Diode-pumped Alkali Vapor Lasers Research Articles

Fast online rubidium DPAL atomic concentration measurement by 420 nm probe laser.

The alkali atom concentration plays an important role in the performance of a diode pumped alkali vapor laser (DPAL). At the rubidium DPAL operational region, the alkali concentration is as high as 1013-1014cm-3, which is "optically thick," or opaque, for the 780 nm or 795 nm doublet D lines when the traditional scanning absorption spectrum method is used for concentration measurement. To solve this problem, we propose the use of a probe laser of 420 nm, which corresponds to the 52S1/2 to 62P3/2 transition and has a lower absorption cross section compared to the D-line doublet. Due to the moderate absorption strength at a fixed 420 nm probe wavelength, we realized fast, online measurement of the Rb concentration in a real-world DPAL. By combining it with the quasi-two-level model, we further provided the population distribution in the lower three energy levels. This fast, online diagnostic method could be well applied in DPAL concentration measurement, and could show the dynamics of a laser's performance.

Picosecond evolution of pulsed and CW alkali vapor lasers: laser oscillation buildup.

Investigation of the kinetic principle of a diode-pumped alkali vapor laser (DPAL) is key to achieve multifunctional DPALs. In this work, we propose a spatiotemporal model, which combines the time-dependent rate equations of population densities and propagation equations of energies to study the dynamic processes from turn-on to steady-state in DPALs. Time evolution of population densities and pump and laser intensity are resolved on a picosecond time scale to study the build-up process of laser oscillations. For nanosecond-pulse pumping, we obtain a laser pulse of 1.6 ns and a delay time of 2.6 ns at an incident pulse width of 2 ns. This pulse can be stretched by increasing the pump pulse width and delayed by applying a more extended cavity. For CW operation, spiking and relaxation oscillations resulting from a dynamic balance of gain and losses are demonstrated to be much faster than other types of lasers.

Investigation of dual-wavelength pump schemes for optically pumped rare gas lasers.

Optically pumped rare gas lasers (OPRGLs) have shown great potential to generate high energy laser radiation with high beam quality. As an alternative to the diode-pumped alkali vapor lasers (DPALs), they have similar working principles and characteristics, but OPRGLs have the advantage that the gain medium is chemically inert and is appropriate for closed-cycle operation. One of the challenges OPRGLs are faced with is the bottleneck caused by the slow 1s4-1s5 collisional relaxations at room temperature. A 1s4-2p10 dual-wavelength pump method had been proposed to transfer the populations pooled on the 1s4 level to the lasing cycle using a steady-state laser model. We explored this method further through 1s4-2p8 and 1s4-2p7 dual-wavelength pump schemes. The enhancement efficiencies at room temperature for a repetitively pulsed discharge, CW dual-wavelength pump system were examined using a dynamic model, and an experiment with a pulsed secondary pump was conducted for qualitative evaluations.

高功率循环流动型半导体泵浦碱金属蒸汽激光器研究进展（特邀）

高功率循环流动型半导体泵浦碱金属蒸汽激光器研究进展（特邀）

高功率循环流动型半导体泵浦碱金属蒸汽激光器研究进展（特邀）

高功率循环流动型半导体泵浦碱金属蒸汽激光器研究进展（特邀）

Hyperfine-state dependence of highly efficient amplification from diode-pumped cesium vapor.

We report optical amplification with an optical-to-optical conversion efficiency of 70 ± 1% from a diode-pumped Cs vapor cell. When pump (852 nm; D2-line) and signal (895 nm; D1-line) lasers with a narrow spectral width of ∼2 MHz are resonant on the hyperfine states (F = 3 or 4) of the 6S1/2 state, we observe that the amplification factors are significantly changed according to the hyperfine-state combination of the pump and signal lasers. We find that the optical frequencies of the pumping and signal lasers need to be controlled near the hyperfine state of 6S1/2 (F = 4) to obtain an efficient diode-pumped alkali amplifier (DPAA). To realize highly efficient optical gain conditions, both the spatial modes of the pump and signal lasers are made to overlap in the Cs vapor cell with the use of a single-mode optical fiber. An amplification factor of 430 ± 15 is achieved under the following conditions: cell temperature of 90 °C, signal power of 0.1 mW, and pump power of 200 mW. We believe that our results can aid in the development of highly efficient diode-pumped alkali-vapor lasers and amplifiers.

