Tunable Terahertz Source Research Articles

Broadband terahertz frequency-domain emission spectroscopy of DAST with a widely tunable quasi-monochromatic source and sensitive up-conversion detection

A continuous 4–32 THz emission spectrum of organic crystal DAST is obtained through a widely tunable quasi-monochromatic terahertz source and sensitive up-conversion detection. The spectrum is characterized by a frequency resolution of ∼0.05 THz and a highest signal-to-noise ratio of ∼65 dB. Terahertz signals are detectable at room temperature even in the high absorption regions of DAST, thus most of the absorption peaks of DAST are clearly located. The results verify the findings of previous works well, including density functional theory calculations and other similar experiments. This paper provides a highly sensitive instrument for broadband terahertz spectroscopic characterization.

Terahertz emission from diamond nitrogen-vacancy centers.

Coherent light sources emitting in the terahertz range are highly sought after for fundamental research and applications. Terahertz lasers rely on achieving population inversion. We demonstrate the generation of terahertz radiation using nitrogen-vacancy centers in a diamond single crystal. Population inversion is achieved through the Zeeman splitting of the S = 1 state in 15 tesla, resulting in a splitting of 0.42 terahertz, where the middle Sz = 0 sublevel is selectively pumped by visible light. To detect the terahertz radiation, we use a phase-sensitive terahertz setup, optimized for electron spin resonance (ESR) measurements. We determine the spin-lattice relaxation time up to 15 tesla using the light-induced ESR measurement, which shows the dominance of phonon-mediated relaxation and the high efficacy of the population inversion. The terahertz radiation is tunable by the magnetic field, thus these findings may lead to the next generation of tunable coherent terahertz sources.

Temperature-Dependent Spin-to-Charge Conversion and Efficient Manipulation of Elliptical THz Waves in Bi2Te3/TbFeCo Heterostructures.

Topological insulators (TIs) with spin-momentum-locked surface states and considerable spin-to-charge conversion (SCC) efficiency are ideal substitutes for the nonmagnetic layer in the traditional ferromagnetic/nonmagnetic (FM/NM) spintronic terahertz (THz) emitters. Here, the TI/ferrimagnetic structure as an effective polarization tunable THz source is verified by terahertz emission spectroscopy. The emitted THz electric field can be separated into two THz components utilizing their opposite symmetry on pump polarization and the magnetic field. TI not only emits a THz electric field via the linear photogalvanic effect (LPGE) but also serves as the medium of SCC via the inverse Edelstein effect (IEE) in the heterostructure. In addition, the amplitude and polarity of the SCC component can be efficiently manipulated by temperature in our ferrimagnetic TbFeCo layer compared with Co or Fe. Once these two THz components are delicately set orthogonally, an elliptical THz wave is generated by the intrinsic phase difference at the THz frequency range. The feasible control of its polarization and chirality is demonstrated by three means: pump polarization, magnetic field, and temperature. These appealing observations may pave the way for the development of elliptical THz wave emitters and polarization-sensitive THz spectroscopy.

Thickness-dependent terahertz emission from Bi2S3 films under excitation below and above the band gap

Two-dimensional (2D) materials demonstrate fascinating thickness-dependent optical properties due to their van der Waals interaction and quantum confinement in the linear optical regime. However, the thickness-dependent nonlinear optical response is more complicated as virtual carriers (dipoles) and real carriers can be generated by below- and above-band-gap excitation, which calls for a more comprehensive understanding of these carriers in 2D materials. Herein, a direct band gap ${\mathrm{Bi}}_{2}{\mathrm{S}}_{3}$ is utilized to investigate the thickness-dependent nonlinear optical response by a terahertz (THz) emission spectroscopy. The results suggest that the THz emission intensity decreases with the increase of band gap energy under an 800-nm femtosecond laser excitation, which can be described by an empirical exponential equation. Under below-band-gap excitation, the optical rectification effect induced by instantaneous polarization (virtual carriers) dominates the THz emission mechanism in thin ${\mathrm{Bi}}_{2}{\mathrm{S}}_{3}$ films. In contrast, under above-band-gap excitation, real carriers are controlled by both resonant optical rectification and surface depletion electric field effects, resulting in shift and drift currents in thick ${\mathrm{Bi}}_{2}{\mathrm{S}}_{3}$ films. The contribution ratio of the shift and drift currents is $\ensuremath{\sim}1:1$ at ${45}^{\ensuremath{\circ}}$ oblique incidence. This competition between shift and drift currents results in the elliptically polarized THz wave generation, and the major axis orientation and ellipticity of the ellipse could be manipulated by changing the polarization of the pump light. In this paper, we imply the potential for designing tunable on-chip THz sources and nonlinear optoelectronic devices based on thickness-dependent 2D materials.

