Single-particle Density Of States Research Articles

Electrodynamics of the Superconducting State in Ultra-Thin Films at THz Frequencies

We report on terahertz frequency-domain spectroscopy (THz-FDS) experiments in which we measure charge carrier dynamics and excitations of thin-film superconducting systems at low temperatures in the THz spectral range. The characteristics of the set-up and the experimental procedures are described comprehensively. We discuss the single-particle density of states and a theory of electrodynamic absorption and optical conductivity of conventional superconductors. We present the experimental performance of the setup at low temperatures for a broad spectral range from 0.1 - 1.1 THz by the example of ultra-thin films of weakly disordered superconductors niobium nitride (NbN) and tantalum nitride (TaN) with different values of critical temperatures. Furthermore, we analyze and interpret our experimental data within the framework of conventional Bardeen-Cooper-Schrieffer (BCS) theory of superconductivity.

C-axis resistivity, pseudogap, superconductivity, and Widom line in doped Mott insulators

Layered doped Mott insulators, such as the cuprates, show unusual temperature dependence of the resistivity. Intriguingly, the resistivity perpendicular to the CuO$_2$ planes, $\rho_c(T)$, shows both metallic ($d\rho_c/dT > 0$) and semi-conducting ($d\rho_c/dT<0$) behavior. We shed light on this puzzle by calculating $\rho_c$ for the two-dimensional Hubbard model within plaquette cellular dynamical mean-field theory and strong-coupling continuous-time quantum Monte Carlo as the impurity solver. The temperature, $T$, and doping, $\delta$, dependencies of $\rho_c$ are controlled by the first-order transition between pseudogap and correlated metal phases from which superconductivity can emerge. On the large doping side of the transition $\rho_c(T)$ is metallic, while on the low-doping side $\rho_c(T)$ changes from metallic to semi-conducting behavior with decreasing $T$. As a function of doping, the jump in $\rho_c$ across the first-order transition evolves into a sharp crossover at higher temperatures. This crossover coincides with the pseudogap temperature $T^*$ in the single-particle density of states, the spin susceptibility and other observables. Such coincidence in crossovers is expected along the continuation of the first-order transition into the super-critical regime, called the Widom line. This implies that not only the dynamic and the thermodynamic properties but also the DC transport in the normal state are governed by the hidden first-order transition. $\rho_c(T)$ has a high-temperature quasi-linear regime where it can exceed the Mott-Ioffe-Regel limit and when it has a minimum it is nearly parallel to the Widom line.

Pseudogap Phenomena of an Ultracold Fermi Gas with a P-wave Feshbach Resonance

We investigate pseudogap phenomena in an ultracold Fermi gas with a p-wave tunable pairing interaction. Including p-wave pairing fluctuations within a strong-coupling T-matrix theory, we calculate the single-particle density of states (DOS) above the superfluid transition temperature Tc. Starting from the weak-coupling regime, we show that, at first, a dip structure gradually appears to become remarkable in DOS with increasing the strength of the p-wave pairing interaction at Tc. However, this pseudogap structure again becomes less remarkable to eventually disappear, as one passes through the intermediate coupling regime to enter the strong-coupling region. This non-monotonic interaction dependence of the pseudogap is quite different from the s-wave case, where the pseudogap size simply increases with increasing a s-wave interaction strength. This difference is found to originate from the momentum dependence of the p-wave interaction. We also determine the pseudogap temperature below which the dip structure in DOS appears and identify the pseudogap regime in the phase diagram of a Fermi gas with respect to the temperature and p-wave interaction strength.

Excitations in a quantum spin liquid with random bonds

We present results of inelastic neutron scattering study on two bond disordered quasi twodimensional quantum magnets (C$_4$H$_12$N$_2$)Cu$_2$(Cl$_{1-x}$Br$_x$)$_6$ with x=0.035 and 0.075. We observe the increase of spin gap, reduction of magnon bandwidth and a decrease of magnon lifetimes compared to x=0 sample. Additional magnon damping is observed at higher energies away from zone center which is found to follow the density of single particle states.

Coulomb Gap Triptych in a Periodic Array of Metal Nanocrystals

The Coulomb gap in the single-particle density of states (DOS) is a universal consequence of electron-electron interaction in disordered systems with localized electron states. Here we show that in arrays of monodisperse metallic nanocrystals, there is not one but three identical adjacent Coulomb gaps, which together form a structure that we call a "Coulomb gap triptych." We calculate the DOS and the conductivity in two- and three-dimensional arrays using a computer simulation. Unlike in the conventional Coulomb glass models, in nanocrystal arrays the DOS has a fixed width in the limit of large disorder. The Coulomb gap triptych can be studied via tunneling experiments.