Pulse operation of linearly polarized diode-pumped cesium-vapor laser based on acousto-optical modulation.

We present a pulse linearly polarized diode-pumped cesium-vapor laser (Cs-DPAL) based on an acousto-optical modulator (AOM) for the first time. The continuous wave (CW) performance of the Cs-DPAL was first investigated, and ~1.05 W linearly polarized CW laser was obtained. Next, we applied a rectangular signal to modulate the AOM. The Cs-DPAL realized a pulse laser output with a maximum repetition rate of 1 MHz and minimum pulse duration of 238 ns. To the best of our knowledge, this is the highest repetition rate reported thus far for a diode-pumped alkali-vapor laser (DPAL). The maximum output power of the pulse laser reached ~0.20 W, and the corresponding Mx 2 and My 2 factors were 1.31 and 1.19, respectively. Finally, we realized code modulation of the Cs-DPAL, with a maximum bit rate of 2 Mb/s.

Dual-wavelength end-pumped Rb-Cs vapor lasers.

Diode-pumped alkali vapor lasers (DPALs) have been rapidly developed because of their excellent performances. However, there have been few reports about DPALs with multiple wavelengths until now. The effects of the output features on the waist size and position of both Rb and Cs pump beams were first theoretically investigated using a kinetic model for an end-pumped dual-wavelength Rb-Cs laser. Then, a continuous-wave (CW) laser was experimentally constructed. Finally, the hybrid CW-modulated output with two wavelengths was also successfully obtained for the first time in development of alkali lasers. The results might be helpful in applications for laser communication and ranging/radar in the future.

Emission spectral diagnosis of argon-helium plasma produced by radio frequency capacitive discharge

Optically pumped metastable rare-gas laser (OPRGL) have been proposed to overcome the shortcomings of diode-pumped alkali-vapor laser in the recent years. The OPRGL promises to realize high-scale output. But how to achieve enough particle density of metastable atoms is still an open problem. Usually, plasma produced by discharge serves as a gain medium of the OPRGL. Here in this paper, we are to reveal the effects of different discharge parameters on the plasma properties, such as particle density of metastable argon atoms. Gas discharge at a radio frequency of 13.56 MHz is adopted to excite argon atoms. Emission spectrum is employed to study argon and helium radio frequency discharge of optically pumped argon laser at high pressure, different powers of discharge and various content of argon. Gas temperature is obtained by analyzing rotational spectrum (A2∑+ → X2Π) of OH radical generated by residual water vapor and comparing simulated spectrum with the measured spectrum. The electronic excitation temperature relating to electron temperature is obtained by the method of Boltzmann's plot. Stark broadening of the spectrum is used to determine the electron density. The results show that gas temperature rises slightly with the increase of pressure and varies little with content and discharge power changing. The electronic excitation temperature increases with the decrease of pressure evidently and decreases slightly with the increase of content. The electron density is on the order of 1015 cm-3 under various conditions controlled by us. Long time discharge test reveals that residual water vapor can lead to the decrease of electron temperature, and thus reducing the yield of argon metastable state. In conclusion, considering that the higher gas temperature can improve the collision relaxation rate of helium and argon, and the higher electron temperature can improve the rate of production of argon metastable state. Thus a proposal is put forward that appropriately heating gas and reducing gas pressure can obtain higher particle density of metastable argon. Furthermore, It can be found from these results that heating and cleaning the gas during discharge may be candidate methods to obtain and sustain the higher particle density in the plasma.

Three-dimensional kinetic and fluid dynamic modeling and three iterative algorithms for side-pumped alkali vapor lasers

Combining the kinetic and fluid dynamic processes in static and flowing-gas diode-pumped alkali vapor lasers, a comprehensive physical model with three cyclically iterative algorithms for simulating the three-dimensional pump and laser intensities as well as temperature distribution in the vapor cell of side-pumped alkali vapor lasers is established. Comparison with measurement of a static side-pumped cesium vapor laser with a diffuse type hollow cylinder cavity, and with classical and modified models is made. Influences of flowed velocity and pump power on laser power are calculated and analyzed. The results have demonstrated that for high-power side-pumped alkali vapor lasers, it is necessary to take into account the three-dimensional distributions of pump energy, laser energy and temperature in the cell to simultaneously obtain the thermal features and output characteristics. Therefore, the model can deepen the understanding of the complete kinetic and fluid dynamic mechanisms of a side-pumped alkali vapor laser, and help with its further experimental design.