Tunable and coherent terahertz source based on CdSiP2 crystal via collinear difference frequency generation.

CdSiP2 (CSP) crystals have attracted increasing attention as efficient optical conversion media. Herein, the optical properties of a CSP crystal grown with the vertical Bridgman method are measured by a terahertz time-domain spectrometer (THz-TDS) at 0.2-3 THz. For the first time, to the best of our knowledge, the broadband, tunable, coherent, monochromatic THz radiation from 0.08 to 1.68 THz (3775-178 µm) is generated experimentally via this crystal, which is pumped by a nanosecond Q-switched Nd:YAG laser and an optical parametric oscillator (OPO) and based on difference frequency generation (DFG) technology. The output power and its corresponding conversion efficiency at 0.74 THz are 26.6 mW and 1.4 × 10-7, respectively. Our work demonstrates that the CSP crystal is a potential efficient terahertz DFG candidate for out-of-door applications.

THz generation by optical rectification of femtosecond laser pulses in a liquid crystal

In this study, we propose the generation of broadband terahertz (THz) radiation from a liquid crystal with large birefringence in the THz range, pumped by 800 nm femtosecond laser pulses based on optical rectification. Our measurements revealed that the THz amplitude depends on the orientation of the liquid crystal relative to the polarization of the femtosecond pump. Additionally, it was found that the THz peak intensity is linearly dependent on the pump fluence. Furthermore, an elliptically polarized THz wave pattern was observed. The results may lead to a new type of tunable THz source.

Resonance-enhanced spectral funneling in Fabry-Perot resonators with a temporal boundarymirror.

A temporal boundary refers to a specific time atwhich the properties of an optical medium are abruptly changed. When light interacts with the temporal boundary, its spectral content can be redistributed due to the breakingof continuous time-translational symmetry of themedium where light resides. In this work, we use this principle todemonstrate, at terahertz (THz) frequencies, the resonance-enhanced spectral funneling of light coupled to a Fabry-Perot resonator with a temporal boundary mirror. To produce a temporal boundary effect, we abruptly increase the reflectance of a mirror constituting the Fabry-Perot resonator and, correspondingly, its quality factor in a step-like manner. The abrupt increase in the mirror reflectance leads to a trimming of the coupled THz pulse that causes the pulse to broaden in the spectral domain. Through this dynamic resonant process, the spectral contents of the input THz pulse are redistributed into the modal frequencies of the high-Q Fabry-Perot resonator formed after the temporal boundary. An energy conversion efficiency of up to 33% was recorded for funneling into the fundamental mode with a Fabry-Perot resonator exhibiting a sudden Q-factor change from 4.8 to 48. We anticipate that the proposed resonance-enhanced spectral funneling technique could be further utilized in the development of efficient mechanically tunable narrowband terahertz sources for diverse applications.

