Dirac Fluid Research Articles

Electronic interactions in Dirac fluids visualized by nano-terahertz spacetime interference of electron-photon quasiparticles.

Ultraclean graphene at charge neutrality hosts a quantum critical Dirac fluid of interacting electrons and holes. Interactions profoundly affect the charge dynamics of graphene, which is encoded in the properties of its electron-photon collective modes: surface plasmon polaritons (SPPs). Here, we show that polaritonic interference patterns are particularly well suited to unveil the interactions in Dirac fluids by tracking polaritonic interference in time at temporal scales commensurate with the electronic scattering. Spacetime SPP interference patterns recorded in terahertz (THz) frequency range provided unobstructed readouts of the group velocity and lifetime of polariton that can be directly mapped onto the electronic spectral weight and the relaxation rate. Our data uncovered prominent departures of the electron dynamics from the predictions of the conventional Fermi-liquid theory. The deviations are particularly strong when the densities of electrons and holes are approximately equal. The proposed spacetime imaging methodology can be broadly applied to probe the electrodynamics of quantum materials.

(Invited) Flow of Charge and Heat in Ultra-Clean Graphene

Over the past two decades our understanding of the charge and heat transport properties of graphene has evolved progressively as the quality of graphene devices improved. In this talk, I shall present some new experimental result on the electrical and thermal transport measurements in graphene devices of unprecedented electrical mobility (> 1 million cm2/V.s). We show that the transport in such graphene devices is limited by intrinsic acoustic phonons and their scattering with electrons, rather than charged impurities – which is the case in conventional disordered graphene devices. This manifests in a rather striking violation of the Wiedemann-Franz law and density-dependent variation of the effective Lorenz number over six orders of magnitude. We find that the transport properties of ultra-clean graphene are quantitatively consistent with that of a hydrodynamic Dirac fluid.

Investigation of transport properties of graphene Dirac fluid by holographic two-current axion coupling model

Recently, there has been great interest in the phenomenon of severe violation of the Wiedemann–Franz law in graphene Dirac fluids around 75 K, due to the strong coupling relativistic plasma near the neutral point, where traditional perturbation theory fails. To explain this phenomenon, this article proposes a holographic dual two-current axion coupling model, describing the interaction between electrons and holes in graphene near the charge neutrality point (CNP) and revealing the related physical mechanism. The study shows that the holographic two-current model aligns with experimental results at 100 μ\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\upmu $$\\end{document}m-2\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$^{-2}$$\\end{document}, and correctly predicts conductivity as temperature increases. Additionally, the article explores the behavior of β+γ\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\beta +\\gamma $$\\end{document} and its impact on conductivity and thermal conductivity. The results suggest a frictional effect between electrons and holes. Consequently, this study provides us with a clearer understanding of the properties of graphene Dirac fluids and further confirms the reliability of the holographic duality method.

Holographic hydrodynamics of tilted Dirac materials

We present a gravity dual to a quantum material with tilted Dirac cone in 2+1 dimensional spacetime. In this many-body system the electronics degrees of freedom are strongly-coupled, constitute a Dirac fluid and admit an effective hydrodynamic description. The holographic techniques are applied to compute the thermodynamic variables and hydrodynamic transports of a fluid on the boundary of an asymptotically anti de Sitter spacetime with a boosted black hole in the bulk. We find that these materials exhibit deviations from the normal Dirac fluid which rely on the tilt of the Dirac cone. In particular, the shear viscosity to entropy density ratio is reduced and the KSS bound is violated in this system. This prediction can be experimentally verified in two-dimensional quantum materials (e.g. organic α-(BEDT-TTF)2I3 and 8Pmmn borophene) with tilted Dirac cone.