Modeling of time evolution of power and temperature in single-pulse and multi-pulses diode-pumped alkali vapor lasers.

A physical model combining rate, power propagation, and transient heat conduction equations for diode-pumped alkali vapor lasers (DPAL) is applied to a pulsed Rb-CH4 DPAL, which agrees well with the time evolution of laser power and temperature measured by K absorption spectroscopy. The output feature and temperature rise of a multi-pulse DPAL are also calculated in the time domain, showing that if we energize the pump light when the temperature rise decays to 1/2, rather than 1/e of its maximum, we can increase the duty cycle and obtain more output energy. The repetition rate of >100Hz is high enough to achieve QCW (quasi-continuous-wave) laser pulses.

Modeling of Steady-State Temperature Distribution in Diode-Pumped Alkali Vapor Lasers: Analysis of the Experimental Results

Combining the first-order ordinary differential equations of pump and laser power and the second-order ordinary differential equation of temperature, an optical model for diode-pumped alkali vapor lasers in two pumped configurations, is reported. This model, taking into account the axial distributions of pump and laser beam radii and the radial distributions of intensities and temperature, shows good agreement between the calculated and experimental results. An observed maximum temperature rise of ~58 K corresponding to a pump power of 20 W is reproduced, and a wide region of heat source density of quenching is predicted by the model. The heat production of relaxation and of quenching are demonstrated to be within an order of magnitude, indicating that quenching is as important as relaxation in the temperature calculation. It can also be deduced that the peak of the temperature profile is mainly dominated by relaxation, whereas its width can be attributed to thermal diffusion and quenching. In addition, dependencies of laser and thermal power on the pump beam waist are calculated, and an optimal ratio of 0.7 between the pump and laser beam waist is obtained.

Modeling of pulsed Cs vapor lasers in transversely pumped configuration

By means of combining the transverse differential equation of pump intensity and the longitudinal differential equation of laser power, an optical model for transversely pumped diode-pumped alkali vapor lasers (DPALs) is established. The spatial distributions of both radius and intensities are considered in the model for pump and laser beams. The simulation results are in good agreement with the experiment ones as compared to the reported pulsed transversely pumped Cs DPALs. Influences of pump power, temperature, cell length, and beam waist on output performance are investigated, which suggests a set of parameters for efficient DPAL operation. In particular, the optimal ratio of the beam waist between the laser and pump beam is demonstrated to be 0.81, which can increase the laser power by 85% larger than the current experimental result.

Comparative study of diode-pumped alkali vapor laser and exciplex-pumped alkali laser systems and selection principal of parameters

A theoretical model based on common pump structure is proposed to analyze the output characteristics of a diode-pumped alkali vapor laser (DPAL) and XPAL (exciplex-pumped alkali laser). Cs-DPAL and Cs-Ar XPAL systems are used as examples. The model predicts that an optical-to-optical efficiency approaching 80% can be achieved for continuous-wave four- and five-level XPAL systems with broadband pumping, which is several times the pumped linewidth for DPAL. Operation parameters including pumped intensity, temperature, cell’s length, mixed gas concentration, pumped linewidth, and output coupler are analyzed for DPAL and XPAL systems based on the kinetic model. In addition, the predictions of selection principal of temperature and cell’s length are also presented. The concept of the equivalent “alkali areal density” is proposed. The result shows that the output characteristics with the same alkali areal density but different temperatures turn out to be equal for either the DPAL or the XPAL system. It is the areal density that reflects the potential of DPAL or XPAL systems directly. A more detailed analysis of similar influences of cavity parameters with the same areal density is also presented.

Removal of Rb(6(2)P) by H(2), CH(4), and C(2)H(6).