Hat-Top Beams for Generating Tunable THz Radiations Using a Medium of Conducting Nanocylinders

There are a large number of studies for terahertz (THz) radiation generation, but tunable THz sources are still a challenge since it is difficult to tune frequency, focus and intensity of the radiation simultaneously. The present work proposes the THz generation by the interaction of two hat-top laser beams with a host medium of argon gas containing graphite nanocylinders, as these beams result in highly nonlinear interaction because of a smooth dip in their peak intensity and a fast rise and fall in the overall intensity pattern. Such an interaction produces nonlinear current (6.7 × 108 A/m2) because of the electron cloud of the nanocylinders, which can be modulated by the laser and medium properties for realizing tunable THz radiation. The orientation of basal planes of nanocylinders is shown to be important for this mechanism, though it may be challenging for the experimentalists. The resonant excitation takes place when the plasmon frequency matches the beating frequency of the laser beams, and in the proposed mechanism one can have longitudinal surface plasmon resonance (~12 THz) and transverse surface plasmon resonance (~40 THz), leading to frequency-tunable THz radiation. The role of height and inter particle distance between the adjacent nanocylinders on the THz field amplitude and the efficiency of the mechanism is uncovered by controlling the aspect ratio in the nanocylinders. For example, reducing the inter particle distance from 180 nm to 60 nm leads to the enhancement of THz field from 1 × 108 V/m to 5.48 × 108 V/m. The profile of the emitted THz radiation is investigated in detail under the effect of various parameters in order to prove the practicality of the proposal. The proposed design and mechanism would be attractive for electromagnetic and communication societies which are dealing with millimeter-waves and THz components in addition to its medical application.

Phonon-Related Monochromatic THz Radiation and its Magneto-Modulation in 2D Ferromagnetic Cr2 Ge2 Te6.

Searching multiple types of terahertz (THz) irradiation source is crucial for the THz technology. In addition to the conventional fermionic cases, bosonic quasi‐/particles also promise energy‐efficient THz wave emission. Here, by utilizing a 2D ferromagnetic Cr2Ge2Te6 crystal, first a phonon‐related magneto‐tunable monochromatic THz irradiation source is demonstrated. With a low‐photonic‐energy broadband THz pump, a strong THz irradiation with frequency ≈0.9 THz and bandwidth ≈0.25 THz can be generated and its conversion efficiency could even reach 2.1% at 160 K. Moreover, it is intriguing to find that such monochromatic THz irradiation can be efficiently modulated by external magnetic field below 160 K. According to both experimental and theoretical analyses, the emergent THz irradiation is identified as the emission from the phonon‐polariton and its temperature and magnetic field dependent behaviors confirm the large spin‐lattice coupling in this 2D ferromagnetic crystal. These observations provide a new route for the creation of tunable monochromatic THz source which may have great practical interests in future applications in photonic and spintronic devices.

Terahertz laser diode using field emitter arrays

High-power and broad-tunable terahertz wave generating source on chip, which has broad application prospects, remains an unachieved goal of researchers after decades of pursuing. Here, we propose a concept of terahertz laser diode, which is a dc-biased self-excited microelectronic laser oscillator using collectively modulated free electrons emitted by field-emitter-arrays as the active medium and using an inherent Fabry-P\'erot interferometer formed by port reflections as the frequency selector. It is sub-millimeter to centimeter in size and can generate continuous-wave coherent terahertz radiation with several watts of power per square millimeter. Its frequency can be tuned to cover a wide terahertz band by changing the cathode-to-anode distance and the bias voltage. It has the potential to outperform the conventional free-electron or solid-state terahertz devices in terms of portability, tunability, and output power, signifying a promising class of tunable and high-power terahertz source on chip.

Narrow-band and tunable intense terahertz pulses for mode-selective coherent phonon excitation

We generate frequency-tunable narrow-band intense fields in the terahertz (THz) range by optical rectification of a temporally modulated near-infrared laser pumping a nonlinear organic crystal. Carrier-frequency tunability between 0.5 and 6.5 THz is achieved by changing the modulation period of the laser pump. This tunable narrow-band THz source allows the selective coherent excitation of adjacent vibrational modes, which are demonstrated for two phonons with a frequency offset of 0.8 THz in single-crystal SrCu2(BO3)2. Our compact and scalable source enables an effective approach for the advanced manipulation of low-energy collective modes in condensed matter and has the potential to reveal the coupling of specific lattice vibrations with other degrees of freedom.