Quantum Coulomb gap in low dimensions

We study the single-particle density of states of one-dimensional and two-dimensional quantum disordered systems with long-range interactions. We consider a $1/\sqrt{r}$ interaction in one dimension and a Coulomb interaction in two dimensions, which produce linear gaps in the density of states in both cases. We focus on the strong localization regime where the localization length is small but non-zero. We use an exact diagonalization technique for small system sizes and a perturbation approach for larger sizes. We find that, with both methods, the inclusion of a finite hopping contribution does not change the linear character of the gap, but reduces its slope, widening the gap.

Atypical BCS-BEC crossover induced by quantum-size effects

Quantum-size oscillations of the basic physical characteristics of a confined fermionic condensate are a well-known phenomenon. Its conventional understanding is based on the single-particle physics, whereby the oscillations follow the size-dependent changes in the single-particle density of states. Here we present a study of a cigar-shaped ultracold superfluid Fermi gas, which demonstrates an important many-body aspect of the quantum-size effects, overlooked previously. The many-body physics is revealed in the atypical crossover from the Bardeen-Cooper-Schrieffer (BCS) superfluid to the Bose-Einstein condensate (BEC) induced by the size quantization of the particle motion. Quantized perpendicular spectrum results in the formation of single-particle subbands (shells) so that the aggregate fermionic condensate becomes a coherent mixture of subband condensates. Each time when the lower edge of a subband crosses the chemical potential, the BCS-BEC crossover is approached in this subband, and the aggregate condensate contains both the BCS and BEC-like components.

Microscopic theory for a ferromagnetic nanowire/superconductor heterostructure: Transport, fluctuations, and topological superconductivity

Motivated by the recent experiment of Wang et al. [Nature Physics 6, 389 (2010)], who observed a highly unusual transport behavior of ferromagnetic Cobalt nanowires proximity-coupled to superconducting electrodes, we study proximity effect and temperature-dependent transport in such a mesoscopic hybrid structure. It is assumed that the asymmetry in the tunneling barrier gives rise to the Rashba spin-orbit-coupling in the barrier that enables induced p-wave superconductivity in the ferromagnet to exist. We first develop a microscopic theory of Andreev scattering at the spin-orbit-coupled interface, derive a set of self-consistent boundary conditions, and find an expression for the p-wave minigap in terms of the microscopic parameters of the contact. Second, we study temperature-dependence of the resistance near the superconducting transition and find that it should generally feature a fluctuation-induced peak. The upturn in resistance is related to the suppression of the single-particle density of states due to the formation of fluctuating pairs, whose tunneling is suppressed. In conclusion, we discuss this and related setups involving ferromagnetic nanowires in the context of one-dimensional topological superconductors. It is argued that to realize unpaired end Majorana modes, one does not necessarily need a half-metallic state, but a partial spin polarization may suffice. Finally, we propose yet another related class of material systems -- ferromagnetic semiconductor wires coupled to ferromagnetic superconductors -- where direct realization of Kitaev-Majorana model should be especially straightforward.

Elementary excitations and avalanches in the Coulomb glass

We study numerically the statistics of elementary excitations and charge avalanches in the classical Coulomb glass model of localized charges with unscreened Coulomb interaction and disorder. We compute the single-particle density of states with an energy minimization algorithm for systems of up to 1003 sites. The shape of the Coulomb gap is consistent with a power-law with exponent δ ≃ 2.4 and marginally consistent with exponential behavior. The results are also compared with a recently proposed self-consistent approach. We then analyze the size distribution of the charge avalanches produced by a small perturbation of the system. We show that the distribution decays as a power law in the limit of large system size, and explain this behavior in terms of the elementary excitations. Similarities and differences with the scale-free avalanches observed in mean-field spin glasses are discussed.

Effect of nonlocal interactions on the disorder-induced zero-bias anomaly in the Anderson-Hubbard model

To expand the framework available for interpreting experiments on disordered strongly correlated systems, and in particular to explore further the strong-coupling zero-bias anomaly found in the Anderson-Hubbard model, we ask how this anomaly responds to the addition of nonlocal electron-electron interactions. We use exact diagonalization to calculate the single-particle density of states of the extended Anderson-Hubbard model. We find that for weak nonlocal interactions the form of the zero-bias anomaly is qualitatively unchanged. The energy scale of the anomaly continues to be set by an effective hopping amplitude renormalized by the nonlocal interaction. At larger values of the nonlocal interaction strength, however, hopping ceases to be a relevant energy scale and higher energy features associated with charge correlations dominate the density of states.

