map obtained by this algorithm well reflects the fine-spatial-resolution changes in AOD distribution. These results suggest that the improved high-resolution AOD retrieval algorithm is robust and has the potential advantage of retrieving high-resolution AOD over urban areas.

Coupling Coordination Degree of AOD and Air Pollutants in Shandong Province from 2015 to 2020

In order to reveal the correlation between aerosols and pollution indicators, the MODIS aerosol optical depth (AOD) was used to investigate the distribution of AOD in 16 prefecture-level cities in Shandong Province from 2015 to 2020. This study quantitatively analyzed the coupling degree and the coupling coordination degree between AOD and pollution indicators based on the coupling coordination model. The results showed that: (1) The annual average AOD in Shandong Province showed a rapid downward trend with a mean value of 0.615. The seasonal AOD of Shandong Province and prefecture-level cities was characterized by spring and summer &gt; autumn and winter. The distribution of AOD in Shandong Province showed a spatial pattern of high in the west and low in the east, and high in the surrounding area and low in the middle. The decreasing rate of AOD was high in the west and low in the east. (2) The annual average AOD and Air Quality Index (AQI) were in a highly coupled and coordinated state. Their spatial distribution pattern decreased from west to east. There were certain fluctuations with seasonal changes, with the largest fluctuation in winter. (3) Except for O3, the overall coupling and coordination level between AOD and each pollutant was relatively high. The coupling coordination effect was as follows: C (PM2.5, AOD) and C (PM10, AOD) &gt; C (NO2, AOD) &gt; C (SO2, AOD), and C (CO, AOD) &gt; C (O3, AOD). Except for the O3, its distribution was characterized by highs in the west and lows in the east. The degree of coupling between each pollution indicator and the seasonal average AOD was high. The study showed that there was a high degree of coupling and coordination between pollutant concentration indicators and AOD, and remote sensing AOD data can be used as an effective supplement to regional pollutant monitoring indicators.

The Role of Midlatitude Cyclones in the Emission, Transport, Production, and Removal of Aerosols in the Northern Hemisphere

AbstractWe examine the distribution of aerosol optical depth (AOD) across 27,707 northern hemisphere (NH) midlatitude cyclones for 2005–2018 using retrievals from the Moderate Resolution Spectroradiometer (MODIS) sensor on the Aqua satellite. Cyclone‐centered composites show AOD enhancements of 20%–45% relative to background conditions in the warm conveyor belt (WCB) airstream. Fine mode AOD accounts for 68% of this enhancement annually. Relative to background conditions, coarse mode AOD is enhanced by more than a factor of two near the center of the composite cyclone, co‐located with high surface wind speeds. Within the WCB, MODIS AOD maximizes in spring, with a secondary maximum in summer. Cyclone‐centered composites of AOD from the Modern Era Retrospective analysis for Research and Applications, version 2 Global Modeling Initiative (M2GMI) simulation reproduce the magnitude and seasonality of the MODIS AOD composites and enhancements. M2GMI simulations show that the AOD enhancement in the WCB is dominated by sulfate (37%) and organic aerosol (25%), with dust and sea salt each accounting for 15%. MODIS and M2GMI AOD are 60% larger in North Pacific WCBs compared to North Atlantic WCBs and show a strong relationship with anthropogenic pollution. We infer that NH midlatitude cyclones account for 355 Tg yr−1 of sea salt aerosol emissions annually, or 60% of the 30–80°N total. We find that deposition within WCBs is responsible for up to 35% of the total aerosol deposition over the NH ocean basins. Furthermore, the cloudy environment of WCBs leads to efficient secondary sulfate production.