The saturated hydrocarbons methane and ethane are often used as collisional energy transfer agents in diode-pumped alkali vapor lasers (DPALs). Problems are encountered because the hydrocarbons eventually react with the optically pumped alkali atoms, resulting in the contamination of the gas lasing medium and damage of the gas cell windows. The reactions require excitation of the more highly excited states of the alkali atoms, which can be generated in DPAL systems by energy pooling processes. Knowledge of the production and loss rates for the higher excited states is needed for a quantitative understanding of the photochemistry. In the present study, we have used experimental and theoretical techniques to characterize the removal of Rb(6P2) by hydrogen, methane, and ethane.

Experimental evaluation of temperature distribution of a vapor cell using a Hilbert transform procedure

A diode-pumped alkali vapor laser (DPAL) is one of the most promising candidates of the next-generation high-powered laser source. As the saturated number density of alkali vapor is highly dependent on the temperature inside a vapor cell, the temperature distribution in the cross-section of a cell will greatly affect the homogeneity of a laser medium and the output characteristics of a DPAL. In this paper, we developed an algorithm based on the regime concluding quasi-Hilbert transform to evaluate the phase aberration of a wavefront when the probe beam passes through the vapor cell placed in one arm of a Mach–Zehnder interference setup. According to the theoretical algorithm, we deduced the temperature distribution of a cesium vapor cell for different heating conditions. The study is thought to be useful for development of a high-powered laser.

Theoretical model and simulations for a cw exciplex pumped alkali laser.

The Exciplex Pumped Alkali Laser (XPAL) system, which is similar to DPAL (Diode Pumped Alkali vapor Laser), has been demonstrated in mixtures of Cs vapor, Ar, with and without ethane. Unlike DPAL, it uses the broadband absorption blue satellite of the alkali D2 line, created by naturally occuring collision pairs. For example, Cs-Ar collision pairs have an absorption width which is as wide as the one of commercial semiconductor diode lasers. A continuous wave XPAL four-level theoretical model is presented in this paper. More factors are considered, such as the spectral dependence of pumped laser absorption for broadband pumping and the longitudinal population variation. Some intra-cavity details, such as longitudinal distributions of pumped laser and alkali laser, can also be solved well. The predictions of optical-to-optical efficiency as a function of temperature and pumped laser intensity are presented. The model predicts that there is an optimum value of temperature or pumped laser intensity. The analysis of the influence of cell length on optical-to-optical efficiency shows that a better performance can be achieved when using longer cell. The prediction of influence of Ar concentration and reflectivity of output coupler shows that higher optical-to-optical efficiency could be achieved if lower reflectivity of output coupler and higher Ar concentration are used. The optical-to-optical efficiency as high as 84% achieved by optimizing configuration with the pumped intensity of 5 × 10⁷ W/cm² presented shows that broadband pumped four-level XPAL system has a potential of high optical-to-optical efficiency.

Kinetics of optically pumped Kr metastables.

Optically-pumped atomic gas lasers that utilize metastable excited states of rare gas atoms (Rg(*)) have been demonstrated using both pulsed and CW pump sources. These devices resemble diode-pumped alkali vapor lasers, but have the advantage of using a chemically inert lasing medium. Collisional energy transfer is needed to sustain a population inversion, and He is used as the transfer agent. Consequently, values for the Kr(*)+He state-to-state energy transfer rate constants are needed for the analysis and prediction of laser performance characteristics. In the present study, we report He energy transfer rate constants for Kr(*) in the 5p[5/2](2), 5p[5/2](3), 5p[1/2](1), and 5s[3/2](1) states.

Modeling of a diode four-side symmetrically pumped alkali vapor amplifier.

Considering the amplified spontaneous emission, the saturation effect and the energy distributions of the incident pump and seed lasers, a physical model is established to describe the kinetic process and the output performance of a four sided diode pumped alkali vapor laser amplifier. According to the experimental parameters of a single-side pumped configuration with a diffuse type hollow cylinder cavity, energy distributions in the cell and influences of several important factors are simulated and analyzed. The model is validated by comparing the simulation result with the experimental data, which shows the model can provide an effective way for designing an efficient diode four-side symmetrically pumped alkali vapor laser amplifier.

考虑抽运光空间分布的半导体抽运碱金属蒸气激光器的模拟计算

考虑抽运光空间分布的半导体抽运碱金属蒸气激光器的模拟计算