The use of portable electronic devices by passengers on intercity transportation services has apparently risen markedly in recent years. To support the use of such devices, carriers have installed Wi-Fi systems, power outlets, and cell-phone signal boosters for passenger use. To gain perspective on the effects of portable electronic technology on intercity travel behavior, this study evaluates newly collected data for 9,005 passengers on bus, train, and air trips. Field researchers conducted visual surveys to measure the use of devices with audio capability, such as music players and cell phones, and those with visual or audiovisual capacity, such as laptop computers and DVD players. The data collection involved field observations in 14 states as well as the District of Columbia and in Canada. Usage between transportation modes differs in a manner consistent not only with the mix of passengers they serve but also their relative attractiveness to technology use. The highest usage was observed on high-speed trains, which offer spacious seating configurations, Wi-Fi, and power outlets. During peak periods, 47.8% of passengers on Amtrak’s Acela Express were using technology at randomly selected points. This compares to 39.4% and 35.8% of passengers on “curbside buses” and Amtrak trains using some form of technology—more than twice the share of conventional bus services and commercial flights. Rail travelers are much more likely to use visual devices than bus and air passengers. Usage tends to be higher on the East Coast than in Midwest states, California, and Canada. Interpreted broadly, the research suggests that the ability to use portable electronics may be a factor offsetting the longer travel times associated with certain bus and train trips. Portable technology appears to be providing a new incentive for travelers to use surface-transportation modes operating to and from the downtown areas of major cities.