Minimal one-dimensional model of bad metal behavior from fast particle-hole scattering

A strongly interacting plasma of linearly dispersing electron and hole excitations in two spatial dimensions (2D), also known as a Dirac fluid, can be captured by relativistic hydrodynamics and shares many universal features with other quantum critical systems. We propose a one-dimensional (1D) model to capture key aspects of the 2D Dirac fluid while including lattice effects and being amenable to non-perturbative computation. When interactions are added to the Dirac-like 1D dispersion without opening a gap, we show that this kind of irrelevant interaction is able to preserve Fermi-liquid-like quasi-particle features while relaxing a zero-momentum charge current via collisions between particle-hole excitations, leading to resistivity that is linear in temperature via a mechanism previously discussed for large-diameter metallic carbon nanotubes. We further provide a microscopic lattice model and obtain numerical results via density-matrix renormalization group (DMRG) simulations, which support the above physical picture. The limits on such fast relaxation at strong coupling are of considerable interest because of the ubiquity of bad metals in experiments.

Observation of hydrodynamic plasmons and energy waves in graphene.

Thermally excited electrons and holes form a quantum-critical Dirac fluid in ultraclean graphene and their electrodynamic responses are described by a universal hydrodynamic theory. The hydrodynamic Dirac fluid can host intriguing collective excitations distinctively different from those in a Fermi liquid1-4. Here we report the observation of the hydrodynamic plasmon and energy wave in ultraclean graphene. We use the on-chip terahertz (THz) spectroscopy technique to measure the THz absorption spectra of a graphene microribbon as well as the propagation of the energy wave in graphene close to charge neutrality. We observe a prominent high-frequency hydrodynamic bipolar-plasmon resonance and a weaker low-frequency energy-wave resonance of the Dirac fluid in ultraclean graphene. The hydrodynamic bipolar plasmon is characterized by the antiphase oscillation of massless electrons and holes in graphene. The hydrodynamic energy wave is an electron-hole sound mode with both charge carriers oscillating in phase and moving together. The spatial-temporal imaging technique shows that the energy wave propagates at a characteristic speed of [Formula: see text] near the charge neutrality2-4. Our observations open new opportunities to explore collective hydrodynamic excitations in graphene systems.

Wiedemann-Franz law in graphene

We analyze a well-known experimental work [J. Crossno et al., Science 351, 1058 (2016)] which reported on the failure of the Wiedemann-Franz law in graphene at $T\ensuremath{\sim}10\text{--}100\phantom{\rule{4pt}{0ex}}\mathrm{K}$, attributing this failure to the non-Fermi liquid nature of the Dirac fluid associated with undoped intrinsic graphene. In spite of serious theoretical efforts, the reported observations remain unexplained. Our detailed quantitative analysis based on Fermi liquid considerations, which apply to extrinsic doped graphene, establishes that one possible explanation for the reported observations is the opening of a gap at the Dirac point, induced perhaps by the boron nitride substrate. We suggest that more experiments are necessary to resolve the issue, and we believe that the experiment may not actually have anything to do with Dirac fluid hydrodynamics but relates to finite-temperature low-density bipolar diffusive transport by electrons and holes in the presence of short- and long-range disorder, and phonons.

Vortical effects in Dirac fluids with vector, chiral and helical charges

Helicity of free massless Dirac fermions is a conserved, Lorentz-invariant quantity at the level of the classical equations of motion. For a generic ensemble consisting of particles and antiparticles, the helical and chiral charges are different conserved quantities. The flow of helicity can be modelled by the helicity current, which is again conserved in the absence of interactions. Similar to the axial vortical effect which generates an axial (chiral) current, the helicity current is induced by vorticity in a finite temperature medium with vector (electrical) charge imbalance via the helical vortical effects, leading to new nondissipative transport phenomena. These phenomena lead to the appearance of a new hydrodynamic excitation, the helical vortical wave. Our results suggest the existence of a new type of triangle anomalies in QED which involve the helicity currents in addition to the standard vector and axial currents. Further exploiting the conservation of the helical current, we show that a finite helical chemical potential may be used to characterise thermodynamic ensembles of fermions similarly to, but independently of, the vector charge and chirality. We derive the pressure P for fermions at finite vector, axial and helical chemical potentials and show that the quantities arising in anomalous transport, including various vortical and circular conductivities and the shear-stress coefficients, can be obtained by differentiation of P with respect to the appropriate chemical potentials. Finally, we calculate the helicity relaxation time in the quark-gluon plasma above the crossover and show that it is similar to that for the axial charge.

