The clean and sustainable development of biomass resources has attracted tremendous attention to alleviate the increasingly serious energy depletion and environmental problems. Hence, it is urgently needed to design a green product through a cleaner production strategy to bridge the gap between materials and sustainability toward environmental protection and practicality. Herein, a bamboo fiber/polybutylene succinate (PBS) biocomposite that carries silver nanoparticles (AgNPs) with electromagnetic interference (EMI) shielding and antibacterial activity, as well as the performance of interface reinforcement, were prepared using a green, efficient, and scalable bionic strategy of PDA coupling with minimal environmental footprint. The proposed bamboo fiber/PBS biocomposites, which showed multifunctionality and environmental adaptability, revealed good antibacterial activity, where the average inhibition zone diameters against E. coli and S. aureus bacteria reached 5.37 ± 0.36 and 3.96 ± 0.74 mm, respectively. Simultaneously, gains in the EMI shielding effectiveness (∼29.72 dB) and mechanical properties (improved by 24.58% in tensile strength, 39.13% in tensile modulus, 14.60% in flexural strength, and 19.67% in flexural modulus) were realized. Overall, this work displays a novel pathway toward eco-friendly and multifunctional nature fiber/polymer composites for high-value utilization.
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