Direct probe of the variability of Coulomb correlation in iron pnictide superconductors

We use core-valence-valence Auger spectra to probe the Coulomb repulsion between holes in the valence band of Fe pnictide superconductors. By comparing the two-hole final-state spectra to density functional theory calculations of the single-particle density of states, we extract a measure of the electron correlations that exist in these systems. Our results show that the Coulomb repulsion is highly screened and can definitively be considered as weak. We also find that there are differences between the 1111 and 122 families and even a small variation as a function of the doping $x$ in Ba(Fe${}_{1\ensuremath{-}x}$Co${}_{x}$)${}_{2}$As${}_{2}$. We discuss how the values of the hole-hole Coulomb repulsion obtained from our study relate to the onsite Coulomb parameter $U$ used in model and first-principles calculations based on dynamical mean field theory and establish an upper bound for its effective value. Our results impose stringent constraints on model-based phase diagrams that vary with the quantity $U$ or $U$/$W$ by restricting the latter to a rather small range of values.

Pseudogap phenomenon in an ultracold Fermi gas with ap-wave pairing interaction

We investigate single-particle properties of a one-component Fermi gas with a tunable p-wave interaction. Including pairing fluctuations associated with this anisotropic interaction within a $T$-matrix theory, we calculate the single-particle density of states, as well as the spectral weight, above the superfluid transition temperature $T_{\rm c}$. Starting from the weak-coupling regime, we show that the so-called pseudogap first develops in these quantities with increasing the interaction strength. However, when the interaction becomes strong to some extent, the pseudogap becomes obscure to eventually disappear in the strong-coupling regime. This non-monotonic interaction dependence is quite different from the case of an s-wave interaction, where the pseudogap simply develops with increasing the interaction strength. The difference between the two cases is shown to originate from the momentum dependence of the p-wave interaction, which vanishes in the low momentum limit. We also identify the pseudogap regime in the phase diagram with respect to the temperature and the p-wave interaction strength. Since the pseudogap is a precursor phenomenon of the superfluid phase transition, our results would be useful for the research toward the realization of p-wave superfluid Fermi gases.

Character of valence-band states in the Kondo surface alloys CeAgx/Ag(111) and CePt5/Pt(111)

The crystal and electronic structures of the CePt${}_{5}$ and CeAg${}_{x}$ surface alloys have been investigated by means of low-energy electron diffraction and angle-resolved photoelectron spectroscopy. From measurements performed near the $4d$-$4f$ absorption edge we were able to infer the weight of the $4f$-electron spectral function with respect to the single-particle density of states. While the typical Kondo features at the Fermi energy (Kondo resonance and spin-orbit partner) in the CePt${}_{5}$ surface alloy were observed, only the ${f}^{0}$ ionization structure and the spin-orbit partner were present in the CeAg${}_{x}$ case. From our experiments, and by comparison to model calculations, we were able to estimate the Kondo temperature in the two systems and investigate parameters contributing to the hybridization strength.

Observations of plasmarons in a two-dimensional system: Tunneling measurements using time-domain capacitance spectroscopy

Calculations of the single-particle density of states (SPDOS) of electron liquids have long predicted that there exist two distinct charged excitations: the usual quasiparticle consisting of an electron or hole, and a plasmaron consisting of a hole resonantly bound to real plasmons in the Fermi sea. Using tunneling spectroscopy to measure the SPDOS of a 2D electronic system, we demonstrate the detection of a plasmaron in a 2D system in which electrons have mass. With the application of a magnetic field we discover unpredicted magnetoplasmarons which resemble Landau levels with a negative index.

Vortex line in spin-orbit coupled atomic Fermi gases

It has recently been shown that the spin-orbit coupling gives rise to topologically nontrivial and thermodynamically stable gapless superfluid phases when the pseudospin populations of an atomic Fermi gas are imbalanced, with the possibility of featuring Majorana zero-energy quasiparticles. In this paper, we consider a Rashba-type spin-orbit coupling, and use the Bogoliubov-de Gennes formalism to analyze a single vortex line along a finite cylinder with a periodic boundary condition. We show that the signatures for the appearance of core- and edge-bound states can be directly found in the density of single-particle states and particle-current density. In particular, we find that the pseudospin components counterflow near the edge of the cylinder, the strength of which increases with increasing spin-orbit coupling.