Electronic viscosity and energy relaxation in neutral graphene

We explore hydrodynamics of Dirac fermions in neutral graphene in the Corbino geometry. In the absence of a magnetic field, the bulk Ohmic charge flow and the hydrodynamic energy flow are decoupled. However, the energy flow does affect the overall resistance of the system through viscous dissipation and energy relaxation that has to be compensated by the work done by the current source. Solving the hydrodynamic equations, we find that local temperature and electric potential are discontinuous at the interfaces with the leads as well as the device resistance and argue that this makes Corbino geometry a feasible choice for an experimental observation of the Dirac fluid.

Interlayer Electron-Hole Friction in Tunable Twisted Bilayer Graphene Semimetal.

Charge-neutral conducting systems represent a class of materials with unusual properties governed by electron-hole (e-h) interactions. Depending on the quasiparticle statistics, band structure, and device geometry these semimetallic phases of matter can feature unconventional responses to external fields that often defy simple interpretations in terms of single-particle physics. Here we show that small-angle twisted bilayer graphene (SA TBG) offers a highly tunable system in which to explore interactions-limited electron conduction. By employing a dual-gated device architecture we tune our devices from a nondegenerate charge-neutral Dirac fluid to a compensated two-component e-h Fermi liquid where spatially separated electrons and holes experience strong mutual friction. This friction is revealed through the T^{2} resistivity that accurately follows the e-h drag theory we develop. Our results provide a textbook illustration of a smooth transition between different interaction-limited transport regimes and clarify the conduction mechanisms in charge-neutral SA TBG.

Coulomb Drag between a Carbon Nanotube and Monolayer Graphene.

We have measured Coulomb drag between an individual single-walled carbon nanotube (SWNT) as a one-dimensional (1D) conductor and the two-dimensional (2D) conductor monolayer graphene, separated by a few-atom-thick boron nitride layer. The graphene carrier density is tuned across the charge neutrality point (CNP) by a gate, while the SWNT remains degenerate. At high temperatures, the drag resistance changes sign across the CNP, as expected for momentum transfer from drive to drag layer, and exhibits layer exchange Onsager reciprocity. We find that layer reciprocity is broken near the graphene CNP at low temperatures due to nonlinear drag response associated with temperature dependent drag and thermoelectric effects. The drag resistance shows power-law dependences on temperature and carrier density characteristic of 1D Fermi liquid-2D Dirac fluid drag. The 2D drag signal at high temperatures decays with distance from the 1D source slower than expected for a diffusive current distribution, suggesting additional interaction effects in the graphene in the hydrodynamic transport regime.

Observation of giant and tunable thermal diffusivity of a Dirac fluid at room temperature

Conducting materials typically exhibit either diffusive or ballistic charge transport. When electron–electron interactions dominate, a hydrodynamic regime with viscous charge flow emerges1–13. More stringent conditions eventually yield a quantum-critical Dirac-fluid regime, where electronic heat can flow more efficiently than charge14–22. However, observing and controlling the flow of electronic heat in the hydrodynamic regime at room temperature has so far remained elusive. Here we observe heat transport in graphene in the diffusive and hydrodynamic regimes, and report a controllable transition to the Dirac-fluid regime at room temperature, using carrier temperature and carrier density as control knobs. We introduce the technique of spatiotemporal thermoelectric microscopy with femtosecond temporal and nanometre spatial resolution, which allows for tracking electronic heat spreading. In the diffusive regime, we find a thermal diffusivity of roughly 2,000 cm2 s−1, consistent with charge transport. Moreover, within the hydrodynamic time window before momentum relaxation, we observe heat spreading corresponding to a giant diffusivity up to 70,000 cm2 s−1, indicative of a Dirac fluid. Our results offer the possibility of further exploration of these interesting physical phenomena and their potential applications in nanoscale thermal management.