Terahertz Dispersion and Amplification under Electron Streaming in Graphene at 300 K

We interpret the recent observations of Otsuji’s team (Sendai) on switching from absorption to amplification at a temperature of T = 300 K during the passage of terahertz radiation through hexagonal boron nitride–graphene sandwiches with multiple gates on the surface with an increase in the electric field in graphene. It is shown that these effects are related to dispersion and negative conductivity near the transit-time frequency of electrons in momentum space under streaming (anisotropic distribution) in graphene in a strong electric field. On the basis of these data, a universal tunable terahertz source is proposed, which has the form of a graphene-containing sandwich with a high-resistance silicon wafer (a cavity) with an applied voltage. This terahertz cavity is a complete analog of the microwave generator implemented on an InP chip by Vorobev’s team (St. Petersburg).

Терагерцовые дисперсия и усиление при стриминге электронов в графене при 300 K

Abstract We interpret the recent observations of Otsuji’s team (Sendai) on switching from absorption to amplification at a temperature of T = 300 K during the passage of terahertz radiation through hexagonal boron nitride–graphene sandwiches with multiple gates on the surface with an increase in the electric field in graphene. It is shown that these effects are related to dispersion and negative conductivity near the transit-time frequency of electrons in momentum space under streaming (anisotropic distribution) in graphene in a strong electric field. On the basis of these data, a universal tunable terahertz source is proposed, which has the form of a graphene-containing sandwich with a high-resistance silicon wafer (a cavity) with an applied voltage. This terahertz cavity is a complete analog of the microwave generator implemented on an InP chip by Vorobev’s team (St. Petersburg).

Investigation of terahertz radiation based on forward and backward wave feedback circuit

A forward and backward wave feedback circuit for a vacuum terahertz radiation source is proposed and demonstrated. In the feedback circuit, two bunched electron beams with different velocities interact with two spatial harmonics, respectively. The simulation reveals that the forward wave and the backward wave form a feedback circuit and affect each other through beam-wave interaction. Furthermore, the maximum gain of the forward wave of the feedback circuit is about 12.4 dB higher than the single beam traveling wave tube. When observing the excitation of the backward wave, it is found that the starting current is 44.4% lower than the traditional backward wave oscillator. The forward and backward wave feedback circuit is a promising choice for the watt-level tunable compact terahertz source that can be potentially used in a transmitter for Terahertz radar detection.

Continuously tunable narrow-band terahertz generation with a dielectric lined waveguide driven by short electron bunches

A continuously tunable narrow-band terahertz source based on Cherenkov wakefield generation in a dielectric lined waveguide driven by short sub-picosecond electron bunches has been experimentally demonstrated. A large tunability range of 0.55--0.95 THz was achieved by implementing the waveguide design as a planar structure with variable 0.15--1.10 mm gap and thin $25\text{ }\text{ }\ensuremath{\mu}\mathrm{m}$ dielectric layers. The source operates essentially in a single mode regime with higher order modes of negligible intensity. THz pulse energy was measured across the tunable range and compared with theory.

Modulation of terahertz radiation from graphene surface plasmon polaritons via surface acoustic wave.

We present a theoretical study of terahertz (THz) radiation induced by surface plasmon polaritons (SPPs) on a graphene layer under modulation by a surface acoustic wave (SAW). In our gedanken experiment, SPPs are excited by an electron beam moving on a graphene layer situated on a piezoelectric MoS2 flake. Under modulation by the SAW field, charge carriers are periodically distributed over the MoS2 flake, and this causes periodically distributed permittivity. The periodic permittivity structure of the MoS2 flake folds the SPP dispersion curve back into the center of the first Brillouin zone, in a manner analogous to a crystal, leading to THz radiation emission with conservation of the wavevectors between the SPPs and the electromagnetic waves. Both the frequency and the intensity of the THz radiation are tuned by adjusting the chemical potential of the graphene layer, the MoS2 flake doping density, and the wavelength and period of the external SAW field. A maximum energy conversion efficiency as high as ninety percent was obtained from our model calculations. These results indicate an opportunity to develop highly tunable and integratable THz sources based on graphene devices.

