The low rank and sparse representation (LRSR) technique has attracted increasing attention for hyperspectral anomaly detection (HAD). Although a large quantity of research based on LRSR for HAD is proposed, the detection performance is still limited, due to the unsatisfactory dictionary construction and insufficient consideration of global and local characteristics. To tackle the above-mentioned concern, a novel HAD method, termed dual collaborative constraints regularized low-rank and sparse representation via robust dictionaries construction, is proposed in this article. Concretely, a robust dictionary construction strategy, which thoroughly excavates the potential of the density estimation model and local outlier factor, is proposed to yield pure and representative dictionary atoms. To fully exploit the global and local characteristics of hyperspectral images, dual collaborative constraints corresponding to the background and anomaly components are imposed on the LRSR model. Notably, two weighted matrices are further exerted on the representation coefficients to improve the effect of collaborative constraints, considering the fact that the surrounding pixels similar to the testing pixel should be given a large weight, otherwise the weight is expected to be small. In this way, the background and anomaly components can be well modeled. Additionally, a nonlinear transformation operation, which combines the output of the density estimation model and local outlier factor with the detection result derived from the LRSR model, is developed to suppress the background. The experiments conducted on one simulated dataset and three real datasets demonstrate the superiority of the proposed method compared with the four typical methods and four state-of-the-art methods.