For the design and certification of wind turbines, it is essential to provide fast and accurate unsteady aerodynamic load prediction models for the whole operational range of angle of attack, up to 180° for vertical-axis and 90° for horizontal-axis wind turbines. This work describes a computationally efficient unsteady forces prediction model based on a deep learning approach, namely the bidirectional long short-term memory (BiLSTM) algorithm, for an airfoil pitched over the full operational range of angles of attack up to 180°. No model has been developed to capture the unsteady forces at high angles of attack. Novel features based on operating conditions and the steady polars of the airfoil are used as inputs for the BiLSTM model. Direct measurements of steady and unsteady forces on a NACA 0021 airfoil model were conducted at reduced frequencies up to 0.075 and a Reynolds number of 120 000 in an open-jet wind tunnel for model learning and testing. The unsteady forces vary significantly from the steady values at high pitching amplitudes and post-stall angles, which, if not accounted for when simulating wind turbine performance, would result in inaccurate predictions. Furthermore, measurements revealed the effect of unsteady vorticity development and shedding on aerodynamic forces under forward and reverse flow conditions. The BiLSTM model is capable of capturing the underlying physics of unsteady aerodynamic forces under extreme operating conditions.