Flux-flow Josephson oscillator as the broadband tunable terahertz source to open space

The flux-flow oscillator (FFO) based on a long Josephson junction has been implemented as a broadband tunable terahertz (THz) source to open space. For this purpose, the transmitting slot antenna has been coupled to the oscillator. Additionally, an elliptical lens with a diameter of 10 mm has been matched to the antenna, forming a narrow output beam of the THz emission. Two designs for the antenna, integrated with the oscillator and developed for operation at different frequency ranges of 0.32–0.55 THz and 0.4–0.7 THz, have been investigated. The FFO has been phase locked to an external reference oscillator by utilizing a harmonic mixer. Its linewidth in the phase-locking regime is determined by the phase noise of the reference oscillator and the number of harmonics used and has been measured to be less than 0.1 MHz. A free-running FFO linewidth from about 2 MHz to several MHz, depending on the operating point, has been obtained. Output emission to open space has been measured by a superconducting integrated spectrometer located in a separate cryostat. The FFO operation as an external source with the achieved emission power and spectral characteristics has demonstrated its applicability for different tasks and purposes where tunable THz sources are required.

Verification of Non-thermal Effects of 0.3–0.6 THz-Waves on Human Cultured Cells

Recent progress has been made in the development of terahertz (THz) waves for practical applications. Few studies that have assessed the biological effects of THz waves have been reported, and the data currently available regarding the safety of THz waves is inadequate. In this study, the effect of THz wave exposure on two cultured cells was assessed using a widely tunable THz source with a 0.3–0.6 THz frequency range, which can be used and increased in one GHz increments. The THz waves applied to the cultured cells were weak enough such that any thermal effects could be disregarded. The influence of THz wave exposure on both the proliferative and metabolic activities of these cells was investigated, as well as the extent of the thermal stress placed on the cells. In this work, no measurable effect on the proliferative or metabolic activities of either cell type was observed following the exposure to THz waves. No differences in the quantity of cDNA related to heat shock protein 70 was detected in either the sham or exposure group. As such, no differences in cellular activity between cells exposed to THz waves and those not exposed were observed.

Over 100-THz bandwidth selective difference frequency generation at LaAlO3/SrTiO3 nanojunctions

The ability to combine continuously tunable narrow-band terahertz (THz) generation that can access both the far-infrared and mid-infrared regimes with nanometer-scale spatial resolution is highly promising for identifying underlying light-matter interactions and realizing selective control of rotational or vibrational resonances in nanoparticles or molecules. Here, we report selective difference frequency generation with over 100 THz bandwidth via femtosecond optical pulse shaping. The THz emission is generated at nanoscale junctions at the interface of LaAlO3/SrTiO3 (LAO/STO) that is defined by conductive atomic force microscope lithography, with the potential to perform THz spectroscopy on individual nanoparticles or molecules. Numerical simulation of the time-domain signal facilitates the identification of components that contribute to the THz generation. This ultra-wide-bandwidth tunable nanoscale coherent THz source transforms the LAO/STO interface into a promising platform for integrated lab-on-chip optoelectronic devices with various functionalities.

Terahertz Cherenkov radiation induced by a self-modulated electron beam in plasma wakefield

In this paper, a novel scheme of generating terahertz radiation is proposed, which considers a relativistic electron beam being modulated by its self-excited plasma wakefield in a plasma-filled slow-wave structure (SWS). Both the dispersion relation and the particle-in-cell simulation show that the self-modulation of the beam can act as a mode-selection method to excite the high-harmonics of the SWS and generate terahertz electromagnetic radiation. The present work gives a new thought for researching high-power and tunable terahertz sources.