Homogenization of hydrodynamic transport in Dirac fluids

Large-scale electrical and thermal currents in ordinary metals are well approximated by effective medium theory: global transport properties are governed by the solution to homogenized coupled diffusion equations. In some metals, including the Dirac fluid of nearly charge neutral graphene, microscopic transport is not governed by diffusion, but by a more complicated set of linearized hydrodynamic equations, which form a system of degenerate elliptic equations coupled with the Stokes equation for fluid velocity. In sufficiently inhomogeneous media, these hydrodynamic equations reduce to homogenized diffusion equations. We re-cast the hydrodynamic transport equations as the infimum of a functional over conserved currents, and present a functional framework to model and compute the homogenized diffusion tensor relating electrical and thermal currents to charge and temperature gradients. We generalize to this system two well-known results in homogenization theory: Tartar's proof of local convergence to the homogenized theory in periodic and highly oscillatory media, and sub-additivity of the above functional in random media with highly oscillatory, stationary and ergodic coefficients.

Nonlocal hydrodynamic transport and collective excitations in Dirac fluids

We study the response of a Dirac fluid to electric fields and thermal gradients at finite wave-numbers and frequencies in the hydrodynamic regime. We find that non-local transport in the hydrodynamic regime is governed by infinite set of kinetic modes that describe non-collinear scattering events in different angular harmonic channels. The scattering rates of these modes $\tau_{m}^{-1}$ increase as $\|m\|$, where $m$ labels the angular harmonics. In an earlier publication, we pointed out that this dependence leads to anomalous, L\'evy-flight-like phase space diffusion (Phys. Rev. Lett. 123, 195302 (2019)). Here, we show how this surprisingly simple, non-analytic dependence allows us to obtain exact expressions for the non-local charge and electronic thermal conductivities. The peculiar dependence of the scattering rates on $m$ also leads to a non-trivial structure of collective excitations: Besides the well known plasmon, second sound and diffusive modes, we find non-degenerate damped modes corresponding to excitations of higher angular harmonics. We use these results to investigate the transport of a Dirac fluid through Poiseuille-type geometries of different widths, and to study the response to surface acoustic waves in graphene-piezoelectric devices.

Imaging viscous flow of the Dirac fluid in graphene

The electron-hole plasma in charge-neutral graphene is predicted to realize a quantum critical system in which electrical transport features a universal hydrodynamic description, even at room temperature1,2. This quantum critical 'Dirac fluid' is expected to have a shear viscosity close to a minimum bound3,4, with an interparticle scattering rate saturating1 at the Planckian time,the shortest possible timescale for particles to relax. Although electrical transport measurements at finite carrier density are consistent with hydrodynamic electron flow in graphene5-8, a clear demonstration of viscous flow at the charge-neutrality point remains elusive. Here we directly image viscous Dirac fluid flow in graphene at room temperature by measuring the associated stray magnetic field. Nanoscale magnetic imaging is performed using quantum spin magnetometers realized with nitrogen vacancy centres in diamond. Scanning single-spin and wide-field magnetometry reveal a parabolic Poiseuille profile for electron flow in a high-mobility graphene channel near the charge-neutrality point, establishing the viscous transport of the Dirac fluid. This measurement is in contrast to the conventional uniform flow profile imaged in a metallic conductor and also in a low-mobility graphene channel. Via combined imaging and transport measurements, we obtain viscosity and scattering rates, and observe that these quantities are comparable to the universal values expected at quantum criticality. This finding establishes a nearly ideal electron fluid in charge-neutral, high-mobility graphene at room temperature4. Our results will enable the study of hydrodynamic transport in quantum critical fluids relevant to strongly correlated electrons in high-temperature superconductors9. This work also highlights the capability of quantum spin magnetometers to probe correlated electronic phenomena at the nanoscale.

