Abstract

PurposeDespite advances in the development of impact categories for ionising radiation, the focus on artificial radionuclides produced in the nuclear fuel cycle means that the potential impacts resulting from increased exposure to naturally occurring radioactive materials (NORM) are still only covered to a limited degree in life cycle assessment (LCA). Here, we present a potential framework for the inclusion of the exposure routes and impact pathways particular to NORM in LCA.MethodsWe assess the potential magnitude of enhanced NORM exposure, particularly in light of the potential use of NORM residues in building materials, and set out the potential exposure routes that may exist. We then assess the current state of the art, in terms of available fate, exposure and damage models, both within and outside of the LCA sphere. Finally, these exposure routes and modelling techniques are combined in order to lay out a potential framework for NORM assessment in LCA, both in terms of impact on humans and ecosystems.Results and discussionIncreased exposure to NORM radionuclides can result either from their release to the environment or their proximity to humans as they reside in stockpiles, landfills or products. The exposure route via products is considered to be increasingly significant in light of current attempts to incorporate technologically enhanced NORMs (TENORM) including bauxite residue into building materials, by groups such as the ETN-MSCA REDMUD project. Impact assessment models for NORM exposure are therefore required to avoid potential burden shifting in the assessment of such TENORM products. Models describing the fate of environmental releases, the exhalation of radon from building products and the shielding effects on landfills/stockpiles are required to assess potential exposure. Subsequently, models relating exposure to radiation sources and the effective internal and external dose received by receptors are required. Finally, an assessment of the damage caused to the receptors is desirable.ConclusionsA sufficient suite of currently existing and internationally recognised models exist that can, with varying degrees of modification, form the building blocks of a comprehensive NORM characterisation method for LCA. The challenge ahead lies in consolidating these models, from disparate fields, into a coherent and generally applicable method for the assessment of enhanced NORM exposure in LCA.

Highlights

  • Prolonged exposure to low-dose ionising radiation is associated with adverse health effects in both humans and nonhuman biota (IAEA 1976; ICRP 2007)

  • We investigate how the potential adverse effects resulting from increased exposure to naturally occurring radioactive materials (NORM) could be comprehensively incorporated into life cycle assessment (LCA), in a way that would allow the assessment of relevant life cycle environmental and health impacts of products and processes where NORM exposure is likely or significant

  • None of the three main NORM radioisotopes are characterised in the ecosystem impact category, while only releases of 238U to air and water are characterised in the human impact category

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Summary

Introduction

Prolonged exposure to low-dose ionising radiation is associated with adverse health effects in both humans and nonhuman biota (IAEA 1976; ICRP 2007). Routine releases from the nuclear fuel cycle account for less than 0.01% of annual per capita effective dose (0.2 μSv a−1) (UNSCEAR 2000). Where human activities have increased the potential for exposure to materials containing these radioactive elements, these materials are classed as naturally occurring radioactive materials (NORM). Increased exposure to NORM has the potential to lead to adverse health effects upon these receptors (UNSCEAR 2000). The two most important naturally occurring isotopes from a radioprotection standpoint are 238U and 232Th (and their decay series), with 40K representing a significant source of terrestrial radioactivity (World Nuclear Association 2014)

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