Formation of magnetic impurities and pair-breaking effect in a superfluid Fermi gas

We theoretically investigate the introduction of magnetic impurities into a superfluid Fermi gas. In the presence of a population imbalance (${N}_{\ensuremath{\uparrow}}&gt;{N}_{\ensuremath{\downarrow}}$, where ${N}_{\ensuremath{\sigma}}$ is the number of Fermi atoms with pseudospin $\ensuremath{\sigma}=\ensuremath{\uparrow},\ensuremath{\downarrow}$), we show that nonmagnetic potential scatterers embedded in the system are magnetized in the sense that some of the excess spin-$\ensuremath{\uparrow}$ atoms are localized around them. They destroy the superfluid order parameter around them, as in the case of the magnetic impurity effect discussed in the superconductivity literature. This pair-breaking effect naturally leads to localized excited states below the superfluid excitation gap. To confirm our idea in a simple manner, we consider an attractive Fermi-Hubbard model within the mean-field theory at $T=0$. We determine consistent superfluid properties around a nonmagnetic impurity, such as the superfluid order parameter, local population imbalance, as well as the single-particle density of states, in the presence of a population imbalance. Since competition between superconductivity and magnetism is one of the most fundamental problems in condensed-matter physics, our results would be useful for the study of this important issue in cold Fermi gases.

Electronic structure of an antiferromagnetic metal: CaCrO3

We report on the electronic structure of the perovskite oxide CaCrO3 using valence-band, core-level, and Cr 2p - 3d resonant photoemission spectroscopy (PES). Despite its antiferromagnetic order, a clear Fermi edge characteristic of a metal with dominant Cr 3d character is observed in the valence band spectrum. The Cr 3d single particle density of states are spread over 2 eV, with the photoemission spectral weight distributed in two peaks centered at ~ 1.2 eV and 0.2 eV below EF, suggestive of the coherent and incoherent states resulting from strong electron-electron correlations. Resonant PES across the Cr 2p - 3d threshold identifies a 'two-hole' correlation satellite and yields an on-site Coulomb energy U ~4.8 eV. The metallic DOS at EF is also reflected through the presence of a well-screened feature at low binding energy side of the Cr 2p core-level spectrum. X-ray absorption spectroscopy (XAS) at Cr L3,2 and O K edges exhibit small temperature dependent changes that point towards a small change in Cr-O hybridization. The multiplet splitting in Cr 2p core level spectrum as well as the spectral shape of the Cr XAS can be reproduced using cluster model calculations which favour a negative value for charge transfer energy between the Cr 3d and O 2p states. The overall results indicate that CaCrO3 is a strongly hybridized antiferromagnetic metal, lying in the regime intermediate to Mott-Hubbard and charge-transfer systems.

Theory of Electron Transport near Anderson–Mott Transitions

We present a theory of the DC electron transport in insulators near Anderson-Mott transitions under the influence of coexisting electron correlation and randomness. At sufficiently low temperatures, the DC electron transport in Anderson-Mott insulators is determined by the single-particle density of states (DOS) near the Fermi energy. Anderson insulators, caused by randomness, are characterized by a nonzero DOS at the Fermi energy. However, recently, the authors proposed that coexisting randomness and short-ranged interaction in insulators open a soft Hubbard gap in the DOS, and the DOS vanishes only at the Fermi energy. Based on the picture of the soft Hubbard gap, we derive a formula for the critical behavior for the temperature dependence of the DC resistivity. Comparisons of the present theory with experimental results of electrostatic carrier doping into an organic conductor kappa-(BEDT-TTF)_2Cu[N(CN)_2]Br demonstrate the evidence for the present soft-Hubbard scaling.

Density of states in an optical speckle potential

We study the single particle density of states of a one-dimensional speckle potential, which is correlated and non-Gaussian. We consider both the repulsive and the attractive cases. The system is controlled by a single dimensionless parameter determined by the mass of the particle, the correlation length and the average intensity of the field. Depending on the value of this parameter, the system exhibits different regimes, characterized by the localization properties of the eigenfunctions. We calculate the corresponding density of states using the statistical properties of the speckle potential. We find good agreement with the results of numerical simulations.

Two-site dynamical mean field theory for the dynamic Hubbard model

At zero temperature, two-site dynamical mean field theory is applied to the Dynamic Hubbard model. The Dynamic Hubbard model describes the orbital relaxation that occurs when two electrons occupy the same site, by using a two-level boson field at each site. At finite boson frequency, the appearance of a Mott gap is found to be enhanced even though it shows a metallic phase with the same bare on-site interaction $U$ in the conventional Hubbard model. The lack of electron-hole symmetry is highlighted through the quasi-particle weight and the single particle density of states at different fillings, which qualitatively differentiates the dynamic Hubbard model from other conventional Hubbard-like models.