Joule—Thomson Cooling in Graphene

Electrons in graphene exhibit hydrodynamic behavior in a certain range of temperatures. We indicate that electric current in this regime can result in cooling of electron fluid due to the Joule-Thomson effect. Cooling occurs in the Fermi liquid regime, while for the Dirac fluid the effect results in heating.

Noncontact Mutual-Inductance-Based Measurement of an Inhomogeneous Topological Insulating State in Bi2Se3 Single Crystals with Defects

Nonmagnetic disorder in a topological insulator (TI) often dopes the material with extra electrical charges, creating a normal electron fluid coexisting with the exotic Dirac electron fluid. As both of these fluids conduct electricity, conventional transport measurements are not convenient for studying the Dirac electron fluid. Therefore the authors develop a technique in which a TI with disorder (here Bi${}_{2}$Se${}_{3}$ with Se vacancies) is used to inductively couple two coils. With this setup they are not only able to specifically identify the contribution from currents induced in the Dirac fluid, but also unravel a complex, temperature-dependent interplay between the two electron fluids.

Enhanced ponderomotive force in graphene due to interband resonance

We analyze intrinsic nonlinearities in two-dimensional (2D) polaritonic materials interacting with an optical wave. Focusing on the case of graphene, we show that the second-order nonlinear optical conductivity due to carrier density fluctuations associated with the excitation of a plasmon polariton is closely related to the ponderomotive force due to the oscillating optical field. A recent study (Sun et al 2018 Proc. Natl Acad. Sci. USA 115 3285–9) derived this force in the hydrodynamic regime of a generic Dirac fluid, and suggested that inclusion of interband transitions could have interesting implications. Here we reproduce the Drude-like result in a more general fashion on the basis of thermodynamics, which makes extension to other regimes straightforward. We find that for zero temperature a diverging nonlinearity is found at the interband threshold. By including finite-temperature effects this is regularized, but remains quite significant even at room temperature. Going further beyond, we include nonlocal corrections as a second potential source of regularization, and find that they do not lead to broadening (as one would usually expect e.g. due to Landau damping), but rather to a splitting of the ponderomotive interband resonance, providing a very characteristic signature of nonlocality. Our analysis should prove useful to the open quest for exploiting nonlinearities in graphene and other 2D polaritonic materials, through effects such as photon drag.

Effects of dissipation on solitons in the hydrodynamic regime of graphene

We use hydrodynamic techniques to analyze the one-dimensional propagation of solitons in gated graphene on an arbitrary uniform background current. Results are derived for both the Fermi liquid and Dirac fluid regimes. We find that these solutions satisfy the Korteweg-de Vries-Burgers equation. Viscous dissipation and ohmic heating are included, causing the solitons to decay. Experiments are proposed to measure this decay and thereby quantify the shear viscosity in graphene.

Quantum-critical conductivity of the Dirac fluid in graphene.

Graphene near charge neutrality is expected to behave like a quantum-critical, relativistic plasma-the "Dirac fluid"-in which massless electrons and holes collide at a rapid rate. We used on-chip terahertz spectroscopy to measure the frequency-dependent optical conductivity of clean, micrometer-scale graphene at electron temperatures between 77 and 300 kelvin. At charge neutrality, we observed the quantum-critical scattering rate characteristic of the Dirac fluid. At higher doping, we detected two distinct current-carrying modes with zero and nonzero total momenta, a manifestation of relativistic hydrodynamics. Our work reveals the quantum criticality and unusual dynamic excitations near charge neutrality in graphene.