Today, hydrogel plugs as a new and effective technology are widely used for temporary oil and gas well plugging. Although, the strength and fluidity of the hydrogels in the oil wells conditions are still most important challenges in their applications in workover operation. In this study, silica nanoparticles were used to improve the network characteristics and strength of hydrogels in addition to reduce the viscosity. It was found that network parameter can be introduced as an effective method for finding the optimum concentration of silica nanoparticles; by application of this method, rheology study is not necessary. The bottle and rheological tests were used to determine the hydrogel strength in desired oil well conditions (high temperature and high salinity). The SEM image of hydrogels showed that the homogenous three-dimensional filler network is formed. The results showed that using 9 wt% of silica nanoparticles decreased the molecular weight between two ties points in network structure in comparison to the neat hydrogels; it also increased the cross-link density of hydrogels (the number of tie points between each entanglement) more than 20 tie points. One of the main findings in this study was considerable increment of strength of hydrogel from 521 Pa to about 26,200 Pa (5000% increasing) that was not reported in other studies. Swelling behavior was also studied in various conditions such as distilled, formation, and tap water and oil solution. Increasing the strength has significantly reduced the hydrogel swelling in the aqueous solution. Based on the results obtained in this study, a polymer hydrogel containing 9 wt% of silica nanoparticles with relatively strong structural strength and thermal stability at 90 °C was proposed for field studies.
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